Land-based Sources Research Articles

Macro marine litter survey of sandy beaches along the Cox's Bazar Coast of Bay of Bengal, Bangladesh: Land-based sources of solid litter pollution

Macro-sized marine litter (>2.5 cm) was collected, characterized, and enumerated along the Cox's Bazar Coast, Bangladesh. Marine litter abundance was converted to density (number of items/m2). Beach cleanliness was evaluated using the clean-coast index (CCI). Plastic polythene bags were the most abundant litter items, followed by plastic cups. Total marine litter abundance was 54,401 ± 184 items. Major sources of marine litter were from tourism, fishery and residential activities. Of 10 sites surveyed, two were classified as dirty, two were moderate, four were clean and two were very clean using the CCI. Marine litter pollution along the Cox's Bazar Coast represents a potential threat to coastal and marine environments. This baseline study will help to establish mitigation strategies that are urgently required to reduce marine litter pollution along the Cox's Bazar Coast.

Characterization of polycyclic aromatic hydrocarbons in the Great Lakes Basin using dreissenid mussels

The National Oceanic and Atmospheric Administration (NOAA), National Centers for Coastal Ocean Science (NCCOS) Mussel Watch Program (MWP), conducts basin-wide monitoring and place-based assessments using dreissenid mussels as bioindicators of chemical contamination in the Laurentian Great Lakes. Polycyclic aromatic hydrocarbons (PAHs) body burden results for the period 2009–2018 were combined into one dataset from multiple MWP studies allowing for a robust characterization of PAH contamination. Patterns in PAH data were identified using descriptive statistics and machine learning techniques. Relationships between total PAH concentration in dreissenid mussel tissue, impervious surface percentages, and PAH relative concentration were identified and used to build a predictive model for the Great Lakes Basin. Significant positive correlation was identified by the Spearman’s rank correlation test between total PAH concentration and percent impervious surface. The findings support the paradigm that PAHs are primarily derived from land-based sources. Offshore and riverine locations had the lowest and highest median total PAH concentrations, respectively. PAH assemblages and ratios indicated that pyrogenic sources were more predominant than petrogenic sources and that PAHs at offshore sites exhibited relatively more weathering compared to inshore sites.

Land-based Nitrogen Pollution Source Structure and Spatial Distribution in Guangdong-Hong Kong-Macao Greater Bay Area

Total nitrogen pollution from land-based sources carried by rivers is the main source of inorganic nitrogen entering the sea. Inorganic nitrogen pollution in the coastal waters of Guangdong-Hong Kong-Macao Greater Bay Area(GBA) is a serious problem. The water quality of an adjacent large area of the sea is classified as poor-category Ⅳ. Therefore, clarification of the scale, structure, and discharge pressure of nitrogen emissions from the land area of the GBA is needed to manage marine nitrogen pollution. Based on multi-source data, including land use, socio-economic statistics, and pollution source census information, the scale, source structure, and regional differences of total nitrogen discharge in GBA and surrounding cities were evaluated using administrative and watershed units. The results show that:①The total nitrogen emissions from the study area are approximately 332500 t. Residential waste is the main source of pollution, accounting for 55.4%, followed by cultivation, with 28.18%, while the contribution from animal husbandry and industrial production is relatively limited. ②The regional differences of total nitrogen emissions are obvious, and the total emissions from GBA(231400 t) are significantly higher than those from neighboring cities(101100 t). ③The distribution of marine pollution and intensity of land-based nitrogen pollution emissions are spatially consistent, which indicates that there is a large number of pollution emissions in the East River Basin, Northwest River Delta Basin, and Tan River Basin; the shoreline sections belonging to the basins carry the greatest emission pressure, lead to serious pollution in the Lingding Sea, Jin Bay, and Huangmao Sea.

Potential microplastic release from beached fishing gear in Great Britain's region of highest fishing litter density

While land-based sources of marine plastic pollution have gained widespread attention, marine-based sources are less extensively investigated. Here, we provide the first in-depth description of abandoned, lost or otherwise discarded fishing gear (ALDFG) on northern and southern beaches of the English Southwest Peninsula, Great Britain's region of highest ALDFG density. Three distinct categories were recorded: twisted rope (0.28 ± 0.14 m−1, 17%), braided rope (0.56 ± 0.28 m−1, 33%) and filament (0.84 ± 0.41 m−1, 50%), which likely correspond to fishing rope, net and line. Estimating the disintegration of ALDFG from length and filament number suggests that it has the potential to generate 1277 ± 431 microplastic pieces m−1, with fishing rope (44%) and net (49%) as the largest emitters. Importantly, ALDFG was over five times more abundant on the south coast, which is likely attributable to the three times higher fishing intensity in that area.

