Gamma Beam Research Articles

Effects of Gamma-Irradiated Recycled Low-Density Polyethylene on the Creep and Recovery Properties of Asphalt

To improve the performance of recycled low-density polyethylene (LDPER), this paper describes the polymer modification of bitumen with gamma-irradiated recycled low-density polyethylene (γ-LDPER). The effects of the γ-LDPER on bitumen were investigated by means of morphological and chemical analyses, including Fourier-transform infrared spectroscopy and multiple stress creep recovery (MSCR) test. The results showed that the surface of the LDPER treated by gamma beam irradiation led to the formation of free radicals and some functional groups that may contribute to the creation of strong chemical bonds between the polymer modifier and bitumen, thus improving the compatibility of the modified asphalt. With the increased use of γ-LDPER, the modified asphalt rutting resistance also increased. However, due to the high γ-LDPER content of the modified asphalt, undertaking the high-temperature performance evaluation of the applicability of MSCR deserves further study.

Energy measurements by means of transition radiation in novel Linacs

Advanced linear accelerator design may use Optical Transition Radiation (OTR) screens to measure beam spot size; for instance, such screens are foreseen in plasma based accelerators (EuPRAXIA@SPARC_LAB) or Compton machines (Gamma Beam Source@ELI-NP). Optical Transition Radiation angular distribution strongly depends on beam energy. Since OTR screens are typically placed in several positions along the Linac to monitor the beam envelope, one may perform a distributed energy measurement along the machine. Furthermore, a single shot energy measurement can be useful in plasma accelerators to measure shot to shot energy variations after the plasma interaction. Preliminary measurements of OTR angular distribution of about 100 MeV electrons have been performed at the SPARC_LAB facility. In this paper, we discuss the sensitivity of this measurement to beam divergence and others parameters, as well as the resolution required and the needed upgrades of conventional OTR diagnostics, using as an example the data collected at SPARC_LAB.

Experiments with brilliant gamma beams at ELI-NP: A glimpse in the future

The emerging experimental program with brilliant gamma beams at the Extreme Light Infrastructure – Nuclear Physics facility (ELI-NP), which is under construction in Magurele, Romania is presented with emphasis on the prepared day-one experiments. Experiments at ELI-NP will cover nuclear resonance fluorescence (NRF) measurements, studies of large-amplitude motions in nuclei, photofission and photonuclear reactions of astrophysics interest, and measurements of photonuclear reaction cross sections. The physics cases of the flagship experiments at ELI-NP are discussed, as well as the related instruments which are under construction for their realization.

Effects of correlations between particle longitudinal positions and transverse plane on bunch length measurement: a case study on GBS electron LINAC at ELI-NP

In high-brightness LINear ACcelerators (LINACs), electron bunch length can be measured indirectly by a radio frequency deflector (RFD). In this paper, the accuracy loss arising from non-negligible correlations between particle longitudinal positions and the transverse plane (in particular the vertical one) at RFD entrance is analytically assessed. Theoretical predictions are compared with simulation results, obtained by means of ELEctron Generation ANd Tracking (ELEGANT) code, in the case study of the gamma beam system (GBS) at the extreme light infrastructure—nuclear physics (ELI-NP). In particular, the relative error affecting the bunch length measurement, for bunches characterized by both energy chirp and fixed correlation coefficients between longitudinal particle positions and the vertical plane, is reported. Moreover, the relative error versus the correlation coefficients is shown for fixed RFD phase 0 rad and rad. The relationship between relative error and correlations factors can help the decision of using the bunch length measurement technique with one or two vertical spot size measurements in order to cancel the correlations contribution. In the case of the GBS electron LINAC, the misalignment of one of the quadrupoles before the RFD between −2 mm and 2 mm leads to a relative error less than 5%. The misalignment of the first C-band accelerating section between −2 mm and 2 mm could lead to a relative error up to 10%.

Collimation and characterization of ELI-NP gamma beam

The ELI-NP facility, currently being built in Bucharest, Romania, will deliver an intense and almost monochromatic gamma beam with tunable energy between 0.2 and 20 MeV. The challenging energy bandwidth of [Formula: see text]0.5% will be adjusted through the collimation system, while the main beam parameters will be measured through a devoted gamma-beam characterization system.[Formula: see text] The gamma-beam characterization system, designed by the EuroGammaS collaboration, consists of four elements: a Compton spectrometer that measures the gamma energy spectrum; a sampling calorimeter for a fast combined measurement of the beam average energy and its intensity, which will be used also as a monitor during machine commissioning and development; a nuclear resonant scattering system for absolute energy inter-calibration of the other detectors; and a gamma beam profile imager to be used for alignment and diagnostics purposes. The collimation and characterization system will be presented in this article. These systems have already been built and tested, while the delivery at ELI-NP facility and the final commissioning is scheduled by Fall 2018.

