Gravity gradients are useful to characterize near mass anomalies since they are much more sensitive to short wavelength anomalies than gravitational accelerations. Estimating gravity gradients from surface gravity data is based on numerical implementations of solutions to geodetic boundary value problem for determination of disturbing potential. One of methods to solve this problem is least-squares collocation which is basically based on data and a defined covariance function. This study deals with estimating gravity gradient tensor components from along track surface gravity anomaly data. The Least-Squares Collocation solution is based on a stationary local covariance function defined for the disturbing potential which allows upward continuation of the observations to a desired altitude. The modeling method is evaluated in using Earth Gravitational Model 2008(EGM2008) and real airborne gravity gradiometry data collected over Southern Texas, Oklahoma region. The results show that modeled gravity gradients estimated in both on the ground and at a certain altitude have basically good agreement with EGM08 gradients. Modeled gradients including horizontal components in the east-west direction exhibit some discrepancies in comparison to the airborne gradiometry data, which may be attributed to some measurement errors in the gradient data.