AbstractThe “thinking face” is a facial signal used to convey being in thought. For androids, the thinking face may be important to achieve natural human–robot interaction. However, the facial pattern necessary for portraying the thinking face remains unclear and has not yet been investigated in androids. The current study aims to (a) identify the facial patterns when people are engaged in answering complex questions (i.e., thinking face) and (b) clarify whether implementing the observed thinking faces in an android can facilitate natural human–robot interaction. In Study 1, we analyze the facial movements of 40 participants after they are prompted with difficult questions and indicate five facial patterns that corresponded to thinking faces. In Study 2, we further focus on the pattern of furrowing of the brows and narrowing of the eyes among the observed thinking facial patterns and implement this pattern in an android. The results show that thinking faces enhance the perception of being in thought, genuineness, human-likeness, and appropriateness in androids while decreasing eeriness. The free-description data also revealed that negative emotions are attributed to the thinking face. In Study 3, we compared the thinking vs. neutral faces in a question–answer situation. The results showed that the android's thinking face facilitated the perception of being in thought and human-likeness. These findings suggest that the thinking face of androids can facilitate natural human–robot interaction.