Terahertz Generation Research Articles

Multi-cycle terahertz generation in lithium niobate wafer stacks via mid-infrared pumping.

Near-infrared laser-pumped optical rectification (OR) using quasi-phase matching (QPM) in lithium niobate (LN) is widely employed to generate multi-cycle terahertz (THz) pulses, which, however, suffer from low efficiency. Here, we demonstrate that mid-infrared pumping is an effective approach to increase the efficiency of multi-cycle THz generation. By using a 2.3-µm laser to pump a QPM macro-crystal composed of ten x-cut lithium niobate wafers, with their ferroelectric Z axis alternately rotated by π, a laser-to-THz conversion efficiency up to ∼0.4% has been achieved at room temperature, more than twice the efficiencies attained with near-infrared pumping. Electro-optic sampling reveals the generation of five-cycle THz pulses at 0.15 THz for 350-µm-thick wafers and 0.22 THz for 250-µm-thick wafers. Such mid-infrared laser-pumped OR in QPM wafer stacks provides an efficient, controllable, and scalable method for generating intense multi-cycle THz pulses suitable for diverse narrow-bandwidth applications.

Generation of Circularly Polarized Strong-Field Terahertz Waves

Abstract Terahertz (THz) circular dichroism (TCD) spectroscopy has been widely used to study the chiral characteristics of biological macromolecules and various other materials. With the rapid development of strong-field THz generation and field-modulated techniques, the advancement of tunable strong-field TCD spectroscopy technology is of great significance. In this work, we built an integrated strong-field TCD spectroscopy system. We employed the tilted-pulse-front technique to generate linearly polarized strong-field THz radiation and a reflective metasurface for linear-to-circular conversion of the strong-field THz radiation. We obtained circularly polarized THz radiation with an ellipticity of over 0.9 in the frequency range from 0.38 THz to 0.61 THz, with a LTC conversion efficiency of over 90%. The peak electric field strength of the obtained strong-field circularly polarized THz radiation exceeded 100 kV/cm. This system is expected to be used to study the chiral characteristics of materials under strong-field conditions, as well as changes in the chiral characteristics under different field conditions.

Advantages of pulse-train excitation in narrow-band terahertz generation: mitigation of undesired nonlinear effects

In this work, we have studied the limitations of narrowband multi-cycle (MC) terahertz (THz) generation via optical rectification (OR) in periodically poled lithium niobate (PPLN) crystals. Detailed investigation of the transmitted beam profile, THz conversion efficiency (CE), and parasitic second-harmonic generation (SHG) strength as a function of incident pump beam size showed that Kerr-lensing is a significant bottleneck in the efficiency scaling of MC THz generation. We have also demonstrated that compared to the usage of a single pump pulse, excitation of the PPLN crystal via a pulse train, not only boosts up THz CE and narrows down the bandwidth of the achieved THz beam but also helps to mitigate the effect of undesired nonlinearities, such as Kerr-lensing and parasitic SHG.

Generation of terahertz radiation with a specified spectral profile from a mosaic combined organic crystal.

We present a method for the generation of terahertz (THz) pulses with a high optical-to-THz conversion efficiency and a smooth spectrum. The method is based on the optical rectification of near-infrared femtosecond laser pulses with a wavelength of 1240 nm in a mosaic combined crystal, consisting of two pieces of nonlinear organic crystals, OH1 and DSTMS. The mosaic combined crystal produces a relatively smooth spectrum in the 0.3-4.5 THz range with no pronounced absorption dips and with a maximum in a spectral amplitude at about 2 THz. The peak field strength is 9.6 MV/cm for an effective crystal diameter of 4.3 mm.

