Magnetic Polarity Research Articles

Altermagnetism Induced by Sliding Ferroelectricity via Lattice Symmetry-Mediated Magnetoelectric Coupling.

Altermagnets, distinct from conventional ferromagnets or antiferromagnets, have recently attracted attention as the third category of collinear magnets, which exhibit the coexistence of zero net magnetization and spin polarization due to their unique lattice symmetries. Meanwhile, the additional layer degrees of freedom in multilayer sliding ferroelectrics offer opportunities for coupling with lattice symmetries, paving the way for an innovative approach to constructing multiferroic lattices. In this study, altermagnetic tuning in SnS2/MnPSe3/SnS2 heterostructures is achieved by breaking and restoration of lattice inversion symmetry through sliding ferroelectric switching. First-principles calculations reveal that the spin density and corresponding time-reversal symmetry of MnPSe3 can be manipulated by lattice symmetry, triggering phase transitions between antiferromagnetism and altermagnetism. This research establishes a novel form of magnetoelectric coupling mediated by lattice symmetry and provides a theoretical basis for the design of miniature information processing and memory devices based on altermagnetism.

An efficient and miniaturized ultra-thin tunable UWB graphene metasurface absorber for terahertz gap regime

This work introduces an ultra-thin tunable ultra-wideband (UWB) metasurface absorber (MSA) for the terahertz (THz) gap. The polarization-insensitive MSA provides an absorptivity (A(f)) ≥ 90% from 0.1 to 11.5 THz, corresponding to 196.6% fractional bandwidth. The usage of resonant slots engraved on top patterned graphene sheet (Gpat) and strong plasmonic coupling in the Fabry-Perot cavity formed between top Gpat and bottom continuous graphene (Gcont) in bilayer stack configuration ensures absorptivity over a UWB THz spectrum. An equivalent circuit model (ECM) closely follows the A(f) response of the proposed MSA. The proposed DC-biasing mechanism can regulate the chemical potential (μc) of the connected Gcont efficiently. A DC bias voltage of 0 to 6.1 V is adequate to vary μc of Gcont from 0 to 0.6 eV for achieving tunable A(f). The structure maintains its ultra-thin nature and has a thickness of only λ0/1500, where λ0 is the free space wavelength calculated at 0.1 THz. In addition, the periodicity is only λ0/300. The MSA also provides stable absorption response from 0.1 to 11.5 THz with A(f) ≥ 80% for incidence angle (θ) up to 60∘ under both transverse magnetic (TM) and transverse electric (TE) polarization.

Magnetic field-augmented photoelectrochemical water splitting in Co3O4 and NiO nanorod arrays

Effective charge separation is crucial for improving the sensitivity of photoelectrochemical studies. Here, we provide an immense magnetic field-based electron spin polarization approach for an efficient charge carrier separation. We have fabricated NiO and Co3O4 thin film and nanorod arrays by electron beam evaporation glancing angle method followed by annealing in a two-zone furnace. The photoelectrochemical performance was investigated for NiO and Co3O4 samples in the presence and absence of a magnetic field. The NiO and Co3O4 nanorods array samples exhibit better absorption compared with the thin film samples. The Co3O4 and NiO nanorod arrays showed the highest photocurrent density of 0.12 and 0.55 mA/cm2 in a magnetic field. The superior photoelectrochemical response of NiO and Co3O4 nanorods in a magnetic field could be ascribed to the limitation of non-radiative recombination of carriers manipulated by Lorentz force and spin polarization. Furthermore, the electrochemical impedance spectra of NiO and Co3O4 nanorod arrays in a magnetic field show the least charge transfer resistance. This study sheds light on the interaction process between external fields and radiative/non-radiative recombination of manipulating carriers. Thus, the application of a magnetic field presents an efficient and versatile approach to enhance the performance of photoelectrodes in solar water splitting.

High-field pulsed EPR spectroscopy under magic angle spinning.

In this work, we demonstrate the first pulsed electron paramagnetic resonance (EPR) experiments performed under magic angle spinning (MAS) at high magnetic field. Unlike nuclear magnetic resonance (NMR) and dynamic nuclear polarization (DNP), commonly performed at high magnetic fields and under MAS to maximize sensitivity and resolution, EPR is usually measured at low magnetic fields and, with the exception of the Spiess group work in the late 1990s, never under MAS, due to great instrumentational challenges. This hampers the investigation of DNP mechanisms, in which electron spin dynamics play a central role, because no experimental data about the latter under DNP-characteristic conditions are available. We hereby present our dedicated, homebuilt MAS-EPR probehead and show the pulsed MAS-EPR spectra of P1 center diamond defect recorded at 7 tesla. Our results reveal unique effects of MAS on EPR line shape, intensity, and signal dephasing. Time-domain simulations reproduce the observed changes in the line shapes and the trends in the signal intensity.

