The Three Gorges Hydropower Station, the largest in the world, plays a pivotal role in hydroelectric power generation, flood control, navigation, and ecological conservation. The water level of the Three Gorges Reservoir has a direct impact on these aspects. Accurate prediction of the reservoir’s water level, especially in the dam area, is of utmost importance for downstream regions’ safety and economic development. This study investigates the application and performance of four distinct deep-learning models in predicting water levels. The models evaluated include the Long Short-Term Memory (LSTM), Bidirectional Long Short-Term Memory (BiLSTM), Convolutional Neural Network–Long Short-Term Memory (CNN–LSTM), and Convolutional Neural Network–Attention–Long Short-Term Memory (CNN–Attention–LSTM). The performance of these models was assessed using several metrics, namely the Coefficient of Determination (R2), Mean Absolute Error (MAE), Root Mean Squared Error (RMSE), and Mean Absolute Percentage Error (MAPE). The findings indicate that the CNN–Attention–LSTM model outperforms the others in all metrics, achieving an R2 value of 0.9940, MAE of 0.5296, RMSE of 0.6748, and MAPE of 0.0032. Moreover, the CNN–LSTM model exhibited exceptional predictive accuracy for lower water levels. These results underscore the potential of deep-learning models in water-level forecasting, particularly highlighting the efficacy of attention mechanisms in enhancing predictive accuracy. Precise water-level predictions are instrumental in optimizing hydropower generation and providing a scientific basis for effective flood control and water resource management.