Design and Analysis of Ship Exhaust Boiler Flue Cleaning System Based on Computer

In recent years, the country for ship emissions of exhaust gas control is relatively loose, but also relatively lack of specific and effective supervision and scientific exhaust emissions and treatment technology, so China’s air pollution is increasingly serious. With the implementation of regulations on the emission of air pollutants from land-based sources such as motor vehicles and power stations, researchers have found that exhaust pollution from ships accounts for an increasing proportion of the overall air pollution, especially in port cities and coastal areas, causing great damage. In order to effectively reduce ship exhaust pollution in China, the Ministry of Transport through the establishment of ship emission control area program, stage by stage and regional limits on the sulfur content of fuel used by ships sailing in China’s ports and coastal inland river waters. Through the implementation of the regulations of the ship discharge control area, all kinds of pollutants discharged by ships have been significantly reduced, and the environment of the port area has been improved to a certain extent. At the same time, it is also necessary to use the computer and other high-tech constantly develop new ship exhaust cleaning mode to deal with the increasingly serious environmental pollution problem.

Anthropogenic nitrogen loading and risk of eutrophication in the coastal zone of Atlantic Canada

Nutrient pollution derived from human land-use activities remains a major cause of the eutrophication of coastal ecosystems around the world. In this study, we conduct a nutrient loading analysis for the coastal watersheds bordering the Bay of Fundy and Scotian Shelf of Atlantic Canada, a cold temperate region of the Northwest Atlantic that exhibits strong gradients in oceanographic conditions and human uses of the coastal zone, and where coastal development is expected to increase in the coming decades. Our objective was to apply the Nitrogen Loading Model (NLM) framework to determine the regional distribution and intensity of nitrogen inputs from land-based sources (wastewater, atmospheric deposition, land use, fertilizer applications, and regional industries) to coastal marine environments, and subsequently identify coastal embayments at risk of developing symptoms of eutrophication. Across all 109 watersheds examined, the estimated mean total nitrogen load varied by three orders of magnitude. The largest loads occurred in the most heavily urbanized and densely populated watersheds, where wastewater inputs contributed the most (>80%) to loading rates. Where the footprint of human activity was small, atmospheric deposition of nitrogen was an important contributor to the total load; however, localized point sources (i.e. seafood processing, fur farming) were significant contributors to the total load in smaller sized watersheds. Coastal embayments with small surface areas and low tidal exchange volumes were most likely to have estuarine loading rates that exceeded previously established thresholds for the loss of submerged aquatic vegetation (e.g., eelgrass). In contrast, none of the embayments were deemed likely to develop anoxia. This analysis enables a novel comparison of nitrogen loading from watersheds across a range of land cover types, watershed characteristics, and human land-use activities, while providing a baseline for the detection of future environmental change in the region. Overall, we emphasize the importance of including human activities that occur on the landscape in future marine coastal planning.

Strategies to Overcome Marine Pollution Caused by Plastic Waste to Protect Marine Environment in Indonesia

Nowadays marine pollution become a serious problem in the world espesially in Indonesia. Marine scientists have found harmful impact of marine pollution to marine environment, ecosystem and humans, there-quarter of all marine debris is plastic, a persistent and potentially hazardous pollutan. Plastic can be chemically harmful to wildlife, either because themselves potentially toxic or other toxic pollutan, the situation become worse when it come to marrine pollution caused by micro plastic, micro plastic is very dangerous for the ecosystem and the human in the world. Public awaarness to participate in maintaining the marine environment is decreasing day by day. Some people do not realise that microplastic are so danger to marine environment because most plastics in the ocean break up into very small particles, plastic is one of the kind of marine debris and it can come in all shapes and size, but those that are less than five millimeter in length. Indonesia is the second-biggest-contributor to ocean after China, with some estimates suggesting it is source of about 10% of global plastic pollution, if this problem can not be solved, there could be more plastic than fish in the ocean. Unfortunetly up to present we do not have any effective methode to clean up the ocean, the only thing that we can do is reduce the use of plastic in daily life. Marine pollution is become global problem so that is why we need some strategies to solved this problem, based on internatinal frame work Indonesia and others contries should do cooperation with others country and based on national legal frame works government should make special regulation to protect marine environment. Pollution from land-based sources, either direcly by urban or argiculuture discharger or indirecly through water. Keyword: Marrine, Pollution, ASEAN

Trend analysis of anthropogenic activities affecting trace metals deposition in core sediments from the coastal and four rivers estuary of Sarawak, Malaysia.