Square & H metasurfaces for SPR Increasing in long Wave-IR absorber

In the long-wave infrared (LWIR) spectrum, this paper suggests an electromagnetic (EM) waveband absorber design based on metamaterials. Germanium, gold, and magnesium oxide layers are arranged in a layered structure from top to bottom in the suggested model. Our proposed metamaterial structure’s upper surface is composed of metallic metasurfaces with H and square forms from various studies. The finite element method is used to evaluate the metamaterials’ electromagnetic properties in terms of absorbance and reflectance. It is observed that there is a particular size of the metamaterial at which extremely localized electromagnetic resonance occurs. Quantitative findings indicate that the suggested metamaterial design’s average absorption reaches 90 % in the 10 μm to 14 μm range across a wide variety of incidence angles (00 to 400 & 00 to 800) for both transverse electric (TE) and transverse magnetic (TM) polarization. It is evident from these data that the suggested model configuration has broad potential applications in manyoptoelectronic fields of study.

Magnetostratigraphy and rock magnetic studies on the Cretaceous‐Paleogene transition strata along the Um Sohryngkew River, Therriaghat, Meghalaya, India

A combination of magnetic polarity and rock magnetic analysis on the well‐documented section of the Um Sohryngkew River (USR) in the south Shillong Plateau, NE India, produced a sharp reversal marking the C29r‐C29n geomagnetic polarity transition at approximately 65.688 Ma. The rock magnetic studies indicate ferrimagnetic dominant mineralogy with abundance of SSD grains, with an anomalous peak in susceptibility coinciding with Ir‐rich limonitic layer. The magnetic reversal occurs precisely 61 m above the Ir‐rich distinct in situ limonitic layer, indicating that the C29r‐C29n geomagnetic reversal post‐dates the widely accepted Ir‐anomaly based K‐Pg boundary by approximately 355 Ka. Furthermore, the rock magnetic studies indicate its frequency dependence coinciding with the Ir‐rich limonitic layer suggesting a possible dust/aerosol source, while akaganéite is reported from the interval approximately 1 m below peak susceptibility, indicating signature of Deccan volcanism. This study infers the completeness of the USR section with a high rate of sedimentation of approximately 17 cm/ka among the marine K‐Pg boundary sections in the world.

Hybrid ferrofluid flow on a stretching sheet with Stefan blowing and magnetic polarization effects in a porous medium

PurposeThis study investigates the behavior of viscous hybrid ferromagnetic fluids flowing through plain elastic sheets with the magnetic polarization effect. It examines flow in a porous medium using Stefan blowing and utilizes a versatile hybrid ferrofluid containing MnZnFe2O4 and Fe3O4 nanoparticles in the C2H2F4 base fluid, offering potential real-world applications. The study focuses on steady, laminar and viscous incompressible flow, analyzing heat and mass transfer aspects, including thermal radiation, Brownian motion, thermophoresis and viscous dissipation with convective boundary condition.Design/methodology/approachThe governing expression of the flow model is addressed with pertinent non-dimensional transformations, and the finite element method solves the obtained system of ordinary differential equations.FindingsThe variations in fluid velocity, temperature and concentration profiles against all the physical parameters are analyzed through their graphical view. The association of these parameters with local surface friction coefficient, Nusselt number and Sherwood number is examined with the numerical data in a table.Originality/valueThis work extends previous research on ferrofluid flow, investigating unexplored parameters and offering valuable insights with potential engineering, industrial and medical implications. It introduces a novel approach that uses mathematical simplification techniques and the finite element method for the solution.

Chirality-Induced Magnetic Polarization by Charge Localization in a Chiral Supramolecular Crystal.

