AbstractInjection molding is widely used for making intricate plastic products due to its precision, cost efficiency, and fast production. Industries like consumer electronics, aerospace, and medical, demand high mechanical properties from these parts. However, high‐performance polymers face challenges in flowability. Ultrasonic‐assisted injection molding offers a solution, but its impact on flowability and mechanical properties is not fully understood. We propose a novel injection mold design with in‐mold ultrasonic vibration to address this. By applying high‐frequency shear forces to the melt, it alters polymer chain alignment, enhancing flow and microstructure. Employing polyphenylene sulfide (PPS) resin as the primary material, this study systematically explores the impact of varying ultrasonic vibration durations and stages on melt filling behavior and product performance. Compared with conventional molds, ultrasonic‐assisted molds reduce melt viscosity by 38% and improve mechanical properties by 10.21%, with a 17.1% increase in crystallinity. This technology shows promise for improving flowability and mechanical properties in injection molding, with potential for wide industrial application.