Hot-electron Currents Research Articles

Néel vector switching and terahertz spin-wave excitation in Mn2Au due to femtosecond spin-transfer torques

Efficient and fast manipulation of antiferromagnets has to date remained a challenging task, hindering their application in spintronic devices. For ultrafast operation of such devices, it is highly desirable to be able to control the antiferromagnetic order within picoseconds - a timescale that is difficult to achieve with electrical circuits. Here, we demonstrate that bursts of spin-polarized hot-electron currents emerging due to laser-induced ultrafast demagnetization are able to efficiently excite spin dynamics in antiferromagnetic Mn$_2$Au by exerting a spin-transfer torque on femtosecond timescales. We combine quantitative superdiffusive transport and atomistic spin-model calculations to describe a spin-valve-type trilayer consisting of Fe$|$Cu$|$Mn$_2$Au. Our results demonstrate that femtosecond spin-transfer torques can switch the Mn$_2$Au layer within a few picoseconds. In addition, we find that spin waves with high frequencies up to several THz can be excited in Mn$_2$Au.

Theory of superdiffusive spin transport in noncollinear magnetic multilayers

Ultrafast demagnetization induced by femtosecond laser pulses in thin metallic layers is caused by the outflow of spin-polarized hot-electron currents describable by the superdiffusive transport model. These laser-generated spin currents can cross the interface into another magnetic layer and give rise to magnetization dynamics in magnetic spin valves with noncollinear magnetizations. To describe ultrafast transport and spin dynamics in such nanostructures, we develop here the superdiffusive theory for general noncollinear magnetic multilayers. Specifically, we introduce an Al/Ni/Ru/Fe/Ru multilayer system with noncollinear Ni and Fe magnetic moments and analyze how the ultrafast demagnetization and spin-transfer torque depend on the noncollinearity. We employ ab initio calculations to compute the spin- and energy-dependent transmissions of hot electrons at the interfaces of the multilayer. Taking into account multiple electron scattering at interfaces and spin mixing in the spacer layer, we find that the laser-induced demagnetization of the Ni layer and the magnetization change of the Fe layer strongly depend on the angle between their magnetizations. Similarly, the spin-transfer torques on the Ni and Fe layers and the total spin momentum absorbed in the Ni and Fe layer are found to vary markedly with the amount of noncollinearity. These results suggest that by changing the amount of noncollinearity in magnetic multilayers, one can efficiently control the hot-electron spin transport, which may open a way toward achieving fast, laser-driven spintronic devices.

Enhanced polarized proton acceleration driven by femtosecond laser pulses irradiating a micro-structured solid–gas target

Herein, we propose a scheme based on collision-less shock acceleration (CSA) involving the use of composite targets comprising a micro-structured foil and a pre-polarized gas for obtaining high-energy polarized proton beams. Femtosecond laser pulses irradiate a microwire-array (MWA) target and efficiently heat the dense plasma, which moves toward the dilute plasma. Shocks are then introduced in the pre-polarized gas to accelerate upstream spin-polarized protons to relativistic velocities. Based on particle-in-cell simulations with added spin dynamics, protons with energies of 30–300 MeV are produced, and the polarization rate of protons in the high-energy region exceeds 90%. The simulations demonstrate an evident increase in the temperature and number of hot electrons owing to the presence of MWA structures, which increase both the longitudinal electric field strength associated with the shock and the energy of the reflected protons. During CSA, the bipolar magnetic field driven by hot-electron currents demonstrates a weak effect on the polarization level of the accelerated protons, resulting in a high polarization rate. The relationship between the energy of the polarized proton beam and the hot-electron temperature enables an optimization of the micro-structured target and other target components to enhance proton quality via the CSA process.

