With the advancements in deep learning and neural network technologies within the engine technology domain, intelligent control of exhaust after-treatment systems has become viable. The exhaust temperature significantly affects the NOx conversion efficiency of the SCR system. In this study, a time-series prediction model for exhaust temperature and NOx emissions was first developed using the LSTM neural network based on experimental data, and a Multi-Head Attention Mechanism was introduced to enhance the model’s predictive performance (LSTM-MA model). Subsequently, a dual-stage SCR system’s ammonia-to-NOx ratio control method (LSTM-ANR) was developed based on LSTM-MA model. The potential of the dual-stage SCR system using the LSTM-ANR control method to reduce NOx emissions during the WHTC cycle was analyzed using GT-Power and Simulink software. Finally, the experimental results show that the cold-state and hot-state WHTC cycle’ weighted NOx emission and conversion efficiency are 0.165 g/kW·h and 98.6%, respectively. Compared to the original data from the engine, NOx emission was reduced by 64.13%. This proves that the control method can effectively lower NOx emission.
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