Magneto-optical Trap Research Articles

External-cavity diode laser at 2.6 µm and its frequency stabilization with a scanning Fabry-Pérot cavity

We report on the construction of an external cavity diode laser at 2.6 µm wavelength and its frequency stabilization with an external scanning Fabry-Pérot cavity using Pound-Drever-Hall (PDH) frequency stabilization technique. We discuss the frequency noise characteristics of the laser using the PDH residual error signal analysis and the locking performance. We have achieved a 2.5 x 105 suppression factor in the frequency noise power spectral density at Fourier frequencies lower than 100 Hz when the laser is stabilized. The laser is employed to observe resonant excitation on the 5s5p3P0 →5s4d3D1 transition in cold 88Sr atoms trapped in a magneto-optical trap. We have observed an enhancement in the trapped atom number by a factor of 8.3 compared to the case when a single laser at 707 nm is employed for repumping.

Enabling Photonic Integrated 3D Magneto-Optical Traps for Quantum Sciences and Applications

Enabling Photonic Integrated 3D Magneto-Optical Traps for Quantum Sciences and Applications

Absolute frequency measurements on the 5s5p3P0 → 5s6d3D1 transition in strontium

We report the first absolute frequency measurements for the 5s5p3P0→5s6d3D1 transition at 394 nm for all the stable strontium isotopes by utilizing repumping induced spectroscopy in a magneto-optical trap. Absolute transition frequency is measured to be 760524409251(25) kHz for Sr88. With reference to Sr88, the isotope shifts are measured to be 91052(35), 54600(33), and 51641(28) kHz for Sr84, Sr86, and Sr87, respectively. We calculate the hyperfine constants A and B for the fermionic isotope Sr87 at kHz level. Furthermore, we perform King plot analysis by combining isotope shifts on the 689-nm transition to our data. Published by the American Physical Society 2024

Limitation of single-repumping schemes for laser cooling of Sr atoms

We explore the efficacy of two single-repumping schemes, 5s5pP23−5p2P23 (481nm) and 5s5pP23−5s5dD23 (497nm), for a magneto-optical trap (MOT) of Sr atoms. We reveal that the enhancement in the MOT lifetime is limited to 26.9(2) for any single-repumping scheme. Our investigation indicates that the primary decay path from the 5s5pP11 state to the 5s5pP03 state proceeds via the 5s4dD13 state, rather than through the upper states accessed by the single-repumping lasers. We estimate that the branching ratio for the 5s5pP11→5s4dD13→5s5pP03 decay path is 1:3.9(1.5)×106 and the decay rate for the transition from the 5s5pP11 state to the 5s4dD13 state is 83(32)s−1. This outcome underscores the limitation on atom number in the MOT for long loading times (≳1s) when employing a single-repumping scheme. These findings will contribute to the construction of field-deployable optical lattice clocks. Published by the American Physical Society 2024

An atomic beam of titanium for ultracold atom experiments.

We generate an atomic beam of titanium (Ti) using a "Ti-ball" Ti-sublimation pump, which is a common getter pump used in ultrahigh vacuum systems. We show that the sublimated atomic beam can be optically pumped into the metastable 3d3(4F)4sa5F5 state, which is the lower energy level in a cycling optical transition that can be used for laser cooling. We measure the atomic density and transverse and longitudinal velocity distributions of the beam through laser fluorescence spectroscopy. We find a metastable atomic flux density of 4.3(2) × 109s-1cm-2 with a mean forward velocity of 773(8) m/s at 2.55cm directly downstream of the center of the Ti-ball. Owing to the details of optical pumping, the beam is highly collimated along the transverse axis parallel to the optical pumping beam and the flux density falls off as 1/r. We discuss how this source can be used to load atoms into a magneto-optical trap.

Three-dimensional, multi-wavelength beam formation with integrated metasurface optics for Sr laser cooling.

We demonstrate the formation of a complex, multi-wavelength, three-dimensional laser beam configuration with integrated metasurface (MS) optics. Our experiments support the development of a compact Sr optical-lattice clock, which leverages magneto-optical trapping at 461 nm and 689 nm without bulk free-space optics. We integrate six mm-scale metasurfaces on a fused silica substrate and illuminate them with light from optical fibers. The metasurfaces provide full control of beam pointing, divergence, and polarization to create the laser configuration for a magneto-optical trap. We report the efficiency and integration of the visible laser beam configuration, demonstrating the suitability of metasurface optics for atomic laser cooling.

