Magnonic Spin Currents Research Articles

Understanding spin currents from magnon dispersion and polarization: Spin-Seebeck effect and neutron scattering study on Tb3Fe5O12

Magnon spin currents in the ferrimagnetic garnet Tb3Fe5O12 with 4f electrons were examined through the spin-Seebeck effect and neutron scattering measurements. The compound shows a magnetic compensation, where the spin-Seebeck signal reverses above and below Tcomp=249.5(4) K. Unpolarized neutron scattering unveils two major magnon branches with finite energy gaps, which are well explained in the framework of spin-wave theory. Their temperature dependencies and the direction of the precession motion of magnetic moments, i.e., magnon polarization, defined using polarized neutrons, explain the reversal at Tcomp and decay of the spin-Seebeck signals at low temperatures. We illustrate an example that momentum- and energy-resolved microscopic information is a prerequisite to understand the magnon spin current.

Electric Field Switching of Magnon Spin Current in a Compensated Ferrimagnet.

Manipulation of directional magnon propagation, known as magnon spin current, is essential for developing magnonic devices featuring nonvolatile functionalities and ultralow power consumption. Magnon spin current can usually be modulated by magnetic field or current-induced spin torques. However, these approaches may lead to energy dissipation due to Joule heating. Electric-field switching of magnon spin current without charge current is highly preferred but challenging to realize. By integrating magnonic and piezoelectric materials, the manipulation of the magnon spin current generated by the spin Seebeck effect in the ferrimagnetic insulator Gd3Fe5O12 (GdIG) film on a piezoelectric substrate is demonstrated. Reversible electric-field switching of magnon polarization without applied charge current is observed. Through strain-mediated magnetoelectric coupling, the electric field induces the magnetic compensation transition between two magnetic states of the GdIG, resulting in its magnetization reversal and the simultaneous switching of magnon spin current. This work establishes a prototype material platform that paves the way for developing magnon logic devices characterized by all electric field reading and writing and reveals the underlying physics principles of their functions.

Thermal generation of spin current in a quantum dot coupled to magnetic insulators

In this work, we study thermally-generated spin current in the system consisting of a quantum dot connected to two magnetic insulators. The external leads are kept at different temperatures which leads to an imbalance of magnon populations in two magnetic insulators resulting in the flow of the magnon (spin) current. We take into account many-body magnon interactions and incorporate energy-dependent density of states of the magnetic insulators. Both features can strongly affect magnon distribution in the magnetic insulators and the coupling strengths between the leads and the dot, and thus, the thermally generated spin current. All the calculations are carried out in the weak coupling regime. We show, that results obtained with a density of states being a function of energy differ significantly from the ones obtained with a density of states taken as a constant. In turn, magnon interactions in the leads proved to be important at high temperatures and large values of energy of transported spin waves.

Spin swapping for an exchange magnon spin current

Spin swapping for an exchange magnon spin current

Coherent magnon-induced domain-wall motion in a magnetic insulator channel.

Advancing the development of spin-wave devices requires high-quality low-damping magnetic materials where magnon spin currents can efficiently propagate and effectively interact with local magnetic textures. Here we show that magnetic domain walls can modulate spin-wave transport in perpendicularly magnetized channels of Bi-doped yttrium iron garnet. Conversely, we demonstrate that the magnon spin current can drive domain-wall motion in the Bi-doped yttrium iron garnet channel device by means of magnon spin-transfer torque. The domain wall can be reliably moved over 15-20 µm distances at zero applied magnetic field by a magnon spin current excited by a radio-frequency pulse as short as 1 ns. The required energy for driving the domain-wall motion is orders of magnitude smaller than those reported for metallic systems. These results facilitate low-switching-energy magnonic devices and circuits where magnetic domains can be efficiently reconfigured by magnon spin currents flowing within magnetic channels.

Highly tunable spin Hall magnetoresistance in room-temperature magnetoelectric multiferroic, Sr3Co2Fe24O41|Pt hybrids

