Landslides are the utmost damaging natural along with anthropogenic hazards which cause huge damage to assets and human lives in hilly environments all over the world. The key aim of this study is to explore landslide susceptibility (LS) maps along highways (SH-12 and NH-717A) in the Darjeeling Himalayas, India. Four data-driven bivariate statistical models (BSMs) were used to develop LS maps based on geospatial techniques. A total of 90 (100%) polygons with different size of landslide locations were identified to develop landslide inventory/distribution (LI/LD) map by incorporating Google Earth and satellite imageries, and filed investigation through the global positioning system (GPS). The LI/LD map is distributed into testing 30% (27 landslide locations), and training 70% (63 landslide locations) of the models. Eighteen landslide causative factors (LCFs) were selected to develop LS maps. Multicollinearity analysis showed that there is no collinearity problem in the LCFs. The receiver operating characteristics (ROC) curve and frequency ratio (FR) value techniques were applied for validation. The relative importance of each LCF for each model has been measured using Jack-knife test. The LS maps were divided into six landslide susceptibility zones (LSZs). The ROC curve showed the accuracy of the LSZ maps is 93.50% for FR, 85.90% for evidential belief functions (EBFs), 81.80% for fuzzy membership (FM) using FR, and 77.20% for FM using cosine amplitude (CA) approaches respectively. Among all models, the FR model showed the highest percentage of accuracy for LS assessment and prediction. The FR values of six LSZs rise from very low to very high LSZs which indicate a positive correlation between LSZs and FR values. The results of Jack-knife test showed that terrain ruggedness index (TRI) factor has the highest relative importance for all models in LSZ mappings. The study findings will help to the planner, and policymakers for spatial planning, implement slope management strategies, land use management in mountainous environments.