Local Black Carbon Research Articles

Strong Haze‐Black Carbon‐Climate Connections Observed Across Northern and Eastern China

AbstractRadiative absorption of black carbon (BC) is of great importance in air quality and climate change. Simultaneous mitigation of haze pollution and climate warming requires an in‐depth understanding of haze‐BC‐climate connections based on direct observations. We simultaneously performed measurements in the North China Plain (NCP) and the Yangtze River Delta (YRD) during the winter of 2018–2019, when cross‐regional haze transport frequently occurred. We found that BC particles exhibited a thick coating thickness (100–120 nm) under haze pollution conditions in the NCP and were then transported to the YRD with regional haze development. BC particles in the downwind region showed a bimodal distribution of core‐size‐resolved aging degree, which can be used to separate and quantify local and regional BC. The results showed that the regional haze transport from the NCP brought 1–3 μg m−3 BC into the YRD. These regional BC particles exhibited ∼1.6 times stronger absorption efficiency than locally emitted BC. The direct radiative effects of BC in the downwind region were estimated to be enhanced by ∼2 times when regional haze pollution was transported from the NCP to the YRD. The amplification of BC's climate effect during regional haze pollution was attributed to the increases in both the mass concentrations and light absorption efficiency of BC, which were responsible for 40%–50% and 50%–60%, respectively. Our work identified strong haze‐BC‐climate connections across the NCP and YRD and highlighted the importance of BC in the effects of haze pollution on regional climate.

Black carbon in contrasting environments in India: Temporal variability, source apportionment and radiative forcing

Analyses of black carbon (BC) data from three different environments in India - Delhi megacity, Srinagar metropolitan and Gulmarg hill station, showed that Delhi had the highest annual average BC concentration (12.3 ± 10.2 μg m−3), followed by Srinagar (4.3 ± 5 μg m−3) and Gulmarg (2.4 ± 2 μg m−3). The inflow of aerosols from the neighboring agricultural regions, notably during Winter, causes Delhi to have the highest seasonal average BC (16.8 μg m−3). Srinagar had the highest average seasonal BC during autumn (6.3 μg m−3) due to the burning of horticulture residue and hardwood for charcoal making and residential heating. At Gulmarg, on the other hand, the winter season's high BC (2.2 μg m−3) is due to the increased emissions from the tourist traffic, snowmobile/ATVs and wood burning for residential heating. BC concentrations in Delhi and Srinagar were roughly in line with their population size. However, compared to sites with the similar population, BC at Gulmarg was roughly twice higher than the other sites. There was a higher contribution to BC from fossil fuels than biomass burning at all three sites, which indicates that cars are the primary source of BC. Overall, values of BC aerosol optical properties in Delhi are much higher than those in Srinagar and Gulmarg. During the cold season, continental air masses transport BC from the neighboring areas to Delhi and westerlies enhance the local BC loading at Srinagar and Gulmarg. The predominant presence of absorbing aerosols, particularly BC, during late autumn and winter at all three sites leads to an increase in aerosol optical depth (AOD), a reduction in single scattering albedo (SSA) and an increase in asymmetry parameter (AP). As a result, there is a significant increase in the radiative forcing of the atmosphere (RFATM), with the highest values observed in January in Delhi (+71.5 W m−2) and Srinagar (+56.05 W m−2), and in November at Gulmarg (+18.5 W m−2). These findings suggest that small rural towns that are affected by seasonal emissions, low planetary boundary layers, and frequent temperature inversions, can contribute to a substantial amount of radiative forcing. This study provides a larger perspective on increasing BC in Delhi, and urban-rural fringe areas in the Indian Himalayas, which is crucial for identifying what actions must be taken to control BC emissions to reduce impacts on cryosphere, human health and other sectors.

Spatiotemporal Analysis of Black Carbon Sources: Case of Santiago, Chile, under SARS-CoV-2 Lockdowns.

