Radionuclide Concentrations Research Articles

Assessment of radiological contamination due to gold mining in soil and food crops of Babban Tsauni, Gwagwalada, Nigeria.

This work assessed the activity concentrations of 238U(226Ra), 232Th, and 40K and their associated radiological risks due to exposure to soil and consumption of food crops in Babban Tsauni artisanal gold mine, Gwagwalada, Nigeria, using the gamma spectrometry technique. The mean activity concentrations of 226Ra, 232Th, and 40K in the mine soil were 60.2±9.9, 161.4±16.2, and 664.6±138.2, while they were 46.4±4.9, 79.9±39.3, 266.4±185.4 for tubers and 46.9±15.7, 100.5±35.8, 311.4±132.7 (Bq/kg) for grains, respectively. The results reveal that the activity concentrations of radionuclides in all samples exceeded the recommended values set by United Nations Scientific Committee on the Effects of Atomic Radiation (33, 45, and 420 Bq/kg) except 40K, which fell within the acceptable limit in all food crop sample types. Estimated results for radiological hazard parameters, radium equivalent, annual effective dose due to ingestion, and excess life cancer risk were within safe limits, while the annual effective dose due to external gamma radiation in soil and annual gonadal equivalent dose were significantly high in all investigated samples; these call for constant radiological monitoring.

Evaluation of Radioactivity Concentration and Hazard Indices in ash Some Hospitals Incinerators in Baghdad / Al Resafa

Due to their harmful effects on human health and their tendency to cause cancer, radionuclide concentrations and risk indicators have been measured in hospital incinerator ash. This was done by collecting samples ash of Hospitals Incinerators, examining them, and identifying the risks that emerged from the examination. Three samples Only taken for the study from certain hospitals affiliated with the Baghdad Al-Rusafa Health Department. High purity germanium gamma spectrometer (HPGe) were used to analyze the samples. The concentrations of potassium isotopes (K-40) range from (147.1±16.5 to 214.4±21.1 Bq/kg), While the range of concentrations for Ra-226 isotopes is (7.52±1 to 19±1.8 Bq/kg), and lead (Pb-212) isotope concentrations ranged from (10.1±1.1 to 11.1±1.5 Bq/kg). In addition, the isotope concentration of actinium (Ac-228) is 8.05±1. Radium equivalent (), risk index , annual effective dose equivalent radioactivity level index ), absorbed dose rate D, and lifetime cancer risk were calculated. The results showed that no radiation risk Only indicated by any of the risk indicators. This indicates that the ash from the hospital incinerator does not pose any radioactive danger.

Problems of management of patient biological waste in radionuclide diagnostics

Biological excretion from patients (urine) generated during radionuclide diagnostics enters directly into the hospital sewage system. The establishment of new clearance level according to Resolution of the Government of the Russian Federation No. 1069 of October 19, 2012 may entail amendments to regulatory documents for radionuclide diagnostics departments. One of these requirements is a mandatory dedicated sewage system. Establishment of the requirement may lead to an increase the cost of the radionuclide diagnostic examinations, and to a decrease the accessibility of radionuclide diagnostic. The aim of this study was to estimate the activity of radionuclides in patient urine after radionuclide diagnostic and activity concentration in sewage water in the hospital and in the transport tank of toilet for evaluation of paths of waste manage. Based on published literature data, models of biological excretion were constructed for the following radiopharmaceuticals: 99mTc-pyrophosphate, 64Cu-Labeled Monoclonal Antibody, 18F-FDG, 68Ga-PSMA-617. The activity of radionuclides in the patient waste in the hospital and in public transport during the patient transportation to home was calculated. Various scenarios of patient transportation were considered. The values of the excreted activity, activity concentration and dose rate at 1 m from the tank with sewage water for each type of transport were calculated. The calculated values of the radionuclide activity concentration in sewage water in transport tank of toilet for the majority scenarios exceed the clearance level (up to 180 times for 68Ga-PSMA-617 when traveling by bus). According the regulatory requirements, it is necessary to collect patient excretions after radionuclide diagnostic examinations and hold it for decay. However, estimated effective doses of individuals from the public from contact with biological patient waste do not exceed the acceptable value. This is due to the short half-life of diagnostic radionuclides. The paths of management system of biological patient waste were proposed.

