This study investigates the seismic behavior of composite shear walls reinforced with post-casting Ultra-High Performance Concrete (UHPC) boundary elements and Colded-Rolled Ribbed Bars (CRB600H). The research aims to explore the synergistic effects of UHPC and CRB600H bars on seismic performance. Six shear wall specimens with a shear span ratio of 1.56 were subjected to cyclic loading to evaluate their failure modes, crack patterns, hysteresis behavior, stiffness degradation, ductility, residual deformation, and energy dissipation capacity. The results demonstrated that the use of CRB600H bars in boundary elements of normal concrete specimens improved post-yield stiffness and reduced residual deformation. Conversely, incorporating UHPC in boundary elements enhanced load-bearing capacity and crack control but slightly reduced ductility due to the weaker interfacial connection between UHPC and the foundation. Additionally, CRB600H bars in the web region improved load-bearing capacity while maintaining ductility comparable to HRB400 bars. The findings suggest that substituting CRB600H for HRB400 in shear-dominant regions can enhance the seismic performance of shear walls. Finally, the multi-layer shell element numerical model validated by the experimental results was encouraged to conduct parametric analysis in the future. This research supports the development of more resilient building structures by integrating high-performance materials in key structural components.