Frequency-entangled Photon Research Articles

Quantum and coherent signal transmission on a single-frequency channel via the electro-optic serrodyne technique.

Fiber-optical networks are well established to accommodate global data traffic via coherent information transmission. The next generation of telecommunications will require the integration of quantum information into fiber-optic networks, e.g., for quantum key distribution. A promising and scalable route to enable quantum networking is encoding quantum information into the frequency of photons. While the cointegration of frequency-entangled photons with coherent information transmission is achieved via spectral multiplexing, more resource-efficient approaches are required. In this work, we introduce and experimentally demonstrate a transceiver concept that enables the transmission of coherent and frequency-entangled photons over a single-frequency channel. Our concept leverages the serrodyne technique via electro-optic phase modulation leading to very different dynamics for entangled and coherent photons. This enables temporal multiplexing of the respective signals. We demonstrate the preservation of entanglement over the channel in the presence of coherent light. Our approach reveals a strong potential for efficient bandwidth use in hybrid networks.

Single-pass generation of widely-tunable frequency-domain entangled photon pairs.

We demonstrate a technique that generates frequency-entangled photon pairs with strong polarization correlation by using a single-period nonlinear crystal and single pass configuration. The technique is based on the simultaneous occurrence of two spontaneous parametric down-conversion processes satisfying independent type-II collinear quasi-phase matching conditions in periodically poled stoichiometric lithium tantalate. The generated photon pairs exhibit non-degenerate Hong-Ou-Mandel interference, indicating the presence of quantum entanglement in the frequency domain. This method provides a light source capable of wide-range quantum sensing and quantum imaging or high-dimensional quantum processing.

Delayed-choice quantum erasure with nonlocal temporal double-slit interference

Wave–particle duality is a counterintuitive nature of quantum physics that challenges many common-sense assumptions, and Young’s double-slit interference is a prototypical example. While most quantum erasure experiments emphasized the choice of erasing or marking the which-path information of one quantum system, we use frequency entanglement to report a nonlocal temporal double-slit interferometer such that the which-time information determines the wave-like or particle-like behaviors. Since frequency-entangled photons are created simultaneously by using spontaneous parametric down conversion, the mark of temporal distinguishability is readily prepared by delaying one of the entangled photons, and its quantum eraser is implemented by using spectrally resolved detection with a tunable delayed choice. These results may provide an alternative aspect and insight into the role of the temporal degree in quantum-light complementarity and photon interference.

Role of indistinguishability and entanglement in Hong-Ou-Mandel interference and finite-bandwidth effects of frequency-entangled photons

We investigate the relation between indistinguishability and quantum entanglement in Hong-Ou-Mandel interference experiments theoretically and relate these quantum mechanical principles to the theorem of entanglement monogamy. Employing Glauber's theory of quantum coherence we compute the detection statistics in HOM interference of frequency-entangled photons and find an additional term in the coincidence detection probability, which is related to the spectral indistinguishability of the considered photons that arises from finite-bandwidth effects and therefore is relevant in the limit of low-frequency separations or large single-photon bandwidths. Compared to previous work in that context we treat all photonic degrees of freedom on equal footing.

Spatial separation of collinearly emitted broadband frequency-correlated photon pairs

The authors demonstrate the efficient separation of broadband frequency-entangled photon pairs generated in the same spatial and polarization mode. Entangled photons with a broad bandwidth of 90 nm are successfully separated using time-reversed Hong-Ou-Mandel interference.

Silicon source of frequency-bin entangled photons.

We demonstrate an integrated source of frequency-entangled photon pairs on a silicon photonics chip. The emitter has a coincidence-to-accidental ratio exceeding 103. We prove entanglement by showing two-photon frequency interference with a visibility of 94.6% ± 1.1%. This result opens the possibility of on-chip integration of frequency-bin sources with modulators and the other active and passive devices available in the silicon photonics platform.