InAs Terahertz Metalens Emitter for Focused Terahertz Beam Generation

Metasurfaces have opened doors to combining multiple photonic functionalities in a single compact device. In particular, the ability to generate short terahertz (THz) pulses with precise wavefront engineering in a single THz metasurface redefined the role metasurfaces can play in THz systems. Here, an InAs metalens emitter which generates and focuses a THz pulse beam is demonstrated using a 130 nm thick InAs metasurface designed as a binary‐phase Fresnel zone plate. The THz beam is focused to a spot of ≈430 μm at 1 THz with a short focal length of 5 mm and large numerical aperture of 0.5. Nanoscale InAs Mie resonators comprising the metasurface enable THz generation with an amplitude as high as 20 times compared to plasmonic THz emitters and several times compared to a 1 mm thick ZnTe crystal. This InAs metasurface emitter provides a new paradigm for designing THz imaging, spectroscopy, and communication systems, where THz beam generation and shaping are performed with a single device without compromising the generation efficiency, while eliminating losses and avoiding limitations of phase matching of conventional nonlinear optics approaches.

Multi-resonance terahertz (THz) generation from magnetized cylindrical and spherical nanoclusters of AlAs and InP nanoparticles

We report a theoretical model for THz generation from the interaction of Gaussian laser beams with semiconductor nanoparticles suspended in argon gas in the presence of a DC magnetic field. Our investigations include two different shapes of nanoparticles [spherical (SNPs) and cylindrical (CNPs)]. The laser fields ionize nanoparticles converting them into plasma, which takes the form of spherical and cylindrical periodic nanoclusters with the electron density profile n=n0+nqeiqz, where q is the wave number of the density ripple and nq is the amplitude of density modulation. In our investigations, nanoparticles of AlAs and InP semiconductors are considered. Resonance condition is obtained when the laser beat frequency matches with the surface plasmon frequency of nanoparticles. We obtain resonances at two different frequencies when we apply a DC magnetic field. The resonance frequencies of THz fields shift with the nanoparticles' shape and orientation. THz field amplitude varies with material properties, spacing, size, and orientation of the nanoparticles. The applied magnetic field enhances the THz field and also helps in controlling the field profile. A THz field ∼0.1GV/cm with ∼2% efficiency is obtained for an optimized set of parameters for CNPs.

Cryogenically cooled periodically poled lithium niobate wafer stacks for multi-cycle terahertz pulses

We report on the generation of high-power narrow-bandwidth terahertz (THz) pulses by cryogenic cooling of hand-made periodically poled lithium niobate (PPLN) wafer stacks. As a proof-of-concept, we cool stacks with up to 48 wafers down to 97 K and achieve few-percent bandwidths at a center frequency of 0.39 THz, with pulse energy up to 0.42 mJ and average power of 21 mW. Supported by modeling, we observe effective cooling of PPLN wafer stacks that not only reduces terahertz absorption but critically maintains the micrometer-scale inter-wafer gaps for optimal terahertz transmission. Our results unlock the potential for scaling these large-area sources to greater numbers of wafers to push both the energy and bandwidth beyond current capability, opening up possibilities in areas such as terahertz-driven particle acceleration, terahertz imaging, and control over material properties.

Mid-infrared laser pulse excitation for terahertz generation from organic liquids molecules

Strong laser field is able to rotate gas molecules and the rotated gas molecules would emit electromagnetic waves when these molecules transition to the lower rotational energy levels. However, related investigation on liquid molecule rotation has not been reported, let alone the radiation falls in terahertz (THz) range. Here, a theoretical model is proposed to study the mid-infrared femtosecond laser driving organic liquid molecules such as methanol, ethanol, and acetic acid molecules to emit THz radiation. The interaction between laser electric field and liquid molecules are analyzed based on quantum mechanics theory. It is found that the spectrum of the THz radiation from methanol molecules range from 0.1 to 5 THz, while the spectra from ethanol and acetic acid molecules show nearly the same frequency range of 0.1–2 THz. These results indicate that broadband THz radiation can be generated through the transitions of rotational energy levels of the rotational liquid molecules excited by a linear polarization mid-infrared laser.

