Kinetic Magnetoelectric Effect Research Articles

Spontaneous Inversion Symmetry Breaking and Emergence of Berry Curvature and Orbital Magnetization in Topological ZrTe_{5} Films.

ZrTe_{5} has recently attracted much attention due to the observation of intriguing nonreciprocal transport responses which necessitate the lack of inversion symmetry (I). However, there has been debate on the exact I-asymmetric structure and the underlying I-breaking mechanism. Here, we report a spontaneous I breaking in ZrTe_{5} films, which initiates from interlayer sliding and is stabilized by subtle intralayer distortion. Moreover, we predict significant nonlinear anomalous Hall effect (NAHE) and kinetic magnetoelectric effect (KME), which are attributed to the emergence of Berry curvature and orbital magnetization in the absence of I symmetry. We also explicitly manifest the direct coupling between sliding ferroelectricity, NAHE, and KME based on a sliding-dependent k·p model. By studying the subsurface sliding in ZrTe_{5} multilayers, we speculate that surface nonlinear Hall current and magnetization would emerge on the natural cleavage surface. Our findings elucidate the sliding-induced I-broken mechanism in ZrTe_{5} films and open new avenues for tuning nonreciprocal transport properties in Van der Waals layered materials.

Universal responses in nonmagnetic polar metals

We demonstrate that two phenomena, the kinetic magnetoelectric effect and the nonlinear Hall effect, are universal to polar metals as a consequence of their coexisting and contraindicated polarization and metallicity. We show that measurement of the effects provides a complete characterization of the nature of the polar metal, in that the nonzero response components indicate the direction of the polar axis, and the coefficients change signs on polarization reversal and become zero in the nonpolar phase. We illustrate our findings for the case of electron-doped PbTiO3 using a combination of density functional theory and model Hamiltonian-based calculations. Our model Hamiltonian analysis provides crucial insight into the microscopic origin of the effects, showing that they originate from inversion-symmetry-breaking-induced interorbital hoppings that correlate to an asymmetric charge density quantified by odd-parity charge multipoles. Our paper both heightens the relevance of the kinetic magnetoelectric and nonlinear Hall effects, and broadens the platform for investigating and detecting odd-parity charge multipoles in polar metals. Published by the American Physical Society 2024

Kinetic magnetoelectric effect in topological insulators

The kinetic magnetoelectric effect is an orbital analog of the Edelstein effect and offers an additional degree of freedom to control magnetization via the charge current. Here we theoretically propose a gigantic kinetic magnetoelectric effect in topological insulators and interpret the results in terms of topological surface currents. We construct a theory of the kinetic magnetoelectric effect for a surface Hamiltonian of a topological insulator, and show that it well describes the results by direct numerical calculation. This kinetic magnetoelectric effect depends on the details of the surface, meaning that it cannot be defined as a bulk quantity. We propose that Chern insulators and Z2 topological insulators can be a platform with a large kinetic magnetoelectric effect, compared to metals by 5–8 orders of magnitude, because the current flows only along the surface. We demonstrate the presence of said effect in a topological insulator, identifying Cu2ZnSnSe4 as a potential candidate.

Electrical magnetochiral effect and kinetic magnetoelectric effect induced by chiral exchange field in helical magnetics