We present spin transport studies on a low-field, room-temperature magnetoelectric multiferroic polycrystalline Sr3Co2Fe24O41|Pt heterostructure wherein a highly tunable transverse conical magnetic phase is responsible for static and dynamic magnetoelectric coupling. We measured angular dependence of spin Hall magnetoresistance (SMR) at constant magnetic fields (H) in the range; 50–100 kOe. Application of field below the critical value (Hc1 ≈ 2.5 kOe), yielded negative SMR and the H-evolution of normalized SMR ((ΔR∕R0) × 100 %) exhibited a negative gradient. Further, an increase in H resulted in the positive slope of (ΔR∕R0) × 100 % Vs. H and later at higher H around 14 kOe, a crossover from negative to positive SMR was observed. We employed a simple model for estimating the equilibrium magnetic configuration and computed the SMR modulation at various values of H. We argue that the tilting of the cone is dominant and in turn responsible for the observed nature of SMR below 2.5 kOe while, the closing of the cone-angle is pronounced at higher fields causing a reversal in sign of the SMR from negative to positive. Importantly, SMR experiments revealed that a change in the helicity with a reversal of the magnetic field has no influence on the observed SMR. Longitudinal spin Seebeck effect (LSSE) signal was measured to be ≈ 500 nV at 280 K, under application of thermal gradient, ΔT = 23 K and field, 60 kOe. The observed LSSE signal, originating from pure magnon spin current, showed a similar H-dependent behavior as that of the magnetization of Sr3Co2Fe24O41. Our detailed spin transport studies on polycrystalline Sr3Co2Fe24O41|Pt heterostructure demonstrate high tunability of the amplitude and the sign of the SMR, highlighting its potential for novel spintronic devices such as SMR-based spin valves and voltage-controlled spin transport devices.

Nonlinear spin current of photoexcited magnons in collinear antiferromagnets

We study the nonlinear magnon spin current induced by an ac electric field under light irradiation in collinear antiferromagnets with broken inversion symmetry. For linearly polarized light, we find that a dc spin current appears through ``the magnon spin shift current" mechanism, which is driven by a spin polarization generation in the two magnon creation process and has a close relationship to the geometry of magnon bands through Berry connection. For circularly polarized light, a dc spin current appears through ``the spin injection current" mechanism, which is proportional to the relaxation time of magnons and can be large when the magnon lifetime is long. We demonstrate generation of the magnon spin shift and injection currents, based on a few toy models and a realistic model for a multiferroic material M$_2$Mo$_3$O$_8$.

Theoretical Study of Magnon Spin Currents in Chromium Trihalide Hetero-bilayers: Implications for Magnonic and Spintronic Devices

The intriguing magnetic behavior of two-dimensional chromium trihalide materials holds great promises for spintronics and magnonics. Here, we study the stacking-dependent magnetism in (CrBr3/CrI3) hetero-bilayers by using first-principles calculations. We find that different stackings yield ferromagnetic ground states or favor an antiferromagnetic (AFM) interlayer coupling. Starting from ab initio results, we study the magnonic spectra and magnon spin textures in the hetero-bilayer. Based on our findings, we propose an experimental setup for the optical generation and electric detection of pure magnon spin currents in layered AFM (LAFM) (CrBr3/CrI3) hetero-bilayers. Furthermore, we propose a device to simultaneously realize magnon spin currents and topological domain walls in the hetero-bilayers. The advantages of (CrBr3/CrI3) hetero-bilayers over the (CrI3)2 homo-bilayers to realize magnon spin currents are highlighted. The interesting features of magnons in LAFM hetero-bilayers and their potential for spin-charge conversion could pave the way for their implementation in spin-based transistors and logic devices.

Spin transport modified by magnetic order

Spintronics has developed over the years from initially generating spin-polarized charge currents from exchange interaction in ferromagnets, into a more general concept, where electronic spin current can be generated and manipulated by spin–orbit interactions and in addition magnonic spin currents can occur in magnetically ordered materials even if they are insulating. Thus the interplay between spin transport and magnetic order has been a very active research field, which has developed many new ideas, such as thermal spin transport and electronic spin currents with unusual symmetries generated by magnetically ordered materials. This article discusses a few selected examples in order to illustrate some of the complexities that can be encountered in these systems. A particular focus is on the contributions from Chia-Ling Chien and his research group, who often explored many of the topics at the forefront of spintronics research, while critically examining unproven assumptions made by other researchers in the field.

