In-plane Emission Research Articles

Mirror-coupled plasmonic nanostructures for enhanced in-plane magnetic dipole emission

Abstract Self-assembling of plasmonic nanoparticles into an oligomer can produce optical nanoantennas with resonant magnetic responses, which constitutes a promising platform to study magnetic light-matter interactions at the nanoscale. However, these self-assembled magnetic nanostructures typically feature a flat-lying geometric configuration, giving rise to out-of-plane magnetic dipole (MD) moments that cannot couple to the far-field light efficiently. Herein, we propose a new geometric configuration of plasmonic nanoantennas to realize in-plane MD responses. This is achieved by elegantly coupling a plasmonic nanoparticle oligomer to one or more adjacent metal mirrors, virtually forming a vertically standing nanoparticle tetramer or trimer, yet with in-plane MD moments. We verified this design strategy by numerically simulating the resonance responses of three typical mirror-coupled nanostructures, all exhibiting pronounced resonant MD characters. Furthermore, optical magnetic emitters can be readily coupled to these plasmonic nanoantennas and gain an emission enhancement of two orders of magnitude while simultaneously featuring a high emission directionality (collection efficiency up to ∼ 70 % evaluated with common microscopy optics). We believe these mirror-enabled magnetic nanoantennas could lead to novel nanophotonic devices fully exploiting the magnetic nature of light.

Microcavity-enhanced photoacoustic vibrational spectroscopy of single particles

Confinement and manipulation of photons using microcavities have triggered intense research interest in both fundamental and applied photonics for more than two decades. Prominent examples are ultrahigh-Q whispering gallery microcavities which confine photons using continuous total internal reflection along a curved and smooth surface. The long photon lifetime, strong field confinement, and in-plane emission characteristics make them promising candidates for enhancing light-matter interactions on a chip. In this talk, I will focus on single-particle photoacoustic vibrational spectroscopy using optical microcavities.

Momentum correlation of light nuclei in Au + Au collisions at [formula omitted] GeV

Within the Ultra-relativistic Quantum Molecular Dynamics model (UrQMD) coupled with nucleon coalescence model and Mini-Spanning-Tree model, the yields of light nuclei have been stimulated in Au + Au collisions over an energy range of sNN=2.0∼7.7GeV and the momentum correlation functions of light nuclei pairs have been calculated by both the Lednický-Lyuboshitz and the Correlation After Burner methods. We compare the yields of light nuclei and their momentum correlation functions at midrapidity in this energy region with experimental data. It is found that there are differences between the results of the two models, and the coalescence method seems less valid at low collision energy. Furthermore, both the peak values of proton-proton correlation functions and the transition point of elliptic flows from out-of-plane to in-plane emission show a turning point around 3-4 GeV, which suggests that there is a relation between momentum correlation function and collective flow of particles.

In-plane emission manipulation of random optical modes by using a zero-index material.

In this work, we have proposed to implement a zero-index material (ZIM) to control the in-plane emission of planar random optical modes while maintaining the intrinsic disordered features. Light propagating through a medium with near-zero effective refractive index accumulates little phase change and is guided to the direction determined by the conservation law of momentum. By enclosing a disordered structure with a ZIM based on all-dielectric photonic crystal (PhC), broadband emission directionality improvement can be obtained. We find the maximum output directionality enhancement factor reaches 30, around 6-fold increase compared to that of the random mode without ZIM. The minimum divergence angle is ∼6° for single random optical mode and can be further reduced to ∼3.5° for incoherent multimode superposition in the far field. Despite the significant directionality enhancement, the random properties are well preserved, and the Q factors are even slightly improved. The method is robust and can be effectively applied to the disordered medium with different structural parameters, e.g., the filling fraction of scatterers, and different disordered structure designs with extended or strongly localized modes. The output direction of random optical modes can also be altered by further tailoring the boundary of ZIM. This work provides a novel and universal method to manipulate the in-plane emission direction as well as the directionality of disordered medium like random lasers, which might enable its on-chip integration with other functional devices.

Direct nano-imaging of light-matter interactions in nanoscale excitonic emitters

Strong light-matter interactions in localized nano-emitters placed near metallic mirrors have been widely reported via spectroscopic studies in the optical far-field. Here, we report a near-field nano-spectroscopic study of localized nanoscale emitters on a flat Au substrate. Using quasi 2-dimensional CdSe/CdxZn1-xS nanoplatelets, we observe directional propagation on the Au substrate of surface plasmon polaritons launched from the excitons of the nanoplatelets as wave-like fringe patterns in the near-field photoluminescence maps. These fringe patterns were confirmed via extensive electromagnetic wave simulations to be standing-waves formed between the tip and the edge-up assembled nano-emitters on the substrate plane. We further report that both light confinement and in-plane emission can be engineered by tuning the surrounding dielectric environment of the nanoplatelets. Our results lead to renewed understanding of in-plane, near-field electromagnetic signal transduction from the localized nano-emitters with profound implications in nano and quantum photonics as well as resonant optoelectronics.