The chirality-induced spin selectivity (CISS) effect is a fascinating phenomenon that correlates the molecular structure with electron spin-polarization (SP). Experimental procedures to quantify the spin-filtering magnitude have extensively used magnetic-field-dependent conductive AFM. In this work chiral crystals of imide-substituted coronene bisimide ((S)-CBI-GCH) are studied to explain the dynamics of the current-voltage I - V spectra and the origin of superimposed peaks are investigated. A dynamic voltage-sweep rate-dependent phenomenon can give rise to complex I - V curves. The redox group, capable of localization of charge, acts as a localized state that interferes with the continuum of the π - π stacking, giving rise to Fano resonances. A novel mechanism for dynamic transport is introduced, which provides insight into the origin of spin-polarized charge in crystallized CBI-GCH molecules after absorption on a metallic substrate, guided by transient charge polarization. Crucially, interference between charge localization and delocalization during transport may be important properties in understanding the magnetochiral phenomena observed by electrostatic force microscopy. Finally, it is observed that charge trapping sensitively modifies the injection barrier from direct tunneling to Fowler-Nordheim tunneling transport supporting nonlinearity in CISS for this class of molecules.

Design and experimental demonstration of a high-performance all-silicon transverse magnetic polarizer using tilted-elliptical-hole arrays

This study presents the design and experimental demonstration of a high-performance all-silicon transverse magnetic (TM) polarizer. The tilted-elliptical-hole arrays are designed to effectively reflect transverse electric (TE) modes while propagating TM modes with low loss. The device bandwidth (BW) is controlled by changing the tilting angle of the elliptical hole or by combining it with changes in other parameters. The device operates beyond 326 nm (1385–1711 nm) in BW, achieving an average insertion loss (IL) below 1.0 dB and a polarization extinction ratio (PER) over 20 dB. A 20 nm shift in BW can be obtained with a 30° deflection, and an 80 nm shift can be achieved with multiple parameter changes. The experimental results confirm the theoretical analysis. The present device with the advantages of simple structure, flexible design, and broad BW has great potential applications in silicon photonics.

Micron-resolution fiber mapping in histology independent of sample preparation.

Detailed knowledge of the brain's nerve fiber network is crucial for understanding its function in health and disease. However, mapping fibers with high resolution remains prohibitive in most histological sections because state-of-the-art techniques are incompatible with their preparation. Here, we present a micron-resolution light-scattering-based technique that reveals intricate fiber networks independent of sample preparation for extended fields of view. We uncover fiber structures in both label-free and stained, paraffin-embedded and deparaffinized, newly-prepared and archived, animal and human brain tissues - including whole-brain sections from the BigBrain atlas. We identify altered microstructures in demyelination and hippocampal neurodegeneration, and show key advantages over diffusion magnetic resonance imaging, polarization microscopy, and structure tensor analysis. We also reveal structures in non-brain tissues - including muscle, bone, and blood vessels. Our cost-effective, versatile technique enables studies of intricate fiber networks in any type of histological tissue section, offering a new dimension to neuroscientific and biomedical research.

LAPOD, Latin-American paleomagnetic online database: An online interface to access paleomagnetic data from Latin America

We present the Latin-American Paleomagnetic Online Database (LAPOD), which includes an online tool for consulting and visualizing paleomagnetic data. This platform allows users to search, filter, and query over 2000 paleomagnetic data entries from locations across Latin America, including North America (Mexico and the Southwestern USA), Central America, and South America. Paleomagnetic data has been pre-validated for geographic locations and ages, enhancing its reliability for users.The platform features a robust database engine with up to 26 filters, allowing users to perform queries with high precision and avoiding data duplication, and to download data in various formats for personal use. It also offers graphical visualization of some data directly on screen. Color indicators are used to indicate data quality and magnetic polarity. All data included in LAPOD are properly referenced to their original authors, with links to the original published articles.LAPOD is proposed as a community-driven platform, allowing users to contribute their data and provide comments on their own and others' data. This fosters discussion about the reliability of paleomagnetic data and finally enhances our knowledge of the Earth's magnetic field in the region. This collaborative approach supports the development of new regional models of paleosecular variation with improved reliability. It may be repeated for other regions in the world, and ultimately lead to improved global field models. To access the platform, please visit: https://paleomagnetismo.org/pmagdb/

Tailored Magnetic Spatial Confinement with Enhanced Polarization and Magnetic Response for Electromagnetic Wave Absorption.