Entangled photons from composite cascade emitters.

One of the most versatile sources for entangled photons are emitters that interact via more than one tunable mechanism. Here, we demonstrate how hybridization and dipole-dipole interactions-potentially simultaneously available in colloidal quantum dots and molecular aggregates-leveraged in conjunction can couple simple, well understood emitters into composite emitters with flexible control over the level structure. We show that cascade decay through carefully designed level structures can result in emission of frequency-entangled photons with Bell states and three-photon GHZ states as example cases. These results pave the way toward rational design of quantum optical emitters of entangled photons.

Ghost imaging as loss estimation: Quantum versus classical schemes

Frequency correlations are a versatile and powerful tool which can be exploited to perform spectral analysis of objects whose direct measurement might be unfeasible. This is achieved through a so-called ghost spectrometer, that can be implemented with quantum and classical resources alike. While there are some known advantages associated to either choice, an analysis of their metrological capabilities has not yet been performed. Here we report on the metrological comparison between a quantum and a classical ghost spectrometer. We perform the estimation of the transmittivity of a bandpass filter using frequency-entangled photon pairs. Our results show that a quantum advantage is achievable, depending on the values of the transmittivity and on the number of frequency modes analyzed.

Highly Coherent Frequency-Entangled Photons Based on Parametric Instability in Active Fiber Ring Cavity

Highly Coherent Frequency-Entangled Photons Based on Parametric Instability in Active Fiber Ring Cavity

Spectral characterization of photon-pair sources via classical sum-frequency generation.

Tailoring spectral properties of photon pairs is of great importance for optical quantum information and measurement applications. High-resolution spectral measurement is a key technique for engineering spectral properties of photons, making them ideal for various quantum applications. Here we demonstrate spectral measurements and optimization of frequency-entangled photon pairs produced via spontaneous parametric downconversion (SPDC), utilizing frequency-resolved sum-frequency generation (SFG), the reverse process of SPDC. A joint phase-matching spectrum of a nonlinear crystal around 1580 nm is captured with a 40 pm resolution and a > 40 dB signal-to-noise ratio, which is significantly improved compared to traditional frequency-resolved coincidence measurements. Moreover, our scheme is applicable to collinear degenerate sources whose characterization is difficult with previously demonstrated stimulated difference frequency generation (DFG). We also illustrate that the observed phase-matching function is useful for finding an optimal pump spectrum to maximize the spectral indistinguishability of SPDC photons. We expect that our precise spectral characterization technique will be useful tool for characterizing and tailoring SPDC sources for a wide range of optical quantum applications.

Fourier domain quantum optical coherence tomography.

Quantum optical coherence tomography (Q-OCT) is the non-classical counterpart of optical coherence tomography (OCT), a high-resolution 3D imaging technique based on white-light interferometry. Because Q-OCT uses a source of frequency-entangled photon pairs, not only is the axial resolution not affected by dispersion mismatch in the interferometer but is also inherently improved by a factor of two. Unfortunately, practical applications of Q-OCT are hindered by image-scrambling artefacts and slow acquisition times. Here, we present a theoretical analysis of a novel approach that is free of these problems: Fourier domain Q-OCT (Fd-Q-OCT). Based on a photon pair coincidence detection as in the standard Q-OCT configuration, it also discerns each photon pair by their wavelength. We show that all the information about the internal structures of the object is encoded in the joint spectrum and can be easily retrieved through Fourier transformation. No depth scanning is required, making our technique potentially faster than standard Q-OCT. Finally, we show that the data available in the joint spectrum enables artefact removal and discuss prospective algorithms for doing so.

Probing excited-state dynamics with quantum entangled photons: Correspondence to coherent multidimensional spectroscopy.

Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission measurement of frequency-entangled broadband photon pairs generated via parametric down-conversion with a monochromatic laser. It is observed that state-to-state dynamics in the system under study are temporally resolved by adjusting the path difference between the entangled twin beams when the entanglement time is sufficiently short. The non-classical photon correlation enables time-resolved spectroscopy with monochromatic pumping. It is further demonstrated that the signal corresponds to the spectral information along anti-diagonal lines of, for example, two-dimensional Fourier-transformed photon-echo spectra. This correspondence inspires us to anticipate that more elaborately engineered photon states would broaden the availability of quantum light spectroscopy.

Quantification of nonlocal dispersion cancellation for finite frequency entanglement.

Benefiting from the unique quantum feature of nonlocal dispersion cancellation (NDC), the strong temporal correlation of frequency-entangled photon pair source can be maintained from the unavoidable dispersive propagation. It has thus played a major role in many fiber-based quantum information applications. However, the limit of NDC due to finite frequency entanglement has not been quantified. In this study, we provide a full theoretical analysis of the NDC characteristics for the photon pairs with finite frequency entanglement. Experimental examinations were conducted by using two spontaneous parametric down-conversion photon pair sources with frequency correlation and anticorrelation properties. The excellent agreement demonstrates the fundamental limit on the minimum temporal correlation width by the nonzero two-photon spectral correlation width of the paired photons, which introduces an inevitable broadening by interaction with the dispersion in the signal path. This study provides an easily accessible tool for assessing and optimizing the NDC in various quantum information applications.

Engineering two-photon wavefunction and exchange statistics in a semiconductor chip

High-dimensional entangled states of light provide novel possibilities for quantum information, from fundamental tests of quantum mechanics to enhanced computation and communication protocols. In this context, the frequency degree of freedom combines the assets of robustness to propagation and easy handling with standard telecommunication components. Here, we use an integrated semiconductor chip to engineer the wavefunction and exchange statistics of frequency-entangled photon pairs directly at the generation stage, without post-manipulation. Tailoring the spatial properties of the pump beam allows generating frequency-anticorrelated, correlated and separable states, and to control the symmetry of the spectral wavefunction to induce either bosonic or fermionic behaviors. These results, obtained at room temperature and telecom wavelength, open promising perspectives for the quantum simulation of fermionic problems with photons on an integrated platform, as well as for communication and computation protocols exploiting antisymmetric high-dimensional quantum states.

Inherent resolution limit on nonlocal wavelength-to-time mapping with entangled photon pairs.

Nonlocal wavelength-to-time mapping between frequency-entangled photon pairs generated with the process of spontaneous parametric down-conversion is theoretically analyzed and experimentally demonstrated. The spectral filtering pattern experienced by one photon in the photon pair will be non-locally mapped into the time domain when the other photon propagates inside a dispersion-compensation fiber with large group velocity dispersion. Our work, for the first time, points out that the spectral bandwidth of the pump laser will become the dominated factor preventing the improvement of the spectral resolution when the involved group velocity dispersion is large enough, which provides an excellent tool for characterizing the resolution of a nonlocal wavelength-to-time mapping for further quantum information applications.

Quantum soliton evaporation

Quantum evaporation may occur in a variety of systems such as superfluids, Bose-Einstein condensates, and gravitational black holes (Hawking radiation). However, to date all predictions are based on semiclassical models, e.g., the Einstein equations and classical space-time metric for a black hole and only the fluctuations are quantized. Here we use a fully quantized dynamical equation, the quantum nonlinear Schr\odinger equation, to study the evolution of quantum solitons. As a result of quantum fluctuations in the center-of-mass position, the expectation value of the quantum soliton width increases and concomitantly evaporates through the emission of frequency-entangled photon pairs. The frequency of this emission decreases as the soliton evaporates due to the soliton spreading. In the final phase, the soliton mean field collapses irreversibly into a state with zero mean amplitude. These results may provide insight to quantum evaporation in other systems where a full quantum description is still to be developed and highlights that even classically stable systems may also be subject to quantum evaporation.

