More recently, the ability of the coprime array to yield large array apertures and high degrees of freedom in comparison with the uniform linear array (ULA) has drawn an enormous amount of attention. In light of this, we propose a low-rank matrix completion algorithm via minimization of the ratio of the nuclear norm and the Frobenius norm (N/F) to solve the two-dimensional (2D) direction finding problem for the L-shaped coprime array (LsCA). Specifically, we first interpolate the virtual co-array signal related to the cross-correlation matrix (CCM) and utilize the interpolated virtual signal for Toeplitz matrix reconstruction. Then, the N/F method is employed to perform low-rank matrix completion on the reconstructed matrix. Finally, exploiting the conjugate symmetry characteristics of the completed matrix, we further develop a direction-finding algorithm that enables 2D angle estimation. Remarkably, the 2D angles are able to be automatically paired by the proposed algorithm. Numerical simulation findings demonstrate that the proposed N/F algorithm generates excellent angular resolution and computational complexity. Furthermore, this algorithm yields better estimation accuracy compared to the competing algorithms.