Rectification of the spin Seebeck current in noncollinear antiferromagnets

In the absence of an external magnetic field and a spin-polarized charge current, an antiferromagnetic system supports two degenerate magnon modes. An applied thermal bias activates the magnetic dynamics, leading to a magnon flow from the hot to the cold edge (magnonic spin Seebeck current). Both degenerate bands contribute to the magnon current but the orientations of the magnetic moments underlying the magnons are opposite in different bands. Therefore, while the magnon current is nonzero, the net spin current is zero. To obtain a nonzero net spin current, one needs to apply either a magnetic field or a spin-polarized charge current that lifts the bands' degeneracy. Here, attaching a thermal contact to one edge of a helical nanowire, we study three different magnonic spin currents: (i) the exchange, and (ii) Dzyaloshinskii--Moriya spin currents flowing along the helical nanowire, and (iii) magnonic spin current pumped into the adjacent normal-metal layer. We find that the combination of Dzyaloshinskii--Moriya interaction and external magnetic field substantially enhances the spin current compared to the current generated solely through a magnetic field. Due to nonreciprocal magnons and magnon dichroism effect, the Dzyaloshinskii--Moriya and exchange spin currents show left-right propagation asymmetry, with $20%$ of current rectification. The spin pumping current shows a slight asymmetry only in the case of a strong Dzyaloshinskii--Moriya interaction. The observed effects are explained in terms of the magnon dispersion relations and the magnon Doppler effect.

Magnon drag in a metal–insulating antiferromagnet bilayer

We study a bilayer structure consisting of an antiferromagnetic insulator and a normal metal. An electron current is driven in the normal metal with direction parallel to the interface between the materials. Due to interfacial exchange coupling between the localized spins in the antiferromagnet and the itinerant electrons in the normal metal, a magnon current can then be induced in the antiferromagnet. Using an uncompensated antiferromagnetic interface, creating an asymmetry in the interfacial coupling to the two degenerate magnon modes, we find that it is possible to generate a magnon spin current. The magnon spin current can be enhanced by increasing the temperature or by spin-splitting the magnon modes.

Direct and alternating magnon spin currents across a junction interface irradiated by linearly polarized laser

The developments in the field of quantum optics raise expectations that laser-matter coupling is a promising building block for magnonics. Here, we propose a method for the generation of direct and alternating spin currents of magnons across the junction interface irradiated by linearly polarized laser. In a junction of ferromagnetic insulators with a large electronic gap, the spin angular momentum is exchanged during the tunneling process of magnons across the junction interface. The advanced technology in the field of plasmonics and metamaterials realizes that spins irradiated by the laser field interact only with the magnetic component of the laser through the Zeeman coupling. Using an analytic perturbation theory, we provide a general formula for magnon transport induced by the inversion symmetry breaking across the junction interface. Then, we show that those spin currents are enhanced by the ferromagnetic resonance, and the period of the ac spin current is one-half of that of the laser magnetic field. Finally, we estimate the magnitude of the spin current, and find that it will be within experimental reach.

A perspective on magnon spin Nernst effect in antiferromagnets

Magnon excitations in antiferromagnetic materials and their physical implications have helped to facilitate the emergence of device concepts not presently available in ferromagnets. A unique characteristic of antiferromagnetic magnons is the coexistence of opposite spin polarization, which mimics the electron spin in a variety of transport phenomena. Among them, the most prominent spin-contrasting phenomenon is the magnon spin Nernst effect (SNE), which refers to the generation of a transverse pure magnon spin current through a longitudinal temperature gradient. We introduce selected recent progress in the study of magnon SNE in collinear antiferromagnets with focus on its underlying physical mechanism entailing profound topological features of magnon band structures. By reviewing how the magnon SNE has inspired and enriched the exploration of topological magnons, we offer our perspective on this emerging frontier that holds potential in future spintronic nano-technology.

Magnon transport in Y3Fe5O12/Pt nanostructures with reduced effective magnetization

For applications making use of magnonic spin currents damping effects, which decrease the spin conductivity, have to be minimized. We here investigate the magnon transport in an yttrium iron garnet thin film with strongly reduced effective magnetization. We show that in a three-terminal device the effective magnon conductivity can be increased by a factor of up to six by a current applied to a modulator electrode, which generates damping compensation above a threshold current. Moreover, we find a linear dependence of this threshold current on the applied magnetic field. We can explain this behavior by the reduced effective magnetization and the associated nearly circular magnetization precession.

Magnon Spin Current Induced by Triplet Cooper Pair Supercurrents.

At the interface between a ferromagnetic insulator and a superconductor there is a coupling between the spins of the two materials. We show that when a supercurrent carried by triplet Cooper pairs flows through the superconductor, the coupling induces a magnon spin current in the adjacent ferromagnetic insulator. The effect is dominated by Cooper pairs polarized in the same direction as the ferromagnetic insulator, so that charge and spin supercurrents produce similar results. Our findings demonstrate a way of converting Cooper pair supercurrents to magnon spin currents.

Electric field control of magnon spin currents in an antiferromagnetic insulator.