Apparatus for producing single strontium atoms in an optical tweezer array

Abstract We outline an experimental setup for efficiently preparing a tweezer array of $^{88}$Sr atoms. Our setup uses permanent magnets to maintain a steady-state two-dimensional magneto-optical trap (MOT) which results in a loading rate of up to $10^{8}$ s$^{-1}$ at 5 mK for the three-dimensional blue MOT. This enables us to trap $2\times10^{6}$ $^{88}$Sr atoms at 2 $\mu$K in a narrow-line red MOT with the $^{1}$S$_{0}$ $\rightarrow$ $^{3}$P$_{1}$ intercombination transition at 689 nm. With the Sisyphus cooling and pairwise loss processes, single atoms are trapped and imaged in 813 nm optical tweezers, exhibiting a lifetime of 2.5 minutes. We further investigate the survival fraction of a single atom in the tweezers and characterize the optical tweezer array using a release and recapture technique. Our experimental setup serves as an excellent reference for those engaged in experiments involving optical tweezer arrays, cold atom systems, and similar research.

Experimental realization of multiple frequency photoassociation in an optical dipole trap.

The generation of cold molecules is an important topic in the field of cold atoms and molecules and has received relevant advanced research attention in ultracold chemistry, quantum computation, and quantum metrology. With a high atomic phase space density, optical dipole traps have been widely used to prepare, trap, and study cold molecules. In this work, Rb2 molecules were photoassociated in a magneto-optical trap to obtain a precise rovibrational spectrum, which provided accurate numerical references for the realization of multiple frequency photoassociation. By meeting the harsh requirements of photoassociation in optical dipole traps, the cold molecule photoassociation process was well explored, and different photoassociation resonances were simultaneously addressed in a single optical dipole trap. This method can be universally extended to simultaneously photoassociate cold molecules with different internal states or atomic species in a single optical dipole trap, thus advancing generous cold molecule studies such as cold molecule collision dynamics.

Three-Dimensional Magneto-Optical Trapping of Barium Monofluoride.

As a heavy molecule, barium monofluoride (BaF) presents itself as a promising candidate for measuring permanent electric dipole moment. Here we report the realization of three-dimensional magneto-optical trapping (MOT) of BaF molecules. Through the repumping of all the vibrational states up to v=3, and rotational states up to N=3, we effectively close the transition to a leakage level lower than 10^{-5}. This approach enables molecules to scatter a sufficient number of photons required for laser cooling and trapping. By employing a technique that involves chirping the slowing laser frequency, BaF molecules are decelerated to near-zero velocity, resulting in the capture of approximately 3×10^{3} molecules in a MOT. Our findings represent a significant step towards the realization of ultracold BaF molecules and the conduct of precision measurements with cold molecules.

Reinforcement learning in cold atom experiments

Cold atom traps are at the heart of many quantum applications in science and technology. The preparation and control of atomic clouds involves complex optimization processes, that could be supported and accelerated by machine learning. In this work, we introduce reinforcement learning to cold atom experiments and demonstrate a flexible and adaptive approach to control a magneto-optical trap. Instead of following a set of predetermined rules to accomplish a specific task, the objectives are defined by a reward function. This approach not only optimizes the cooling of atoms just as an experimentalist would do, but also enables new operational modes such as the preparation of pre-defined numbers of atoms in a cloud. The machine control is trained to be robust against external perturbations and able to react to situations not seen during the training. Finally, we show that the time consuming training can be performed in-silico using a generic simulation and demonstrate successful transfer to the real world experiment.

Use of the 5P3/2→6P3/2 electric dipole forbidden transition in Rb as a non-perturbing probe of atom dynamics in an operating magneto-optical trap

