Laser-driven Source Research Articles

Kapitza Stabilization of Quantum Critical Order

Dynamical perturbations modify the states of classical systems in surprising ways and give rise to important applications in science and technology. For example, Floquet engineering exploits the possibility of band formation in the frequency domain when a strong, periodic variation is imposed on parameters such as spring constants. We describe here Kapitza engineering, where a drive field oscillating at a frequency much higher than the characteristic frequencies for the linear response of a system changes the potential energy surface so much that maxima found at equilibrium become local minima, in precise analogy to the celebrated Kapitza pendulum where the unstable inverted configuration, with the mass above rather than below the fulcrum, actually becomes stable. Our starting point is a quantum field theory of the Ginzburg-Devonshire type, suitable for many condensed matter systems, including particularly ferroelectrics and quantum paralectrics. We show that an off-resonance oscillatory electric field generated by a laser-driven terahertz source can induce ferroelectric order in the quantum-critical limit. Heating effects are estimated to be manageable using pulsed radiation; “hidden” radiation-induced order can persist to low temperatures without further pumping due to stabilization by strain. We estimate the Ginzburg-Devonshire free-energy coefficients in SrTiO3 using density-functional theory and the stochastic self-consistent harmonic approximation accelerated by a machine-learned force field. Although we find that SrTiO3 is not an optimal choice for Kapitza stabilization, we show that scanning for further candidate materials can be performed at the computationally convenient density-functional theory level. We suggest second harmonic generation, soft-mode spectroscopy, and x-ray diffraction experiments to characterize the induced order. Published by the American Physical Society 2024

Acceleration mechanisms of energetic ion debris in laser-driven tin plasma EUV sources

Laser-driven tin plasmas are driving new-generation nanolithography as sources of extreme ultraviolet (EUV) radiation centered at 13.5 nm. A major challenge facing industrial EUV source development is predicting energetic ion debris produced during the plasma expansion that may damage the sensitive EUV channeling multilayer optics. Gaining a detailed understanding of the plasma dynamics and ion acceleration mechanisms in these sources could provide critical insights for designing debris mitigation strategies in future high-power EUV sources. We develop a fully kinetic model of tin-EUV sources using one-dimensional particle-in-cell simulations to study ion debris acceleration, which will be valuable for cross-validation of radiation-hydrodynamic simulations. An inverse-bremsstrahlung heating operator is used to model the interaction of a tin target with an Nd:YAG laser, and thermal conduction is included through a Monte Carlo Coulomb collision operator. While the large-scale evolution is in reasonable agreement with analogous hydrodynamic simulations, the significant timescale for collisional equilibration between electrons and ions allows for the development of prominent two-temperature features. A collimated flow of energetic ions is produced with a spectrum that is significantly enhanced at high energies compared to fluid simulations. The dominant acceleration mechanism is found to be a large-scale electric field supported mainly by the electron pressure gradient, which is enhanced in the kinetic simulations due to the increased electron temperature. We discuss the implications of these results for future modeling of tin-EUV sources and the development of debris mitigation schemes.

Cryogenic solid deuterium target formation to realize highly pure deuteron acceleration by high-intensity laser

In recent years, laser-driven neutron sources have attracted attention for their applications such as nondestructive analysis and the production of medical radioisotopes. One of the efficient neutron production methods is the use of the 9Be(d, n)10B reaction on a beryllium target with deuterons accelerated by laser–plasma interactions, since this is an exothermic reaction. For efficient deuteron acceleration, we have developed a formation system for solid deuterium targets. A millimeter thick solid deuterium target can be formed with the system. Before the laser shot, the solid deuterium target in the laser chamber can be mechanically moved to the laser irradiation point. We have demonstrated deuteron acceleration by the LFEX laser, and a highly pure deuteron pulse with energies of up to 6.2 MeV was measured with a Thomson parabola ion spectrometer.

