In this paper, a hybrid control method with adaptive phase-shifting modulation (PSM) and pulse-frequency modulation (PFM) is proposed to optimize the steady-state performance of an LLC resonant converter in wide voltage-gain range application. For the primary-side switches under the hybrid control method, zero-voltage switching (ZVS) performance is maintained over wide voltage-gain range and the turn-off loss is reduced; therefore, the converter reconciles wide voltage-gain range and high efficiency. Mode characteristics under different phase-shifting-angle-θ and switching-frequency-fs combinations is analyzed, and then the soft-switching characteristic is revealed. By introducing time domain analysis, the turn-on current of the primary-side switches is calculated, and thus the ZVS boundary of different θ and fs combinations is inferred. In addition, to acquire the optimum steady-state operation of the converter, the turn-off current is calculated; by making the converter work near to the minimum turn-off current operating point, the turn-off loss can be reduced greatly. With the principles of achieving ZVS performance and minimizing turn-off current, the phase-shifting angle θ of PSM is designed to be adaptive to the reference output voltage, no additional circuits are needed, and the two control degrees (θ and fs) are simplified to one (fs). The simulation and experiment are developed to verify the feasibility and effectiveness of the hybrid control method; the results show that ZVS performance is maintained at wide voltage-gain range and the turn-off current of the hybrid control method is reduced to that of the single PFM, and thus the turn-off loss is reduced. The efficiency comparison validates the fact that the hybrid control method has less power loss than single PSM and single PFM.