Gamma-beam photofission experiments at ELI-NP: The future is emerging

At the Extreme Light Infrastructure - Nuclear Physics facility (ELI-NP), high-power laser systems together with high-brilliance gamma beams are the main research tools. The status of the construction of the facility is reported. The emerging photofission experimental program with brilliant gamma beams at ELI-NP is presented with emphasis on the prepared day-one experiments. The physics cases of the flagship experiments at ELI-NP are discussed, as well as the related instruments which are under construction for their realization.

Production of neutron-rich nuclei approaching r-process by gamma-induced fission of 238U at ELI-NP

The investigation of neutron-rich exotic nuclei is crucial not only for nuclear physics but also for nuclear astrophysics. Experimentally, only few neutron-rich nuclei near the stability have been studied, however, most neutron-rich nuclei have not been measured due to their small production cross sections as well as short half-lives. At ELI-NP, gamma beams with high intensities will open new opportunities to investigate very neutron-rich fragments produced by photofission of 238U targets in a gas cell. Based on some simulations, a novel gas cell has been designed to produce, stop and extract 238U photofission fragments. The extraction time and efficiency of photofission fragments have been optimized by using SIMION simulations. According to these simulations, a high extraction efficiency and a short extraction time can be achieved for 238U photofission fragments in the gas cell, which will allow one to measure very neutron-rich fragments with short half-lives by using the IGISOL facility proposed at ELI-NP.

Nuclear Physics Research at ELI-NP

The new research facility Extreme Light Infrastructure – Nuclear Physics (ELI-NP) is under construction in Romania, on the Magurele Physics campus. Valued more than 300 Meuros the center will be operational in 2019. The research center will use a high brilliance Gamma Beam and a High-power Laser beam, with unprecedented characteristics worldwide, to investigate the interaction of very intense radiation with matter with specific focus on nuclear phenomena and their applications. The energetic particle beams and radiation produced by the 2x10 PW laser beam interacting with matter will be studied. The precisely tunable energy and excellent bandwidth of the gamma-ray beam will allow for new experimental approaches regarding nuclear astrophysics, nuclear resonance fluorescence, and applications. The experimental equipment is presented, together with the main directions of the research envisioned with special emphasizes on nuclear physics studies.

Photodisintegration reactions for nuclear astrophysics studies at ELI-NP

Extreme Light Infrastructure - Nuclear Physics facility will come online in Bucharest-Magurele, Romania, in 2018 and will deliver high intensity laser and brilliant gamma beams. We present the physics cases and instruments proposed at ELI-NP to measure capture reactions by means of the inverse photodisintegration reaction. We propose to study the 16O(γ, α)12C reaction using a Time Projection Chamber detector with electronic readout. Several other reactions, such as 24Mg(γ, α)20Ne and reactions on heavy nuclei relevant in the p-process, are central to stellar evolution and will be investigated with a proposed Silicon Strip Detector array and a 4π neutron detector. The status of the experimental facilities and first-day experiments will be presented in detail.

Progress of the development of the ELI-NP GBS high level applications

The Gamma Beam System (GBS) is a high brightness LINAC to be installed in Magurele (Bucharest) at the new ELI-NP (Extreme Light Infrastructure — Nuclear Physics) laboratory. The accelerated electrons, with energies ranging from 280 to 720 MeV, will collide with a high power laser to produce tunable high energy photons (0.2–20 MeV ) with high intensity (1013 photons/s), high brilliance and spectral purity (0.1%BW), through the Compton backscattering process. This light source will be open to users for nuclear photonics and nuclear physics advanced experiments. Tested high level applications will play an important role in commissioning and operation. In this paper we report the progress and status of the development of dedicated high level applications. We also present the results of the test on the FERMI LINAC of the electron trajectory control method based on Dispersion Free Steering.