Estimation of radiological health risks due to 226Ra, 232Th, and 40K in foods consumed in Iraqi Kurdistan Region

ABSTRACT This study investigates the activity concentration of natural radionuclides in a diverse range of food samples in the Koya district markets food baskets, including both domestic and imported products. The samples cover annual crops (e.g. coffee, tea, kidney beans), tree nuts (e.g. almonds, pistachios), and other items (e.g. beef, fish, milk) by using a high-purity germanium (HPGe) detector. This research addresses a notable gap by providing baseline data on radionuclide concentrations and assessing potential health risks. Average activity concentrations for ²²⁶Ra, ²³²Th, and ⁴⁰K were 0.943, 0.367, and 191.8 Bq kg−1, respectively. Radium equivalent activity values ranged from 2.88–58.48 Bq kg−1, all below the safety limit. The average excess lifetime cancer risk (ELCR) was 0.154 mSv a−1, indicating safety for most samples, though coffee and tea showed higher levels. This study provides new data crucial for future research and regulatory monitoring, underscoring the need for further investigation into geological impacts on radionuclide levels.

Influence of earthworms on the mobility and bioavailability of metals, metalloids and radionuclides in historically contaminated soil

While soil characteristics such as pH, cation exchange capacity and organic matter are known to influence the mobility of pollutants in soil and the transfer to vegetation, far less attention has been paid to the possible non-trophic influence of organisms on pollutant transfer to other species. When pollutants are present in a bound unavailable form in the mineral or organic fraction, they can be made available through bio-weathering and decomposition of organic material. Within this study, the impact of earthworms on the mobility of metal(loid)s and radionuclides in soil and their transfer to vegetation was evaluated and the pathways through which earthworms work were studied. Soil from a Belgian field, historically contaminated with metal(loid)s and radionuclides, was used and microcosm systems were applied to mimic the natural interactions between soil, earthworms (Lumbricus terrestris) and vegetation (Lolium perenne). Metal and radionuclide concentrations were determined in soil, pore water and grass. In addition, soil pH, (chromophoric) dissolved organic matter, the ionic composition of pore water and the soil microbial activity were analysed. In general, earthworm presence significantly increased the concentration of most pollutants in soil pore water. This could be a direct consequence of decreased soil pH and increased humification. The latter also lead to higher nutrient concentrations in pore water that were depleted in the root zone due to high accumulation by plants. Indications were found for earthworm-induced effects on the soil microbial activity. The results show that earthworm activity can increase leaching of metal(loid)s and radionuclides and enhance dispersion into the environment and transfer to other biota and the food chain. Biologically induced release or remobilization of pollutants in the soil should therefore be considered in the context of risk assessment and site management strategies.

Distribution and in situ bioaccumulation test of radioecologically relevant metals in boreal freshwater sediments

Sediments act as important sinks for metals and their radionuclides in aquatic environments and play a crucial role in their transfer and uptake to aquatic organisms. Traditional radioecological models use radionuclide concentrations in water to predict concentrations in aquatic organisms. In this study, we investigated the distribution of radioecologically important metals (Ba, Co, Ni, Sr, U) among sediment, porewater and hypolimnion over seasons. We also studied the uptake of these metals to benthic organisms and importance of sediment as an uptake source by conducting a 28-day in situ bioaccumulation experiment with oligochaete worms (Lumbriculus variegatus). The studied metals were chosen based on common occurrence of their radioactive isotopes in nuclear fuel cycle. Measurements of total elemental concentration were used as proxies to study the behavior of specific radionuclides. Sediment and water samples were collected from two small lakes connected to a former uranium mine in Eastern Finland, and from a nearby reference lake connected to a different drainage area. Environmental characteristics and concentrations measured from sediment, porewater and overlying water indicated only minor changes between seasons. Measured metals were highly associated with sediment particles, rather than porewater or hypolimnion. Both the distribution of metals and in situ experiment indicated the importance of sediment as the main source of bioaccumulation. Significant differences in Ba, Ni and U concentrations between treatments containing contaminated sediment and reference sediment were noted, regardless of water concentrations. Additionally, as U contaminated lakes lacked seasonal overturn during our monitoring period, metal distribution and environmental conditions remained unchanged in deeper parts of those lakes. Lastly, the results of this in situ bioaccumulation experiment are in line with the findings of our previous laboratory study using sediments from these same lakes.