Refractive Index Resolved Imaging Enabled by Terahertz Time-Domain Spectroscopy Ellipsometry

Material characterization in the terahertz range is an interesting topic of research due to its great applications in material science, health monitoring, and security applications. Advances in terahertz generation, detection, and data acquisition have contributed to improved bandwidth, signal power, and signal-to-noise ratio. This enables advanced material characterization methods such as ellipsometry, which has been little explored in the terahertz frequency range, yet. Here, we introduce a comparison between material characterization with terahertz time-domain spectroscopy in transmission geometry and ellipsometry reflection geometry. Terahertz ellipsometry images were taken, showing spatially resolved refractive index estimation in the far field and higher image quality compared to single-polarization imaging.

Magnetic field enhanced terahertz emission from metallic nanostructures with response to laser spatial profile distribution

This communication proposes an analytical model that exhibits terahertz (THz) radiation generation from spatially corrugated noble-metal spherical and cylindrical nanoparticles (NPs) placed under the influence of an externally applied static magnetic field. This scheme involves the resonant excitation of THz radiation through the beat-wave of two lasers in the presence of ponderomotive nonlinearities. Effect of magnetic field as well as laser intensity profiles, which include super, cosh, flat-top and ring-shaped Gaussian profiles, have been investigated. The incorporation of the magnetic field induces substantially more dynamic laser-metal coupling and influences the surface plasmon resonance condition associated with electrons of the NPs, thereby leading to stronger THz emission. Our results also demonstrate that the spatial profile of the laser affects the THz output, as it impacts the excitation and dynamics of the NPs. Additionally, we find that both the shape, size and interparticle-separation of NPs play crucial roles in enhancing THz generation. Furthermore, we explore the effects of varying other parameters like electric field strength and beam waist of incident lasers. These findings provide valuable insights for the design and optimization of THz sources based on NP systems, offering new avenues for applications in spectroscopy, imaging, communication and biomedical sciences.

Plasmonic Crystals for Terahertz Detection, Amplification, and Generation

Plasmonic Crystals for Terahertz Detection, Amplification, and Generation

Harnessing complexity: Nonlinear optical phenomena in L-shapes, nanocrescents, and split-ring resonators.

We conduct systematic studies of the optical characteristics of plasmonic nanoparticles that exhibit C2v symmetry. In particular, we analyze three distinct geometric configurations: an L-type shape, a crescent, and a split-ring resonator shaped like the Greek letter π. Optical properties are examined using the finite-difference time-domain method. It is demonstrated that all three shapes exhibit two prominent plasmon modes associated with the two axes of symmetry. This is in addition to a wide range of resonances observed at high frequencies corresponding to quadrupole modes and peaks due to sharp corners. Next, to facilitate nonlinear analysis, we employ a semiclassical hydrodynamic model, where the electron pressure term is explicitly accounted for. This model goes beyond the standard Drude description and enables capturing nonlocal and nonlinear effects. Employing this model enables us to rigorously examine the second-order angular resolved nonlinear optical response of these nanoparticles in each of the three configurations. Two pumping regimes are considered, namely, continuous wave (CW) and pulsed excitations. For CW pumping, we explore the properties of the second harmonic generation (SHG). Polarization and angle-resolved SHG spectra are obtained, revealing strong dependence on the nanoparticle geometry and incident wave polarization. The C2v symmetry is shown to play a key role in determining the polarization states and selection rules of the SHG signal. For pulsed excitations, we discuss the phenomenon of broadband terahertz (THz) generation induced by the difference-frequency generation . It is shown that the THz emission spectra exhibit unique features attributed to the plasmonic resonances and symmetry of the nanoparticles. The polarization of the generated THz waves is also examined, revealing interesting patterns tied to the nanoparticle geometry. To gain deeper insight, we propose an analytical theory that agrees very well with the numerical experiments. The theory shows that the physical origin of the THz radiation is the mixing of various frequency components of the fundamental pulse by the second-order nonlinear susceptibility. An expression for the far-field THz intensity is derived in terms of the incident pulse parameters and the nonlinear response tensor of the nanoparticle. The results presented in this work offer new insights into the linear and nonlinear optical properties of nanoparticles with C2v symmetry. The demonstrated strong SHG response and efficient broadband THz generation hold great promise for applications in nonlinear spectroscopy, nanophotonics, and optoelectronics. The proposed theoretical framework also provides a valuable tool for understanding and predicting the nonlinear behavior of other related nanostructures.