Virtual source approach for maximizing resolution in high-penetration gamma-ray imaging

High-energy gamma-ray radiography has exceptional penetration ability and has become an indispensable nondestructive testing (NDT) tool in various fields. For high-energy photons, point projection radiography is almost the only feasible imaging method, and its spatial resolution is primarily constrained by the size of the gamma-ray source. In conventional industrial applications, gamma-ray sources are commonly based on electron beams driven by accelerators, utilizing the process of bremsstrahlung radiation. The size of the gamma-ray source is dependent on the dimensional characteristics of the electron beam. Extensive research has been conducted on various advanced accelerator technologies that have the potential to greatly improve spatial resolution in NDT. In our investigation of laser-driven gamma-ray sources, a spatial resolution of about 90 µm is achieved when the areal density of the penetrated object is 120 g/cm2. A virtual source approach is proposed to optimize the size of the gamma-ray source used for imaging, with the aim of maximizing spatial resolution. In this virtual source approach, the gamma ray can be considered as being emitted from a virtual source within the convertor, where the equivalent gamma-ray source size in imaging is much smaller than the actual emission area. On the basis of Monte Carlo simulations, we derive a set of evaluation formulas for virtual source scale and gamma-ray emission angle. Under optimal conditions, the virtual source size can be as small as 15 µm, which can significantly improve the spatial resolution of high-penetration imaging to less than 50 µm.

Three-dimensional particle-in-cell simulations of laser-driven multiradiation sources based on double-layer targets.

Double-layer targets (DLTs), made of a low-density foam on top of a solid substrate, can efficiently convert the energy of a high-intensity laser to provide sources of photons and protons. We investigate a 30-fs pulse with a peak intensity of I∼8.7×10^{20}W/cm^{2} and a peak power of ∼120 TW interacting with a DLT using three-dimensional (3D) particle-in-cell simulations. We focus on providing quantitative results in full 3D geometry on the foam thickness dependence; on the competition between two photon-generating processes in DLTs, i.e., nonlinear inverse Compton scattering (NICS) and bremsstrahlung (BS); and on the acceleration of protons via enhanced target-normal sheath acceleration. We discuss conversion efficiency, average energy, and angular distributions of such multiradiation sources. We find that NICS can prevail over BS if the DLT's substrate is thin enough (∼µm) and that the optimal foam thickness that maximizes the conversion efficiency in NICS and BS photons and the proton cutoff energy, among those considered, is the same (15µm). These results show that DLTs constitute an excellent tool for developing relatively compact and optimized laser-driven multicomponent radiation sources.

Narrow bandwidth, low-emittance positron beams from a laser-wakefield accelerator

The rapid progress that plasma wakefield accelerators are experiencing is now posing the question as to whether they could be included in the design of the next generation of high-energy electron-positron colliders. However, the typical structure of the accelerating wakefields presents challenging complications for positron acceleration. Despite seminal proof-of-principle experiments and theoretical proposals, experimental research in plasma-based acceleration of positrons is currently limited by the scarcity of positron beams suitable to seed a plasma accelerator. Here, we report on the first experimental demonstration of a laser-driven source of ultra-relativistic positrons with sufficient spectral and spatial quality to be injected in a plasma accelerator. Our results indicate, in agreement with numerical simulations, selection and transport of positron beamlets containing Ne+≥105\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$N_{e+}\\ge 10^5$$\\end{document} positrons in a 5% bandwidth around 600 MeV, with femtosecond-scale duration and micron-scale normalised emittance. Particle-in-cell simulations show that positron beams of this kind can be guided and accelerated in a laser-driven plasma accelerator, with favourable scalings to further increase overall charge and energy using PW-scale lasers. The results presented here demonstrate the possibility of performing experimental studies of positron acceleration in a laser-driven wakefield accelerator.

Laser-driven broadband near-infrared light source with watt-level output

Laser-driven broadband near-infrared light source with watt-level output

Laser-driven quasi-static B-fields for magnetized high-energy-density experiments

We present measurements of magnetic fields generated in laser-driven coil targets irradiated by laser pulses of nanosecond duration, 1.053 μm wavelength, 500 J energy, and ∼1015 W/cm2 intensity, at the LULI2000 facility. Using two perpendicular probing axes, proton deflectometry is used to characterize the coil current and static charge at different times. Results reveal various deflection features that can be unambiguously linked to a looping quasi-steady current of well-understood polarity or to a static charging of the coil surface. Measured currents are broadly consistent with predictions from a laser-driven diode-current source and lumped circuit model, supporting the quasi-steady assessment of the discharges. Peak magnetic fields of ∼50 T at the center of 500-μm-diameter coils, obtained at the moderate laser intensity, open up the use of such laser-driven coil targets at facilities worldwide to study numerous phenomena in magnetized high-energy-density plasmas, and its potential applications.