Radiation doses assessment and radon exhalation rate from the soils of Albyda area, Yemen

This work focuses on evaluating the potential health hazards posed by natural radionuclides in soil samples collected from 20 different sites in the Albyda area, Yemen. The activity concentrations of 226Ra, 232Th and 40K and radon exhalation rates in the soil samples were investigated. Alpha GUARD detector was used to estimate 222Rn concentration, while activity levels for natural radionuclides were measured by HPGe detector. The average values obtained for 226Ra, 232Th, and 40K were 27.60 ± 2.40 Bq/kg, 35.07 ± 2.45 Bq/kg, and 544.71 ± 48 Bq/kg, respectively, and for 222Rn concentrations were 135 ± 15 Bq/m3. Our findings show that the concentrations of radionuclides were within the limits of the world average established by UNSCEAR, except the concentrations of 40K, which was slightly higher than the world average (420 Bq/kg), while the average 222Rn concentration was lower than the ICRP reference level of 300 Bq/m3, and the average area exhalation rate 3.46 × 10−5 Bq m−2 s−1 was lower than the UNSCEAR world average of 0.016 Bq m−2 s−1. Therefore, the soil in this study does not pose any radiological hazard to the population due to the harmful effects of ionizing radiation. The results of the current study highlight the potential health hazard posed by radon and radioactivity levels in the soil samples from Albyda area, Yemen, which will help to increase awareness of the radiological hazard and the data could also be used as a reference for future research on radioactivity mapping in the study area.

Environmental Radioactivity Monitoring and Radiological Impact Assessment of Agbara Industrial Area, Ogun State, Nigeria

This study assessed the naturally occurring radioactivity of 40K, 238U, and 232Th, which pose a significant threat to human health, particularly when their concentrations exceed the threshold. Background radiation levels were measured at two specific locations, Access Bank and Market areas, across a total of forty (40) sample points. The measurements were taken using a calibrated RS125 Gamma Spectrometer (a portable NaI [Tl] detector) designed in Canada, in conjunction with a global positioning system (GPS) to accurately record the research coordinates within the Agbara industrial area, Ogun State, Nigeria. The mean activity concentrations of the primordial radionuclides were 177.87 Bqkg-1, 20.01 Bqkg-1, and 52.90 Bqkg-1 for 40K, 238U, and 232Th, respectively. More so, the in-situ measured dose rate (DR) ranges between 12.18 nGyh-1 (Access Bank area) and 97.95 nGyh-1 (Market area), with an average value of 47.22 nGyh-1. The average measured and estimated absorbed dose rates were within the safe limit of 57 nGyh-1 provided by UNSCEAR. However, the measured dose rates exceeded the recommended limit in ten locations, while measured activity for thorium exceeded the world average value for over half of the study locations. Although all estimated radiological parameters were within recommended threshold values, suggesting the low risk of exposure to higher levels of ionising radiation in most locations in the Agbara industrial area, there is a potential cancer risk for individuals who have resided in the area for 70 years or more due to long-term exposure to ionising radiation.