The SARS-CoV-2 pandemic has temporarily decreased black carbon emissions worldwide. The use of multi-wavelength aethalometers provides a quantitative apportionment of black carbon (BC) from fossil fuels (BCff) and wood-burning sources (BCwb). However, this apportionment is aggregated: local and non-local BC sources are lumped together in the aethalometer results. We propose a spatiotemporal analysis of BC results along with meteorological data, using a fuzzy clustering approach, to resolve local and non-local BC contributions. We apply this methodology to BC measurements taken at an urban site in Santiago, Chile, from March through December 2020, including lockdown periods of different intensities. BCff accounts for 85% of total BC; there was up to an 80% reduction in total BC during the most restrictive lockdowns (April-June); the reduction was 40-50% in periods with less restrictive lockdowns. The new methodology can apportion BCff and BCwb into local and non-local contributions; local traffic (wood burning) sources account for 66% (86%) of BCff (BCwb). The intensive lockdowns brought down ambient BC across the city. The proposed fuzzy clustering methodology can resolve local and non-local contributions to BC in urban zones.

Compilation of a city-scale black carbon emission inventory: Challenges in developing countries based on a case study in Brazil

Black carbon (BC) inventories for cities are scarce, especially in developing countries, despite their importance to tackle climate change and local air pollution. Here, we draw on results from a case study in a Brazilian city to discuss the challenges of compiling a BC inventory for different activity sectors. We included traditionally inventoried sectors, such as industries and on-road transportation, other less reported sectors (food establishments and aviation), and open burning of household solid waste (HSW), typically found in developing countries. We present a machine-learning technique (Random Forest) as a novel approach to obtain HSW burning activity using a set of spatial predictors. The BC inventory was based on PM2.5 emissions weighted by the fraction of PM2.5 emitted as BC and developed for the year 2018. We also reported the disaggregated spatial PM2.5 emissions for the same combustion sources, and documented the databases used for activity data and emission factors (EF). The total estimated BC and PM2.5 emissions amounted to 57.88 and 234.75 tons, respectively, with on-road vehicle exhaust emissions and industrial combustion as the main BC sources (63 and 22%, respectively). For PM2.5 emissions, on-road transportation (exhaust and non-exhaust) contributed 48%, followed by industrial combustion (21%) and food establishments (20%). Population density, number of vacant lots, and property tax values were identified as the most important features to predict the HSW fire activity. A comparison with other inventories revealed that the BC emission profile of Londrina is similar to the profile reported for Greater Mexico City, another Latin American city. Thus, the methodology used in this study could be extended to other cities with similar local BC sources. Finally, we highlight that the lack of local activity data, representative EF, and even methodology may undermine the development of reliable BC inventories, and intensive research should be conducted to characterize the emission sources.

Relative contributions of fossil fuel and biomass burning sources to black carbon aerosol on the Southern Atlantic Ocean Coast and King George Island (Antarctic Peninsula).

Carbonaceous aerosols can affect climate, especially particles containing black carbon (BC). BC originated from the incomplete combustion of fossil fuel and biomass, which can heat the atmosphere and increase ice melting, but little is known about BC sources to Antarctica. We quantified the contribution of distant origin (biomass burning) and local emissions (fossil fuel) to atmospheric BC concentration in the King George Island (Antarctic Peninsula) and the Southern Ocean. We examine the BC concentrations using a multi-wavelength Aethalometer AE-33 and AE-42 aboard the Brazilian Oceanographic Research Ship Almirante Maximiano. The results indicate that the region is influenced by local sources and air masses coming from surrounding continents. Fossil fuel combustion was the major source of carbonaceous aerosols in the region, whereas the total average concentration was 41.8 ± 22.8 ng m-3. The findings indicate a contribution of biomass burning coming from low and mid-latitudes of South America over the Antarctic Peninsula and the Southern Ocean around 62ºS latitude. We demonstrated that fossil fuel is the main contributor to atmospheric BC concentration for the Austral summer and autumn. Scientific stations, local tourism, and traffic are possible local BC sources. Our work invokes the urgency of questionable sustainability issues about Antarctica exploration.

