High-dimensional Quantum Information Research Articles

Nonlinear parametric generation and optical vortex transfer in graphene ensemble under Landau quantization

We explore the dynamics of nonlinear parametric generation and light beam propagation in a Landau-quantized graphene structure with three energy levels interacting with two laser pulses, utilizing the Maxwell-Bloch equations. By applying a laser field to one transition of the graphene sample while keeping the second beam initially absent, the distinctive preparation of the graphene sample, coupled with its weak interaction with laser radiation, results in the parametric generation of a new laser beam in a different transition. We investigate the influence of diverse system parameters on both the efficiency of the generated beam and the propagation dynamics of both beams. Our findings reveal that manipulating these parameters can induce oscillations in the intensity of propagated beams, mitigate absorption losses during propagation allowing for earlier relaxation, and enhance the efficiency of energy transfer from the initial to the generated beam. Additionally, we demonstrate the transfer of optical vortices within the graphene ensemble by introducing an optical vortex to the initial beam. This scheme holds promise for applications in high-dimensional quantum information processing.

Empowering a qudit-based quantum processor by traversing the dual bosonic ladder

High-dimensional quantum information processing has emerged as a promising avenue to transcend hardware limitations and advance the frontiers of quantum technologies. Harnessing the untapped potential of the so-called qudits necessitates the development of quantum protocols beyond the established qubit methodologies. Here, we present a robust, hardware-efficient, and scalable approach for operating multidimensional solid-state systems using Raman-assisted two-photon interactions. We then utilize them to construct extensible multi-qubit operations, realize highly entangled multidimensional states including atomic squeezed states and Schrödinger cat states, and implement programmable entanglement distribution along a qudit array. Our work illuminates the quantum electrodynamics of strongly driven multi-qudit systems and provides the experimental foundation for the future development of high-dimensional quantum applications such as quantum sensing and fault-tolerant quantum computing.

High-dimensional two-photon quantum controlled phase-flip gate

High-dimensional quantum systems have been used to reveal interesting fundamental physics and to improve information capacity and noise resilience in quantum information processing. However, it remains a significant challenge to realize universal two-photon quantum gates in high dimensions with high success probability. Here, by considering an ion-cavity QED system, we theoretically propose, to the best of our knowledge, the first high-dimensional, deterministic, and universal two-photon quantum gate. By using an optical cavity embedded with a single trapped Ca+40 ion, we achieve a high average fidelity larger than 98% for a quantum controlled phase-flip gate in four-dimensional space, spanned by photonic spin angular momenta and orbital angular momenta. Our proposed system can be an essential building block for high-dimensional quantum information processing, and also provides a platform for studying high-dimensional cavity QED. Published by the American Physical Society 2024

Spatiotemporal optical vortices with controllable radial and azimuthal quantum numbers

Optical spatiotemporal vortices with transverse photon orbital angular momentum (OAM) have recently become a focal point of research. In this work we theoretically and experimentally investigate optical spatiotemporal vortices with radial and azimuthal quantum numbers, known as spatiotemporal Laguerre-Gaussian (STLG) wavepackets. These 3D wavepackets exhibit phase singularities and cylinder-shaped edge dislocations, resulting in a multi-ring topology in its spatiotemporal profile. Unlike conventional ST optical vortices, STLG wavepackets with non-zero p\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{{{{\\boldsymbol{p}}}}}}$$\\end{document} and l\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{{{{\\boldsymbol{l}}}}}}$$\\end{document} values carry a composite transverse OAM consisting of two directionally opposite components. We further demonstrate mode conversion between an STLG wavepacket and an ST Hermite-Gaussian (STHG) wavepacket through the application of strong spatiotemporal astigmatism. The converted STHG wavepacket is de-coupled in intensity in space-time domain that can be utilized to implement the efficient and accurate recognition of ultrafast STLG wavepackets carried various p\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{{{{\\boldsymbol{p}}}}}}$$\\end{document} and l.\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{{{{\\boldsymbol{l}}}}}}.$$\\end{document} This study may offer new insights into high-dimensional quantum information, photonic topology, and nonlinear optics, while promising potential applications in other wave phenomena such as acoustics and electron waves.

