Laser Wavelength Research Articles

Modeling Study of Si3N4 Waveguides on a Sapphire Platform for Photonic Integration Applications.

Sapphire has various applications in photonics due to its broadband transparency, high-contrast index, and chemical and physical stability. Photonics integration on the sapphire platform has been proposed, along with potentially high-performance lasers made of group III-V materials. In parallel with developing active devices for photonics integration applications, in this work, silicon nitride optical waveguides on a sapphire substrate were analyzed using the commercial software Comsol Multiphysics in a spectral window of 800~2400 nm, covering the operating wavelengths of III-V lasers, which could be monolithically or hybridly integrated on the same substrate. A high confinement factor of ~90% near the single-mode limit was obtained, and a low bending loss of ~0.01 dB was effectively achieved with the bending radius reaching 90 μm, 70 μm, and 40 μm for wavelengths of 2000 nm, 1550 nm, and 850 nm, respectively. Furthermore, the use of a pedestal structure or a SiO2 bottom cladding layer has shown potential to further reduce bending losses. The introduction of a SiO2 bottom cladding layer effectively eliminates the influence of the substrate's larger refractive index, resulting in further improvement in waveguide performance. The platform enables tightly built waveguides and small bending radii with high field confinement and low propagation losses, showcasing silicon nitride waveguides on sapphire as promising passive components for the development of high-performance and cost-effective PICs.

Design and wavelength selection of compact dual-wavelength Yb:YAG lasers with a Z-shaped cavity

The compact dual-wavelength Yb:YAG lasers were designed and developed by employing a Z-shaped cavity. The overall cavity length is about 32 cm, which can be packaged in a device size of 15 × 10 cm2. The oscillating beam radius in the laser crystal varied by the cavity length, and stable dual wavelength laser was achieved. The 1050 nm output of 1.44W was obtained at the highest pump power is 10 W when the oscillating beam radius was 125 μm. The balance dual-wavelength output of 0.93W was achieved with the optical to optical conversion efficiency of 9.3%. The output wavelengths of the Yb:YAG laser depended on the oscillating beam radius, which was consistent with the experimental results. Our findings indicated that while stringent mode matching was ideal, there was a degree of flexibility that can be tolerated without significantly compromising the laser's performance, which can be beneficial for the dual-wavelength oscillation in applications.

Design of 16-wavelength high-power heterogeneous III-V/Si laser arrays with varying stripe width and grating period

Multi-wavelength laser array is currently one of the most attractive technologies to provide high density links for advanced optical communications and computing. The conventional scheme of varying grating period is almost impossible to achieve 8-wavelength or more. And, the optical output power of heterogeneously integrated quantum dot laser can hardly meet the commercial demand. In this paper, we report a 16-wavelength high-power heterogeneously integrated quantum dot distributed feedback laser array. To the best of our knowledge, this is the first heterogeneously integrated quantum dot laser array that tunes the lasing wavelength by combining the scheme of varying the stripe width and grating period of laser units. The effective refractive index of gratings is calculated by eigenmode expansion method. When the grating period is fixed at 198 nm, and the stripe widths of laser units are 2.00 μm, 2.25 μm, 2.60 μm and 3.15 μm, respectively, the corresponding lasing wavelengths are 1307.94 nm, 1308.49 nm, 1309.06 nm and 1309.63 nm, respectively, and the wavelength spacing of the adjacent laser units is about 100 GHz. By additionally adjusting the grating period between 196 nm and 202 nm with 2 nm spacing of grating period, a 16-wavelength QD DFB laser array is designed with the wavelength range from 1294.73 nm to 1336.09 nm. In addition, asymmetric distributed feedback grating is adopted to improve the optical output power at the front-end of laser arrays. The maximum ratio of the output power at the both end of laser units is 19.6 when the grating duty cycles of the front-end and the back-end of the λ/4 phase-shift is 0.7 and 0.5, respectively, and the grating lengths is 250 μm and 450 μm, respectively. This work will promote the performance improvement of heterogeneously integrated quantum dot lasers and develop the quantum dot lasers towards multi-wavelength.