This study reports the concentrations of trace metals in core sediments profile from the coastal and four rivers estuary in the Kuching Division of Sarawak, Malaysia, and the controlling mechanisms influencing their availability in sediments of the studied area. The bonding of trace metals with non-mobile fractions was confirmed with the sequential extraction. Inductively coupled plasma-optical emission spectroscopy (ICP-OES) was used to measure the concentrations of the trace metals. Granulometric analyses were performed using normalized sieve apertures to determine the textural characteristics of the sediments. Enrichment factor was used to evaluate the level of metal enrichment. Heavy metals concentrations in sediment samples varied in the range: Pb (8.9-188.9mg/kg d.w.), Zn (19.4-431.8mg/kg d.w.), Cd (0.014-0.061mg/kg d.w.), Ni (6.6-33.4mg/kg d.w.), Mn (2.4-16.8mg/kg d.w.), Cu (9.4-133.3mg/kg d.w.), Ba (1.3-9.9mg/kg d.w.), As (0.4-7.9mg/kg d.w.), Co (0.9-5.1mg/kg d.w.), Cr (1.4-7.8mg/kg d.w.), Mg (68.8-499.3mg/kg d.w.), Ca (11.3-64.9mg/kg d.w.), Al (24.7-141.7mg/kg d.w.), Na (8.8-29.4mg/kg d.w.), and Fe (12,011-35,124.6mg/kg d.w.). The estimated results of the enrichment factor suggested enrichments of Pb, Zn, and Cu in all the core sediment samples and depths at all sites. The other trace metals showed no enrichments in almost all the sampled stations. Continuous accumulation of Pb, Zn, and Cu metals over a period can be detrimental to living organisms and the ecology. The results obtained from the statistical analyses suggested that the deposition of trace metals in the studied sites is due to anthropogenic inputs from the adjacent land-based sources.

Estimation of land-based emissions during container terminal operations in the Ambarlı Port, Turkey

Many types of mobile vehicles are used simultaneously in container terminal operations. Because most of these mobile vehicles have diesel engines, they emit a significant amount of pollutant emissions into the atmosphere during their operation. They are considered as land-based mobile emission sources (MobES) and should be included in the total port emission inventory. The emission inventory is a basic requirement in developing an environmental management strategy to improve emission control. In this context, this study aims to estimate the emission inventories of mobile vehicles used in terminal operations in the Ambarlı container ports located in the city of Istanbul, which is one of the most populous cities in the world. In this respect, the amounts of the emissions of all the container handling equipment with diesel engines in the port areas, including external trucks delivering/receiving containers to/from the port were estimated using an activity-based method. It has been found that approximately 42.39% of the total CO2 emission is owing to terminal tractors and the total annual CO2 value per TEU (Twenty-foot Equivalent Unit) of MobES is 0.01259 tons. The CO2 value per TEU can serve as a CO2 emission performance indicator for land-based MobES in process of the evaluation of emission inventories in container ports.

Changes in (micro and macro) plastic pollution in the sediment of three sandy beaches in the Eastern Mediterranean Sea, in relation to seasonality, beach use and granulometry

Smaller sized plastics (microplastics or MPs <5 mm) are ubiquitous in nature and have been found to interact in diverse ways with most biotic and abiotic systems globally. Most MPs in the seas have a land-based source, however, little is known about how the transfer occurs. In our study, we used three sandy beaches to describe the process of how MPs travel from accumulation points at the backshore of the beach to the sea, and vice versa. MPs differed significantly in all three beaches (both in quantitative and qualitative terms) between the summer and the winter samplings. During the summer, heavy MPs are the majority, while during the winter, lightweight microplastics are predominant, and the ratio of heavy per lightweight MPs is affected by the sediment median diameter after the summer sampling. Macroplastics follow a similar pattern to MPs and appear to provide a source of MPs for the sea.