Nontrivial evolution and geometric phase for an orbital angular momentum qutrit

Photonic orbital angular momentum (OAM) offers a promising platform for high-dimensional quantum information processing. While geometric phase (GP) is the crucial tool in enabling intrinsically fault-tolerant quantum computation, the measurement of GP using linear optics remains relatively unexplored in the OAM state space. Here, we propose an experimental scheme to detect GP shifts resulting from the cyclic evolution of OAM qutrit states. Distinguished with the conventional evolution along cyclic path on the Poincaré sphere (PS), the nontrivial evolution in our theoretical scheme is along a cyclic path residing within the SU(3)/U(2) parameter space. By employing a combination of X-gates, dove prisms, and double cylindrical lenses, we achieve the cyclic evolution and analyse the resultant GP through our designed Sagnac interferometer. Our theoretical study may find potential in high-dimensional quantum computation using twisted photons and in exploring the geometric structure of such optical systems.

Optical storage of circular airy beam in atomic vapor

Abstract The realization of quantum storage of spatial light field is of great significance to the construction of high-dimensional quantum repeater. In this paper, we experimentally realize the storage and retrieval of circular Airy beams (CABs) by using the Λ-type three-level energy system based on the electromagnetically induced transparency in a hot rubidium atomic vapor cell. The weak probe beam field is modulated with phase distribution of CABs by a spatial light modulator. We store the probe circular Airy beam (CAB) into the rubidium atomic vapor cell and retrieve it after the demanded delay. We quantitatively analyze the storage results and give corresponding theoretical explanations. Moreover, we investigate the autofocusing and self-healing effect of the retrieved CAB, which indicates that the properties and beam shape of CAB maintain well after storage. Our work will have potential applications in the storage of high-dimensional quantum information, and is also useful for improving the channel capacities of quantum internet.

Energy-flow-reversing dynamics in vortex beams: OAM-independent propagation and enhanced resilience

Since their discovery in the 1990s, vortex beams, known for their ability to carry orbital angular momentum (OAM), have found substantial applications in optical manipulation and high-dimensional classical and quantum information communication. However, their inherent diffraction in free space, resulting in OAM-dependent beam expansion, has constrained their utility in spatial mode multiplexing communication, fiber optic transmission, and particle manipulation. These domains necessitate vortex beams with OAM-independent propagation characteristics. Addressing this, we report an approach that employs the energy redistribution mechanism to reverse the radial energy flows of traditional vortex beams, thereby presenting iso-propagation vortex beams (IPVBs) with OAM-independent propagation dynamics. These IPVBs, attributed to their reversed radial energy flows, maintain resilience in diverse environments, from free space to challenging media, including sustaining their form post-damage, retaining consistent intensity in lossy media, and experiencing reduced modal scattering in atmospheric turbulence. Their unique features position IPVBs as promising candidates for applications in imaging, microscopy, optical communication, metrology, quantum information processing, and light-matter interactions. Case studies within optical communication reveal that the IPVB basis potentially unlocks a broader spectrum of data channels, enhancing information capacity over traditional spatial multiplexing techniques.

Time-reversible and fully time-resolved ultra-narrowband biphoton frequency combs

Time-reversibility, which is inherent in many physical systems, is crucial in tailoring temporal waveforms for optimum light–matter interactions. Among the time-reversible atomic systems, narrowband biphoton sources are essential for efficient quantum storage. In this work, we demonstrate time-reversed and fully time-resolved ultra-narrowband single-sided biphoton frequency combs with an average free-spectral range (FSR) of 42.66 MHz and an average linewidth of 4.60 MHz in the telecommunication band. We experimentally observe the fully time-resolved and reversible temporal oscillations by second-order cross correlation and joint temporal intensity measurements. The potential benefits of the time-reversed and fully time-resolved temporal oscillations from our source include enhancing the efficiency of quantum storage in atomic memories and maximizing the utilization of temporal information in multimode biphoton frequency combs. We further verify the heralded single-photon state generation from the multimode biphoton frequency combs by using Hanbury Brown and Twiss interference measurements. To the best of our knowledge, this 42.66 MHz FSR of our photon-pair source represents the narrowest among all of the different configurated biphoton sources reported to date. This ultra-narrow FSR and its 4.60 MHz linewidth provide the highest frequency mode number of 5786 and the longest coherence time among all the singly configurated biphoton sources so far. Our time-reversed and fully time-resolved massive-mode biphoton source could be useful for high-dimensional quantum information processing and efficient time–frequency multiplexed quantum storage toward long-distance and large-scale quantum networks.