On-chip integrated exceptional surface microlaser.

The on-chip integrated visible microlaser is a core unit of high-speed visible-light communication with huge bandwidth resources, which needs robustness against fabrication errors, compressible linewidth, reducible threshold, and in-plane emission. However, until now, it has been a great challenge to meet these requirements simultaneously. Here, we report a scalable strategy to realize a robust on-chip integrated visible microlaser with further improved lasing performances enabled by the increased orders (n) of exceptional surfaces, and experimentally verify the strategy by demonstrating the performances of a second-order exceptional surface-tailored microlaser. We further prove the potential application of the strategy by discussing an exceptional surface-tailored topological microlaser with unique performances. This work lays a foundation for further development of on-chip integrated high-speed visible-light communication and processing systems, provides a platform for the fundamental study of non-Hermitian photonics, and proposes a feasible method of joint research for non-Hermitian photonics with nonlinear optics and topological photonics.

Controllable spin-resolved photon emission enhanced by a slow-light mode in photonic crystal waveguides on a chip.

We report the slow-light enhanced spin-resolved in-plane emission from a single quantum dot (QD) in a photonic crystal waveguide (PCW). The slow light dispersions in PCWs are designed to match the emission wavelengths of single QDs. The resonance between two spin states emitted from a single QD and a slow light mode of a waveguide is investigated under a magnetic field with Faraday configuration. Two spin states of a single QD experience different degrees of enhancement as their emission wavelengths are shifted by combining diamagnetic and Zeeman effects with an optical excitation power control. A circular polarization degree up to 0.81 is achieved by changing the off-resonant excitation power. Strongly polarized photon emission enhanced by a slow light mode shows great potential to attain controllable spin-resolved photon sources for integrated optical quantum networks on chip.

Discovery of Type II Interlayer Trions.

In terms of interlayer trions, electronic excitations in van der Waals heterostructures (vdWHs) can be classified into Type I (i.e., two identical charges in the same layer) and Type II (i.e., two identical charges in the different layers). Type I interlayer trions are investigated theoretically and experimentally. By contrast, Type II interlayer trions remain elusive in vdWHs, due to inadequate free charges, unsuitable band alignment, reduced Coulomb interactions, poor interface quality, etc. Here, the first observation of Type II interlayer trions is reported by exploring band alignments and choosing an atomically thin organic-inorganic system-monolayer WSe2 /bilayer pentacene heterostructure (1L+2L HS). Both positive and negative Type II interlayer trions are electrically tuned and observed via PL spectroscopy. In particular, Type II interlayer trions exhibit in-plane anisotropic emission, possibly caused by their unique spatial structure and anisotropic charge interactions, which is highly correlated with the transition dipole moment of pentacene. The results pave the way to develop excitonic devices and all-optical circuits using atomically thin organic-inorganic bilayers.

Anisotropic photon emission from gluon fusion and splitting in a strong magnetic background: The two-gluon one-photon vertex

Having in mind the pre-equilibrium stage in peripheral heavy-ion collisions as a possible scenario for the production of electromagnetic radiation, we compute the two-gluon one-photon vertex in the presence of an intense magnetic field at one-loop order. The quarks in the loop are taken such that two of them occupy the lowest Landau level, with the third one occupying the first excited Landau level. When the field strength is the largest of the energy (squared) scales, the tensor basis describing this vertex corresponds to two of the three-vector particles polarized in the longitudinal direction whereas the third one is polarized in the transverse direction. However, when the photon energy is of the same order as or larger than the field strength, the explicit one-loop computation contains extra tensor structures that spoil the properties of the basis compared with the case when the field strength is the largest of the energy scales, which signals that the calculation is incomplete. Nevertheless, by projecting the result onto the would-be basis, we show that the squared amplitude for processes involving two gluons and one photon exhibits the expected properties such as a preferred in-plane photon emission and a slightly decreasing strength for an increasing magnetic-field strength. We comment on possible venues to improve the one-loop calculation that include accounting for progressive occupation of the three quarks of the lowest and first-excited Landau levels such that, still working in the large field limit, a more complete description can be achieved when the photon energy increases.