For materials with coexisting phases, the transition from a random to an ordered distribution of materials often generates new mechanisms. Although the magnetic confinement effect has improved the electromagnetic (EM) performance, the transition from random to ordered magnetic confinement positions remains a synthetic challenge, and the underlying mechanisms are still unclear. Herein, precise control of magnetic nanoparticles is achieved through a spatial confinement growth strategy, preparing five different modalities of magnetic confined carbon fiber materials, effectively inhibiting magnetic agglomeration. Systematic studies have shown that the magnetic confinement network can refine CoNi NPs size and enhance strong magnetic coupling interactions. Compared to CoNi@HCNFs on the hollow carbon fibers (HCNFs) outer surface, HCNFs@CoNi constructed on the inner surface induce stronger spatial charge polarization relaxation at the interface and exhibit stronger magnetic coupling interactions at the inner surface due to the high-density magnetic coupling units at the micro/nanoscale, thereby respectively enhancing dielectric and magnetic losses. Remarkably, they achieve a minimum reflection loss (RLmin) of -64.54dB and an absorption bandwidth of 5.60GHz at a thickness of 1.77mm. This work reveals the microscale mechanism of magnetic confinement-induced different polarization relaxation and magnetic response, providing a new strategy for designing magnetic materials.

Design and validation of a novel 2.5‐D miniaturized FSS with angular and superior polarization stability for mobile technology

AbstractThis paper presents a novel 2.5D miniaturized frequency‐selective surface (FSS) measuring 6.1 mm × 6.1 mm, designed to effectively shield smartphones and tablets from unwanted electromagnetic radiation. The FSS is notable for its stable attenuation peaks in the high‐frequency stopband under transverse magnetic (TM) polarization, offering dual‐frequency response and exceptional angular stability in both transverse electric and TM modes. An equivalent circuit analysis, prototype fabrication, and empirical evaluation confirmed its effectiveness. The prototype exhibits superior polarization stability and minimal peak attenuation reduction of just 1.9 dB (10%) across a 0°–60° incidence angle, outperforming similar studies.

Enhancing terahertz magneto-optical effects in wafer-scale RIG single crystal thick films with anti-reflective coatings for improved transmittance

Wafer-scale rare-earth iron garnet (RIG) single crystal thick films were fabricated on 3-in. gadolinium gallium garnet (GGG) substrates using liquid phase epitaxy. The terahertz transmittance of the RIG crystals improved after removing the GGG substrate by polishing. The time-domain spectra at Terahertz (THz) frequencies indicate the existence of a magneto-optical effect in RIG samples. The results indicate that the RIG samples exhibit a high refractive index of ∼4.50 within the 0.1–1.0 THz frequency range, a transmittance of around 40%, and an absorption rate of only 10–50 cm−1. The Faraday rotation angles of the thick single-crystal films of the RIG samples were measured using a THz-TDS system. The RIG has a thickness of ∼330 μm. The Faraday rotation angles of RIG crystals at THz frequencies can reach up to 16° when an external magnetic field of 0.18 T is applied. The Verdet constants of the RIG sample were calculated to be ∼120°/mm/T. To improve the transmittance of the RIG sample, epoxy resin and polymethylpentene (TPX) were used as anti-reflective films. The transmittance of the RIG sample increased by ∼5% for the 80 μm thick epoxy and about 10% for the 320 μm thick TPX. Therefore, this RIG single crystal thick film can achieve a low loss, a high transmittance, and a strong magneto-optical effect in the terahertz region with the cooperation of a reflection-reducing film. It is expected to have wide applications in terahertz magnetic polarization conversion, non-reciprocal phase shifters, and isolators.

The Temporal Evolution of Nonneutralized Electric Currents and the Complexity of Solar Active Regions

We study the evolution of electric currents during the emergence of magnetic flux in the solar photosphere and the differences exhibited between solar active regions of different Hale complexity classes. A sample of 59 active regions was analyzed using a method based on image segmentation and error analysis to determine the total amount of nonneutralized electric current along their magnetic polarity inversion lines. The time series of the total unsigned nonneutralized electric current, I NN,tot, exhibit intricate structure in the form of distinct peaks and valleys. This information is largely missing in the respective time series of the total unsigned vertical electric current I z . Active regions with δ-spots stand out, exhibiting a 1.9 times higher flux emergence rate and 2.6 times higher I NN,tot increase. The median value of their peak I NN,tot is equal to 3.6 × 1012 A, which is more than three times higher than that of the other regions of the sample. An automated detection algorithm was also developed to pinpoint the injection events of nonneutralized electric current. The injection rates and duration of these events were higher with increasing complexity of active regions, with regions containing δ-spots exhibiting the strongest and longest events. These events do not necessarily coincide with increasing magnetic flux, although they exhibit moderate correlation. We conclude that net electric currents are injected during flux emergence but are also shaped drastically by the incurred photospheric evolution as active regions grow and evolve.