Optimized terahertz generation in BNA organic crystals with chirped Ti:sapphire laser pulses.

We report on the efficient generation of intense terahertz radiation from the organic crystal N-benzyl-2-methyl-4-nitroaniline pumped by chirped Ti:sapphire femtosecond laser pulses. The THz energy and spectrum as a function of the pump fluence and duration of the chirped laser pulses are studied systematically. For the appropriate positively chirped pump pulses, a significant boost in the THz generation efficiency by a factor of around 2.5 is achieved, and the enhancement of high-frequency components (>1 THz) shortens the THz pulse duration. Via complete characterization of THz properties and transmitted laser spectra, this nonlinear behavior is attributed to the extended effective interaction length for phase matching as a result of the self-phase modulation of the intense pump laser pulses. Numerical calculations well reproduce the experimental observation. Our results demonstrate a robust, efficient, strong-field (up to several MV/cm) THz source using the common sub-10 mJ and sub-100 fs Ti:sapphire laser systems without optical parametric amplifiers.

Intercalation-enhanced topological material Bi2Se3: Tuning charge carrier and phonon dynamics for advanced optoelectronic and terahertz applications

The field of topological materials (TMs) is experiencing significant advancements due to their unique surface states, which offer considerable potential for optoelectronics and terahertz (THz) applications. Intercalation in TMs can effectively modulate these surface states, thereby altering electronic and optical properties and enhancing functionalities. This approach enables the tailoring of material properties for specific applications, broadening the utility of TMs across various technological domains. This study focuses on understanding the charge carrier and phonon dynamics in bismuth selenide (Bi2Se3) intercalated with various metals (AxBi2Se3, where A = Ag, Cr, Ni, Mn, Sm, Zn). We examine carrier trapping, carrier relaxation through optical and acoustic phonons, charge recombination processes, and variations in carrier temperature with probe delay lifetimes. Additionally, we explore coherent optical phonons (COPs) in MIBS, which oscillate at THz frequencies and have potential applications in THz generation and detection. Achieving tunability in the THz frequency of COP modes is a significant challenge; however, our research establishes a correlation between optical and structural properties and the dependence of COP frequencies on effective metal intercalation. This comprehensive investigation elucidates the intricate interplay between surface carriers and phonon dynamics in intercalated TMs, highlighting promising advancements for diverse technological applications, including spintronics, optoelectronics, and THz technology.

Efficient THz wave generation through intermodal four-wave mixing in the Ge waveguides with different geometries

ABSTRACT Intermodal four-wave mixing (FWM) in photonic waveguides offers a promising approach for efficient terahertz (THz) wave generation, crucial for advanced photonic systems. This study explores the potential of germanium (Ge) waveguides, leveraging their distinct dispersion profiles in transverse electric (TE), and transverse magnetic (TM) modes to achieve phase-matching for FWM. We conducted a numerical analysis of two waveguide geometries, ridge and plane, to optimize THz generation efficiency. Also, by optimizing waveguide geometry, it is possible to achieve higher conversion efficiency and broader THz bandwidth. The results demonstrate that Ge waveguides, particularly when utilizing same-phase laser pulses, can significantly enhance THz radiation and exhibit lower losses compared to traditional silicon-based designs. The findings suggest that integrating these optimized Ge waveguides with existing photonic components could lead to more versatile and efficient THz systems.

