This article addresses the synchronization issue for inertial neural networks (INNs) with heterogeneous time-varying delays and unbounded distributed delays, in which the state quantization is considered. First, by fully considering the delay and sampling time point information, a modified looped-functional is proposed for the synchronization error system. Compared with the existing Lyapunov-Krasovskii functional (LKF), the proposed functional contains the sawtooth structure term V8(t) and the time-varying terms ex(t-βħ (t)) and ey(t-βħ (t)) . Then, the obtained constraints may be further relaxed. Based on the functional and integral inequality, less conservative synchronization criteria are derived as the basis of controller design. In addition, the required quantized sampled-data controller is proposed by solving a set of linear matrix inequalities. Finally, two numerical examples are given to show the effectiveness and superiority of the proposed scheme in this article.