Staring laser situation awareness technology with wide-FOV and high-angle positioning accuracy based on two-dimensional grating and two-channels

Current and future battlefields face the emerging threat of laser weapon development. Existing laser situation awareness technology cannot provide simultaneous operation of wide field-of-view (FOV) and high angle positioning accuracy. This study introduces a system employing a two-dimensional grating and dual-channel approach that offers high precision in situation awareness about laser wavelengths and angle positioning across a wide FOV. The system consists of two main components: an approximate measurement channel and an accurate measurement channel. The former includes a wide-FOV lens and a focal plane array detector (FPA1), acquiring preliminary angle information of the laser. The latter, comprising a two-dimensional grating, a narrow-FOV lens, and a FPA2, captures the incoming laser’s wavelength and precise azimuth and pitch through the analysis of diffraction spot position and distance. Experimental findings confirm that the accuracies of angle and central wavelength measurements exceed 0.05° and 8 nm, respectively, for a FOV of 120°.

Aggregation of One‐Dimensional Wires: The Case of Long Oligoynes

AbstractWe show an unexpected aggregation phenomenon of a long oligoyne (Py[16]) with 16 contiguous triple bonds and endcapped with bulky 3,5‐bi(3,5‐bis‐tert‐butylphenyl)pyridine groups. Aggregation of 1D π‐conjugated oligoyne chains is rare given the minimal π–π intermolecular interactions as well as its flexibility that works against self‐assembly. In dilute solutions, the reversible aggregation of Py[16] initiates at low temperature in the range of 140–180 K, and is not observed for shorter oligoynes in this series. Cryogenic UV/Vis electronic absorption spectra and vibrational Raman spectra with different laser wavelength lines tuning from in‐resonance to off‐resonance conditions have been used to extract the vibrational features characterizing the monomer and aggregate species. Theoretical calculations complement the spectroscopic findings.

Aggregation of One-Dimensional Wires: The Case of Long Oligoynes.

We show an unexpected aggregation phenomenon of a long oligoyne (Py[16]) with 16 contiguous triple bonds and endcapped with bulky 3,5-bi(3,5-bis-tert-butylphenyl)pyridine groups. Aggregation of 1D π-conjugated oligoyne chains is rare given the minimal π-π intermolecular interactions as well as its flexibility that works against self-assembly. In dilute solutions, the reversible aggregation of Py[16] initiates at low temperature in the range of 140-180 K, and is not observed for shorter oligoynes in this series. Cryogenic UV/Vis electronic absorption spectra and vibrational Raman spectra with different laser wavelength lines tuning from in-resonance to off-resonance conditions have been used to extract the vibrational features characterizing the monomer and aggregate species. Theoretical calculations complement the spectroscopic findings.

Solid-state laser (266 nm) as an alternative to ArF excimer laser (193 nm) for corneal reshaping: Comparative numerical study of the thermal effect.

Laser corneal reshaping is a safe and effective technique utilized to treat common vision disorders. An advanced laser delivery system equipped with a pulsed UV laser with specific parameters is used to ablate parts of the cornea surface to correct the existing refractive error. The argon fluoride (ArF) excimer pulsed gas laser at 193 nm is the most employed type in the commercial devices for such treatments. This laser is generated using a mixture of Argon, Fluorine, and a significant amount of Neon gases. However, due to the ongoing Russian-Ukraine war, the availability of Neon gas is currently very limited, as this region is considered the primary supplier of pure Neon gas. Consequently we suggest replacing the common ArF laser source in the commercial devices with a solid-state (forth harmonic neodymium-doped yttrium aluminum garnet laser at 266 nm). This replacement uses the same operation parameters, optics, and scanning algorithm. Parameters from five commercial devices (Zeiss MEL 90, Technolas TENEO 317, Alcon Wave Light EX 500, Schwind Amaris 750 s, OptoSystems MICROSCAN VISUM) were compared with those of the i-ablation device, a research device that uses a 266 nm laser source. Our goal is to reduce production costs through a simple modification that has a significant impact. Consequently, the present study aims to find an alternative laser source for the current ArF laser without exchanging the complete system's design. This recommendation is based on a numerical simulation study. The thermal effect on a human cornea model was numerically evaluated using finite-element solutions of Pennes' bioheat equation on the COMSOL platform by applying two laser wavelengths. The results demonstrated that changing the laser source significantly impacts the thermal effect, even with the same laser settings. All studied devices showed a reduction in the thermal effect to below 40°C, compared with nearly 100°C under ordinary conditions.