Free-electron terahertz radiation based on silicon gratings with in-plane waveguide emission

We present a method utilizing the coupling between a pre-bunched electron beam and a silicon subwavelength grating to generate coherent terahertz waves. The grating that is connected to two opposite-traveling in-plane waveguides functions as a resonator. An example operating around 2 THz shows that, when the velocity and repetition frequency of the electron bunches respectively match the phase velocity and resonant frequency of the Bragg resonance in the grating, the strong electron-wave coupling leads to coherent radiation through the waveguide. The repetition frequency of the electron bunches can be halved by using its second harmonic to match the resonant frequency. This study might offer a potential approach for on-chip terahertz sources.

Perovskite micro-nano lasers and on-chip integration

<p indent="0mm">With the rapid development of photonic technologies and micro-nano fabrication technologies, optoelectronic devices tend to be miniaturized and integrated. Photonic integrated circuits (PICs) can adress the bottleneck problems of electronic chips, such as high-power consumption and slow computing speed. Micro-nano lasers are an important part in PICs, and they are the key device to generate optical signals. Perovskites are direct band gap semiconductor materials with high exciton binding energy and low defect densities. Therefore, they have high photoluminescence quantum yield and can be used as gain materials for micro-nano lasers. In addition, perovskite materials also have advantages of low non-radiation recombination rate, low manufacturing cost, tunable bandgap width, solution treatment, and so on. Because of these advantages, perovskite materials have been widely used in micro-nano lasers and other fields. At present, researchers have developed a variety of micro-nano fabrication methods to fabricate perovskite micro-nano structures. A variety of perovskite micro-nano lasers have been obtained by using perovskite micro-nano structures under the pump of pulses or continuous lasers. In PICs, it is necessary to use optical waveguides to couple laser sources to other photonic devices to form a complete photonic circuit. This paper first summarizes the synthesis methods of perovskite materials, including spin coating methods, cooling crystallization methods, inversion crystallization methods, antisolvent crystallization methods, space limited methods, and gas phase epitaxial growth methods. Among these synthesis methods, spin coating methods are simple, but only polycrystalline perovskite materials can be prepared. Single crystal perovskites can be prepared by cooling crystallization methods, inversion crystallization methods, antisolvent crystallization methods, space limited methods, and gas phase epitaxial growth methods. Next, fabrication methods of perovskite micro-nano structures are introduced, including space limited synthetic growth methods, nano imprinting methods, focused ion beam etching methods, and electron beam exposure methods. Space limited synthetic growth methods and nano imprinting methods have no damage to perovskite materials. Electron beam exposure methods have small damage to perovskite materials, and focused ion beam etching methods cause great damage to perovskite materials. Then, perovskite micro-nano lasers, including out-plane emission lasers and in-plane emission lasers, are introduced. Out-plane emission lasers emit the laser towards the free space, and they are not favorite for on-chip integration. In-plane emission lasers emit the laser towards the in-plane space, and they are easy to be integrated with the waveguide. In addition, the combination of perovskites and metal structures is expected to reduce the size of the laser to subwavelength scales based on plasmonic effects. We also introduce the on-chip integration of perovskite micro-nano lasers, including tip manipulation methods, overlay alignment methods, and transfer printing methods. Tip manipulation and overlay alignment methods can damage perovskite materials. Transfer printing methods do not cause damage to perovskite materials. Finally, the development trends of perovskite materials and micro-nano lasers are discussed. Although perovskite micro-nano lasers have made great progress, there are still some problems to be addressed. For example, lead in perovskite materials is toxic, so it is necessary to develop lead-free perovskite materials. Perovskite materials have poor stability, and their stability should be improved. Moreover, the realization of electrically pumped micro-nano lasers and on-chip integration is also a great challenge.

Large In-Plane Anisotropic Terahertz Emission Induced by Asymmetric Polarization in Low-Symmetric PdSe2.

Palladium diselenide (PdSe2) exhibits air stability, low symmetry, and high carrier mobility, resulting in unique in-plane anisotropy for polarized optoelectronic devices. However, the relationship of the symmetry and the terahertz (THz) radiation remains elusive yet significant for both the THz source in technology and nonlinear optical physics in science. Herein, we observed large in-plane anisotropic THz radiation from multilayer PdSe2 under femtosecond laser excitation. The THz emission demonstrates 2α dependence on the optical polarization angle from the resonant optical rectification combined with a background from the photocarrier acceleration under the surface depletion field. Interestingly, the in-plane THz emission along and perpendicular to the puckered direction demonstrates large anisotropy. Furthermore, the THz time-domain signals exhibit reversed polarities along the positive and negative puckered directions. This asymmetric polarization could relate to the bonding of Pd-Se, resulting in the unidirectional photon-induced current. Our results bridge the gap between the low-symmetry two-dimensional materials and the THz technology, which could promote the development of THz-polarized devices based on low-symmetry layered materials.