Sources of black carbon at residential and traffic environments obtained by two source apportionment methods

Abstract. This study investigated the sources of black carbon (BC) at two contrasting urban environments in Helsinki, Finland: residential area and street canyon. The measurement campaign in the residential area was conducted in winter–spring 2019, whereas in the street canyon the measurements were carried out in autumn 2015. The sources of BC were explored by using positive matrix factorization (PMF) for the organic and refractory black carbon (rBC) mass spectra collected with a soot particle aerosol mass spectrometer (SP-AMS). Based on the PMF analysis, two sites had different local BC sources; the largest fraction of BC originated from biomass burning at the residential site (38 %) and from the vehicular emissions in the street canyon (57 %). Also, the mass size distribution of BC diverged at the sites as BC from traffic was found at the particle size of ∼100–150 nm whereas BC from biomass combustion was detected at ∼300 nm. At both sites, a large fraction of BC was associated with urban background or long-range-transported BC indicated by the high oxidation state of organics related to those PMF factors. The results from the PMF analysis were compared with the source apportionment from the Aethalometer model calculated with two pairs of absorption Ångström values. It was found that several PMF factors can be attributed to wood combustion and fossil fuel fraction of BC provided by the Aethalometer model. In general, the Aethalometer model showed less variation between the sources within a day than PMF, indicating that it was less responsive to the fast changes in the BC sources at the site, or it could not distinguish between as many sources as PMF due to the similar optical properties of the BC sources. The results of this study increase understanding of the limitations and validity of the BC source apportionment methods in different environments. Moreover, this study advances the current knowledge of BC sources and especially the contribution of residential combustion in urban areas.

Effects of local and remote black carbon aerosols on summer monsoon precipitation over India

In this study, we perform idealized climate model simulations to assess the relative impacts of an increase in local black carbon (BC) aerosols (located over the Indian region) and the remote BC aerosols (located outside the Indian region) on the summer monsoon precipitation over India. We decompose the precipitation changes into fast adjustments triggered by the introduction of the forcing agent and slow response that is associated with the global mean temperature change. We find that a 60-fold increase in the ‘present-day’ global distribution of BC aerosols leads to an increase in precipitation over India, which is mainly contributed by an increase in remote BC aerosols. When remote BC aerosols are increased, the fast adjustments contribute to an increase in precipitation in association with the warming of the northern hemisphere land and the related northward Intertropical Convergence Zone (ITCZ) shift. For an increase in local aerosols too, by enhancing the upper tropospheric temperature meridional gradient in the Indian region, the fast adjustments contribute to an increase in precipitation over India. The slow response contributions in both cases are related to the regional patterns of SST change and the resulting changes to meridional temperature gradient in the Indian region and zonal circulation changes. The net precipitation change over India is an increase (decrease) for an increase in remote (local) BC aerosols. As the interpretation of our results relies on ITCZ shift related to planetary energetics, differing land-ocean response and meridional temperature gradients in the Indian region, the results from our study are likely to be robust across climate models.

Concentration and Physical Characteristics of Black Carbon in Winter Snow of Beijing in 2015

In Beijing, the probability of snowfall is decreasing as a result of global warming. At the same time, Beijing has suffered severe air pollution. In this paper, the concentration and particle size characteristics of BC (Black Carbon) in snow during the winter of 2015 in Beijing were analyzed by the SP2 method. The average concentration of BC in snow meltwater in Beijing is 82 ng/mL, with a minimum value of 62.9 ng/mL and a maximum of 210.6 ng/mL. The BC particle size in snow and ice in the Beijing area is mostly concentrated in the range of 70–400 nm. After log-normal, the BC particle size above 600 nm is still small, which should be closely related to the nature of the local BC emission source. The concentration of BC in snow is highly susceptible to meteorological conditions and local pollution levels. When Beijing is under the control of the east wind or the southeast wind, aerosols in the urban areas can easily accumulate in the northwestern mountains and then settle or participate in the snowfall process, resulting in an increase in BC aerosol accumulation in the snow, thus further changing the optical properties of snow in the Beijing area.

