Probe Laser Beam Research Articles

Ultrafast 2D-IR spectroscopy of intensely optically scattering pelleted solid catalysts.

Solid, powdered samples are often prepared for infrared (IR) spectroscopy analysis in the form of compressed pellets. The intense scattering of incident light by such samples inhibits applications of more advanced IR spectroscopic techniques, such as two-dimensional (2D)-IR spectroscopy. We describe here an experimental approach that enables the measurement of high-quality 2D-IR spectra from scattering pellets of zeolites, titania, and fumed silica in the OD-stretching region of the spectrum under flowing gas and variable temperature up to ∼500 ◦C. In addition to known scatter suppression techniques, such as phase cycling and polarization control, we demonstrate how a bright probe laser beam comparable in strength with the pump beam provides effective scatter suppression. The possible nonlinear signals arising from this approach are discussed and shown to be limited in consequence. In the intense focus of 2D-IR laser beams, a free-standing solid pellet may become elevated in temperature compared with its surroundings. The effects of steady state and transient laser heating effects on practical applications are discussed.

Dynamic Optical Grating Based on a Photomechanical Molecular Crystal

AbstractOrganic photomechanical crystals transform molecular‐scale photoisomerization events into largescale crystal shape changes. The results in this paper demonstrate that this photomechanical motion can be harnessed to reconfigure reflective elements on the crystal surface to actively control light propagation. This is accomplished by using a single organic photomechanical crystal composed of 1,2‐bis(2,4‐dimethyl‐5‐phenyl‐3‐thienyl)‐3,3,4,4,5,5‐hexafluoro‐1‐cyclopentene, which undergoes a reversible ring‐open to ring‐closed photoisomerization. Electron beam lithography patterning followed by a sublimation development step leaves periodically positioned, 120 nm deep grooves that are coated with gold metal to form a reflective grating on the crystal surface. Under UV irradiation, expansion of the bulk crystal increases the grating period by ≈5% and changes the diffraction angle of a 633 nm probe laser beam by 0.7° (first order) and 1.3° (second order). The grating period change can be reversed by visible light exposure and repeated for multiple cycles. The crystal expansion and thus the diffraction angle can also be continuously tuned by controlling the duration of light exposure. Anisotropic crystal expansion and contraction due to molecular photoisomerization enables low‐power light sources to steer light beams continuously over a range of diffraction angles.

Optimization of beam shaping and error quantification of calibration approach using E-FISHG based electric field measurements

Electric-field measurement based on the electric-field-induced second-harmonic generation (E-FISHG) method is a promising tool for a noncontact field measurement in plasmas and gases. For the E-FISHG method, a probing laser beam is focused at the measurement target by a lens, and the signals integrated along the laser path are acquired. Although the signal is frequently calibrated under uniform electric fields, the yielded value is erroneous if one does not consider the difference in the electric-field-profiles between the calibration and measurement. In this paper, we review the calibration and measurement targets of relevant studies, assess the error in the conventional method for the streamer discharge measurement, and give guidelines on which calibration approach to use depending on the electric field profile to be measured. Our approach uses cylindrical-to-cylindrical electrodes and multipoint measurement corresponding to the target length along the optical path, gas, and pressure.

STUDY OF NEGATIVE REFRACTIVE INDEX IN Rb FOUR-LEVEL N-TYPE ATOMIC GAS MEDIUM

In this work, we study the generation of a negative refractive index based on electromagnetically induced transparency (EIT) in a Rb four-level N-type atomic gas medium. We derive analytic expressions for the relative permittivity and relative permeability of the medium according to the parameters of the probe, pump, and signal laser fields. We then investigate the variation of the real parts of the relative permittivity and relative permeability with respect to the intensity and frequency of the pump and signal laser fields. In the presence of the pump laser beam, the medium becomes transparent to the probe laser beam even in the resonant region. At the same time, the real parts of the relative permittivity and relative permeability are simultaneously negative (i.e., the medium exhibits a negative refractive index) in the EIT spectral domain. In the presence of the signal laser beam, the EIT effect occurs over two different frequency domains of the probe beam, so a negative refractive index is also generated in these two frequency domains. The investigation of the real parts of the relative permittivity and relative permeability with intensity and frequency of the pump and signal laser fields allowed us to find the laser parameters for the appearance of the negative refractive index, which can be useful for experimental observations.