Measurement of natural radiation levels in some soil samples from the ancient city of Borsippa in Babylon Governorate, Iraq

Abstract In the present study, the activity concentration of natural radionuclides was determined for 40K, 232Th, and 238U. Some samples of soil from the ancient city of Borsippa in Babylon Governorate. The detector sodium iodide activated by Thallium NaI (Tl) has been used to perform the radioactivity measurements. 15 samples had their natural radioactivity levels assessed. 40K, 232Th, and 238U had average specific activities of (167.86±1.19, 25.15±1.09, and 11.75±0.457) Bq/kg. The average radium equivalent (61.17±2.10) Bq/kg. Average internal and external risk factors were (0.15±0.00007, and 0.19±0.00027), As for the average value of the index of representative levels (Iᵧ) was (0.44±0.018) The average absorbed dose level in (nGy/h) (28.19±1.18). The results of this study were within the internationally permissible limits, according to the report of the United Nations Scientific Committee on the Effects of Atomic Radiation.

Safety assessment of introducing radioactive waste incineration facilities in Korea: An off-site resident dose evaluation

As nuclear power technology advances, radioactive waste accumulation rises, necessitating measures to alleviate strain on disposal facilities and minimize waste management costs. Analysis of radioactive waste composition revealed that combustible waste comprised the largest proportion (45 %), with incineration demonstrating high reduction efficiency for this fraction. In order for a radioactive waste incineration facility to be introduced, it is necessary to evaluate the safety of gas radioactive effluent generated during city operation. Evaluation criteria have already been established and methodologies also exist, but these results greatly depend on the area where the incineration facilities are located, the waste to be treated, the operation method of the facilities. Accordingly, this study assumed annual throughput and radionuclide concentrations based on the radioactive waste stored and generated in Korea. The centralized operation method at a specific site was compared with the decentralized operation method employed at all sites. Post-incineration, the impact of radionuclides released from the facilities was analyzed against Nuclear Safety and Security Commission standards, confirming the discharge standards and doses for single facilities and entire sites.

Statistical Computational Model of Fission Products Composition of Irradiated Nuclear Fuel and Their Contribution to Gas-aerosol Emissions of Nuclear Power Plants

Based on the assumption that the radionuclide composition of gas-aerosol emissions from nuclear power plants (NPPs) into the environment is determined by the composition of the fuel in the reactor (but not identical to it), an analysis of the probability of the occurrence of various isotopes in possible emissions is conducted in this paper. It is confirmed that the activity of nuclear fuel, and consequently the emissions, are determined by uranium fission fragments, proving that the decay rate of radionuclides is proportional to the probability of the appearance of radionuclides with certain mass numbers. It is also shown that there is no functional relationship between the mass yield of radionuclides and their atomic mass, as the variability (fluctuations) in the content of radionuclides in VVER-440 reactor fuel and consequently in NPP emissions reaches 20 orders of magnitude, which prevents the application of computational methods for processing the results. This paper proves that, in order to determine the yield of radionuclides from their observable activity, applying a Zipf-Mandelbrot type distribution in “rank - size” coordinates, it is possible to carry out the mathematical modeling based on the appropriate processing of the obtained results.

Blending phosphogypsum to mitigate radionuclide leaching for sustainable road base applications

Production of phosphoric acid generates a calcium sulfate byproduct known as phosphogypsum (PG). PG is not considered a suitable standalone road base material because of concerns such as strength and presence of radionuclides. This paper investigates the latter, specifically the influence of blending PG with common alkaline road base aggregates – limerock (LR) and recycled concrete aggregate (RCA) – on radionuclide leaching. Radionuclide leaching from several PG sources was assessed for gross alpha, gross beta, uranium, and combined radium (226 + 228). Solution pH affected Ra226 mobility, with minimum concentrations exhibited at a pH in the range of 6 to 8. Mobile Ra226 concentrations in RCA blends decreased compared to original PG; Ra226 mobility initially increased at low LR replacements but decreased with increasing mass of LR (50 %–75 %). The data suggest an additional mechanism beyond pH alone impacted Ra226 mobility from the blends, possibly the binding or substitution of radium by elevated concentrations of Ba, Sr, or Ca. Blending with RCA resulted in radionuclide concentrations below respective drinking water thresholds, mitigating leaching concern from PG-RCA road base blends. PG-LR blends can meet regulatory limits when incorporating appropriate PG sources, providing an avenue for PG-amended road base materials. The blending approach reduced Ra226 mobility from PG-amended base, accommodating more PG use, serving as an alternative scenario to end-of-life stacking.