Exciton-Phonon Interaction-Induced Large In-Plane Optical Anisotropy in Two-Dimensional All-Inorganic Perovskite Crystals.

Two-dimensional (2D) perovskites are an emerging class of layered materials with unique optoelectronic properties. To date, most 2D perovskites with Ruddlesden-Popper (RP) phase reported are organic- inorganic hybrid perovskites with long organic spacers. Here, we report a high-quality all-inorganic 2D perovskite, Cs2PbI2Cl2, synthesized by an aqueous method. The as-synthesized perovskite crystals exhibit large in-plane emission and reflection optical anisotropy. The maximum in-plane linear dichroic ratio is up to 9.6 for exciton emission and 2.0 for reflection at 77 K. The large in-plane optical anisotropy may be ascribed to the strong electron-phonon interaction-induced lattice distortion. The large optical anisotropy enables us to construct a polarization-sensitive photodetector based on this perovskite, for which the linear dichroic ratio of photoresponse is about 1.2. Our study provides an alternative avenue to achieve in-plane optical anisotropy in an isotropy structure and thus would be of great importance for polarization-associated applications.

Identification of Brillouin Zones by In-Plane Lasing from Light-Cone Surface Lattice Resonances.

Because of translational symmetry, electromagnetic fields confined within 2D periodic optical structures can be represented within the first Brillouin zone (BZ). In contrast, the wavevectors of scattered electromagnetic fields outside the lattice are constrained by the 3D light cone, the free-photon dispersion in the surrounding medium. Here, we report that light-cone surface lattice resonances (SLRs) from plasmonic nanoparticle lattices can be used to observe the radiated electromagnetic fields from extended BZ edges. Our coupled dipole radiation theory reveals how lattice geometry and induced surface plasmon dipole orientation affect angular distributions of the radiated fields. Using dye molecules as local dipole emitters to excite the light-cone SLR modes, we experimentally identified high-order BZ edges by directional, in-plane lasing emission. These results provide insight into nanolaser architectures that can emit at multiple wavelengths and in-plane directions simply by rotating the nanocavity lattice.

Lasing at the nanoscale: coherent emission of surface plasmons by an electrically driven nanolaser

Abstract Plasmonics offers a unique opportunity to break the diffraction limit of light and bring photonic devices to the nanoscale. As the most prominent example, an integrated nanolaser is a key to truly nanoscale photonic circuits required for optical communication, sensing applications and high-density data storage. Here, we develop a concept of an electrically driven subwavelength surface-plasmon-polariton nanolaser, which is based on a novel amplification scheme, with all linear dimensions smaller than the operational free-space wavelength λ and a mode volume of under λ 3/30. The proposed pumping approach is based on a double-heterostructure tunneling Schottky barrier diode and gives the possibility to reduce the physical size of the device and ensure in-plane emission so that the nanolaser output can be naturally coupled to a plasmonic or nanophotonic waveguide circuitry. With the high energy efficiency (8% at 300 K and 37% at 150 K), the output power of up to 100 μW and the ability to operate at room temperature, the proposed surface plasmon polariton nanolaser opens up new avenues in diverse application areas, ranging from ultrawideband optical communication on a chip to low-power nonlinear photonics, coherent nanospectroscopy, and single-molecule biosensing.

Supertransport of excitons in atomically thin organic semiconductors at the 2D quantum limit

Long-range and fast transport of coherent excitons is important for the development of high-speed excitonic circuits and quantum computing applications. However, most of these coherent excitons have only been observed in some low-dimensional semiconductors when coupled with cavities, as there are large inhomogeneous broadening and dephasing effects on the transport of excitons in their native states in materials. Here, by confining coherent excitons at the 2D quantum limit, we first observed molecular aggregation-enabled ‘supertransport’ of excitons in atomically thin two-dimensional (2D) organic semiconductors between coherent states, with a measured high effective exciton diffusion coefficient of ~346.9 cm2/s at room temperature. This value is one to several orders of magnitude higher than the values reported for other organic molecular aggregates and low-dimensional inorganic materials. Without coupling to any optical cavities, the monolayer pentacene sample, a very clean 2D quantum system (~1.2 nm thick) with high crystallinity (J-type aggregation) and minimal interfacial states, showed superradiant emission from Frenkel excitons, which was experimentally confirmed by the temperature-dependent photoluminescence (PL) emission, highly enhanced radiative decay rate, significantly narrowed PL peak width and strongly directional in-plane emission. The coherence in monolayer pentacene samples was observed to be delocalised over ~135 molecules, which is significantly larger than the values (a few molecules) observed for other organic thin films. In addition, the supertransport of excitons in monolayer pentacene samples showed highly anisotropic behaviour. Our results pave the way for the development of future high-speed excitonic circuits, fast OLEDs, and other optoelectronic devices.