Diagnosing X-pinch and cylindrical wire array Z-pinch with an all-optical framing camera on the “QiangGuang-I” facility

An all-optical framing camera has been established on the 1-MA “QiangGuang-I” facility for investigating the imploding dynamics of the X-pinch and the cylindrical wire array Z-pinch. This camera measures the photons flux distribution by detecting the photon-induced refractive index changes in the InP semiconductor with a probe laser beam. The InP-based imaging sensor with a 100 nm thick Al film and a 10 μm thick gold transmission grating of 20 μm spatial period was fabricated based on the lithography method. Two sequential frames with 1.5 ns time resolution and 13 ns inter frame separation time can be recorded in one single shot. Framing images indicating the plasma generation and dissipation of the X-pinch and the cylindrical wire array Z-pinch have been obtained, showing that this framing camera is a promising technique for investigating the mechanisms of the Z-pinch and other high energy density physics.

Systematic 1D electric field induced second harmonic measurement on primary-to-secondary transition phase of positive streamer discharge in atmospheric-pressure air

The electric field induced second harmonic generation (E-FISH) technique has been widely utilized for the electric field measurement of atmospheric-pressure nonthermal plasmas. However, the measurement accuracy has not been quantified. Further, the E-FISH signal generation that is necessary to the evaluation of the measurement accuracy has been formulated only for the probe laser beam focused by a spherical lens and not for the cylindrical lens. Here, the E-FISH method utilizing the focusing cylindrical lens was studied for accurate one-dimensional (1D) electric field measurement of the primary-to-secondary transition phase of a single-filament positive streamer discharge generated in atmospheric-pressure air. A combination of numerical analysis and the E-FISH signal measurement was used to establish the radial distribution of the electric field vectors and the accompanying measurement accuracy. The E-FISH methodology captured a distinct evolution in the 1D electric field varying over timescales of ns and length scales of 100 µm. At the instant when the primary streamer arrived at the cathode, the electric field at 3 mm above the cathode surface was found to be as high as 225 Td, while the field at 10 mm above the cathode surface was as low as 5 Td. At the final stage of the primary-to-secondary transition phase completed in 3 ns from the primary streamer arrival at the cathode, the electric field at 3 mm above the cathode was found to be lower than that observed at 10 mm from the cathode; this finding is consistent with predictions made based on a previous model describing the initiation of the secondary streamer discharge and previously published electron density measurement.

Measurement of the temperature dependency of the linewidths and amplitudes of the sub-Doppler resonances of the 87Rb D2 line with π (π) polarized pump (probe) laser beams

Measurement of the temperature dependency of the linewidths and amplitudes of the sub-Doppler resonances of the 87Rb D2 line with π (π) polarized pump (probe) laser beams

Linear and nonlinear Bragg diffraction by electromagnetically induced gratings with PT symmetry and their active control in a Rydberg atomic gas

Due to its myriad applications in many fields of science and technology, novel light diffraction from specially designed optical gratings is a subject of great interest. Here, we propose a scheme to realize the linear and nonlinear Bragg diffractions from an electromagnetically induced grating (EIG) with parity-time $(\mathcal{PT})$ symmetry in a cold Rydberg atomic gas, where the Rydberg-Rydberg interaction between atoms are mapped to strong and long-range interaction between photons, characterized by a giant nonlocal Kerr nonlinearity. We show that a probe laser beam with very low light intensity incident upon the $\mathcal{PT}$-symmetric EIG can display distinctive asymmetric diffraction patterns, which can be actively manipulated through tuning the gain-absorption coefficient of the EIG and the input power of the laser beam. We also show that the intensity distribution among different diffraction orders depends significantly on the $\mathcal{PT}$-symmetry property of the EIG and on the magnitude and nonlocality degree of the Kerr nonlinearity. In addition, we demonstrate that such Bragg diffraction patterns can be controlled by an external gradient magnetic field, which provides a different way of diffraction control. The research results reported here are not only useful for understanding the unique properties of linear and nonlinear Bragg diffractions by $\mathcal{PT}$-symmetric gratings but may also be promising for designing optical devices applicable in optical information processing and transmission.