Spatio-temporal variability in black carbon concentrations at highway toll plaza: Comparison between manual and electronic toll lanes

The quantification of the differences in the magnitudes of black carbon (BC) concentrations between electronic and manual toll lanes is necessary to understand the impacts of toll plazas to air pollution. This study investigated the space-time distribution of BC concentrations and compared the BC pollution profiles between traffics and toll collection lanes of an urban highway toll plaza in Shanghai. Experiments were carried out between August 15 and August 22, 2019. The mean BC concentrations at east-westbound manual toll collection (MTC) lanes were 17.8 and 14.8 μg m−3, respectively, while the counterpart values for the electronic toll collection (ETC) lanes were 7.7 and 9.2 μg m−3, respectively. Moreover, parallel measurements at urban background site yielded mean BC level ranges between 3.4 and 2.8 μg m−3. The traffic volumes through the east-westbound ETC and MTC lanes were estimated as 489 and 347 vehicles h−1, respectively. Although ETC-lane traffic was ~1.4 times higher than that of the MTC lanes, owing to the toll collection method, the BC concentrations at the MTC lanes were 1.6–2.3 times higher than those at the ETC lanes and 4.8–5.9 times higher than that of the urban background site. As per multivariate regression analysis, it was found that the variations in BC concentrations were caused by traffic emissions and influenced by the local background BC levels, influences of wind speed and humidity were also determined. This study found that at highway toll plazas, when compared with MTC lanes, ETC lanes can contribute to reducing BC emissions by ~50%.

Importance of Local Black Carbon Emissions to the Fate of Glaciers of the Third Pole.

Importance of Local Black Carbon Emissions to the Fate of Glaciers of the Third Pole.

An observational study on the variation of black carbon aerosol and source identification over a tropical station in south India

Abstract Continuous and high temporal resolution surface based measurements of Black Carbon (BC) concentrations have been carried out during 1st September 2014 to 30th April 2017 at Thiruvananthapuram (8.5°N, 76.9°E), a near equatorial tropical coastal station, in South India. High diurnal and seasonal variations of BC aerosols in relation to changes in the regional meteorological conditions are examined. The BC exhibited well defined diurnal cycle with a bimodal peak one in the morning (07.00–08.00 LST) and other in evening (21.00–23.00 LST). Relative humidity of 60–90% and 70–90% favours the BC mass concentration in daytime and nighttime respectively. BC mass concentration is considerably less for the relative humidity category of 90–100%. BC greater than 10 μg m−3 are mostly associated with low wind speed (less than 2 ms−1). Hence the local BC emissions are not well mixed or transported to a larger distance in calm or low wind speed. In high wind speed local emissions are quickly and well mixed in the air. Coherence wavelet analysis between BC and rainfall shows periodicities in the synoptic scale of less than 10 days and in the between 16–32 days. This shows the importance of intra seasonal rainfall scavenging on BC concentration over the tropical region. Synoptic systems over the monsoon region shows high scavenging relation. The bivariate analysis pointed that the local emission from northeast sector contributes the black carbon aerosol to the observational site. HYSPLIT trajectory model reveals that the long range transport of airmass is through northwest India and Bay of Bengal in winter season.