Magnetic field enhanced terahertz generation from shape-dependent metallic nanoparticles

Abstract This communication deals with the analytical study of terahertz (THz) generation via frequency-difference mechanism using two circularly symmetric Gaussian laser beams with slightly different frequencies ω 1 and ω 2 and wave vectors k → 1 and k → 2 simultaneously propagating through a mixture of spatially corrugated noble-metal nanoparticles. The mixture, consisting of spherical nanoparticles (SNPs) and cylindrical nanoparticles (CNPs), is placed in a host medium under the influence of an externally applied static magnetic field. The two co-propagating laser beams impart a nonlinear ponderomotive force on the electrons of the NPs, causing them to experience nonlinear oscillatory velocity. Furthermore, the consequent nonlinear current density excites THz radiation at the beat frequency ω ( = ω 1 − ω 2 ) . Magnetic fields influence the surface plasmon resonance condition associated with electrons of the nanoparticles due to enhancement in ponderomotive nonlinearities, thereby causing an increment in the amplitude of the generated THz field. It is observed that the generated THz radiation has a strong dependence on the shape and size of the NPs in addition to the magnetic field strength. CNPSs provide greater THz amplitude than SNPs due to additional resonance modes, and combining both kinds of nanostructures further enhances the amplitude. THz radiation plays an important role in biomedical and pharmaceutical fields, communications, security and THz spectroscopy.

Enhanced terahertz generation via plasma modulation on two bunches

Enhanced terahertz generation via plasma modulation on two bunches

Spectral programmable mid-infrared optical parametric oscillator

A spectral programmable, continuous-wave mid-infrared (MIR) optical parametric oscillator (OPO), enabled by a self-developed high-power spectral tailorable fiber laser, was proposed and realized. While operating at a single-wavelength, the maximum idler power reached 5.53 W at 3028 nm, with a corresponding pump-to-idler conversion efficiency of 14.7%. The wavelength number switchable output was available from one to three. The single idler was tunable in a range of 528 nm (2852–3380 nm). In a dual-wavelength operation, the interval between two idlers could be flexibly tuned for 470 nm (53–523 nm), and the intensity of each channel was controllable. Triple-wavelength idler emission was realized, meanwhile exhibiting spectral custom-tailored characteristics. Furthermore, we balanced the parametric gain through the pre-modulating broadband multi-peak pump spectra, enabling a 10 dB bandwidth adjustment of the idler emission from 20 to 125 nm. This versatile mid-infrared laser, simultaneously featuring wide tuning, multi-wavelength operation, and broad bandwidth manipulation, has great application potential in composition detection, terahertz generation, and speckle-free imaging.

THz generation by AlGaAs/GaAs heterostructured p-i-n diode

The generation of terahertz radiation by heterostructure p-i-n AlxGa1−xAs/GaAs diodes excited by femtosecond optical pulses was studied experimentally and using the Monte Carlo method. It is shown that when the reverse bias varies, the terahertz generation mechanism changes. With a positive bias on the p-i-n diode, the THz generation mechanism is due to the reflection of the photoexcited electrons from the interface. With a large internal electric field, THz generation in the p-i-n diode occurs due to the acceleration of electrons at the ballistic stage of their movement in the electric field to velocities significantly exceeding the steady state velocity (“velocity overshoot”). The subsequent sharp decrease in velocity of electrons is associated with their inter-valley transitions from the Γ-valley to the L-valley of the conduction band. At electric fields less than 22 kV/cm, the effect of electric field screening by photoexcited carriers has a significant impact on the formation of photocurrent and, accordingly, on the THz generation mechanism. As the reverse bias decreases, this effect leads to a shift in the maximum of the THz pulse toward shorter times and it begins to dominate at electric fields less than 10 kV/cm.

Generation of the vortex terahertz radiation by the interaction of two-color Laguerre–Gaussian laser with plasmas in the presence of a static magnetic field

The generation of vortex terahertz (THz) radiation by the interaction of a two-color Laguerre–Gaussian (LG) laser with plasmas under an external magnetic field is investigated theoretically and numerically. It is found that the vortex THz radiation with good monoenergetic properties can be generated successfully, and the orbital angular momentum of the LG lasers can be transferred to the radiation. In this scheme, the external magnetic field can not only enhance the intensity but can also break the spatial distribution symmetry of the vortex THz radiation. With the increase in the initial plasma density, the intensity of the vortex THz radiation increases significantly before reaching saturation and the spatial period of the radiation decreases, which indicates the monoenergetic peak of the vortex THz radiation can be well controlled through the initial plasma density. The relevant conclusions are verified by two-dimensional particle-in-cell simulations.