We present geochronological, geochemical, and isotopic data on Statherian–Calymmian metaplutonites located within the Alto Moxotó Terrane (Borborema Province, Brazil). The Carnoió Suite occurs within a large area of this terrane. It is characterized by slightly deformed syenogranites and quartz-syenites, which present a geochemical signature typical of within-plate magmas. In contrast, the Coloete Suite occurs in the northern border area of the terrane. Its petrographic and geochemical characteristics vary between those of granodiorite and syenogranite, while its geochemistry suggests an arc-related/syn-collisional origin. There are few Statherian A-type granites in the Borborema Province and in its African counterpart. Zircon crystals recovered from the Carnoió Suite (dated 1638 Ma) and from the Coloete Suite (dated 1652 Ma; LA-ICP-MS) provide some clues about magma volume and concentration during the Statherian-Calymmian transition. Coeval collisional magmas are scarce in this region: they are interpreted worldwide as a product of peripheral convergences and coeval with the fragmentation of cratonic blocks. Our results suggest that the Alto Moxotó Terrane was part of an ancient block affected by an intraplate event during at the Statherian-Calymmian transition; moreover, its northern limits might have experienced accretion during a crust-reworking episode.