Source attribution of black carbon and its direct radiative forcing in China

Abstract. The source attributions for mass concentration, haze formation, transport and direct radiative forcing of black carbon (BC) in various regions of China are quantified in this study using the Community Earth System Model (CESM) with a source-tagging technique. Anthropogenic emissions are from the Community Emissions Data System that is newly developed for the Coupled Model Intercomparison Project Phase 6 (CMIP6). Over north China where the air quality is often poor, about 90 % of near-surface BC concentration is contributed by local emissions. Overall, 35 % of BC concentration over south China in winter can be attributed to emissions from north China, and 19 % comes from sources outside China in spring. For other regions in China, BC is largely contributed from nonlocal sources. We further investigated potential factors that contribute to the poor air quality in China. During polluted days, a net inflow of BC transported from nonlocal source regions associated with anomalous winds plays an important role in increasing local BC concentrations. BC-containing particles emitted from East Asia can also be transported across the Pacific. Our model results show that emissions from inside and outside China are equally important for the BC outflow from East Asia, while emissions from China account for 8 % of BC concentration and 29 % in column burden in the western United States in spring. Radiative forcing estimates show that 65 % of the annual mean BC direct radiative forcing (2.2 W m−2) in China results from local emissions, and the remaining 35 % is contributed by emissions outside of China. Efficiency analysis shows that a reduction in BC emissions over eastern China could have a greater benefit for the regional air quality in China, especially in the winter haze season.

Local biomass burning is a dominant cause of the observed precipitation reduction in southern Africa.

Observations indicate a precipitation decline over large parts of southern Africa since the 1950s. Concurrently, atmospheric concentrations of greenhouse gases and aerosols have increased due to anthropogenic activities. Here we show that local black carbon and organic carbon aerosol emissions from biomass burning activities are a main cause of the observed decline in southern African dry season precipitation over the last century. Near the main biomass burning regions, global and regional modelling indicates precipitation decreases of 20–30%, with large spatial variability. Increasing global CO2 concentrations further contribute to precipitation reductions, somewhat less in magnitude but covering a larger area. Whereas precipitation changes from increased CO2 are driven by large-scale circulation changes, the increase in biomass burning aerosols causes local drying of the atmosphere. This study illustrates that reducing local biomass burning aerosol emissions may be a useful way to mitigate reduced rainfall in the region.

Air quality and climate responses to anthropogenic black carbon emission changes from East Asia, North America and Europe

East Asia, North America and Europe are the world largest emitters of anthropogenic black carbon (BC). In this study, the role of each region's anthropogenic BC emissions on domestic air quality and climate is investigated. A ten-year six-member parallel simulation (i.e., with anthropogenic emissions in each region reduced by 0%, 50% or 100%, or increased by 200%, 500% or 1000%) is conducted based on the state-of-the-art Community Earth System Model (CESM). Linearity of the emission-response relationship is examined for a variety of air quality and climate indicators. Generally, a change in BC emissions tend to linearly influence BC concentrations over both source and nearby downwind regions even taking into account the effect of BC-induced climate perturbations. Aerosol optical depth (AOD) and the net radiative flux perturbation at top of atmosphere (TOA) tend to preserve a similar linear relationship to local BC emission changes, with a robust signal confined only to the source areas. However, the response of temperature in most places is inconsistent to BC emission changes. Though the presence of BC in the atmosphere absorbs solar and terrestrial radiation which has a tendency to warm the atmosphere, the perturbed atmospheric circulation induces substantial meridional exchanges of warm and cold air masses, which overpasses the warming tendency of BC exerted on the atmosphere. This indicates that reducing/increasing regional BC emissions immediately ameliorate/deteriorate local air quality proportionally, but the associated effects on climate perturbation may lack a clear trend within the initial 10-year time span.