Demonstration of a robust laser-driven X-ray source for CT

Demonstration of a robust laser-driven X-ray source for CT

Development of a Time-Gated Epithermal Neutron Spectrometer for Resonance Absorption Measurements Driven by a High-Intensity Laser

The advance of laser-driven neutron sources (LDNSs) has enabled neutron resonance spectroscopy to be performed with a single shot of a laser. In this study, we describe a detection system of epithermal (∼eV) neutrons especially designed for neutron resonance spectroscopy. A time-gated photomultiplier tube (PMT) with a high cut-off ratio was introduced for epithermal neutron detection in a high-power laser experiment at the Institute of Laser Engineering, Osaka University. We successfully reduced the PMT response to the intense hard X-ray generated as a result of the interaction between laser light and the target material. A time-gated circuit was designed to turn off the response of the PMT during the laser pulse and resume recording the signal when neutrons arrive. The time-gated PMT was coupled with a 6Li glass scintillator, serving as a time-of-flight (TOF) detector to measure the neutron resonance absorption values of 182W and 109Ag in a laser-driven epithermal neutron generation experiment. The neutron resonance peaks at 4.15 eV of 182W and 5.19 eV of 109Ag were detected after a single pulse of laser at a distance of 1.07 m.

Low-energy spin-polarized electrons: their role in surface physics

Low-energy (∼100eV) electrons have been employed for more than half a century to investigate physical, chemical and electronic phenomena in condensed matter and surface physics. A particular role may be attributed to a purely quantum-mechanical property of the electron–its spin or intrinsic angular momentum. Since the 1970s the electron spin has been indispensable in determining the role of spin-dependent interactions, such as exchange interaction and spin-orbit coupling and their consequences. Most recently, the aspect of topology and its role in condensed matter systems has given a new drive to the investigation of the electron spin and spin textures in such materials. New results on time-dependent ultrafast phenomena may become available by the availability of new intense lasers and laser-driven sources.

Advancing lithium neutron capture therapy: 6Li-loaded nanoparticles and laser-driven neutron sources

We report on 6Li neutron capture therapy (LiNCT) in anticipation of using carbon nanoparticles to deliver targeted, high linear energy transfer radiation to non-resectable tumors. Our investigations show that, compared with existing 10B neutron capture therapy (BNCT), 6Li offers similar dose potential for equal mass density (DLi∼DB when mLi=mB), for capture products that span 7 times more range and approximately three cell lengths. Consequently, 6Li-filled nanoparticles dispersed more than half-a-cell-length apart, better convey high doses and ultra-high dose-rates, as LiNCT generates substantially less γ-rays and becomes more targeted than BNCT. To this end, we propose a neutron production scheme involving laser-plasma driven protons incident on various 7Li targets, capable of producing >109 n/sr/pulse. For high repetition frequency, efficient neutron moderation, and ideal 6Li concentration, the modality offers greater precision than existing neutron capture therapy.

Reconstruction of lateral coherence and 2D emittance in plasma betatron X-ray sources

X-ray sources have a strong social impact, being implemented for biomedical research, material and environmental sciences. Nowadays, compact and accessible sources are made using lasers. We report evidence of nontrivial spectral-angular correlations in a laser-driven betatron X-ray source. Furthermore, by angularly-resolved spectral measurements, we detect the signature of spatial phase modulations by the electron trajectories. This allows the lateral coherence function to be retrieved, leading to the evaluation of the coherence area of the source, determining its brightness. Finally, the proposed methodology allows the unprecedented reconstruction of the size of the X-ray source and the electron beam emittance in the two main emission planes in a single shot. This information will be of fundamental interest for user applications of new radiation sources.

A Platform for Laser-Driven Ion Sources Generated with Nanosecond Laser Pulses in the Intensity Range of 1013–1015 W/cm2

An experimental platform for laser-driven ion (sub-MeV) acceleration and potential applications was commissioned at the HiLASE laser facility. The auxiliary beam of the Bivoj laser system operating at a GW level peak power (~10 J in 5–10 ns) and 1–10 Hz repetition rate enabled a stable production of high-current ion beams of multiple species (Al, Ti, Fe, Si, Cu, and Sn). The produced laser–plasma ion sources were fully characterized against the laser intensity on the target (1013–1015 W/cm2) by varying the laser energy, focal spot size, and pulse duration. The versatility and tuneability of such high-repetition-rate laser–plasma ion sources are of potential interest for user applications. Such a statistically accurate study was facilitated by the large amount of data acquired at the high repetition rate (1–10 Hz) provided by the Bivoj laser system.