Spin-polarized hot electron transport versus spin pumping mediated by local heating

A ‘toy model’—aimed at capturing the essential physics—is presented that jointly describes spin-polarized hot electron transport and spin pumping driven by local heating. These two processes both contribute to spin-current generation in laser-excited magnetic heterostructures. The model is used to compare the two contributions directly. The spin-polarized hot electron current is modeled as one generation of hot electrons with a spin-dependent excitation and relaxation scheme. Upon decay, the excess energy of the hot electrons is transferred to a thermalized electron bath. The elevated electron temperature leads to an increased rate of electron-magnon scattering processes and yields a local accumulation of spin. This process is dubbed as spin pumping by local heating. The built-up spin accumulation is effectively driven out of the ferromagnetic system by (interfacial) electron transport. Within our model, the injected spin current is dominated by the contribution resulting from spin pumping, while the hot electron spin current remains relatively small. We derive that this observation is related to the ratio between the Fermi temperature and Curie temperature, and we show what other fundamental parameters play a role.

Regulation of UV light on the hot-electron current of Au/TiO2:Tb3+ Schottky diodes

Tb3+-doped TiO2 (TiO2:Tb3+) films are synthesized by a facile sol–gel method. The hot-electron current of Au/TiO2:Tb3+ Schottky diodes was enhanced by UV light decreasing the height of Schottky barrier. Compared with pure TiO2, doping Tb3+ can reduce the background current originating from the internal photoelectric effect in TiO2, and improve the on/off ratio. This is due to the energy and charge transfer mechanism from TiO2 to Tb3+. Photogenerated electrons in TiO2:Tb3+ films excited by UV light can be consumed by radiative electron transitions from the level 5D4 to the 7Fj (j = 6, 5, 4, 3) for Tb3+. This is beneficial and effective to regulate the electronic state of optoelectronic materials.

2D MHD simulation of spontaneous magnetic fields generated during interaction of 1315.2-nm laser radiation with copper slabs at 1016 W/cm2

Multidimensional modeling of phenomena and processes occurring during the expansion of the laser-produced plasma for different irradiation conditions related to both the laser beam parameters and the target constructions is a very complex issue, especially when modeling requires consideration of kinetic processes associated with the development of various types of microscopic instability. Multidimensional PIC codes create such a possibility, but their use is limited to modeling phenomena even in a very narrow timescale due to the limited computational capabilities of current supercomputers. For this reason, the paper attempts to interpret the results of the spontaneous magnetic field (SMF) measurements obtained during the PALS (Prague Asterix Laser System) experiment [Pisarczyk et al., AIP Adv. 10, 115201 (2020); Pisarczyk et al., Phys. Plasmas 22, 102706 (2015)] based on the 2D magneto-hydrodynamic (MHD) model [Jach et al., Computer Modeling of Dynamic Interaction of Bodies by Free Point Method (PWN, Warsaw, 2011)]. The MHD equations were used with included arbitrary (i) current of hot electrons treating it as an additional external current and (ii) ion-sound instability responsible for the increase in anomalous resistance in areas with high temperature and low-density plasma. The spatial distribution of magnetic fields and current density obtained from 2D modeling are in acceptable agreement with the experimental results [Pisarczyk et al., Plasma Phys. Controlled Fusion 62, 115020 (2020); Zaraś-Szydłowska et al., AIP Adv. 10, 115201 (2020); Pisarczyk et al., Phys. Plasmas 22, 102706 (2015)]. The inclusion of temporal changes in anomalous resistance in modeling allowed us to explain the persistence of high SMF amplitude at the level of several megagauss after the laser pulse ended due to the effect of magnetic field freezing.

Estimate of pre-thermal quench non-thermal electron density profile during Ar pellet shutdowns of low-density target plasmas in DIII-D

The radial density profile of pre-thermal quench (pre-TQ) early-time non-thermal (hot) electrons is estimated by combining electron cyclotron emission and soft x-ray data during the rapid shutdown of low-density (ne≲1019 m−3) DIII-D target plasmas with cryogenic argon pellet injection. This technique is mostly limited in these experiments to the pre-TQ phase and quickly loses validity during the TQ. Two different cases are studied: a high (10 keV) temperature target and a low (4 keV) temperature target. The results indicate that early-time, low-energy (∼10 keV) hot electrons form ahead of the argon pellet as it enters the plasma, affecting the pellet ablation rate; it is hypothesized that this may be caused by rapid cross field transport of argon ions ahead of the pellet or by rapid cross field transport of hot electrons. Fokker–Planck modeling of the two shots suggests that the hot electron current is quite significant during the pre-TQ phase (up to 50% of the total current). Comparison between modeled pre-TQ hot electron current and post-TQ hot electron current inferred from avalanche theory suggests that hot electron current increases during the high-temperature target TQ but decreases during the low-temperature target TQ. The uncertainties in this estimate are large; however, if true, this suggests that TQ radial loss of hot electron current could be larger than previously estimated in DIII-D.