The features of spin and charge transport in conductive helimagnets, which are due to the action of an inhomogeneous exchange magnetic field on the spin of conduction electrons, are theoretically studied. The interaction between the spin of moving particles and an inhomogeneous external magnetic field was first recorded in the famous Stern-Gerlach experiment that investigated the quantum nature of spin. In the present paper, we have demonstrated that two physical effects---the electrical magnetochiral effect (EMChE) and the kinetic magnetoelectric effect (KMEE)---can be explained through the interaction of the spins of itinerant electrons in chiral helimagnets with spatially inhomogeneous effective magnetic field of exchange origin. All parameters of the EMChE and KMEE are presented in terms of both the characteristic frequencies of spin relaxation of conduction electrons in a helimagnet and the frequencies of their Larmor precession in external and internal exchange fields. It has been shown that the effective frequency of conduction-electron spin relaxation in a helimagnet contains three components: (i) the rate of spin-lattice relaxation caused by spin-orbit scattering of conduction electrons by defects of the crystal lattice, (ii) the rate of change in the average spin of electrons due to their ``diffusion'' escape from a region with a given direction of the average spin to a region with a different direction of spin density, and (iii) the contribution of the Larmor precession of the spins of electrons moving in the helimagnet's exchange field that assigns the precession axis altering its direction in space. The peculiarities of the EMChE and KMEE that substantially depend on the ratio of the above-listed spin relaxation rates and the angular frequencies of electron precession are described. The numerical estimates performed show that the mechanism of generating EMChE provides the effect magnitude sufficient to be experimentally detected in metallic helimagnets. The frequency regions of spin relaxation and spin precession are determined to observe a giant electrical magnetochiral effect and resonant behavior of the chiral magnetoresistance. We have called the appropriate effect ``magnetochiral kinetic resonance'' (MChKR). The physical nature of MChKR is elucidated. The latter arises due to the coincidence of the Larmor precession frequency of an electron in the effective field and the phase change frequency of the helicoidal exchange field acting on the electron moving along the helicoid's axis with a speed equal to that of the electron flow. We have demonstrated how the experimental studies of the KMEE can be used to directly determine the chirality of helimagnets.

Orbital Edelstein effect from density-wave order

Coupling between charge and spin, and magnetoelectric effects more generally, have been an area of great interest for several years, with the sought-after ability to control magnetic degrees of freedom via charge currents serving as an impetus. The orbital Edelstein effect (OEE) is a kinetic magnetoelectric effect consisting of a bulk orbital magnetization induced by a charge current. It is the orbital analogue of the spin Edelstein effect in spin-orbit coupled materials, in which a charge current drives nonzero electron spin magnetization. The OEE has recently been investigated in the context of Weyl semimetals and Weyl metals. Motivated by these developments, we study a model of electrons without spin-orbit coupling which exhibits line nodes that get gapped out by via symmetry breaking due to an interaction-induced charge density wave order. This model is shown to exhibit a temperature dependent OEE, which appears due to symmetry reduction into a gyrotropic crystal class.

Magnetoelectric effect in band insulator–ferromagnet heterostructures

We theoretically study magnetoelectric effects in a heterostructure of a generic band insulator and a ferromagnet. In contrast to the kinetic magnetoelectric effect in metals, referred to as the Edelstein effect or the inverse spin galvanic effect, our mechanism relies on virtual interband transitions between the valence and conduction bands and therefore immune to disorder or impurity scattering. By calculating electric field-induced magnetization by the linear response theory, we reveal that the magnetoelectric effect shows up without specific parameter choices. The magnetoelectric effect qualitatively varies by changing the direction of the magnetic moment in the ferromagnet: the response is diagonal for the out-of-plane moment, whereas it is off-diagonal for the inplane moment. We also find out that in optical frequencies, the magnetoelectric signal can be drastically enhanced via interband resonant excitations. Finally, we estimate the magnitude of the magnetoelectric effect for a hybrid halide perovskite semiconductor as an example of the band insulator and compare it with other magnetoelectric materials. We underscore that our mechanism is quite general and widely expectable, only requiring the Rashba spin-orbit coupling and exchange coupling. Our result could potentially offer a promising method of Joule heating-free electric manipulation of magnetic moments in spintronic devices.

Pancharatnam-Berry phase and kinetic magnetoelectric effect in trigonal tellurium

We study the kinetic magnetoelectric effect (current-induced magnetization including both the orbital and spin contributions) in three-dimensional conductors, specializing to the case of p-doped trigonal tellurium. We include both intrinsic and extrinsic contributions to the effect, which stem from the band structure of the crystal, and from disorder scattering, respectively. Specifically, we determine the dependence of the kinetic magnetoelectric response on the hole doping in tellurium, and show that the intrinsic and extrinsic effects dominate for low and high levels of doping, respectively. The results of this work imply that three-dimensional helical metals are promising for spintronics applications, in particular, they can provide robust control over current-induced magnetic torques.