Impact of dual wavelength laser therapies in the treatment of hypertrophic scars and keloids: a systematic review

Impact of dual wavelength laser therapies in the treatment of hypertrophic scars and keloids: a systematic review

Exceptional point sensing via energy loss profile in a non-Hermitian system

The heightened sensitivity observed in non-Hermitian systems at exceptional points (EPs) has garnered significant attention. Typical EP sensor implementations rely on precise measurements of spectra and importantly, for real time sensing measurements, the EP condition ceases to hold as the perturbation increases over time, thereby preventing the use of high sensitivity at the EP point. In this work, we present an new approach to EP sensing which goes beyond these two traditional constraints. Firstly, instead of measuring the spectra, our scheme of EP based sensing is based on the observation of decay length of the optical mode in finite size gratings, which is validated via coupled mode theory as well as full wave electrodynamic simulations. Secondly, for larger perturbation strengths, the EP is spectrally shifted instead of being destroyed — this spectral shift of the EP is calibrated and using this look-up table, we propose continuous real time detection by varying the excitation laser wavelength. As a proof of principle of our technique, we present an application to the sensing of coronavirus particles, which shows unprecedented limit of detection. Furthermore, our analysis includes calculation of the signal-to-noise ratio, revealing that EP sensors offer advantage when classical technical noise dominates over fundamental noise. These findings will contribute to the expanding field of exceptional point based sensing technologies for real time applications beyond spectral measurements.

Tongue squamous cell carcinoma treated by 5-aminolevulinic acid administrated through Microdrop method

BackgroundPostoperative recurrence of tongue squamous cell carcinoma (TSCC) has always been a clinical problem for patients and doctors. Surgery and radiotherapy are the main treatment methods for TSCC, but reoperation often leads to functional impairment. Side effects of radiotherapy include mucosal gland damage, dry mouth, weakened or lost taste. Improved treatment is needed. ObjectiveTo evaluate the clinical outcome of a patient with TSCC treated with Microdrop aminolevulinic acid (ALA) photodynamic treatment (PDT) twice. MethodsALA was dissolved in 5 % lidocaine and the concentration of ALA was 20 % by Microdrop method. Then, the tumor tissue was expanded 1 cm outward, and the injection points were evenly distributed with an upper and lower left and right interval of 2–3 mm. The 1 ml syringe was used to perform the injection in the skin of the tumor area, and there was a small cuticle at each injection point. A pathologically confirmed patient with TSCC received twice Microdrop ALA-PDT treatments, which were evaluated at 1 month and 4 months later. ResultsAfter 3 h of Microdrop ALA injection, the wavelength of semiconductor laser was set to 630 nm, and the energy of 300 mW /cm2 was irradiated for 30 min. After two treatments, the lesions were not visible, and no recurrence occurred after 4 months of follow-up. The patient's tongue function was well preserved and the cosmetic effect was good. ConclusionMicrodrop ALA-PDT may be effective in the salvage treatment of select tongue squamous cell carcinoma.

Efficacy of low-level laser therapy enhances the rate of canine retraction by increasing β glucoronidase and pentraxin – 3 in gingival crevicular fluid: A clinical study

The aim of the study was to evaluate the efficacy of low-level laser therapy in enhancing the rate of orthodontic tooth movement using β glucoronidase and pentraxin-3 (TNF) biomarkers in gingival crevicular fluid.A split-mouth design was used in 16 subjects (8 experimental and 8 controlled) aged 14 to 25 years, who’s maxillary first premolars were extracted. A gallium-aluminium-arsenide semiconductor diode laser (wavelength, 810 nm; energy density, 10 J/cm2; power output, 100 mW) delivered low-level laser therapy to the experimental canine undergoing distalization at 10 points. The control canine was distalized without low-level laser therapy. The experimental and control canines were distalized using a force of 150 g provided by nickel-titanium closed coil springs. Gingival crevicular fluid was collected at 5 time points from the control and experimental sides, and the levels of β glucoronidase and pentraxin-3 were analysed by enzyme-linked immuno-sorbent assay (ELISA). The rate of canine retraction was calculated by using ortho analyser software.Increased levels of β glucoronidase and pentraxin-3 were observed in the experimental canines compared with the control canines (P <0.001). Cumulative tooth movements over an 8-week experimental period were greater for the experimental canines compared with the control canines. A positive correlation existed between the β glucoronidase and pentraxin-3 levels and the amounts of tooth movement across all time intervals.Low level laser therapy in adjunct with continuous and light forces leads to increase in β glucoronidase and pentraxin-3 leading to accelerated orthodontic tooth movement.: Low-level laser therapy fastens the rate of canine retraction thus accelerating the orthodontic tooth movement. The levels of β glucoronidase and Pentraxin 5 are increased significantly after laser irradiation which aids in accelerating orthodontic tooth movement.