Abstract Results of spectroscopy experiments using the $5P_{3/2} \to 6P_{3/2}$ electric dipole forbidden transition in cold rubidium atoms are presented. Production of this forbidden transition is detected by observing the emission of the $420 $ nm fluorescence photons that result from the decay of the $6P_{3/2} $ state into the ground state. The experiments are performed under the steady state operation conditions of a magneto-optical trap (MOT), and thus provide non-perturbing information on the atom-light system. The hyperfine structure of the $6P_{3/2}$ level is completely resolved, and the fluorescence peaks show the expected Autler-Townes (AT) splitting of the emission lines. This hyperfine structure is used to calibrate the frequency scale of all spectra recorded. A combination of this absolute frequency scale and an expression for the AT profile allows an absolute determination of the effective Rabi frequency and detuning of the MOT. The behavior of these AT doublets is studied as a function of frequency detuning and also as a function of the trapping light intensity.
The experiments also take full advantage of the strong polarization dependence of the relative intensities of the hyperfine fluorescence components.
This study results in a sensitive probe of the relative populations of the magnetic sublevel projections relative to the trapping magnetic field gradient.
An almost isotropic population distribution was found, but small deviations from isotropy could be determined with this electric dipole forbidden probe.

Ratchet loading and multi-ensemble operation in an optical lattice clock

We demonstrate programmable control over the spatial distribution of ultra-cold atoms confined in an optical lattice. The control is facilitated through a combination of spatial manipulation of the magneto-optical trap and atomic population shelving to a metastable state. We first employ the technique to load an extended (5 mm) atomic sample with uniform density in an optical lattice clock (OLC), reducing atomic interactions and realizing remarkable frequency homogeneity across the atomic cloud. We also prepare multiple spatially separated atomic ensembles, and realize multi-ensemble clock operation within the standard one-dimensional (1D) OLC architecture. Leveraging this technique, we prepare two oppositely spin-polarized ensembles that are independently addressable, offering a platform for implementing spectroscopic protocols for enhanced tracking of local oscillator phase. Finally, we demonstrate a relative fractional frequency instability at one second of 2.4(1)×10−17 between two ensembles, useful for characterization of intra-lattice differential systematics.

Realization of a single-beam, detachable, cascaded 2D magneto-optical trap based modular cesium source

We present a detachable, cascaded modular cesium loading source based on a 2D magneto-optical trap (MOT). Our design utilizes only a single beam of mixed cooling and repumping light that is split evenly into five discrete trapping regions, each with horizontal and vertical beams. The pre-aligned, single-beam design makes our module suitable for miniaturization. The generated cold atomic beam serves to load a 3D MOT, whose loading rate we use to characterize the efficiency of our design. The effect of individual trapping regions relative to the differential tube and to each other on the loading rate has also been examined. Experimental results were compared with a numerical simulation. We are able to obtain an experimental loading rate of nearly 8×107atoms/s and a vapor density of about 3×1015atoms/m3 in our 2D MOT module.

Realization of a chip-based hybrid trapping setup for 87Rb atoms and Yb+ ion crystals.

Hybrid quantum systems integrate laser-cooled trapped ions and ultracold quantum gases within a single experimental configuration, offering vast potential for applications in quantum chemistry, polaron physics, quantum information processing, and quantum simulations. In this study, we introduce the development and experimental validation of an ion trap chip that incorporates a flat atomic chip trap directly beneath it. This innovative design addresses specific challenges associated with hybrid atom-ion traps by providing precisely aligned and stable components, facilitating independent adjustments of the depth of the atomic trapping potential, and positioning trapped ions. Our findings include the simultaneous loading of the ion trap with linear Yb+ ion crystals and the loading of neutral 87Rb atoms into a mirror magneto-optical trap.

Effect of light-assisted tunable interaction on the position response function of cold atoms.

The position response of a particle subjected to a perturbation is of general interest in physics. We study the modification of the position response function of an ensemble of cold atoms in a magneto-optical trap (MOT) in the presence of tunable light-assisted interactions. We subject the cold atoms to an intense laser light tuned near the photoassociation (PA) resonance and observe the position response of the atoms subjected to a sudden displacement. Surprisingly, we observe that the entire cold atomic cloud undergoes collective oscillations. We use a generalized quantum Langevin approach to theoretically analyze the results of the experiments and find good agreement.

Compact magneto-optical traps using planar optics

Abstract Magneto-optical traps (MOTs) composed of magnetic fields and light fields have been widely utilized to cool and confine microscopic particles. Practical technology applications require miniaturized MOTs. The advancement of planar optics has promoted the development of compact MOTs. In this article, we review the development of compact MOTs based on planar optics. First, we introduce the standard MOTs. We then introduce the grating MOTs with micron structures, which have been used to build cold atomic clocks, cold atomic interferometers, and ultra-cold sources. Further, we introduce the integrated MOTs based on nano-scale metasurfaces. These new compact MOTs greatly reduce volume and power consumption, and provide new opportunities for fundamental research and practical applications.

