Coherent Pulses Research Articles

Novel method for the generation of stable radiation from free-electron lasers at high repetition rates

For more than a decade free-electron lasers (FELs) have been in operation, providing scientists from many disciplines with the benefits of ultrashort, nearly transversely coherent radiation pulses with wavelengths down to the \AA{}ngstrom range. If no further techniques are applied, the FEL will only amplify radiation from the stochastic distributed electron density in the electron bunch. Contemporary developments aim at producing stable and single-mode radiation by preparing an electron bunch with favorable longitudinal electron density distributions using magnets and conventional laser pulses (seed), hence the name ``seeding.'' In recent years, short wavelength FELs at high electron beam energies and high repetition rates were proposed and built. At those repetition rates, an external seed with sufficient power to manipulate the electron beam cannot be provided by present state-of-the-art laser systems, thus no external seeding scheme could be applied yet. In this paper, we present ways to seed FELs to generate short wavelength radiation at high repetition rates, making use of tested electron beam manipulation schemes. For our parameter study, we used the parameters of FLASH, the free-electron laser in Hamburg. First simulations are presented, showing the feasibility of the method proposed.

Enhanced Self-Seeding with Ultrashort Electron Beams.

We describe a new method to produce intensity stable, highly coherent, narrow-band x-ray pulses in self-seeded free electron (FEL) lasers. The approach uses an ultrashort electron beam to generate a single spike FEL pulse with a wide coherent bandwidth. The self-seeding monochromator then notches out a narrow spectral region of this pulse to be amplified by a long portion of electron beam to full saturation. In contrast to typical self-seeding where monochromatization of noisy self-amplified spontaneous emission pulses leads to either large intensity fluctuations or multiple frequencies, we show that this method produces a stable, coherent FEL output pulse with statistical properties similar to a fully coherent optical laser.

Dynamics of Many-Body Photon Bound States in Chiral Waveguide QED

We theoretically study the few- and many-body dynamics of photons in chiral waveguides. In particular, we examine pulse propagation through a system of $N$ two-level systems chirally coupled to a waveguide. We show that the system supports correlated multi-photon bound states, which have a well-defined photon number $n$ and propagate through the system with a group delay scaling as $1/n^2$. This has the interesting consequence that, during propagation, an incident coherent state pulse breaks up into different bound state components that can become spatially separated at the output in a sufficiently long system. For sufficiently many photons and sufficiently short systems, we show that linear combinations of $n$-body bound states recover the well-known phenomenon of mean-field solitons in self-induced transparency. For longer systems, however, the solitons break apart through quantum correlated dynamics. Our work thus covers the entire spectrum from few-photon quantum propagation, to genuine quantum many-body (atom and photon) phenomena, and ultimately the quantum-to-classical transition. Finally, we demonstrate that the bound states can undergo elastic scattering with additional photons. Together, our results demonstrate that photon bound states are truly distinct physical objects emerging from the most elementary light-matter interaction between photons and two-level emitters. Our work opens the door to studying quantum many-body physics and soliton physics with photons in chiral waveguide QED.

Fault-tolerant quantum error correction code preparation in UBQC

The universal blind quantum computation (UBQC) is a scheme to allow a client to delegate a computation to a remote server while concealing the input, output and algorithm. However, the qubit errors are inevitable in the practical application. In this paper, a fault-tolerant quantum error correction code preparation protocol with weak coherent pulses is proposed for fault-tolerant UBQC. Furthermore, the $$\epsilon $$ -correctness and $$\epsilon $$ -blindness of the protocol are fully proven. The simulation results show that the required number of pulses in our protocol is much less than that of the remote blind qubit state preparation protocol with two decoy states in case of the same probability of successful preparation, and is closer to asymptotic case.