A wavelength analyzer using laser self-mixing interferometry

In this paper, we propose a simple yet effective method to measure the operating wavelength of a laser using laser self-mixing interferometry (SMI). Analyzing the self-mixing interference signals acquired from external objects with known motion patterns allows us to deduce the laser's operating wavelength. To validate the accuracy of our method further, we constructed a laser self-mixing linear motion sensing system. This system captured the self-mixing interference signals generated as external targets moved at a uniform linear velocity under various laser wavelengths. By conducting FFT analysis, we obtained the signal frequency, which was then converted from laser Doppler frequency to optical frequency, ultimately determining the laser's wavelength. Our experiment specifically focused on analyzing the impact of frequency doubling on the results, discussing its causes and potential solutions. Numerical analysis indicates that the laser's working wavelength parameter is precisely measured from external targets moving at a uniform speed of 0.4 to 2.4 mm/s. Additionally, the experimental results show a absolute error of less than 1.230 nm and an relative error of less than 0.12 %. In conclusion, our experimental, simulation, and theoretical analysis results mutually validate each other, confirming the accuracy and practicality of the measurement method.

Measurement of engine exhaust plume temperature and concentration distributions with tomographic absorption spectroscopy and learning-based absorbance recovery

Measuring the spatial distribution of temperature and species concentration is important to the thermodynamic analysis and validation of modern combustion systems. In this work, we developed a measurement method based on tomographic absorption spectroscopy (TAS) for the quantitative measurement of two-dimensional distributions of gas temperature and concentration. A learning-based absorbance recovery method was proposed and incorporated into TAS to address the baseline error induced distortion of absorbance and improve the accuracy of single path measurement. The developed TAS system, consisting of 12 laser beams, was demonstrated on a diesel fueled small turbojet engine. Temperature and H2O concentration distributions of the exhaust plume were measured with laser wavelength scan rates of 20 kHz. Temperature variations in microsecond-scale were captured and the time-averaged center temperature agreed well with thermocouple measurements. The developed TAS method demonstrates the feasibility of real-time and accurate tomographic imaging for practical combustion flows, which could be effectively applied for widespread combustion diagnostics.

Wavelength-influenced electrical performance of laser-written flexible copper-based structures

The one-step direct laser writing process has been an efficient strategy for constructing flexible metal structures. However, the effect of laser wavelength on the structuring process remains unclear, thus restricting the universal manufacturing process development. In this work, the feasibility of one-step writing of flexible Cu structures with different wavelength continuous diode lasers has been verified. Here, photothermal reactions dominate in the decomposition of the reducing agent to form copper structures. Differences in the wavelength primarily affect the photothermal reaction amplitude for structuring, resulting in a variation in the formation of Cu structures. Under our processing conditions, the photothermal reaction induced by 532 nm laser is higher than 808 nm laser, a higher reduced-joining degree of the Cu structure can be achieved by 532 nm laser. This results in a superior conductivity, adhesion, and bendability of Cu structures fabricated by 532 nm laser than that of 808 nm laser. Furthermore, strain sensors that can detect different bending angles and bending frequencies have been fabricated by 532 nm laser-written structures to demonstrate their practical applications.

Evaluation of Thermal Transport Characteristics of Three-Dimensional Self-Ordered Multilayered Silicon-Germanium Nanodots