Collective Mie Resonances for Directional On-Chip Nanolasers.

A highly efficient nanocavity formed by optically coupled nanostructures is achieved by optimization of the collective Mie resonances in a one-dimensional array of semiconductor nanoparticles. Analysis of quasi-normal multipole modes enables us to reveal the close relation between the collective Mie resonances and Van Hove singularities. On the basis of these concepts, we experimentally demonstrate a directional GaAs nanolaser at cryogenic temperatures with well-defined, in-plane emission, which, moreover, can be controlled by selective excitation. The lasing threshold is shown to be significantly reduced by optimizing the interparticle gap such that the optimal near-field confinement is achieved at a resonant wavelength corresponding to the highest gain of GaAs. We show that the lasing performance of this nanolaser is orders of magnitude better than a nanowire-based laser of the same dimensions. The present work provides design guidelines for high performance in-plane emission nanolasers, which may find applications in future photonic integrated circuits.

Dislocation emission and crack growth in 3D bcc iron crystals under biaxial loading by atomistic simulations

This paper is devoted to the study of the ductile-brittle behavior of a central nanocrack (1¯10)[110] (crack plane/crack front) under biaxial loading via free 3D molecular dynamics (MD) simulations, as well as the comparison of MD results with continuum predictions concerning T-stress. The so called T-stress is a constant stress component acting along the crack plane, which should be considered (together with the stress intensity factor K) in the assessment of brittle-ductile behavior, namely, in the case of the short cracks. Previous 2D atomistic simulations under plane strain conditions indicated that the level of T-stress (controlled by the biaxiality ratio σB/σA from the external loading) affects dislocation emission from the crack and can cause the ductile-brittle transition. The plane strain simulations using the periodic or translational boundary conditions in the bcc lattice have certain limitations: they enable the in-plane dislocation emission (Burgers vector lies in the observation plane), but they do not allow the complete dislocation emission on the all slip systems favored by the shear stress. As presented, our new free 3D atomistic simulations (without periodic or symmetry conditions) enable the activity of the all favored slip systems. Thus, they offer a more realistic insight into the microscopic processes generated by the crack itself in dependence on the T-stress level.

Improving the Efficiency of Transverse Magnetic Polarized Emission from AlGaN Based LEDs by Using Nanowire Photonic Crystal

AlGaN-based deep ultraviolet (UV) light-emitting diodes (LEDs) are attractive for a wide range of applications. To date, however, the best reported external quantum efficiency (EQE) for LEDs operating in the wavelength range of ~240 nm is well below 1%. In this paper, we have performed detailed studies of the EQE of AlGaN nanowire photonic crystal LEDs in this wavelength range by finite-difference time-domain simulation. By coupling in-plane emission to vertical emission, light-extraction efficiency (LEE) over 90% can, in principle, be expected from the device top surface for transverse magnetic polarized photons that was not previously possible in conventional planar quantum well devices. Taken into account practical limitations including the absorptive p-Al(Ga)N contact and the presence of metal contact grid, LEE in the range of 30-40% is also expected. Moreover, due to the Purcell effect, the radiative recombination rate and, therefore, internal quantum efficiency (IQE) can be significantly modified in nanowire photonic crystal structures. We have established the design principles and ultimate efficiency limit of AlGaN nanowire photonic crystal LEDs: For AlGaN LEDs with very high IQE, EQE >70% can, in principle, be expected by operating near the Γ point of nanowire photonic crystals, whereas for structures with relatively low IQE it is preferred to operate near the M point to enhance the IQE while maintaining reasonably high LEE.

Vertical‐Cavity Silicon‐Integrated Laser with In‐Plane Waveguide Emission at 850 nm (Laser Photonics Rev. 12(2)/2018)

Silicon-Integrated Lasers In article number 1700206, Sulakshna Kumari and co-workers experimentally demonstrate a hybrid vertical-cavity silicon-integrated laser (VCSIL) with in-plane emission into a silicon nitride (SiN) waveguide. The inset shows the optical micrograph of the fully processed VCSIL. A weak SiN grating is placed inside the cavity to couple the vertically amplified light inside the cavity into an in-plane SiN waveguide. The grating also sets the polarization of the lasing output and provides transverse mode control.