Pure spin currents can be generated via thermal excitations of magnons. These magnon spin currents serve as carriers of information in insulating materials, and controlling them using electrical means may enable energy efficient information processing. Here, we demonstrate electric field control of magnon spin currents in the antiferromagnetic insulator Cr2O3. We show that the thermally driven magnon spin currents reveal a spin-flop transition in thin-film Cr2O3. Crucially, this spin-flop can be turned on or off by applying an electric field across the thickness of the film. Using this tunability, we demonstrate electric field–induced switching of the polarization of magnon spin currents by varying only a gate voltage while at a fixed magnetic field. We propose a model considering an electric field–dependent spin-flop transition, arising from a change in sublattice magnetizations via a magnetoelectric coupling. These results provide a different approach toward controlling magnon spin current in antiferromagnets.

Exceptional sign changes of the nonlocal spin Seebeck effect in antiferromagnetic hematite

Low power spintronic devices based on the propagation of pure magnonic spin currents in antiferromagnetic insulator materials offer several distinct advantages over ferromagnetic components including higher frequency magnons and a stability against disturbing external magnetic fields. In this work, we make use of the insulating antiferromagnetic phase of iron oxide, the mineral hematite $\alpha$-Fe$_2$O$_3$ to investigate the long distance transport of thermally generated magnonic spin currents. We report on the excitation of magnons generated by the spin Seebeck effect, transported both parallel and perpendicular to the antiferromagnetic easy-axis under an applied magnetic field. Making use of an atomistic hematite toy model, we calculate the transport characteristics from the deviation of the antiferromagnetic ordering from equilibrium under an applied field. We resolve the role of the magnetic order parameters in the transport, and experimentally we find significant thermal spin transport without the need for a net magnetization.

Theory for phonon pumping by magnonic spin currents

In recent years several experimental observations and theoretical predictions of unique phenomena involving the interplay between spin currents and the coupled magnetization-elastic dynamics have invigorated the field of spintronics. One important experiment reported several years ago showed that elastic waves can produce spin pumping, that is, generation of spin currents in a metallic film in contact with a ferromagnetic material. Very recently the Onsager reciprocal of this effect has been observed in samples made of a film of the insulating ferrimagnet yttrium iron garnet in contact with a platinum strip with nanoscopic silver particles that is known to exhibit a giant spin Hall effect. By passing an electric current through the metallic strip, the spin current generated by the spin Hall effect produces a large magnonic spin current that excites phonons with microwave frequency, observed by Brillouin light scattering. Here we show that these experiments are explained by a theory based on a process in which one magnon in the spin current creates one phonon and another magnon, with conservation of energy and momentum. The theoretical value of the critical charge current in the metallic strip necessary to drive phonons and the values of the phonon frequencies are in good agreement with the values measured experimentally.

Interlayer coupling effect on skyrmion dynamics in synthetic antiferromagnets

Skyrmions in synthetic antiferromagnets (SAFs) could be immune to the skyrmion Hall effect and are, thus, promising in spintronics applications. We introduce breathing modes that can be realized by changing the magnetocrystalline anisotropy periodically in time to generate spin waves around a deformed SAF skyrmion. The net momentum transferred from the magnon spin currents results in a motion of the SAF skyrmion, which is two orders of magnitude faster than that of a ferromagnetic skyrmion. We also reveal that the velocity of the SAF skyrmion can be manipulated by the strength of antiferromagnetic coupling between layers, which is different from ferromagnetic and antiferromagnetic systems. This phenomenon originates from the damping-like character of the antiferromagnetic coupling and offers a dimension to optimize skyrmion dynamics in SAFs.

Evidence of phonon pumping by magnonic spin currents

Spin current phenomena are at the heart of the active research field of spintronics that aims to develop new perspectives for emerging information technologies. In recent years, several groups reported experiments in which spin currents are used to excite coherent magnetization dynamics in magnetic nanostructures. Here, we show experimentally two effects of the large spin current generated by the giant spin Hall effect in a platinum strip with nanoscopic silver particles adjacent to a film of the insulating ferrimagnet yttrium iron garnet (YIG). The first, demonstrated by ferromagnetic resonance (FMR) experiments, is the dramatic reduction of the magnon damping measured by the FMR linewidth due to the spin torque produced by the spin current. The second, observed by Brillouin light scattering (BLS), is the excitation of quasi-particles in the YIG film with frequencies that do not vary with the applied magnetic field. We interpret the BLS signal as due to phonons excited by the magnonic spin current injected into the YIG film, in a process that is the Onsager reciprocal of the spin pumping by coherent elastic waves.