Tempering Multichannel Photon Emission from Emitter-Coupled Holographic Metasurfaces.

On-chip manipulation of photon emission from quantum emitters (QEs) is crucial for quantum nanophotonics and advanced optical applications. At the same time, the general design strategy is still elusive, especially for fully exploring the degrees of freedom of multiple channels. Here, the vectorial scattering holography (VSH) approach developed recently for flexibly designing QE-coupled metasurfaces is extended to tempering the strength of QE emission into a particular channel. The VSH power is demonstrated by designing, fabricating, and optically characterizing on-chip QE sources emitted into six differently oriented propagation channels, each representing the entangled state of orthogonal circular polarizations with different topological charges and characterized with a specific relative strength. We postulate that the demonstration of tempered multichannel photon emission from QE-coupled metasurfaces significantly broadens the possibilities provided by the holographic metasurface platform, especially those relevant for high-dimensional quantum information processing.

Multiplication of orbital angular momentum via multi-plane light conversion.

The multiplication of orbital angular momentum (OAM) modes using optical coordinate transformation is useful for OAM optical networks, but the scalability of this scheme is limited by the ray model. Here, we propose an alternative scheme for the scalable multiplication of OAM modes based on modified multi-plane light conversion (MPLC) that can extend azimuthal and radial indices of OAM modes supported by the multipliers and unlock a new degree of freedom for radial high-order OAM states that has been restricted in the zero order. The multiplication for 20 OAM modes with radial index p = 0 and 10 OAM modes with radial index p = 1 is performed in simulation and experiment. The 3-dB optical bandwidth corresponding to the purity of OAM modes covers the entire C-band experimentally. This novel, to the best of our knowledge, approach to manipulating OAM states provides valuable insights and flexible strategies for high-capacity OAM optical communication and high-dimensional optical quantum information processing.

Highly Efficient Storage of 25-Dimensional Photonic Qudit in a Cold-Atom-Based Quantum Memory.

Building an efficient quantum memory in high-dimensional Hilbert spaces is one of the fundamental requirements for establishing high-dimensional quantum repeaters, where it offers many advantages over two-dimensional quantum systems, such as a larger information capacity and enhanced noise resilience. To date, it remains a challenge to develop an efficient high-dimensional quantum memory. Here, we experimentally realize a quantum memory that is operational in Hilbert spaces of up to 25 dimensions with a storage efficiency of close to 60% and a fidelity of 84.2±0.6%. The proposed approach exploits the spatial-mode-independent interaction between atoms and photons which are encoded in transverse-size-invariant vortex modes. In particular, our memory features uniform storage efficiency and low crosstalk disturbance for 25 individual spatial modes of photons, thus allowing the storing of qudit states programmed from 25 eigenstates within the high-dimensional Hilbert spaces. These results have great prospects for the implementation of long-distance high-dimensional quantum networks and quantum information processing.

Simulation of quantum walks on a circle with polar molecules via optimal control.