Исследование экологической безопасности автоклавного золопенобетона, полученного с использованием золы от сжигания осадка сточных вод

The article presents the research of ecological safety of autoclaved ash-foam concrete using ash from sewage sludge incineration in the constructed and operated production building. It is shown that after more than eighteen years of operation, the building made of autoclaved ash-foam concrete obtained using ash from sewage sludge incineration plant turned out to be environmentally safe for humans. Purpose: ash from sewage sludge incineration has high average specific radioactivity (radium and thorium), which strongly limits its further use. Earlier it was found that the use of ash from sewage sludge incineration as a raw material in autoclaved ash-foam concrete in different proportions affects the content of natural radionuclides in the finished product. The paper considers the environmental safety of autoclaved ash-foam concrete after prolonged operation. Methods: the research was carried out at the operating facility using a verified dosimeter-radiometer ATOMEX MKC-AT6130. Results: it was found that in all samples of autoclaved ash-foam concrete produced with ash from sewage sludge incineration the generated radiation background was below the norm, on the border of threshold values. Practical significance: the results of the work are important for construction, as they expand the ideas about the peculiarities of autoclaved ash-foam concrete and the possibility of safe use of ash from sewage sludge incineration in construction.

Radiological characterization of materials used in the Italian heritage buildings

Building materials (BMs) can cause significant gamma dose indoors due to their natural radionuclide content. In 2013, the European Directive 59/2013/EURATOM introduced, in annex XIII, a list of types of BMs of interest for the content of gamma-emitting radionuclides among which materials or additives of natural igneous origin, such as granitoids, tuff and lava, are included. These materials have been largely employed for decorative and structural purposes in the course of centuries in the Italian heritage buildings. Aim of this study is to assess the contribute of BMs in terms of alpha exposure. Six samples of different materials, characterized in a previous study by the authors in terms of radiological content by means of a gamma spectrometry, have been analyzed in order to determine the specific exhalation rate of 222Rn, the radon emanation coefficient and excess in indoor radon concentration. Results confirm that BMs of natural igneous origin can play an important role in terms of alpha radiation dose and internal exposure due to the inhalation of the alpha particles emitted.

Assessment of Radioactivity Levels in Bottled Drinking Water Consumed by Different Age Groups of People in Kampala City, Uganda

The activity concentrations of natural radionuclides in drinking water may be enhanced depending on the geological strata from which it is extracted. The demand and consumption of bottled drinking water is increasing every year in Uganda mainly in Kampala city. Therefore, the study was purposed to assess the levels of natural radioactivity using a gamma spectrometer in commonly bottled drinking water in Kampala City. The mean specific activities for Ra-226, Th-232, and K-40 in bottled drinking water were 4.45±0.20, 1.32±0.27, and 46.33±0.24 Bq/l respectively which exceeded the specific World Health Organization recommended guidance level of 1.0 Bq/l except for K-40. The mean activity concentrations were however comparable to the mean concentration of tap water used in Kampala City, that is 4.00±0.16, 1.4±0.19, and 47.05±0.21 Bq/l for Ra-226, Th-232, and K-40 respectively. The annual effective dose contributed by two radionuclides of Ra-226 and Th-232 in the bottled water exceeded the maximum dose limit of 0.1 mSv/y recommended by the World Health Organization (WHO). The mean estimated excess lifetime cancer risk due to Ra-226 (0.00177) exceeded the recommended limit of 0.001 while that due to Th-232 (0.0001) was below the recommended limit. Therefore, the main contributor to the total annual ingestion dose was Ra-226. Due to the high solubility and toxicity of Ra-226, there is a significant concern warranting further investigation. Finally, the results from the study revealed that there was not any trace of contamination from artificial radionuclides in the bottled drinking water manufactured and consumed within Kampala City. With the growing populational demand for bottled drinking water, it's recommended that radioactivity levels comply with the WHO recommended radioactivity levels. Therefore, this study contributes to the revision of standards and development of regulations for radiological protection of the public and the environment from risks of radiation exposure associated with bottled drinking water.