Reliability of Sub-20 nm Black Phosphorus Trench (BP-T) MOSFET in High-Temperature Harsh Environment

In this work, the high-temperature reliability of the Black Phosphorus Trench (BP-T) MOSFET device has been analyzed. When the temperature is very high (500 K), the proposed device (BP-T-MOSFET) shows very high reliability with less effects in the device performance. The device is also calibrated with the experimental data. All the simulation has been performed using ATLAS-3D device simulator. BP-T-MOSFET shows high-temperature reliability in terms of reduced sub-threshold current, hot-electron injection gate current, and impact ionization substrate current. Further, higher switching ratio (Ion/Ioff), electron mobility, and electron velocity have also been observed owing to the electrical properties of black phosphorus used in the trench gate which shows the potential in a high-temperature environment. Owing to trench structure and electrical properties of black phosphorus, BP-T-MOSFET has significant device efficiency and low leakage currents at high temperatures which prove as highly shrieked MOS device applications in harsh temperature environment.

Magnetic field generation from a coil-shaped foil by a laser-triggered hot-electron current

A strong electron current triggered by a femtosecond relativistically intense laser pulse in a foil coil-like target is shown to be able to generate a solenoidal-type extremely strong magnetic field. The magnetic field lifetime sufficiently exceeds the laser pulse duration and is defined mainly by the target properties. The process of the magnetic field generation was studied with 3D PIC simulations. It is demonstrated that the pulse and the target parameters allow controlling the field strength and duration. The scheme studied is of great importance for laser-based magnetization technologies.

Ultrafast dynamics of magnetic vortices and pulse collapse in a laser-under dense plasma interaction

The energy of an intense ultrashort laser pulse interacting with high density (still under dense) plasma is typically transformed into electron heating and in excitation of nonlinear coherent structures such as magnetic vortices, solitons, or post-solitons. Using 33 TW 30 fs laser pulses and a high-density nitrogen gas jet, we experimentally investigated magnetic vortices in the laser pulse collapse region where electrons are efficiently accelerated and heated. Those vortices, which are associated with rapidly decaying magnetic fields, are found to be immobile and persist for several picoseconds. A collisionless plasma was formed due to the quasi-static field ionization of the gas associated with the hot and fast electron currents. The evolution dynamics of such nonlinear plasma phenomena have been monitored by using a 30-fs probe laser beam through employing the polarimetric and shadowgraphic techniques. Our experimental results are also supported by particle-in-cell simulations.

A Comparison of Pt/Si and Pt3Cu/Si Schottky nano-heterojunctions: enhanced direct methanol energy converter based on non-adiabatic system and molecular adsorption

In order to utilize the miniaturization exothermic oxidation of methanol in the microelectronic device as an energy source rather than industrial waste, nano-heterojunctions between Si and 20 nm ultra-thin catalyst Pt3Cu or Pt film were fabricated to investigate the energy conversion of methanol in this study. Methanol was catalyzed by Pt3Cu or Pt to release energy, then electrons were excited and passed through the Schottky barrier of Pt3Cu/Si or Pt/Si, which were calculated to be 0.43 and 0.80 eV, respectively. Thereupon, hot electron current was formed in a ballistic transport mode. Pt3Cu, Pt and Si have good high temperature stability. Pt3Cu has a higher crystallinity and better electronic structure than Pt and is dominated by (111) crystal orientation. Thus, Pt3Cu has higher catalytic activity and stronger ability to overcome the toxicity of CO, making it easier to obtain stable hot electron current. The factors that affect the hot electron current are varied from chemical reaction rate to Au electrode structure with the increase of temperature. This work is likely to provide a new reference to enhance the methanol’s direct conversion effectively with a stable current in the solid-state way at different temperature. Herein we report for the first time achieving methanol as hot electron energy source. Therefore, the maximum utilization of energy could be realized by turning waste methanol into treasure.