Line Scanning with Gas-Coupled Laser Acoustic Detection

The Gas-Coupled Laser Acoustic Detection (GCLAD) is an optical technique for ultrasonic detection based on the deviation that a laser beam sustains when travelling in a fluid that features refractive index fluctuations. If the laser beam is perpendicular to the wave propagation direction, the technique enables simultaneous detection of direct waves in mechanical components and eventual echoes from defects to be achieved.The technique is applied to the inspection of elements predominantly extending in one/two dimensions as bars and axisymmetric pieces, exploiting a signal enhancement effect occurring in defects’ proximity. The phenomenon, namely constructive interference between wave crests of a direct Rayleigh ultrasound and those associated with reflections on a defect flank, is first illustrated numerically. The effect of parameters like the angle between wave propagation direction and source-receiver distance on the GCLAD sensitivity is then experimentally highlighted. The technique is finally implemented to B-scan a steel plate with 1 mm wide, 20 mm long, and 3 mm deep surface defects.Since the GCLAD probe laser beam insists on an entire line, defects present on that line can be identified without moving the device along such direction. This reduces the monitoring time compared to techniques leveraging on traditional air-coupled transducers or more sophisticated methods (Scanning Laser Source).

Spatial evolution of nitric oxide in ns-discharges using a 250 kHz optical parametric oscillator

In this article we present burst-mode nitric oxide laser-induced fluorescence (LIF) measurements at 250 kHz probing the first 500 µs evolution of a nanosecond repetitively pulsed discharge in the spark regime. The discharge energy was varied from 140 µJ to 180 µJ by adjusting the excitation voltage. The probe laser beam at 226 nm was produced by doubling the 452 nm output of an optical parametric oscillator (OPO) pumped by 355 nm output of a burst-mode laser. It was observed that the nitric oxide produced by the discharge developed a toroidal distribution around the electrode central axis over the first 200 µs after the last spark discharge with the maximum local nitric oxide concentration of 1.8 × 1024 m−3. The expansion of the toroidal distribution was tracked over time and space by the pulse-burst laser pumped OPO system for the first time.

Experimental observation of partial parity-time symmetry and its phase transition with a laser-driven cesium atomic gas

Realization and manipulation of parity-time (PT) symmetry in multidimensional systems are highly desirable for exploring nontrivial physics and uncovering exotic phenomena in non-Hermitian systems. Here, we report the first experimental observation of partial PT (pPT) symmetry in a cesium atomic gas coupled with laser fields, where a two-dimensional pPT-symmetric optical potential for probe laser beam is created. A transition of the pPT symmetry from an unbroken phase to a broken one is observed through changing the beam-waist ratio of the control and probe laser beams, and the domains of unbroken, broken, and non-pPT phases are also discriminated unambiguously. Moreover, we develop a technique to precisely determine the location of the exceptional point of the pPT symmetry breaking by measuring the asymmetry degree of the probe-beam intensity distribution. The findings reported here pave the way for controlling multidimensional laser beams in non-Hermitian systems via laser-induced atomic coherence, and have potential applications for designing new types of light amplifiers and attenuators

Satellite-assisted laser magnetometry with mesospheric sodium

Magnetic field sensing provides crucial insights into various geophysical phenomena such as atmospheric currents, crustal magnetism, and oceanic circulation. In this paper, a method for remote detection of magnetic fields using mesospheric sodium with an assisting satellite is proposed. Sodium atoms in the mesosphere are optically pumped with a ground-based laser beam. A satellite-borne detector is used to measure magneto-optical rotation of the polarization of a probe laser beam by the sodium atoms. This sensitive magnetometry method benefits from direct detection of laser photons and complements existing space- and aircraft-borne techniques by probing magnetic fields at upper-atmospheric altitudes inaccessible to those.