Radioactivity Levels, Spatial Distribution, and Radiological Risk Assessment of 226Ra, 228Ra, 40K, and 3H in Water Samples from Dhaka City and Savar, Bangladesh.

This investigation was conducted to measure the radioactivity levels of 226Ra, 228Ra, 40K, and 3H in the 13 most popular branded bottled mineral water (BMW), 12 groundwater sources consumed in Dhaka city, Bangladesh, and six water samples collected from the nuclear object site at Savar, adjacent to Dhaka. The activity of 3H was measured by using a liquid scintillation counter, and a gamma-ray spectrometer with an HPGe detector was used to measure the activity of other radionuclides. The average activity concentrations of 226Ra, 228Ra, 40K, and 3H in BMW samples and groundwater were found to be 1.81 ± 0.43, 1.74 ± 0.40, 43.08 ± 6.23, 2.42 ± 0.16, and 1.61 ± 0.51, 1.69 ± 0.45, 57.42 ± 3.16, and 3.02 ± 0.19 Bq/L, respectively. In addition, the activity concentrations of identified radionuclides in water samples collected from Savar were found to be 1.59 ± 0.43, 1.53 ± 0.50, 99.83 ± 3.05, and 2.95 ± 0.20 Bq/L. With the exception of 3H, the activity concentration and the annual effective dose of 40K, 226Ra, and 228Ra surpassed the acceptable thresholds of the WHO. The combined activity of radium (Rac) also exceeds the USEPA recommended maximum permissible limit of 0.185 Bq/L. The excess lifetime cancer risk results were below the permissible threshold of 10-3 for radiological risks. Groundwater was subjected to an AAS analysis for common metals (Na, Mg, and Ca) and heavy metals (Fe, Cr, Cu, and Pb). The results showed that the heavy metals were below the detection limit. Radionuclide contents in groundwater of Dhaka city were mapped spatially using a GIS technique. Statistical analyses such as one-way ANOVA, one sample t test, and Pearson's correlation analysis were also performed. According to Pearson's correlation analysis, 228Ra is mostly responsible for radiation risk in BMW and groundwater.

Concentrations of radionuclides and trace elements in wetlands.

Environmental risks in wetlands are considered with radionuclides and trace elements to understand pollution accumulation. In this study, we aimed to determine the levels of radiation and heavy metals in water systems and assess pollution configurations. Radionuclides (222Rn, 210Pb and 210Po) and trace elements (Ag, As, Ba, Be, Cd, Co, Cr, Cu, Fe, Li, Mo, Ni, Pb, V and Zn) were measured to evaluate anthropogenic factors. Water pollution in wetlands was indicated by mean concentrations of 66.2mBq/L for 222Rn, 3mBq/L for 210Pb, 42mBq/L for 210Po, 41ppb for Zn, 37ppb for Ba, 190ppb for Fe and 481ppb for Sr. These pollutants may be related to industrial facilities in Kırklareli city, Türkiye.

Background activity of naturally occurring and reference values of fallout radionuclides in soils of mountainous areas (Armenia)

ABSTRACT Complex mountainous relief and diverse geology that are common for the whole territory of Armenia are strong limiting factors for regional scale geochemical survey, for assessment of the geochemical background of naturally occurring radionuclides (226Ra, 232Th, 40K) and reference values of artificial 137Cs. Sampling transects spanned by altitude in mountain ridges and massifs, representing the main geological formations of the area, are informative enough for a pilot assessment of background and reference activity of radionuclides in soils. A total of 131 undisturbed soil samples were collected from 8 mountain ranges and massifs throughout Armenia. HPGe detector-based gamma spectrometry was used for the quantification of radionuclide activity concentrations. Geology and soil type were the main factors in the formation of radionuclide composition in the soil. The reasonably close estimates of naturally occurring radionuclide background activity were obtained from the application of ‘Median ± 2MAD’ and Tukey’s boxplot methods. The results yielded by both methods could be employed as a background, contingent upon the specific objectives being addressed. The distribution of 137Cs exhibits strong dependence on the altitude and therefore, its reference activity concentrations were estimated at distinct elevation intervals applying the ‘Median ± 2MAD’ method.