1. Background and purpose Silicon-germanium (SiGe) alloys have much lower thermal conductivity than Si and Ge single crystals and are expected to be candidates for next-generation thermoelectric device materials of internet of things society. It is important to achieve both high carrier mobility and low thermal conductivity on the basis of the dimensionless figure of merit [1]. There are several studies on the thermoelectric properties of SiGe with low-dimensional structures such as superlattice and nanodots [2,3] to dramatically decrease thermal conductivity. However, the relationship between the nanoscale thermal properties and the phonon scattering mechanism of self-ordered multilayer SiGe nanodots with high uniformity grown by Stranski-Krastanov [4] mode is unclear. In this study, we demonstrated the thermal transport characteristics of the self-ordered multilayer SiGe nanodots. 2. Experiments Si/SiGe superlattice and nanodots samples were fabricated by reduced pressure chemical vapor deposition. We set to 20 cycles of Si0.65Ge0.35 / Si superlattice, the staggered Si0.65Ge0.35 nanodots (alternately stacked) and the dot-on-dot Si0.65Ge0.35 nanodots (vertically stacked) by changing growth temperature and precursors for Si spacer growth [4], as shown in Fig. 1. Thermal properties were evaluated by the Time Domain Thermoreflectance (TDTR) method. The strain states and Ge fraction were evaluated by Raman spectroscopy. The focal length and wavenumber resolution of the Raman spectrometer were 2,000 mm and 0.1 cm-1, respectively. The excitation light source was a green laser (wavelength: 532 nm). We obtained the Raman spectra of Si-Si, Si-Ge, and Ge-Ge vibrational modes derived from the SiGe regions. 3. Results and discussion Figure 2 shows the thermal conductivity for the SiGe region of the superlattice and nanodots (dot-on-dot and staggered structures) obtained by TDTR method. We found that the SiGe nanodots with the dot-on-dot structure have the highest thermal conductivity, while the SiGe nanodots with the staggered structure and SiGe superlattice have almost the same thermal conductivity. We consider that the heat flow easily penetrates from the top (surface) to the bottom (Si substrate interface) in the dot-on-dot structures. On the other hand, it is possible that the staggered SiGe nanodots can play a sufficient role as a phonon scatterer compared to the dot-on-dot structures since the superlattice structure and the staggered SiGe nanodots have almost the same thermal properties. In conclusion, we demonstrated the possibility of controlling phonon scattering by changing the arrangement of the self-ordered multilayer SiGe nanodots. Acknowledgement This work was supported by JSPS KAKENHI Grant Number 21K14201, Japan.

Low-Temperature Synthesis of Linear Carbon Chain inside Single-Walled Carbon Nanotubes

Linear carbon chain (LCC) has attracted much interest concerning its structure and applications. It has been reported that LCC possesses higher strength, elastic modulus, and stiffness than any known material, which provides a possibility for LCC as a new composite material, yet its chemical stability remains an issue [1]. Therefore, finding a method to efficiently synthesize LCC has become a meaningful research topic in recent years. A landmark study on LCC synthesis was given by using double-walled carbon nanotubes (DWCNTs) as the template combined with a high-temperature annealing treatment at 1460°C to acquire long chains composed of more than 6,000 carbon atoms [2]. Except for DWCNTs, LCC synthesis starting from single-walled carbon nanotubes (SWCNT) as templates was also reported. However, given the instability of SWCNTs at higher temperature [2] the synthesis efficiency is not as good as for DWCNTs. As far as we know, there is still no report on an efficient LCC synthesis inside SWCNTs. Herein, we report the low-temperature (400°C) efficient LCC synthesis starting from a SWCNT template.To this end, a SWCNT dispersion [3] underwent a surfactant exchange process and was fabricated into a SWCNT film by the filtration method. The SWCNT film was annealed under 400°C in an argon atmosphere to synthesize LCC. Raman spectroscopy (laser wavelength 532 nm) was used to characterize the efficiency of the LCC synthesis. A strong peak at 1863 cm-1 appeared after annealing, originating from the well-known C-mode of the linear carbon chain [4] thereby confirming its existence inside SWCNTs. SWCNTs synthesized by a low-pressure alcohol catalytic chemical vapor deposition (ACCVD) method [5] were also adopted for the LCC synthesis template, resulting in a similar LCC Raman peak at 1863 cm-1. We attribute this successful low-temperature LCC synthesis to the appropriate surfactant which could be encapsulated inside CNTs and converted to LCC during the annealing process.Keywords: Linear Carbon Chain, Single-walled Carbon Nanotubes, Surfactants

Effect of laser wavelength on ablation propulsion and plasma characteristics with acrylonitrile butadiene styrene target

Propulsion performance produced by laser ablation of polymer made of acrylonitrile butadiene styrene is experimentally investigated using the first, second, and third harmonics of a Nd: YAG laser. A ballistic pendulum is employed to assess the impulse and coupling coefficient for laser propulsion application. Fast photography, target ablation, and optical emission spectroscopy are proposed to analyze the energy coupling characteristic. The impulse and coupling coefficient under different pressures are demonstrated to depend on the target ablation and plasma properties which are relevant to laser wavelength. As the laser wavelength decreases, the crater depth and ablation mass are enhanced. Meanwhile, the plasma plume separates at atmospheric pressure and its length extends continuously in the low-pressure range. As a result, plasma including more ejected particles with higher velocity contributes to obtaining excellent impulse and coupling coefficient. In addition, the decreased electron density and temperature indicate higher collision frequency and photoionization dominate rather than inverse bremsstrahlung absorption at shorter laser wavelengths. This work provides a better understanding of the energy conversion mechanism and a reference for improving propulsion performance.