Enhanced vibrational-mode-selective two-step excitation using ultrabroadband frequency-entangled photons

We theoretically investigate strongly enhanced vibrational-mode-selective two-step excitation by ultrabroadband frequency-entangled photons. A diatomic molecule having three sets of vibronic states is used to evaluate the excitation efficiency of the two-step excitation. We show that the photon entanglement has little influence on the populations of intermediate vibrational modes of intermediate states but selectively increases the population of a single vibrational mode of excited states, resonant with the total energy of the entangled photons. For an ultrashort pulse close to a monocycle with high degree of entanglement, the population of the vibrational mode is enhanced 2500 times more than by uncorrelated photons, and the selectivity nearly reaches unity. Our results indicate that the two-step excitation with ultrabroadband frequency-entangled photons can achieve highly selective and strongly enhanced excitation of a single vibrational mode.

Optical sectioning in induced coherence tomography with frequency-entangled photons

We demonstrate a different scheme to perform optical sectioning of a sample based on the concept of induced coherence [Zou et al., Phys. Rev. Lett. 67, 318 (1991)]. This can be viewed as a different type of optical coherence tomography scheme where the varying reflectivity of the sample along the direction of propagation of an optical beam translates into changes of the degree of first-order coherence between two beams. As a practical advantage the scheme allows probing the sample with one wavelength and measuring photons with another wavelength. In a bio-imaging scenario, this would result in a deeper penetration into the sample because of probing with longer wavelengths, while still using the optimum wavelength for detection. The scheme proposed here could achieve submicron axial resolution by making use of nonlinear parametric sources with broad spectral bandwidth emission.

Performance optimization for quantum key distribution in lossy channel using entangled photons**Project supported by the National Natural Science Foundation of China (Grant Nos. 61573059, 61401340, and 61172138), the Natural Science Basic Research Plan in Shaanxi Province of China (Grant No. 2016JM6035), and the Fundamental Research Funds for the Central Universities, China (Grant No. JB161303).

In quantum key distribution (QKD), the times of arrival of single photons are important for the keys extraction and time synchronization. The time-of-arrival (TOA) accuracy can affect the quantum bit error rate (QBER) and the final key rate. To achieve a higher accuracy and a better QKD performance, different from designing more complicated hardware circuits, we present a scheme that uses the mean TOA of M frequency-entangled photons to replace the TOA of a single photon. Moreover, to address the problem that the entanglement property is usually sensitive to the photon loss in practice, we further propose two schemes, which adopt partially entangled photons and grouping-entangled photons, respectively. In addition, we compare the effects of these three alternative schemes on the QKD performance and discuss the selection strategy for the optimal scheme in detail. The simulation results show that the proposed schemes can improve the QKD performance compared to the conventional single-photon scheme obviously, which demonstrate the effectiveness of the proposed schemes.

Generation of broadband ultraviolet frequency-entangled photons using cavity quantum plasmonics

Application of quantum entangled photons is now extending to various fields in physics, chemistry and biology. In particular, in terms of application to molecular science, broadband ultraviolet frequency-entangled photons are desired because molecules inducing photochemical reactions of interest often have electronic transition energies in the ultraviolet region. Recent standard method for generating such entangled photons is a chirped quasi-phase-matching method, however this method is not suitable for the generation of ultraviolet frequency-entangled photons because it requires down-conversion of a photon with a wavelength shorter than ultraviolet into an entangled photon pair. Here we propose a simple method for generating broadband ultraviolet frequency-entangled photons using cavity quantum plasmonics, in which conventional cavity quantum electrodynamics theory is applied to quantum plasmonics. We introduce a cavity-plasmon system in which localised surface plasmon (LSP) is coupled to the cavity fields of a state-of-the-art microcavity. Using this system, we theoretically show that broadband ultraviolet frequency-entangled photons can be generated simply by utilising the absorption saturation effect of LSP.