Stranded marine debris on the touristic beaches in the south of Bali Island, Indonesia: The spatiotemporal abundance and characteristic

Stranded marine debris (MD) has become a hot topic on Bali Island because it threatens coastal tourism sustainability. This study aims to investigate the spatiotemporal abundance and characteristics of MD on 14 touristic beaches in Bali Island. Sampling is carried out twice every season by adapting methods from NOAA's MD program. We found that the average MD abundance and weight were 0.356 ± 0.366 items/m2 and 4.057 ± 3.892 g/m2, respectively. Plastic dominated the MD based on abundance (86.9%) and weight (40.1%). Plastic bags, straws, and plastic cups are the most common items among plastics. The MD is originated from Indonesia and is dominated by land-based sources. The beaches are categorized as dirty in the rainy seasons and clean in the dry seasons. Statistically, the MD based on abundance, weight, category, source, and level of cleanliness varied significantly between seasons.

Modeling the Pathways and Accumulation Patterns of Micro- and Macro-Plastics in the Mediterranean

The Mediterranean is considered a hot-spot for plastic pollution, due to its semi-enclosed nature and heavily populated coastal areas. In the present study, a basin-scale coupled hydrodynamic/particle drift model was used to track the pathways and fate of plastics from major land-based sources (coastal cities and rivers), taking into account of the most important processes (advection, stokes drift, vertical and horizontal mixing, sinking, wind drag, and beaching). A hybrid ensemble Kalman filter algorithm was implemented to correct the near- surface circulation, assimilating satellite data (sea surface height, temperature) in the hydrodynamic model. Different size classes and/or types of both micro- and macroplastics were considered in the model. Biofouling induced sinking was explicitly described, as a possible mechanism of microplastics removal from the surface. A simplified parameterization of size-dependent biofilm growth has been adopted, as a function of bacterial biomass (obtained from a biogeochemical model simulation), being considered a proxy for the biofouling community. The simulated distributions for micro- and macroplastics were validated against available observations, showing reasonable agreement, both in terms of magnitude and horizontal variability. An 8-year simulation was used to identify micro- and macroplastics accumulation patterns in the surface layer, water column, seafloor and beaches. The impact of different processes (vertical mixing, biofouling, and wind/wave drift) was identified through a series of sensitivity experiments. For both micro- and macroplastics, distributions at sea surface were closely related to the adopted sources. The microplastics concentration was drastically reduced away from source areas, due to biofouling induced sinking, with their size distribution dominated by larger (&amp;gt;1 mm) size classes in open sea areas, in agreement with observations. High concentration patches of floating plastics were simulated in convergence areas, characterized by anticyclonic circulation. The distribution of macroplastics on beaches followed the predominant southeastward wind/wave direction. In the water column, a sub-surface maximum in microplastics abundance was simulated, with increasing contribution of smaller particles in deeper layers. Accumulation of microplastics on the seafloor was limited in relatively shallow areas (&amp;lt;500 m), with bottom depth below their relaxation depth due to defouling. The simulated total amount of floating plastics (∼3,760 tonnes) is comparable with estimates from observations.

Effect of Physical Characteristics and Hydrodynamic Conditions on Transport and Deposition of Microplastics in Riverine Ecosystem

Microplastic disposal into riverine ecosystems is an emergent ecological hazard that mainly originated from land-based sources. This paper presents a comprehensive review on physical processes involved in microplastics transport in riverine ecosystems. Microplastic transport is governed by physical characteristics (e.g., plastic particle density, shape, and size) and hydrodynamics (e.g., laminar and turbulent flow conditions). High-density microplastics are likely to prevail near riverbeds, whereas low-density particles float over river surfaces. Microplastic transport occurs either due to gravity-driven (vertical transport) or settling (horizontal transport) in river ecosystems. Microplastics are subjected to various natural phenomena such as suspension, deposition, detachment, resuspension, and translocation during transport processes. Limited information is available on settling and rising velocities for various polymeric plastic particles. Therefore, this paper highlights how appropriately empirical transport models explain vertical and horizontal distribution of microplastic in riverine ecosystems. Microplastics interact, and thus feedback loops within the environment govern their fate, particularly as these ecosystems are under increasing biodiversity loss and climate change threat. This review provides outlines for fate and transport of microplastics in riverine ecosystems, which will help scientists, policymakers, and stakeholders in better monitoring and mitigating microplastics pollution.