Kinetic orbital moments and nonlocal transport in disordered metals with nontrivial band geometry

We study the effects of spatial dispersion in disordered noncentrosymmetric metals. These include the kinetic magnetoelectric effect, natural optical activity of metals, as well as the so-called dynamic chiral magnetic effect as a particular case of the latter. These effects are determined by the linear in the wave vector of an electromagnetic perturbation contribution to the conductivity tensor of a material, and stem from the magnetic moments of quasiparticles near the Fermi surface. We identify new disorder-induced contributions to these magnetic moments that come from the skew scattering and side jump processes, familiar from the theory of anomalous Hall effect. We show that at low frequencies the spatial dispersion of the conductivity tensor comes mainly either from the skew scattering or intrinsic contribution, and there is always a region of frequencies in which the intrinsic mechanism dominates. Our results imply that in clean three-dimensional metals, current-induced magnetization is in general determined by impurity skew scattering, rather than intrinsic contributions. Intrinsic effects are expected to dominate in cubic enantiomorphic crystals with point groups $T$ and $O$, and in polycrystalline samples, regardless of their mobility.

The kinetic magnetoelectric effect in laterally boundary-confined ballistic two-dimensional hole gases

A theoretical investigation is presented on the characteristics of the kinetic magnetoelectric effect in laterally boundary-confined ballistic two-dimensional hole gases. It was shown that, though the momentum-dependent effective magnetic fields felt by charge carriers due to the spin-orbit interaction are in-plane orientated in such systems, both in-plane polarized and normal polarized nonequilibrium spin polarization densities could be electrically induced by the kinetic magnetoelectric effect, and the induced nonequilibrium spin polarizations exhibit some interesting characteristics. The characteristics we found indicate that there may be some possible relation between this effect and some recent experimental findings.

A unified semiclassical description for kinetic magnetoelectric effect in both k-linear and k-cubic two-dimensional Rashba models

We propose a unified semiclassical description for the kinetic magnetoelectric effect in both k -linear and k -cubic two-dimensional Rashba model in the thermodynamic limit, which takes into account the effects of both spin coherence and spin dephasing by a closed set of Boltzman-like kinetic equations. Based on this unified description, we show that in contrary to the case found in the studies of intrinsic spin Hall effect in such systems, in the linear response regime the kinetic magnetoelectric effect would vanish for the k -cubic Rashba model in the thermodynamic limit but be robust for the k -linear Rashba model in the thermodynamic limit.

Kinetic magnetoelectric effect in a two-dimensional semiconductor strip due to boundary-confinement-induced spin-orbit coupling

In a thin strip of a two-dimensional semiconductor electronic system, spin-orbit coupling may be induced near both edges of the strip due to the substantial spatial variation of the confining potential in the boundary regions. In this paper we show that, in the presence of boundary-confinement induced spin-orbit coupling, a longitudinal charge current circulating through a 2D semiconductor strip may cause \textit{strong} non-equilibrium spin accumulation near both edges of the strip. The spins will be polarized along the normal of the 2DEG plane but in opposite directions at both edges of the strip. This phenomenon is essentially a kinetic magnetoelectric effect from the theoretical points of view, but it manifests in a very similar form as was conceived in a spin Hall effect.

Controllable kinetic magnetoelectric effect in two-dimensional electron gases with both Rashba and Dresselhaus spin-orbit couplings

A microscopic model calculation of the electric-field-induced nonequilibrium spin accumulation due to kinetic magnetoelectric effect in two-dimensional electron gases with both Rashba and Dresselhaus spin-orbit couplings is presented. The results show that by modulating the relative strength of the two different spin-orbit couplings, both the magnitude and the polarization direction of the nonequilibrium spin accumulation can be effectively controlled.