Development and prospect on driving laser for attosecond pulse

<p indent="0mm">Attosecond light source is a new type of light source that was born at the beginning of the 21st century, which has a short pulse, broad spectrum, high temporal and spatial coherence and wide tunability, thus being widely employed in various research fieds. From ultrafast motion of electrons in atoms to charge transfer in biological macromolecules, attosecond pulses is currently the only tool that can track and capture these ultrafast dynamics. Attosecond pulse enables us to investigate ultrafast dynamics of micro-world both in nanometer and attosecond scales. However, the mechanism of attosecond pulse generation is completely different from general ultrafast lasers. Instead, attosecond pulse is generated by a highly nonlinear interaction between strong ultrafast femtosecond laser and matter, which is called high-order harmonic generation (HHG). The mechanism of HHG can be understood by a classical three step model. First, an electron is ionized from an atom by a strong laser electric field through tunnel ionization. Then the free electron is accelerated by the laser field and gains energy. Finally, the electron recombines with the parent ion when the laser field changes its sign with emission of a photon, whose energy equals its kinetic energy gained in the laser field plus ionization potential of the atom. Apparently, HHG is strongly affected by the laser waveform. Several key parameters of driving laser, such as wavelength, intensity, and carrier envelope phase strongly affect the process of HHG. Thus, the characteristics of attosecond pulses are determined by the driving laser. The rapid development of attosecond pulse technology strongly depends on the development of driving laser technology. In the beginning, chirped pulse amplification (CPA) technology greatly promoted the development of attosecond light sources. The femtosecond CPA systems based on Ti:sapphire crystal has been the main driving laser to generate attosecond light pulses. The driving laser wavelength is in the near infrared region near <sc>800 nm,</sc> which generally has a pulse duration of multiple optical cycles. By employing post-compression technology to shorten pulse durations of CPA systems to few-cycle, isolated attosecond pulses in the extreme ultraviolet (XUV) can be generated, which is called the first generation of attosecond light source. Recently, optical parametric amplification (OPA) systems have been widely used as driving laser due to its flexible wavelength tunability. Using OPA, longer driving laser wavelength up to the midinfrared (MIR) can be obtained, which pushes the attosecond pulses to the soft X-ray region, and has been called the second generation of attosecond light sources. Due to broad spectrum and higher photon energy, attosecond pulses have a shorter duration in the soft X-ray region compared with XUV region, given that the temporal chirp is properly compensated. In 2017, reseachers generated soft X-ray isolated attosecond pulses, which was driven by mid-infrared pulses centered at <sc>1.8 µm.</sc> These attosecond pulses, whose duration reaches 53 as and spectrum surpasses carbon K-edge, provide a tool for studying the ultrafast dynamics of diamond, graphene and other carbon materials. In this paper, we start with the principle of attosecond pulses generation based on HHG. Then, we introduce different technologies and their development for obtaining driving laser pulses for HHG. Finally, we introduce prospect on development of driving laser pulses for attosecond pulses generation.

Supercontinuum generation in all-normal dispersion suspended core fiber infiltrated with water

Octave spanning all-normal dispersion supercontinuum generation (SCG) was experimentally demonstrated in a solid, suspended-core fiber (SCF) infiltrated with water. Replacement of air with water in the cladding air-holes leads to a dramatic modification of the dispersion profile of the fiber, significantly flattening the characteristic over the visible and much of the near-infrared wavelength range at normal values. In such a fiber infiltrated with water, all-normal dispersion supercontinuum was generated with the spectral coverage from 435 nm to 1330 nm using femtosecond pumping with the output peak power of 150 kW and 800 nm central wavelength. The SCF without water infiltration – air in the cladding region – had a zero-dispersion wavelength at 760 nm and enabled the generation of the anomalous dispersion dynamics-based SCG in the wavelength range from 450 nm to 1250 nm. We also numerically calculated the coherence of simulated supercontinuum pulses with one-photon-per-mode noise seeds and point out that the all-normal dispersion SCG in suspended-core fiber infiltrated with water has the potential for high temporal coherence, while the fiber without water infiltration shows gradual decoherence of generated supercontinuum pulses with increasing pump power, over similar peak power range.