Femtosecond laser plane-by-plane inscription of ultra-short DBR fiber lasers for sensing applications

We propose and demonstrate the inscription of ultra-short distributed Bragg reflector fiber lasers (DBR-FLs) in Er/Yb co-doped fiber (EYDF) using a femtosecond laser plane-by-plane (Pl-b-Pl) method. By integrating the spherical aberration (SA) with a laser 2D scanning process, a planar refractive index modification (RIM) region can be induced in the fiber core. Thanks to the Pl-b-Pl inscription, a high-quality fiber Bragg grating (FBG) in an EYDF is produced, exhibiting a grating strength exceeding 40 dB and an insertion loss of 0.1 dB. Subsequently, an ultra-short DBR-FL with an entire length of 7.3 mm is fabricated by the Pl-b-Pl inscription. The Pl-b-Pl ultra-short DBR-FL exhibits an improved slope efficiency of 0.7% compared with the DBR-FLs fabricated using another two direct-writing techniques, namely line-by-line (LbL) and point-by-point (PbP) methods. Furthermore, this ultra-short DBR-FL generates single-frequency and single-polarization radiation with a narrow linewidth (9.4 kHz) and a low relative intensity noise (-105.8 dB/Hz). Moreover, a wavelength-division-multiplexed array consisting of eight ultra-short DBR-FLs with distinct lasing wavelengths is successfully created. The Pl-b-Pl ultra-short DBR-FLs with excellent output performances offer significant potential for high-sensitivity sensing applications requiring high spatial resolution.

Implementation of laser-light backscattering imaging for authentication of the geographic origin of Indonesia region citrus

Citrus fruit (Citrus nobilis Lour.) from the Indonesian region is reported to have high economic value due to attractive nutritional, nutraceutical, and sensory attributes. However, authenticating the geographic origins is challenging because of adulteration and similarity in visual appearance. Therefore, this study aimed to develop an effective method based on laser-light backscattering imaging (LLBI) for authentication of the geographic origin of the region citrus. A total of 200 citrus samples were collected from Medan, Malang, Jember, and Banyuwangi regions, which were the four main citrus-producing areas in Indonesia. Approximately three different laser wavelengths, namely 450, 532, and 648 nm were beamed to produce the backscattering image. Furthermore, a combination of the gray-level co-occurrence matrix (GLCM) method and support vector machine (SVM) algorithm was applied to extract texture features and build a classification model, respectively. In this context, three kernel functions, such as linear, radial basis function, and polynomial, were compared in authenticating the geographic origin of citrus. The results showed that the proposed technique achieved 96.667 % accuracy and 3.333 % apparent error for authentication of the geographic origin. The proposed LLBI technique applied a laser wavelength of 450 nm and a polynomial kernel function as the best combination to produce reliable predictive power. This study held valuable implications for advancing sensing technology devices to authenticate geographic origin, specifically citrus fruit.

Femtosecond Laser‐Induced Regulation of Photo‐ and Persistent Luminescence of Perovskite Crystals

AbstractManipulation of photoluminescence (PL) and persistent luminescence (PersL) provides a powerful tool for anti‐counterfeiting applications. Here, Sb3+‐doped CsCdCl3 perovskite single crystals (SCs) can be selectively irradiated via utilizing ultra‐fast femtosecond (fs) laser, creating tunable PL colors and PersL duration with high precision. The PL color of the synthesized SCs changes from cyan to orange along with the wavelength of the fs laser, for the successful regulation of the optical procedure from a single‐photon to a two‐photon absorption process. Moreover, an orange PersL of CsCdCl3:Sb3+ SC is observed after being charged with a fs laser, and the corresponding duration time can be feasibly controlled with the pump wavelength. In particular, CsCdCl3:Sb3+ is capable of ultrafast carrier capture (1 s) under fs laser compared to ultraviolet lamp pre‐irradiation enabling a high‐resolution micro‐PersL in photon trapping/de‐trapping modes. These findings not only give a new solution for the fabrication high‐resolution micro‐PL and trajectory‐writing micro‐PersL patterns, but also provide a deep insight to understand the photon–matter interactions.