Generation and detection of axions using guided structures

We propose a new experimental technique to generate and detect axions in the lab with a good experimental sensitivity over a broad axion mass range. The scheme relies on using laser-based four-wave mixing, which is mediated by the hypothetical axion field. Intense pump and Stokes laser beams that are confined to a waveguide (i.e., for example, an optical fiber) with appropriately chosen frequencies resonantly drive axion generation. Under such a geometry, we predict the existence of guided axion waves, which we refer to as "axitons". These are solutions of the axion Klein-Gordon field equation that are spatially guided by the profiles of the driving pump and Stokes laser beams. These guided axitons can then couple to a nearby fiber and mix with another laser, affecting the propagation of a probe laser beam. A key advantage of the scheme is that the mass range of the hypothetical axion can be scanned by varying the frequencies of the pump and the Stokes laser beams. We predict that, using reasonable parameters, the technique will be able to detect axions in the mass range $10^{-6} $eV $< m<$ $10^{-2} $eV with a sensitivity at the level of $10^{-12}$ GeV$^{-1}$ for the axion-photon coupling constant.

Water-Based Coherent Detection of Broadband Terahertz Pulses.

Both solids and gases have been demonstrated as the materials for terahertz (THz) coherent detection. The gas-based coherent detection methods require a high-energy probe laser beam and the detection bandwidth is limited in the solid-based methods. Whether liquids can be used for THz detection and relax these problems has not yet been reported, which becomes a timely and interesting topic due to the recent observation of efficient THz wave generation in liquids. Here, we propose a THz coherent detection scheme based on liquid water. When a THz pulse and a fundamental laser beam are mixed on a free-flowing water film, a second harmonic (SH) beam is generated as the plasma is formed. Combining this THz-induced SH beam with a control SH beam, we successfully achieve the time-resolved waveform of the THz field with the frequency range of 0.1-18THz. The required probe laser energy is as low as a few microjoules. The sensitivity of our scheme is 1 order of magnitude higher than that of the air-based method under comparable detection conditions. The scheme is sensitive to the THz polarization and the phase difference between the fundamental and control SH beams, which brings direct routes for optimization and polarization sensitive detection. Energy scaling and polarization properties of the THz-induced beam indicate that its generation can be attributed to a four-wave mixing process. This generation mechanism makes simple relationships among the probe laser, THz-induced SH, and THz field, favorable for robustness and flexibility of the detection device.

A laser wakefield acceleration facility using SG-II petawatt laser system.

Laser wakefield acceleration (LWFA) using PW-class laser pulses generally requires cm-scale laser-plasma interaction Rayleigh length, which can be realized by focusing such pulses inside a long underdense plasma with a large f-number focusing optic. Here, we present a new PW-based LWFA instrument at the SG-II 5 PW laser facility, which employs f/23 focusing. The setup also adapted an online probing of the plasma density via Nomarski interferometry using a probe laser beam having 30fs pulse duration. By focusing 1-PW, 30-fs laser pulses down to a focal spot of 230 µm, the peak laser intensity reached a mild-relativistic level of 2.6 × 1018 W/cm2, a level modest for standard LWFA experiments. Despite the large aspect ratio of >25:1 (transverse to longitudinal dimensions) of the laser pulse, electron beams were observed in our experiment only when the laser pulse experienced relativistic self-focusing at high gas-pressure thresholds, corresponding to plasma densities higher than 3 × 1018cm-3.

The Story behind the First Automatic Atomic Force Microscope

Abstract:Over the past three decades, atomic force microscopy (AFM) has undergone a series of design changes to attain a flat XY scan and stable non-contact mode in ambient atmosphere. AFM has evolved into an ideal method for non-destructive scanning of samples with longer probe tip life, high accuracy, repeatability, and automation. Together with self-optimizing algorithms for scan parameters in the non-contact mode, AFM can become as widely adopted as other microscopies such as optical or scanning electron microscopy (SEM). Even full automation of AFM probe tip exchange is now possible with probe type recognition software and laser beam alignment on the cantilever and position-sensitive photo diode (PSPD). By separating the optics stage from the Z stage, an AFM system can be made with low mechanical noise and improved optical vision.