Supercontinuum generation in all-normal dispersion suspended core fiber infiltrated with water

Octave spanning all-normal dispersion supercontinuum generation (SCG) was experimentally demonstrated in a solid, suspended-core fiber (SCF) infiltrated with water. Replacement of air with water in the cladding air-holes leads to a dramatic modification of the dispersion profile of the fiber, significantly flattening the characteristic over the visible and much of the near-infrared wavelength range at normal values. In such a fiber infiltrated with water, all-normal dispersion supercontinuum was generated with the spectral coverage from 435 nm to 1330 nm using femtosecond pumping with the output peak power of 150 kW and 800 nm central wavelength. The SCF without water infiltration – air in the cladding region – had a zero-dispersion wavelength at 760 nm and enabled the generation of the anomalous dispersion dynamics-based SCG in the wavelength range from 450 nm to 1250 nm. We also numerically calculated the coherence of simulated supercontinuum pulses with one-photon-per-mode noise seeds and point out that the all-normal dispersion SCG in suspended-core fiber infiltrated with water has the potential for high temporal coherence, while the fiber without water infiltration shows gradual decoherence of generated supercontinuum pulses with increasing pump power, over similar peak power range.

Two-dimensional spectroscopy of Rydberg gases

Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates, various types of static and dynamic disorder and on relaxation processes. However, two-dimensional spectra can be difficult to interpret without precise knowledge of how the signal components relate to microscopic Hamiltonian parameters and system-bath interactions. Here we show that two-dimensional spectroscopy can be mapped in the microwave domain to highly controllable Rydberg quantum simulators. By porting 2D spectroscopy to Rydberg atoms, we firstly open the possibility of its experimental quantum simulation, in a case where parameters and interactions are very well known. Secondly, the technique may provide additional handles for experimental access to coherences between system states and the ability to discriminate different types of decoherence mechanisms in Rydberg gases. We investigate the requirements for a specific implementation utilizing multiple phase coherent microwave pulses and a phase cycling technique to isolate signal components.

Single-shot transverse coherence measurements with Young's double pinholes at FLASH2

We measured the transverse coherence at FLASH2, a variable gap undulator line at the FLASH free-electron laser user facility at DESY in Hamburg. We demonstrate, theoretically and experimentally, a revised version of Young’s double pinhole approach to perform single-shot, repeatable and non-invasive transverse coherence measurements. At beamline FL24 of FLASH2, the transverse coherence of pulses was systematically characterized at wavelengths of 8, 13.5 and 18 nm for different FEL source settings. We determine degrees of coherence of 57% to 87% in the vertical and horizontal direction, respectively. These measurements can facilitate the planning of novel, coherence-based experiments at the FLASH facility.

Simulation of Excitation by Sunlight in Mixed Quantum-Classical Dynamics.

This paper proposes a method to simulate nonadiabatic dynamics initiated by thermal light, including solar radiation, in the frame of mixed quantum-classical (MQC) methods, like surface hopping. The method is based on the Chenu–Brumer approach, which treats the thermal radiation as an ensemble of coherent pulses. It is composed of three steps: (1) sampling initial conditions from a broad blackbody spectrum, (2) dynamics propagation using conventional methods, and (3) ensemble averaging considering the field and realization time of the pulses. The application of MQC dynamics with pulse ensembles (MQC-PE) to a model system of nucleic acid photophysics showed the emergence of a steady excited-state population. In another test case, modeling retinal photophysics, MQC-PE predicted that although the photoisomerization occurs within 200 fs, it may take tens of microseconds of continuous solar irradiation to photoactivate a single retinal. Such emergent long timescales may impact our understanding of biological and technological phenomena occurring under solar radiation.