Quenching controlled spin exchange interactions and spin selective electron transfer for oxygen evolution reactions

The utilization of magnetic field to enhance electrocatalytic activity has become an effective strategy garnering significant attention in the field of electrocatalysis. Herein, we employ a combination of electrospinning and quenching techniques to successfully synthesize high-entropy oxide (HEO) (FeCoNiCrMn)3O4. The HEO exhibited ferromagnetic properties and further increased the saturation magnetization after the quenching process, primarily due to temperature-mediated magnetic exchange interactions. The OER performance is significantly improved by employing a ferromagnetic ordered catalyst as a spin polarizer in the presence of a magnetic field. The introduction of an exterior magnetic field (∼130 mT) significantly improved the OER performance of HEO-LN (HEO quenching in liquid nitrogen), reducing the overpotential by 39.4 mV at 10 mA cm-2. The improved OER performance is due to the presence of the magnetic field-enhanced electron spin polarization, reducing electron repulsion and enhancing orbital hybridization. These findings not only provide crucial insights into understanding reactions involving magnetic field-induced electrochemistry but also contribute to the rational design of electrocatalysts with magnetic effect.

Effect of Ho3+ Substitution on Magnetic Properties of ZnCr2Se4.

A series of ZnCr2-xHoxSe4 microcrystalline spinels (where x = 0.05, 0.075, and 0.10) containing holmium ions in octahedral coordination were obtained by sintering of adequate reactants at high temperatures. The obtained doped materials were characterized by X-ray diffraction, Scanning Electron Microscopy, UV-Vis-NIR, molecular field approximation, and XPS spectroscopies. Their thermal properties were also investigated. The doping of the ZnCr2S4 matrix with paramagnetic Ho3+ ions with a content of not more than 0.1 and a screened 4f shell revealed a significant effect of orbital and Landau diamagnetism, a strong reduction in short-range ferromagnetic interactions, and a broadening and shift of the peak of the first critical field by simultaneous stabilization of the sharp peak in the second critical field. These results correlate well with FPLO calculations, which show that Cr sites have magnetic moments of 3.19 µB and Ho sites have significantly larger ones with a value of 3.95 µB. Zn has a negligible magnetic polarization of 0.02 µB, and Se induces a polarization of approximately -0.12 µB.

Magnetized tori with magnetic polarization around Kerr black holes: Variable angular momentum disks

Magnetized tori with magnetic polarization around Kerr black holes: Variable angular momentum disks

Thermodynamics of Magnetic Black Holes with Nonlinear Electrodynamics in Extended Phase Space

We study Einstein’s gravity in AdS space coupled to nonlinear electrodynamics. Thermodynamics in extended phase space of magnetically charged black holes is investigated. We compute the metric and mass functions and their asymptotics, showing that black holes may have one or two horizons. The metric function is regular, f(0)=1, and corrections to the Reissner–Nordström solution are in the order of O(r−3) when the Schwarzschild mass is zero. We prove that the first law of black hole thermodynamics and the generalized Smarr relation hold. The magnetic potential and vacuum polarization conjugated to coupling are computed and depicted. We calculate the Gibbs free energy and the heat capacity showing that first-order and second-order phase transitions take place.

A decomposition of light’s spin angular momentum density

Light carries intrinsic spin angular momentum (SAM) when the electric or magnetic field vector rotates over time. A familiar vector equation calculates the direction of light’s SAM density using the right-hand rule with reference to the electric and magnetic polarisation ellipses. Using Maxwell’s equations, this vector equation can be decomposed into a sum of two distinct terms, akin to the well-known Poynting vector decomposition into orbital and spin currents. We present the first general study of this spin decomposition, showing that the two terms, which we call canonical and Poynting spin, are chiral analogies to the canonical and spin momenta of light in its interaction with matter. Like canonical momentum, canonical spin is directly measurable. Both canonical and Poynting spin incorporate spatial variation of the electric and magnetic fields and are influenced by optical vortices. The decomposition allows us to show that a linearly polarised vortex beam, which has no total SAM, can nevertheless exert longitudinal chiral pressure due to equal and opposite canonical and Poynting spins.