A new method for remote detection of ionizing radiation using transient optical absorption

Increasing demand for the detection of high-intensity ionizing radiation, especially the neutron radiation, puts forward the challenge to substantially enhance the radiation hardness of radiation detectors. We suggest an approach to meet this challenge by introducing an all-optical method to gauge the irradiation flux by radiation-induced modulation of the optical absorption coefficient in radiation-hard single crystals. We demonstrate the feasibility of this approach by using the transient absorption modulation caused by nonequilibrium charge carriers created in Gd2Al2Ga3O12:Ce (GAGG:Ce) crystal by the radiation to be detected. To optimize the detection unit, we mimicked the effect of ionizing radiation by using laser pulses to generate the nonequilibrium electron–hole pairs. The best sensitivity was obtained by exploiting multi-pass transitions of the probing laser beam in the GAGG:Ce single crystal with inclined opposite sides. The optimized system was then applied for the detection of X-ray pulses, and sufficient sensitivity and good linearity of its response was demonstrated. In the presented detection scheme, the radiation-hard detecting crystal is the only part of the system exposed to irradiation, enabling the system to be used for monitoring high-intensity neutron sources.

Noncollinear electro-optic sampling detection of terahertz pulses in a LiNbO3 crystal while avoiding the effect of intrinsic birefringence.

We propose and experimentally prove efficient high-resolution electro-optic sampling measurement of broadband terahertz waveforms in a LiNbO3 crystal in the configuration with the probe laser beam propagating along the optical axis of the crystal. This configuration allows one to avoid the detrimental effect of strong intrinsic birefringence of LiNbO3 without any additional optical elements. To achieve velocity matching of the terahertz wave and the probe beam, the terahertz wave is introduced into the crystal through a Si prism at the Cherenkov angle to the probe beam. The workability of the scheme at different wavelengths of the probe optical beam (800 and 1550 nm) is demonstrated.

Non-contact ultrasonic inspection by Gas-Coupled Laser Acoustic Detection (GCLAD)

Gas-Coupled Laser Acoustic Detection (GCLAD) is an ultrasonic, non-contact detection technique that has been recently proven to be applicable to the inspection of mechanical components. GCLAD response raises as the intersection length between the probe laser beam and the acoustic wavefront propagating in the air increases; such feature differentiates the GCLAD device from other optical detection instruments, making it a line detection system rather than a point detector. During the inspection of structures mainly extending in two dimensions, the capability to evidence presence of defects in whichever point over a line would enable moving the emitter and the detector along a single direction: this translates in the possibility to decrease the overall required time for interrogation of components compared to point detectors, as well as generating simpler automated monitoring layouts. Based on this assumption, the present study highlights the possibility of employing the GCLAD device as a line inspection tool. To this end, preliminary concepts are provided allowing maximization of the GCLAD response for the non-destructive testing of components which predominantly extend in two dimensions. Afterwards, the GCLAD device is employed in pulse-echo mode for the detection of artificial defects machined on a 12 mm-thick steel plate: the GCLAD probe laser beam is inclined to be perpendicular to the propagation direction of the airborne ultrasound, generated by surface acoustic waves (SAWs) in the solid which are first reflected by the defect flanks and subsequently refracted in the air. Numerical results are provided highlighting the SAW reflection patterns, originated by 3 mm deep surface and subsurface defects, that the GCLAD should interpret. The subsequent experimental campaign highlights that the GCLAD device can identify echoes associated with surface and subsurface defects, located in eight different positions on the plate. B-scan of the component ultimately demonstrates the GCLAD performance in accomplishing the inspection task.

Bright and Dark Soliton of Probe and Couple Laser Beam in an Electromagnetically Induced Transparency

Bright and Dark Soliton of Probe and Couple Laser Beam in an Electromagnetically Induced Transparency