Quantum walks are the quantum counterpart of classical random walks and have various applications in quantum information science. Polar molecules have rich internal energy structure and long coherence time and thus are considered as a promising candidate for quantum information processing. In this paper, we propose a theoretical scheme for implementing discrete-time quantum walks on a circle with dipole-dipole coupled SrO molecules. The states of the walker and the coin are encoded in the pendular states of polar molecules induced by an external electric field. We design the optimal microwave pulses for implementing quantum walks on a four-node circle and a three-node circle by multi-target optimal control theory. To reduce the accumulation of decoherence and improve the fidelity, we successfully realize a step of quantum walk with only one optimal pulse. Moreover, we also encode the walker into a three-level molecular qutrit and a four-level molecular ququart and design the corresponding optimal pulses for quantum walks, which can reduce the number of molecules used. It is found that all the quantum walks on a circle in our scheme can be achieved via optimal control fields with high fidelities. Our results could shed some light on the implementation of discrete-time quantum walks and high-dimensional quantum information processing with polar molecules.

Multichannel Quantum Emission with On-Chip Emitter-Coupled Holographic Metasurfaces.

Multichannel quantum emission is in high demand for advanced quantum photonic applications such as quantum communications, quantum computing, and quantum cryptography. However, to date, the most common way for shaping photon emission from quantum emitters (QEs) is to utilize free-standing (external) bulky optical components. Here, we develop the multichannel holography approach for flexibly designing on-chip QE-coupled metasurfaces that make use of nonradiatively QE-excited surface plasmon polaritons for generating far-field quantum emission, which propagates in designed directions carrying specific spin and orbital angular momenta (SAM and OAM, respectively). We further design, fabricate, and characterize on-chip quantum light sources of multichannel quantum emission encoded with different SAMs and OAMs. The holography-based inverse design approach developed and demonstrated on-chip quantum light sources with multiple degrees of freedoms, thereby enabling a powerful platform for quantum nanophotonics, especially relevant for advanced quantum photonic applications, e.g., high-dimensional quantum information processing.

High-dimensional time-frequency entanglement in a singly-filtered biphoton frequency comb

High-dimensional quantum entanglement is a cornerstone for advanced technology enabling large-scale noise-tolerant quantum systems, fault-tolerant quantum computing, and distributed quantum networks. The recently developed biphoton frequency comb (BFC) provides a powerful platform for high-dimensional quantum information processing in its spectral and temporal quantum modes. Here we propose and generate a singly-filtered high-dimensional BFC via spontaneous parametric down-conversion by spectrally shaping only the signal photons with a Fabry-Pérot cavity. High-dimensional energy-time entanglement is verified through Franson-interference recurrences and temporal correlation with low-jitter detectors. Frequency- and temporal- entanglement of our singly-filtered BFC is then quantified by Schmidt mode decomposition. Subsequently, we distribute the high-dimensional singly-filtered BFC state over a 10 km fiber link with a post-distribution time-bin dimension lower bounded to be at least 168. Our demonstrations of high-dimensional entanglement and entanglement distribution show the singly-filtered quantum frequency comb’s capability for high-efficiency quantum information processing and high-capacity quantum networks.

Interferometric imaging of amplitude and phase of spatial biphoton states

High-dimensional biphoton states are promising resources for quantum applications, ranging from high-dimensional quantum communications to quantum imaging. A pivotal task is fully characterizing these states, which is generally time-consuming and not scalable when projective measurement approaches are adopted; however, new advances in coincidence imaging technologies allow for overcoming these limitations by parallelizing multiple measurements. Here we introduce biphoton digital holography, in analogy to off-axis digital holography, where coincidence imaging of the superposition of an unknown state with a reference state is used to perform quantum state tomography. We apply this approach to single photons emitted by spontaneous parametric down-conversion in a nonlinear crystal when the pump photons possess various quantum states. The proposed reconstruction technique allows for a more efficient (three orders of magnitude faster) and reliable (an average fidelity of 87%) characterization of states in arbitrary spatial modes bases, compared with previously performed experiments. Multiphoton digital holography may pave the route toward efficient and accurate computational ghost imaging and high-dimensional quantum information processing.