Development and characterization of a laser-driven cold-field emission source

Development and characterization of a laser-driven cold-field emission source

Flux and estimated spectra from a low-intensity laser-driven X-ray source

Abstract Laser-driven X-rays as probes for high-energy-density physics spans an extremely large parameter space with laser intensities varying by 8 orders of magnitude. We have built and characterized a soft X-ray source driven by a modest intensity laser of 4 × 1013 W/cm2. Emitted X-rays were measured by diamond radiation detectors and a filtered soft X-ray camera. A material-dependence study on Al, Ti, stainless steel alloy 304, Fe, Cu and Sn targets indicated 5-μm-thick Cu foils produced the highest X-ray yield. X-ray emission in the laser direction and emission in the reverse direction depend strongly on the foil material and the thickness due to the opacity and hydrodynamic disassembly time. The time-varying X-ray signals are used to measure the material thinning rate and is found to be ∼1.5 μm/ns for the materials tested implying thermal temperature around 0.6 eV. The X-ray spectra from Cu targets peaks at ∼2 keV with no emission >4 keV and was estimated using images with eight different foil filters. One-dimensional hydrodynamic and spectral calculations using HELIOS-CR provide qualitative agreement with experimental results. Modest intensity lasers can be an excellent source for nanosecond bursts of soft X-rays.

Design of a semiconductor-based proton spectrometer for laser-driven sources applications

Design of a semiconductor-based proton spectrometer for laser-driven sources applications

X-ray detector requirements for laser–plasma accelerators

Laser–plasma interactions (LPIs) are an emerging source of a range of energetic radiation. LPI experiments drive ultra-short (< ps) and brilliant sources of X-rays from keV to MeV energies. Designing detectors to maximise the sensitivity and resolution achievable with these sources is paramount to optimising laser-driven accelerators. In this article, we explore the key parameters associated with laser-driven X-ray sources and the detector systems required to characterise them. We present a concise approach to modelling the sensitivity and resolution for indirect detector systems factoring in both the optical collection and the X-ray attenuation within the scintillator.

Ultrabroadband flying-focus using an axiparabola-echelon pair.

Flying-focus pulses promise to revolutionize laser-driven secondary sources by decoupling the trajectory of the peak intensity from the native group velocity of the medium over distances much longer than a Rayleigh range. Previous demonstrations of the flying focus have either produced an uncontrolled trajectory or a trajectory that is engineered using chromatic methods that limit the duration of the peak intensity to picosecond scales. Here we demonstrate a controllable ultrabroadband flying focus using a nearly achromatic axiparabola-echelon pair. Spectral interferometry using an ultrabroadband superluminescent diode was used to measure designed super- and subluminal flying-focus trajectories and the effective temporal pulse duration as inferred from the measured spectral phase. The measurements demonstrate that a nearly transform- and diffraction-limited moving focus can be created over a centimeter-scale-an extended focal region more than 50 Rayleigh ranges in length. This ultrabroadband flying-focus and the novel axiparabola-echelon configuration used to produce it are ideally suited for applications and scalable to >100 TW peak powers.

Flexible tape-drive target system for secondary high-intensity laser-driven sources.

We present the development of a flexible tape-drive target system to generate and control secondary high-intensity laser-plasma sources. Its adjustable design permits the generation of relativistic MeV particles and x rays at high-intensity (i.e., ≥1 × 1018 W cm-2) laser facilities, at high repetition rates (>1Hz). The compact and robust structure shows good mechanical stability and a high target placement accuracy (<4 μm RMS). Its compact and flexible design allows for mounting in both the horizontal and vertical planes, which makes it practical for use in cluttered laser-plasma experimental setups. The design permits ∼170° of access on the laser-driver side and 120° of diagnostic access at the rear. A range of adapted apertures have been designed and tested to be easily implemented to the targetry system. The design and performance testing of the tape-drive system in the context of two experiments performed at the COMET laser facility at the Lawrence Livermore National Laboratory and at the Advanced Lasers and Extreme Photonics (ALEPH) facility at Colorado State University are discussed. Experimental data showing that the designed prototype is also able to both generate and focus high-intensity laser-driven protons at high repetition rates are also presented.