Temporal measurement of MeV pulsed gamma-ray using a diode laser

A single-shot temporal measurement of pulsed gamma ray using a diode laser has been carried out with the MeV gamma beams at “Qiangguang-I” facility. The gamma-ray temporal profile is encoded to the power of a diode laser by the carrier variation in laser cavity. We analyze the dynamic process of carriers induced by gamma rays and derive a sensitivity expression for the detector based on a diode laser. It shows that the sensitivity is determined by both the gain of resonant cavity and the efficiency of gamma-ray deposition in the diode laser. And the efficiency of depositing gamma-ray is estimated with Monte Carlo methods. The experimental results demonstrate that the detection method with diode lasers can be used for the temporal profile measurement of a MeV pulsed gamma ray source. The relative gamma-ray sensitivity of the detector is estimated at about 1.27×10−22Ccm2 from the experimental results, which agrees with the theoretical predictions.

Comparative study of gamma and ion beam irradiation of polymeric nanocomposite on electrical conductivity

ABSTRACTPoly(vinyl alcohol) (PVA) was used to prepare nanocomposites of multi‐wall carbon nanotubes (MWCNT) and functionalized carbon nanotubes (MWCNT‐NH2) in existence of 2‐carboxyethyl acrylate oligomers (CEA). Radiation‐induced crosslinking of the prepared matrix was carried out via gamma and ion beam irradiation. A comparative study of gamma and ion beam irradiation effect on the electrical conductivity of nanocomposite was conducted. The gelation of the gamma irradiated matrix outperforms the ion beam irradiated matrix. The order of gelation is PVA > (PVA/CEA) > (PVA/CEA)‐MWCNT > (PVA/CEA)‐MWCNT‐NH2. There is a significant reduction in the swelling of the nanocomposite. The formation of nanocomposites was confirmed by scanning electron microscopy, energy‐dispersive X‐ray (EDX) and FTIR examinations. The direct current electrical properties of PVA/nanocomposites are examined at room temperature by applying electric voltage from 1 to 20 V. The results revealed that the electrical conductivity is increased by adding the carbon nanotubes and irradiation by gamma and ion beam. At an applied electric voltage 20 V, in the electrical conductivity of the unirradiated PVA was from 9.20 × 10−8 S cm−1. After adding MWCNT an increase up to 4.70 × 10−5 S cm−1 was observed. While after ion beam irradiation, a further increase up to 9.30 × 10−5 S cm−1 was noticed. © 2017 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2018, 135, 46146.

A new method of creating high intensity neutron source

We propose a new scheme of producing an intense neutron beam whose yields may exceed those of the existing facilities by a few to several orders of magnitude in the sub-eV region. This scheme employs a MeV gamma beam extracted from circulating quantum ions, which has been recently proposed. The gamma beam is directed to a deuteron target and the photo-disintegration process generates a neutron beam. The calculated neutron energy spectrum is nearly flat down to the neV range, and thus there exists a possibility to utilize a good quality of neutrons especially in sub-eV energy region without using a moderator.

Highly improved operation of monolithic BGO-PET blocks

In PET scanners both scintillation crystals and photosensors are key components defining the system's performance and cost. Original PET systems used BGO or NaI(Tl) scintillators but achieved limited performance due to its slow decay and relatively low light output. Moreover, NaI(Tl) has low stopping power for 511 keV annihilation photons. In this study we report the possibility to reintroduce BGO crystals, and in particular in the form of monolithic blocks, especially suitable for low-dose large-size PET scanners, offering significantly improved sensitivity at a highly reduced cost compared to LYSO type fast scintillators. We have studied the performance of a monolithic BGO block as large as 50 × 50 × 15 mm3 with black-painted lateral walls to reduce lights spread, enabling accurate photon depth of interaction (DOI) measurements. A directional optical layer, called retro-reflector, was coupled to the entrance face bouncing back the scintillation light in the direction of the emission source and, therefore, adding to the light signal while preserving the narrow light cone distribution. Four configurations namely 12 × 12 and 16 × 16 SiPM arrays (3 mm × 3 mm each) as photosensors, with or without a nanopattern treatment at the crystal exit face, have been studied. This structure consisted of a thin layer of a specific high refractive index material shaped with a periodic nanopattern, increasing the scintillation light extraction. The readout returned information for each SiPM row and column, characterizing the X-Y light distribution projections. We have studied the detector spatial resolution using collimated 22Na sources at normal incidence. The DOI resolution was evaluated using collimated gamma beams with lateral incidence. The overall best detector performance was obtained for the 16× 16 SiPM array offering higher readout granularity. We have determined the spatial resolution for 3 separated DOI layers, obtaining the best results for the DOI region near to the photosensor.