Occurrence of microplastics and phthalate esters in urban runoff: A focus on the Persian Gulf coastline

Urban runoff seems an obvious pathway for the transfer of microplastics (MPs) and phthalate acid esters (PAEs) from land-based sources to the marine environment; an issue that still lacks attention. This study presents the first results on MP and PAE levels in the urban runoff into the northern part of the Persian Gulf during the dry season. Average concentrations of MPs and PAEs in the urban runoff of eight selected sampling sites (N = 72) along the Bushehr coast were 1.86 items/L and 53.57 μg/L, respectively. MPs with a size range of 500-1000 μm had the highest abundance, and the mean levels of PAEs in MPs were 99.77 μg/g. The results of this study show that urban runoff is a main source of MP and PAE contaminants that are discharged into the Persian Gulf. Therefore, to decrease these pollutants from entering the aquatic environment, decision-makers in the area should consider this problem and stop the direct discharging of urban runoff into water bodies.

Traceability and Emission Reduction of Dissolved Inorganic Nitrogen in Minjiang Estuary, China.

The accumulation of dissolved inorganic nitrogen (DIN) in estuaries has become a global environmental problem. A two-dimensional, hydrodynamic water quality model was constructed in this study to investigate the sources of DIN pollution in the Minjiang Estuary. The concentration response field between the stream input and DIN in the estuary was established by using the surveyed source data of the study area. A sharing coefficient method was used to calculate the contribution percentage of each outfall to derive and propose a reasonable nitrogen reduction plan. The results showed that the input of land-based nitrogen into the Minjiang River contributed more than half of the DIN in the near-shore sea; the middle and upper reaches of the Minjiang River largely influenced the estuary area (38.57%). Conversely, the estuary and the coastline accounted for a smaller proportion of only 5.24%, indicating that an integrated DIN reduction should be implemented in the estuary area of the whole river basin. The model calculations showed that the reduction results, after remediation according to the current national standards for wastewater discharge in rivers, were not satisfactory. Thus, a new scheme is proposed in this paper—the total nitrogen (TN) input from land-based sources into the Minjiang Estuary and from the Shuikou Dam to the Min’an section should be reduced to below 31.64%; simultaneously, the DIN concentration discharged from the Shuikou Dam should be controlled and maintained below 0.5 mg·L−1 (TN = 0.8 mg·L−1). These results will provide guidelines for developing strategies for the improvement of DIN and water quality in similar estuaries.

The first baseline estimation of marine litter in Port Elizabeth, South Africa

Data on marine litter is crucial to guide waste management but is scarce in third-world countries such as South Africa. We established the first baseline measurement of litter accumulation on two beaches differing in public access in Port Elizabeth, Eastern Cape, the poorest province in South Africa. Four 10-day surveys were conducted on each beach between June 2019 and June 2020. Results revealed that most of the litter (95.7%) was of South African origin and likely came from local land-based sources (e.g., beachgoers or a local river). Daily accumulation rates at the study sites ranged between 24.58 and 86.54 items·100 m−1·day−1, an order of magnitude lower than rates from other cities in Africa. However, like elsewhere, plastic (including foam) made up the bulk (74.2%) of litter with food packaging contributing a large portion of this. These findings indicate that local interventions are warranted to reduce litter in Port Elizabeth.

Cross-oceanic distribution and origin of microplastics in the subsurface water of the South China Sea and Eastern Indian Ocean

Marine microplastic (MP) pollution is a global environmental problem that has received attention from scientific researchers and the public for the past several decades. However, without a suitably large-volume sampling method, the presence of MPs in subsurface water (< 5 m) is poorly understood. Here, MP content in subsurface water was determined using a pump-underway ship intake system along the cross-oceanic transect from the Pearl River Estuary to the Indian Ocean. The study regions have always been considered as one of the major MPs hotspots in the global oceans and still lack of study. Generally, MP abundance ranged between 0 and 4.97 items m-3, with an overall mean value of 0.40 ± 0.62 items m-3. A total of 679 MP particles were identified using μ-FT-IR. These collections identified polyethylene (PE), polypropylene (PP), and polyester (PET) as the major polymers represented (73.14–88.81%). The presence of MPs in coastal regions was significantly higher than that in the open ocean, revealing the contribution of land-based sources to marine MPs and the ocean dynamics. Therefore, an effective and feasible way to retard the penetration of MPs into the marine environment is to exhibit controls at the source. No significant correlation was found between the MP abundance and the physical and chemical properties of water. The results of the analysis of similarities (ANOSIM) and non-metric multidimensional scaling (NMDS) also showed that MP communities in different environments were significantly greater than the differences in different sites within the same environment. These findings of this study provide reliable information on MP distribution and characterization in cross-oceanic region of South China Sea and Eastern Indian Ocean, which will help to improve our understanding about the fate of MPs in the ocean.