Radioecological characteristics of Siberian roe deer (Capreolus pygargus Pal., 1771) inhabiting locations of nuclear weapon tests.

This paper reports the activity concentrations of 137Cs, 90Sr, 239+240Pu, 241Am, and 3Н in the form of tritiated water (НТО) and organically bound tritium (ОBТ) in the tissues and organs of roe deer (Capreolus pygargus Pal., 1771) that inhabit the 'Degelen' test location of the Semipalatinsk Test Site. Tissues and organs were sampled from six deer by killing. The activity concentrations of specific radionuclides in the samples were measured using γ-, α-, and β-spectrometry. The radionuclide activity concentrations in the tissues and organs showed considerable variation, for example, 0.6-170 Bq kg-1 for 137Cs and 0.3-2.8×103 Bq kg-1 for 90Sr. The activity concentrations of radionuclides in animal muscular tissue did not exceed permissible values for the meat of wild animals. The tissues and organs in the roe deer were arranged as follows in descending order of their ability to accumulate 137Cs and 90Sr: for 137Cs, muscular tissue-kidneys-lungs-spleen-heart-liver-bone tissue; for 90Sr, bone tissue-liver-lungs-muscular tissue-spleen-heart-kidneys. The activity concentrations of 241Am and 239+240Pu did not exceed the minimum detectable activity. Therefore, no quantitative values could be determined for 241Am, and the 239+240Pu activity concentration could be derived for only one sample: 0.5±0.1 Bq kg-1 (liver). The distribution pattern of these radionuclides in the tissues and organs of the roe deer could not be determined because of insufficient data. The HTO volumetric activity in the tissues and organs of the examined animals ranged from 2.6×10-2 to 77 kBq l-1; activity concentration of OBT, 3.0×10-2 to 16 kBq kg-1; and OBT-to-HTO ratios, 2.0×10-3 to 5.3×102. This ratio can serve as an indicator of how long the examined animals stay in radioactively contaminated ecosystems. Within the 'Degelen' site, the activity concentrations of 90Sr and tritium, in the form of HTO and OBT, are expected to be high in the bone tissues, soft tissues, and organs, respectively.

Transfer factors of naturally occurring radionuclides from soil-to-rice cultivated in Bangladesh and associated health implications

This study investigates the uptake of naturally occurring radionuclides (226Ra, 232Th, and 40K) from soil by rice plants in extensively cultivated regions in Bangladesh. It also evaluates the potential radiation risks associated with rice consumption by the Bangladeshi populace. High purity germanium (HPGe) gamma-ray spectrometry was employed to measure the concentrations of radionuclides in both soil and rice samples. For 40K, our results agree with the International Atomic Energy Agency's (IAEA) published value; however, the transfer factors (TF) for the other two radionuclides differ considerably. Despite the fact that the IAEA based its publication of TFs for 226Ra and 232Th on clay soil, the majority of the soil profile in the present study was silty clay with a little alkalinity. Moreover, the data obtained may have been impacted by the growing seasons, cultivation methods, and soil fertility. Additionally, the annual effective dose due to the ingestion of radioactivity resulting from rice consumption was evaluated and the results agree with UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation), 2000. With a few exceptions, the excess lifetime cancer risk (ELCR) values for 226Ra, 232Th, and 40K were below the globally average permissible level (1 × 10−3). In light of this, the current study indicates that consuming rice does not pose an immediate health risk to the general public. By studying TFs among various rice varieties and geographical areas, scientists can develop models to forecast the possible radiation exposure from rice consumption and pinpoint activities or areas that require additional attention.