Inhibiting Sterilization-Induced Oxidation of Large Molecule Therapeutics Packaged in Plastic Parenteral Vials.

For many years, glass has been the default material for parenteral packaging, but the development of advanced plastics such as cyclic olefin polymers and the rapidly increasing importance of biologic drugs have provided new choices, as well as more stringent performance requirements. In particular, many biologics must be stored at non-neutral pH, where glass is susceptible to hydrolysis, metal extraction, and delamination. Plastic containers are not susceptible to these problems, but suffer from higher gas permeability and a propensity for sterilization-induced radical generation, heightening the risk of oxidative damage to sensitive drugs. This study evaluates the properties of a hybrid material, SiOPlas™, in which an ultrathin multilayer coating is applied to the interior of cyclic olefin polymer containers via plasma-enhanced chemical vapor deposition. Our results show that the coating decreases oxygen permeation through the vial walls 33-fold compared to uncoated cyclic olefin polymers, which should allow for improved control of oxygen levels in sensitive formulations. We also measured degradation of two biologic drugs that are known to be sensitive to oxidation, teriparatide and erythropoietin, in gamma and electron beam sterilized SiOPlas™, glass, and uncoated cyclic olefin polymer vials. In both cases, solutions stored in SiOPlas™ vials did not show elevated susceptibility to oxidation compared to either glass or unsterilized controls. Taken together, these results suggest that hybrid materials such as SiOPlas™ are attractive choices for storing high-value biologic drugs.LAY ABSTRACT: One of the most important functions of parenteral drug containers is safeguarding their contents from damage, either chemical or physical. Glass has been the container material of choice for many years, but concerns over breakage and vulnerability to chemical attack at non-neutral pH have spurred the rise of advanced plastics as alternatives. Plastics solve many problems associated with glass but introduce several of their own, including increased gas permeation and generation of oxidizing radicals during sterilization. In this article, we evaluate SiOPlas™, a hybrid material consisting of plastic with a thin multilayer coating applied to the interior, for its ability to overcome these two problems. We find that SiOPlas™ is much less permeable to oxygen than uncoated plastic, and that two biologic drugs stored in gamma and electron beam sterilized SiOPlas™ vials do not display elevated levels of oxidation compared to either glass or unsterilized vials. This suggests that hybrid materials such as SiOPlas™ can exhibit the best qualities of both glass and plastic, making them attractive materials for storing high-value parenteral drugs.

Influence of gamma and electron beam sterilization on the stability of a premixed injectable calcium phosphate cement for trauma indications.

Premixed calcium phosphate cements (CPC's) are becoming the material of choice for injectable cements as a result of their effective delivery to the target implantation site. For orthopaedic use, it is of vital importance that the attributes of these CPC's are not compromised by irradiation sterilization. Therefore, the aim of this study is to determine the influence of irradiation sterilization on a range of premixed CPC's, with an emphasis on improving product shelf life through the use of optimal packaging configurations and annealing steps. Electron spin resonance (ESR) confirmed the presence of free radicals in the inorganic phase of the CPC paste following irradiation. The inclusion of a 24-h annealing step was the only successful method in reducing the degree of free radical formation. Based on the results of injectability force testing, it was revealed that an annealing step greater than 24-h significantly altered the viscosity, however; at 24-h the key attributes of the CPC paste were minimally effected. Overall, it was established that vacuum packing the CPC paste, placing the contents into a foil pouch, gamma irradiating at the minimal dose required and using an annealing step of ≤ 24-h, has the potential to extend the shelf life of the cement.

Effects of energy chirp on bunch length measurement in linear accelerator beams

The effects of assumptions about bunch properties on the accuracy of the measurement method of the bunch length based on radio frequency deflectors (RFDs) in electron linear accelerators (LINACs) are investigated. In particular, when the electron bunch at the RFD has a non-negligible energy chirp (i.e. a correlation between the longitudinal positions and energies of the particle), the measurement is affected by a deterministic intrinsic error, which is directly related to the RFD phase offset. A case study on this effect in the electron LINAC of a gamma beam source at the Extreme Light Infrastructure-Nuclear Physics (ELI-NP) is reported. The relative error is estimated by using an electron generation and tracking (ELEGANT) code to define the reference measurements of the bunch length. The relative error is proved to increase linearly with the RFD phase offset. In particular, for an offset of , corresponding to a vertical centroid offset at a screen of about 1 mm, the relative error is 4.5%.