Potential microplastic release from the maritime industry: Abrasion of rope

While land-based sources of plastic pollution have gained increasing attention in recent years, ocean-based sources have been less well studied. The aim of this study was to compare a variety of ropes (differing in age, wear surface and material) to quantify and characterise the production of microplastic during use. This was achieved by simulating, in laboratory and field experiments, rope hauling activity which is typically performed on board maritime vessels, such as fishing boats. Microplastic generation was quantified by collecting fragments that were released as a consequence of abrasion. Notably, we show that microplastic fragments generated from rope wear during use were characteristically irregular in shape, rather than fibrous such as those assigned to synthetic rope by previous studies. Therefore, we suggest that some of the plastic fragments found in the marine environment may have been falsely attributed to land-based sources but have in fact arisen form the abrasion of rope. Our research found that new and one-year old polypropylene rope released significantly fewer microplastic fragments (14 ± 3 and 22 ± 5) and less microplastic mass (11 ± 2 and 12 ± 3 μg) per metre hauled compared to ropes of two (720 ± 51, 247 ± 18 μg) or ten (767 ± 55, 1052 ± 75 μg) years of age. We show that a substantial amount of microplastic contamination is likely to directly enter the marine environment due to in situ rope abrasion and that rope age is an important factor influencing microplastic release. Our research suggests the need for standards on rope maintenance, replacement, and recycling along with innovation in synthetic rope design with the aim to reduce microplastic emission.

Biodiversity of Upwelling Coastal Systems of the Southern Caribbean Sea Adjacent to Guajira Peninsula

This paper describes the unique natural communities and biodiversity of the upwelling coastal system along the Guajira peninsula in the southern Caribbean Sea. The Guajira peninsula has a small human population with limited infrastructure and limited opportunities for coastal research, yet its coastal upwelling system is unique in the Tropical Western Atlantic region. This report includes both field observations along with a review of literature on the biodiversity of coastal eastern Guajira. In addition, it identifies missing information on the coastal system that is key to its management and conservation. Mangrove wetlands along with submerged aquatic vegetation (SAV) communities in a combination of consolidated and unconsolidated shorelines (e.g., rocky shores, cliffs, and beaches) form unique habitats in eastern Guajira. The diversity of these habitats is illustrated with the Bahia Hondita marine lagoon, where critical nursery habitat for several commercial valuable and endangered fisheries species, including sharks and sea turtles, is observed. Less information is available on more cryptic fauna, invertebrates, and coastal plankton species. Several anthropogenic factors are threatening species diversity in coastal Guajira, including overgrazing, mining, and target-species overfishing. Additional threats, such as extreme weather events (e.g., storms and droughts) as well as changes in coastal water quality, are also impacting species. The protection of the Guajira’s biodiversity would depend on local communities’ governance and empowerment as well as law enforcement for mining and agriculture operations. Management plans can include reducing land-based sources of pollution and building coastal resilience for climate change.

Exposure radius of a local coal mine in an Arctic coastal system; correlation between PAHs and mercury as a marker for a local mercury source

Mercury in the Arctic originates from emissions and releases at lower latitudes and, to a lesser extent, from local and regional sources. The relationship between mercury (Hg) and polycyclic aromatic hydrocarbons (PAHs) in sediment can be applied as an indicator of the mercury source. This research examines the Hg contamination gradient from a land-based coal mine to the surrounding coastal environment to quantify the impact of local sources. Total mercury and PAH (Σ14PAH) were measured in terrestrial and marine sediments as well as in marine biota. Samples were collected at the mine and two reference sites. Mercury and Σ14PAH concentrations in samples collected at the mine site were significantly higher than those at the reference sites. This was also found in the biota samples, although less pronounced. This work addresses the complexities of interpreting data concerning very low contaminant levels in a relatively pristine environment. A clear correlation between PAH and Hg concentration in sediment was found, although a large number of samples had levels below detection limits. PAH profiles, hierarchical clustering, and molecular diagnostic ratios provided further insight into the origin of PAHs and Hg, showing that signatures in sediments from the nearest reference site were more similar to the mine, which was not the case for the other reference site. The observed exposure radius from the mine was small and diluted from land to water to marine biota. Due to low contamination levels and variable PAH profiles, marine biota was less suitable for tracing the exposure radius for this local land-based Hg source. With an expected increase in mobility and availability of contaminants in the warming Arctic, changes in input of PAHs and Hg from land-based sources to the marine system need close monitoring.Graphical abstract