Transport theory for femtosecond laser-induced spin-transfer torques

Ultrafast demagnetization of magnetic layers pumped by a femtosecond laser pulse is accompanied by a nonthermal spin-polarized current of hot electrons. These spin currents are studied here theoretically in a spin valve with noncollinear magnetizations. To this end, we introduce an extended model of superdiffusive spin transport that enables the treatment of noncollinear magnetic configurations, and apply it to the perpendicular spin valve geometry. We show how spin-transfer torques arise due to this mechanism and calculate their action on the magnetization present, as well as how the latter depends on the thicknesses of the layers and other transport parameters. We demonstrate that there exists a certain optimum thickness of the out-of-plane magnetized spin-current polarizer such that the torque acting on the second magnetic layer is maximal. Moreover, we study the magnetization dynamics excited by the superdiffusive spin-transfer torque due to the flow of hot electrons employing the Landau–Lifshitz–Gilbert equation. Thereby we show that a femtosecond laser pulse applied to one magnetic layer can excite small-angle precessions of the magnetization in the second magnetic layer. We compare our calculations with recent experimental results.

Thickness and angular dependence of the magnetocurrent of hot electrons in a magnetic tunnel transistor with crossed anisotropies

We have studied the thickness and angular dependence of the magnetocurrent of hot electrons in a magnetic tunnel transistor (MTT) with crossed magnetic anisotropies. In a first step, we show that the magnetocurrent increases with ferromagnetic layer thickness as for MTTs with collinear magnetic configurations. The maximum magnetocurrent value is obtained to be 85%, which is close to the theoretical maximum value of 100% for MTTs with crossed magnetic configurations. In a second step, we demonstrate that we are able to reproduce both current vs field direction and current vs field intensity measurements in a framework taking into account a reduced number of magnetic parameters and a simple cosine dependence of the hot-electron current on the angle between magnetizations.

Ultrafast probing of magnetic field growth inside a laser-driven solenoid

We report on the detection of the time-dependent B-field amplitude and topology in a laser-driven solenoid. The B-field inferred from both proton deflectometry and Faraday rotation ramps up linearly in time reaching 210 ± 35 T at the end of a 0.75-ns laser drive with 1 TW at 351 nm. A lumped-element circuit model agrees well with the linear rise and suggests that the blow-off plasma screens the field between the plates leading to an increased plate capacitance that converts the laser-generated hot-electron current into a voltage source that drives current through the solenoid. ALE3D modeling shows that target disassembly and current diffusion may limit the B-field increase for longer laser drive. Scaling of these experimental results to a National Ignition Facility (NIF) hohlraum target size (∼0.2cm^{3}) indicates that it is possible to achieve several tens of Tesla.

Dynamics and structure of self-generated magnetics fields on solids following high contrast, high intensity laser irradiation

The dynamics of self-generated magnetic B-fields produced following the interaction of a high contrast, high intensity (I > 1019 W cm−2) laser beam with thin (3 μm thick) solid (Al or Au) targets is investigated experimentally and numerically. Two main sources drive the growth of B-fields on the target surfaces. B-fields are first driven by laser-generated hot electron currents that relax over ∼10–20 ps. Over longer timescales, the hydrodynamic expansion of the bulk of the target into vacuum also generates B-field induced by non-collinear gradients of density and temperature. The laser irradiation of the target front side strongly localizes the energy deposition at the target front, in contrast to the target rear side, which is heated by fast electrons over a much larger area. This induces an asymmetry in the hydrodynamic expansion between the front and rear target surfaces, and consequently the associated B-fields are found strongly asymmetric. The sole long-lasting (>30 ps) B-fields are the ones growing on the target front surface, where they remain of extremely high strength (∼8–10 MG). These B-fields have been recently put by us in practical use for focusing laser-accelerated protons [B. Albertazzi et al., Rev. Sci. Instrum. 86, 043502 (2015)]; here we analyze in detail their dynamics and structure.