Effects of gamma ray and electron beam irradiation on reduction of microbial load and antioxidant properties of Chum-Hed-Thet (Cassia alata (L.) Roxb.)

Considering the growing demands of herbal medicines, Cassia alata (L.) Roxb. has been reported to have various phytochemical activities. It has also been called in Thai as Chum-Hed-Thet. In this study, C. alata (L.) Roxb. powder were exposed to gamma and electron beam irradiation at doses of 0, 5, 10, 15 and 20 kGy. At the dose of 10 kGy, both of gamma and electron beam irradiation were sufficient in reducing microbial load of irradiated samples as specified in Thai pharmacopoeia (2005). These include the total aerobic microbial count of < 5.0x105 CFU/g, total fungi count of < 5.0x104 CFU/g, bile tolerant gram negative bacteria of < 104 (per g). In addition, pathogenic Clostridium spp. (per 10 g), Salmonella spp. (per 10 g), S. aureus (per 1g) and E.coli (per 1g) were absence. In terms of the bioactive molecules, the total phenolic content, DPPH free radical scavenging activity and ferric reducing antioxidant potential of unirradiated and irradiated samples were 19.32-22.44 mg gallic acid equivalent/g, 5.20-7.82 mg ascorbic acid equivalent/g and 69.46-82.06 μmol FeSO4/g, respectively. However, there were no significant differences between unirradiated and irradiated samples (p>0.05). Therefore, both of radiation by gamma ray or electron beam at 10 kGy was sufficient in elimination of microbial flora and did not significantly affected the total phenolic content and antioxidant activities of C. alata (L.) Roxb.

Project for a Source of Polarized Slow Positrons at ELI-NP

We describe the status of a project for obtaining an intense beam of polarized slow positrons at the Extreme Light Infrastructure - Nuclear Physics (ELI-NP) at Magurele (near Bucharest, Romania) [1]. Positrons will be created via pair production and moderated at a tungsten target using the pulsed brilliant gamma beam which will be produced by Compton back-scattering of circularly polarized laser photons on electrons from a warm linac beam [2]. Simulations of the interaction of circularly polarized γ‑rays of energies up to 3.5 MeV and an intensity of 2.4×1010γ/s with the target, moderation of created positrons and beam formation are discussed. The optimization of the target design showed that the primary slow positron beam can be obtained with intensity of 1‑2×106e+/s. The primary beam will be transversally polarized with a degree of polarization of ~30%. We discuss the necessity of changing the e+ beam polarization from transversal to longitudinal by an electrostatic 90˚ bender which is proposed to work in combination with a remoderator. Simulations show that neither the remoderator nor the electrostatic bender will change the degree of e+ beam polarization. The longitudinally polarized e+ can be successfully transported to the sample chambers without depolarization, but with reduced intensity (by approximately one order of magnitude) due to the remoderation. We present a convertor-moderator assembly with a hole which will allow creating positrons in parasitic mode, i.e., simultaneously with the nuclear physics experiments at ELI-NP. The positron spectroscopy laboratory at ELI-NP will be user dedicated and the beam will have the highest intensity of polarized slow positrons for material science in the world and therefore it could become a unique tool for investigation of magnetic samples.

A collimation system for ELI-NP Gamma Beam System – design and simulation of performance

The purpose of this study was to evaluate the performance and refine the design of the collimation system for the gamma radiation source (GBS) currently being realised at ELI-NP facility. The gamma beam, produced by inverse Compton scattering, will provide a tunable average energy in the range between 0.2 and 20MeV, an energy bandwidth 0.5% and a flux of about 108photons/s. As a result of the inverse Compton interaction, the energy of the emitted radiation is related to the emission angle, it is maximum in the backscattering direction and decreases as the angle increase [1,2]. Therefore, the required energy bandwidth can be obtained only by developing a specific collimation system of the gamma beam, i.e. filtering out the radiation emitted at larger angles. The angular acceptance of the collimation for ELI-NP-GBS must be continuously adjustable in a range from about 700 to 60μrad, to obtain the required parameters in the entire energy range. The solution identified is a stack of adjustable slits, arranged with a relative rotation around the beam axis to obtain an hole with an approximately circular shape. In this contribution, the final collimation design and its performance evaluated by carrying out a series of detailed Geant4 simulations both of the high-energy and the low-energy beamline are presented.