Diffractive Theory Study of Twisted Light’s Evolution during Phase-Only OAM Manipulations

Twisted light, or orbital angular momentum (OAM) carrying beams or photons, is a pillar of structured photonics, a booming subfield of modern optics. The generation and transformation of twisted light, which lie with coupling topological charges into target light’s wavefunctions, are usually performed by phase-only OAM manipulations. The practical twisted lights, however, obtained by this method are actually noneigen modes of free space, leading to an evolution through the diffractive propagation. Here, we present a general theoretical frame for accurately describing this evolution. Based on the theory, the whole diffractive propagation history in a typical OAM-manipulation loop, converting Gaussian light into a twisted one and then reconverting back, is demonstrated via a set of exact analytical solutions. These results provide a powerful tool for analyzing the transverse profiles of twisted light through the diffractive evolution, as a guideline for studying the science of structured light, which would provide guidelines for research studies in nonlinear optics and high-dimensional quantum information technology based on OAM-degree of freedom.

High-dimensional quantum information processing on programmable integrated photonic chips

High-dimensional quantum information processing on programmable integrated photonic chips

Time-Resolved Hanbury Brown–Twiss Interferometry of On-Chip Biphoton Frequency Combs Using Vernier Phase Modulation

Biphoton frequency combs (BFCs) are promising quantum sources for large-scale and high-dimensional quantum information and networking systems. In this context, the spectral purity of individual frequency bins will be critical for realizing quantum networking protocols like teleportation and entanglement swapping. Measurement of the temporal autocorrelation function of the unheralded signal or idler photons comprising the BFC is a key tool for characterizing their spectral purity and in turn verifying the utility of the biphoton state for networking protocols. Yet the experimentally obtainable precision for measuring BFC correlation functions is often severely limited by detector jitter. The fine temporal features in the correlation function---not only of practical value in quantum information, but also of fundamental interest in the study of quantum optics---are lost as a result. We propose a scheme to circumvent this challenge through electro-optic phase modulation, experimentally demonstrating time-resolved Hanbury Brown--Twiss characterization of BFCs generated from an integrated 40.5-GHz ${\mathrm{Si}}_{3}{\mathrm{N}}_{4}$ microring, up to a $3\ifmmode\times\else\texttimes\fi{}3$-dimensional two-qutrit Hilbert space. Through slight detuning of the electro-optic drive frequency from the comb's free spectral range, our approach leverages Vernier principles to magnify temporal features, which would otherwise be averaged out by detector jitter. We demonstrate our approach under both continuous-wave and pulsed-pumping regimes, finding excellent agreement with theory. Our method reveals not only the collective statistics of the contributing frequency bins but also their temporal shapes---features lost in standard fully integrated autocorrelation measurements.

Manipulation of continuous variable orbital angular momentum squeezing and entanglement by pump shaping.

Spatially structured quantum states, such as orbital angular momentum (OAM) squeezing and entanglement, is currently a popular topic in quantum optics. The method of generating and manipulating spatial quantum states on demand needs to be explored. In this paper, we generated OAM mode squeezed states of -5.4 dB for the L G0+1 mode and -5.3 dB for the L G0-1 mode directly by an optical parametric oscillator (OPO) for the first time. Additionally, we demonstrated that the OAM mode squeezed and entangled states were respectively generated by manipulating the nonlinear process of the OPO by controlling the relative phase of two beams of different modes, thus making two different spatial multimode pump beams. We characterized the Laguerre-Gaussian (LG) entangled states by indirectly measuring the squeezing for the H G 10(45∘) mode and H G 10(135∘) mode, and directly measuring the entanglement between the L G0+1 and L G0-1 modes. The effective manipulation of the OAM quantum state provides a novel insight into the continuous variable quantum state generation and construction on demand for high-dimensional quantum information and quantum metrology.

Room‐Temperature Generation of Heralded Single Photons on Silicon Chip with Switchable Orbital Angular Momentum (Laser Photonics Rev. 16(12)/2022)

Orbital Angular Momentum In article number 2200388, Shan Zhang, Xue Feng, and colleagues have proposed and demonstrated a heralded single-photon source with switchable orbital angular momentum (OAM) modes on silicon chip. At room-temperature, the heralded single photons are generated through the nonlinear effect and transformed to 11 OAM modes by an OAM emitter, offering a practical platform for high-dimensional quantum information processing.