Hot-Electron Photodetection with a Plasmonic Nanostripe Antenna

Planar metal-oxide-metal structures can serve as photodetectors that do not rely on the usual electron-hole pair generation in a semiconductor. Instead, absorbed light in one of the metals can produce a current of hot electrons when the incident photon energy exceeds the oxide barrier energy. Despite the desirable traits of convenient fabrication and room-temperature operation at zero bias of this type of device, the low power conversion efficiency has limited its use. Here, we demonstrate the benefits of reshaping one of the metallic contacts into a plasmonic stripe antenna. We use measurements of the voltage-dependence, spectral-dependence, stripe-width dependence, and polarization-dependence of the photocurrent to show that surface plasmon excitations can result in a favorable redistribution in the electric fields in the stripe that enhances the photocurrent. We also provide a theoretical model that quantifies the spectral photocurrent in terms of the electrical and optical properties of the junction. This model provides an accurate estimate of the bias dependence of the external quantum efficiency of different devices and shows that both the spatial and vectorial properties of the electric field distribution are important to its operation.

Short Intense Laser Pulse Collapse in Near-Critical Plasma

It is observed that the interaction of an intense ultrashort laser pulse with a near-critical gas jet results in the pulse collapse and the deposition of a significant fraction of the energy. This deposition happens in a small and well-localized volume in the rising part of the gas jet, where the electrons are efficiently accelerated and heated. A collisionless plasma expansion over ~ 150 μm at a subrelativistic velocity (~ c/3) has been optically monitored in time and space, and attributed to the quasistatic field ionization of the gas associated with the hot electron current. Numerical simulations in good agreement with the observations suggest the acceleration in the collapse region of relativistic electrons, along with the excitation of a sizable magnetic dipole that sustains the electron current over several picoseconds.

Ultrafast spin transport as key to femtosecond demagnetization

Irradiating a ferromagnet with a femtosecond laser pulse is known to induce an ultrafast demagnetization within a few hundred femtoseconds. Here we demonstrate that direct laser irradiation is in fact not essential for ultrafast demagnetization, and that electron cascades caused by hot electron currents accomplish it very efficiently. We optically excite a Au/Ni layered structure in which the 30 nm Au capping layer absorbs the incident laser pump pulse and subsequently use the X-ray magnetic circular dichroism technique to probe the femtosecond demagnetization of the adjacent 15 nm Ni layer. A demagnetization effect corresponding to the scenario in which the laser directly excites the Ni film is observed, but with a slight temporal delay. We explain this unexpected observation by means of the demagnetizing effect of a superdiffusive current of non-equilibrium, non-spin-polarized electrons generated in the Au layer.

Cavitation and shock wave formation in dense plasmas by relativistic electron beams

The propagation of a high current relativistic electron beam through a dense plasma, for example, in fast-ignition inertial confinement fusion, produces strong heating and magnetic field generation. The j × B force and thermal pressure gradient that the return current creates may in fact cavitate and cause shock waves in the plasma around the electron beam.Here we investigate this effect in different regimes of plasma density and hot electron current. An analytic model has been developed that gives good estimates of the density, pressure, magnetic field and velocity obtained in the plasma. This model is compared against the results from an MHD code that includes the effects of resistive field growth, Ohmic heating and the j × B force. The strength of the cavitation is found to be dependent upon the ratio between j2 and the initial mass density. It is shown that cavitation is indeed relevant to fast-ignition, and is strong enough to launch shocks in certain circumstances.

Transport of hot electron currents in solid targets irradiated by high intensity short laser pulses

We have analyzed the transport of hot electrons generated in the interaction between a short-pulse, ultra-high intensity laser beam (pulse duration τ<ps, intensity Iλ > 1018 W.cm 2.um2) and a solid or dense target through the use of proton emission imaging. We used targets of different material (Cu, Al, Au) with a regularly modulated rear target surface in order to compare the electron transport in different conditions. As result, we see that the electron transport depends on the target material and on the interaction conditions.