Evaluation of the impact of transportation changes on air quality

Transport regulation at local level for the abatement of air pollution has gained significant traction in the EU. In this work, we analyze the effect of different transportation changes on air quality in two similarly sized cities: Granada (Spain) and Ljubljana (Slovenia). Several air pollutants were measured at both sites before and after the implementation of the changes. In Ljubljana, a 72% reduction of local black carbon (BC), from 5.6 to 1.6 μg/m3, was observed after the restriction was implemented. In Granada, statistically significant reductions of 1.3 μg/m3 (37%) in BC and of 15 μg/m3 (33%) in PM10 concentrations were observed after the public transportation re-organization. However, the improvement observed in air quality was very local since other areas of the cities did not improve significantly. We show that closing streets to private traffic, renewal of the bus fleet and re-organization of the public transportation significantly benefit air quality.

Spatial and temporal assessment of organic and black carbon at four sites in the interior of South Africa

Limited data currently exist for atmospheric organic carbon (OC) and black carbon (BC) in South Africa (SA). In this paper OC and BC measured in SA were explored in terms of spatial and temporal patterns, mass fractions of the total aerosol mass, as well as possible sources. PM10 and PM2.5 samples were collected at five sites in SA operated within the Deposition of Biogeochemical Important Trace Species-IGAC DEBITS in Africa (DEBITS-IDAF) network. OC were higher than BC concentrations at all sites in both size fractions, while most OC and BC occurred in the PM2.5 fraction. OC/BC ratios reflected the location of the different sites, as well as possible sources impacting these sites. The OC and BC mass fraction percentages of the total aerosol mass varied up to 24% and 12%, respectively. A relatively well defined seasonal pattern was observed, with higher OC and BC measured from May to October, which coincides with the dry season in the interior of SA. An inverse seasonal pattern was observed for the fractional mass contributions of OC and BC to the total aerosol mass, which indicates substantially higher aerosol load during this time of the year. The relationship between OC and BC concentrations with the distance that air mass back trajectories passed by biomass burning fires and large point sources proved that biomass burning fires contribute significantly to regional OC and BC during the burning season, while large point sources did not contribute that significantly to regional OC and BC. The results from a highly industrialised and populated site also indicated that household combustion for space heating contributed at least to local OC and BC concentrations.

An AeroCom assessment of black carbon in Arctic snow and sea ice

Abstract. Though many global aerosols models prognose surface deposition, only a few models have been used to directly simulate the radiative effect from black carbon (BC) deposition to snow and sea ice. Here, we apply aerosol deposition fields from 25 models contributing to two phases of the Aerosol Comparisons between Observations and Models (AeroCom) project to simulate and evaluate within-snow BC concentrations and radiative effect in the Arctic. We accomplish this by driving the offline land and sea ice components of the Community Earth System Model with different deposition fields and meteorological conditions from 2004 to 2009, during which an extensive field campaign of BC measurements in Arctic snow occurred. We find that models generally underestimate BC concentrations in snow in northern Russia and Norway, while overestimating BC amounts elsewhere in the Arctic. Although simulated BC distributions in snow are poorly correlated with measurements, mean values are reasonable. The multi-model mean (range) bias in BC concentrations, sampled over the same grid cells, snow depths, and months of measurements, are −4.4 (−13.2 to +10.7) ng g−1 for an earlier phase of AeroCom models (phase I), and +4.1 (−13.0 to +21.4) ng g−1 for a more recent phase of AeroCom models (phase II), compared to the observational mean of 19.2 ng g−1. Factors determining model BC concentrations in Arctic snow include Arctic BC emissions, transport of extra-Arctic aerosols, precipitation, deposition efficiency of aerosols within the Arctic, and meltwater removal of particles in snow. Sensitivity studies show that the model–measurement evaluation is only weakly affected by meltwater scavenging efficiency because most measurements were conducted in non-melting snow. The Arctic (60–90° N) atmospheric residence time for BC in phase II models ranges from 3.7 to 23.2 days, implying large inter-model variation in local BC deposition efficiency. Combined with the fact that most Arctic BC deposition originates from extra-Arctic emissions, these results suggest that aerosol removal processes are a leading source of variation in model performance. The multi-model mean (full range) of Arctic radiative effect from BC in snow is 0.15 (0.07–0.25) W m−2 and 0.18 (0.06–0.28) W m−2 in phase I and phase II models, respectively. After correcting for model biases relative to observed BC concentrations in different regions of the Arctic, we obtain a multi-model mean Arctic radiative effect of 0.17 W m−2 for the combined AeroCom ensembles. Finally, there is a high correlation between modeled BC concentrations sampled over the observational sites and the Arctic as a whole, indicating that the field campaign provided a reasonable sample of the Arctic.