Measurements of cesium PJ-series quantum defect with the microwave spectroscopy.

High-precision microwave spectroscopy has been used to measure the transition frequency of nS1/2 → nPJ (n is the principle quantum number) and further the quantum defect of nPJ states in a standard cesium magneto-optical trap. A microwave field with 30-μs duration coupling the nS1/2 → nP1/2,3/2 transition yields a narrow linewidth microwave spectroscopy with the linewidth approaching the Fourier limit. After carefully compensating the stray electric and magnetic field and using the diluted atomic gas, we extract improved quantum defects of nPJ state, δ0(nP1/2) = 3.59159091(19), δ2(nP1/2) = 0.36092(35) and δ0(nP3/2) = 3.55907153(25), δ2(nP3/2) = 0.37344(47).

Compact structures for single-beam magneto-optical trapping of ytterbium.

At present, the best optical lattice clocks are based on the spectroscopy of trapped alkaline-earth-like atoms such as ytterbium and strontium. The development of mobile or even space-borne clocks necessitates concepts for the compact laser-cooling and trapping of these atoms with reduced laser requirements. Here, we present two compact and robust achromatic mirror structures for single-beam magneto-optical trapping of alkaline-earth-like atoms using two widely separated optical cooling frequencies. We have compared the trapping and cooling performance of a monolithic aluminum structure that generates a conventional trap geometry to a quasi-planar platform based on a periodic mirror structure for different isotopes of Yb. Compared to prior work with strontium in non-conventional traps, where only bosons were trapped on a narrow line transition, we demonstrate two-stage cooling and trapping of a fermionic alkaline-earth-like isotope in a single-beam quasi-planar structure.

Blue-Detuned Magneto-optical Trap of CaF Molecules.

A key method to produce trapped and laser-cooled molecules is the magneto-optical trap (MOT), which is conventionally created using light red detuned from an optical transition. In this work, we report a MOT for CaF molecules created using blue-detuned light. The blue-detuned MOT (BDM) achieves temperatures well below the Doppler limit and provides the highest densities and phase-space densities reported to date in CaF MOTs. Our results suggest that BDMs are likely achievable in many relatively light molecules including polyatomic ones, but our measurements suggest that BDMs will be challenging to realize in substantially heavier molecules due to sub-mK trap depths. In addition to record temperatures and densities, we find that the BDM substantially simplifies and enhances the loading of molecules into optical tweezer arrays, which are a promising platform for quantum simulation and quantum information processing. Notably, the BDM reduces molecular number requirements ninefold compared to a conventional red-detuned MOT, while not requiring additional hardware. Our work therefore substantially simplifies preparing large-scale molecular tweezer arrays, which are a novel platform for simulation of quantum many-body dynamics and quantum information processing with molecular qubits.

Understanding Inner-Shell Excitations in Molecules through Spectroscopy of the 4f Hole States of YbF

Molecules containing a lanthanide atom have sets of electronic states arising from excitation of an inner-shell electron. These states have received little attention but are thought to play an important role in laser cooling of such molecules and may be a useful resource for testing fundamental physics. We study a series of inner-shell excited states in YbF using resonance-enhanced multiphoton ionization spectroscopy. We investigate the excited states of lowest energy, 8474, 9013, and 9090 cm−1 above the ground state, all corresponding to the configuration 4f136s2 F27/2 of the Yb+ ion. They are metastable, since they have no electric dipole allowed transitions to the ground state. We also characterize a state at 31 050 cm−1 that is easily excited from both the ground and metastable states, which makes it especially useful for this spectroscopic study. Finally, we study two states at 48 720 and 48 729 cm−1, which are above the ionization limit and feature strong autoionizing resonances that prove useful for efficient detection of the molecules and for identifying the rotational quantum number of each line in the spectrum. We resolve the rotational structures of all these states and find that they can all be described by a very simple model based on Hund’s case (c). Our study provides information necessary for laser slowing and magneto-optical trapping of YbF, which is an important species for testing fundamental physics. We also consider whether the low-lying inner-shell states may themselves be useful as probes of the electron’s electric dipole moment or of varying fundamental constants, since they are long-lived states in a laser-coolable molecule featuring closely spaced levels of opposite parity. Published by the American Physical Society 2024