Spatio-temporal variations of black carbon concentrations in the Megacity Beijing

The spatial and temporal distribution and the flux of black carbon (BC) concentration in Beijing were continuously investigated over a two-year period at five sites to highlight the relative influence of contributing sources. The results demonstrate firstly that there is significant spatio-temporal variability of BC in Beijing. Highest concentrations occurred during winter primarily due to stagnant meteorological conditions, and seasonal BC sources, such as coal combustion for heating purposes. Biomass burning was identified as a minor seasonal source during the summer months. BC also varied spatially with higher concentrations in the SE of Beijing and lower concentrations in the NW, due to the differing emission intensity of various local BC sources such as traffic and industry. Frequently, overnight BC concentrations were higher due to specific meteorological conditions, such as the lower urban mixing layer height and various anthropogenic activities, such as exclusive night-time heavy duty vehicle traffic in the inner-city.

Arctic climate sensitivity to local black carbon

Recent attention has focused on the impact of black carbon (BC) on Arctic climate. Here, idealized equilibrium climate experiments are conducted to explore the dependence of Arctic temperature change on the altitude and season of local BC forcing. BC residing in the lowest atmospheric layer produces very strong Arctic warming per unit mass and forcing [ 2.8 ± 0.5 K (Wm − 2) − 1] because of low cloud and sea‐ice feedbacks that amplify both summer and winter warming. BC operating only within Arctic snow and sea‐ice also effectively warms the surface, but forcings at 400–750mbar and 210–250mbar cause weak surface warming and cooling, respectively, despite increasing atmospheric moist static energy. This is a consequence of stable atmospheric conditions in the Arctic limiting vertical mixing, and of higher‐altitude BC reducing surface insolation, increasing stability and summer low‐cloud cover, and decreasing poleward energy transport. The current simulated distribution of Arctic atmospheric BC slightly cools the surface, supporting an earlier study, while local atmospheric and cryosphere‐deposited BC warms the Arctic with a sensitivity of + 0.5 ± 0.4 K (Wm − 2) − 1. By season, April–May tropospheric BC induces the greatest mass‐normalized Arctic warming [0.18 K (Gg yr) − 1] because high insolation and surface albedo facilitate large specific forcing during this season. Forcing efficacy, however, increases with summer progression because of decreasing atmospheric stability, leading to a narrow range of mass‐normalized response with season. Although limited by exclusion of aerosol indirect effects, changes in ocean heat transport and forcing by co‐emitted species, these experiments show that Arctic climate response is sensitive to the vertical distribution and deposition efficiency of BC reaching the Arctic.

Delay in the onset of South Asian summer monsoon induced by local black carbon in an AGCM

The influence of local black carbon (BC) on monthly mean precipitation and the associated circulation in South Asia is investigated. The results show that the amplified shortwave radiative heating rate by BC absorption enhances convective activity near the Himalayas and the southern Tibetan Plateau with increased rainfall anomalies in April and May, which is consistent with previous studies. However, the enhanced vertical motions and the precipitation ultimately lead towards cooling of the lower troposphere especially in May, which is extended till June. This favored negative rainfall responses in June, implying delay in the onset of South Asian summer monsoon rainfalls over Arabian Sea and western parts of the subcontinent. The negative precipitation response is further associated with the prevailing anomalous high pressure and the anticyclonic wind circulations induced by BC. Thus, we present here one different feature associated with BC-induced elevated heat pump-like circulations in South Asia.