Generation of intense and coherent sub-femtosecond X-ray pulses in electron storage rings

Temporally short X-ray pulses are an indispensable tool for the study of electron transitions close to the Fermi energy and structural changes in molecules undergoing chemical reactions which take place on a time-scale of hundreds of femtoseconds. The time resolution of experiments at 3rd generation light sources which produce intense synchrotron radiation is limited fundamentally by the electron-bunch length in the range of tens of picoseconds. Here we propose a new scheme for the generation of intense and coherent sub-femtoseconds soft X-ray pulses in storage rings by applying the Echo-Enabled Harmonic Generation (EEHG) method. Many issues for obtaining the EEHG structure such as two modulators and a radiator are solved by a paradigm shift in an achromatic storage ring cell. Numerical demonstration of the feasibility of the scheme for the BESSY II beam parameters is presented.

Ultrafast Creation of Overlapping Rydberg Electrons in an Atomic BEC and Mott-Insulator Lattice.

We study an array of ultracold atoms in an optical lattice (Mott insulator) excited with a coherent ultrashort laser pulse to a state where single-electron wave functions spatially overlap. Beyond a threshold principal quantum number where Rydberg orbitals of neighboring lattice sites overlap with each other, the atoms efficiently undergo spontaneous Penning ionization resulting in a drastic change of ion-counting statistics, sharp increase of avalanche ionization, and the formation of an ultracold plasma. These observations signal the actual creation of electronic states with overlapping wave functions, which is further confirmed by a significant difference in ionization dynamics between a Bose-Einstein condensate and a Mott insulator. This system is a promising platform for simulating electronic many-body phenomena dominated by Coulomb interactions in the condensed phase.

Optical generation and detection of gigahertz shear acoustic waves in solids assisted by a metallic diffraction grating

Absorption of ultrashort laser pulses in a metallic grating deposited on a transparent sample launches in the material both compression/dilatation (longitudinal) and shear coherent acoustic pulses in directions of different orders of acoustic diffraction. The propagation of the emitted acoustic pulses can be monitored by measuring the variation of the optical reflectivity of the time-delayed ultrashort probe laser pulses. The direction of probe light incidence and its polarization relative to the sample surface as well as the orientation of the metallic grating should be specifically chosen for efficient Brillouin scattering of the probe light from shear phonons propagating in the elastically isotropic materials. As theoretically predicted, the obtained experimental data contain multiple frequency components which are due to a variety of possible Brillouin scattering angles for both shear and compression/dilatation coherent acoustic waves. All these different frequency components are explained through multiplexing the propagation directions of probe light and coherent sound by the metallic diffraction grating. Our experimental scheme of time-domain Brillouin scattering with metallic gratings operating in reflection mode provides access to monitoring the shear acoustic waves launched in the direction of the first diffraction order by backward Brillouin scattering process. Applications include simultaneous determination of several different acoustic mode velocities and optical refractive index and, potentially, measurements of the acoustic dispersion of samples with a single direction of possible optical access.

Ghost spintronic THz-emitter-array microscope

Terahertz (THz) waves show great potential in nondestructive testing, biodetection and cancer imaging. Despite recent progress in THz wave near-field probes/apertures enabling raster scanning of an object’s surface, an efficient, nonscanning, noninvasive, deep subdiffraction imaging technique remains challenging. Here, we demonstrate THz near-field microscopy using a reconfigurable spintronic THz emitter array (STEA) based on the computational ghost imaging principle. By illuminating an object with the reconfigurable STEA followed by computing the correlation, we can reconstruct an image of the object with deep subdiffraction resolution. By applying an external magnetic field, in-line polarization rotation of the THz wave is realized, making the fused image contrast polarization-free. Time-of-flight (TOF) measurements of coherent THz pulses further enable objects at different distances or depths to be resolved. The demonstrated ghost spintronic THz-emitter-array microscope (GHOSTEAM) is a radically novel imaging tool for THz near-field imaging, opening paradigm-shifting opportunities for nonintrusive label-free bioimaging in a broadband frequency range from 0.1 to 30 THz (namely, 3.3–1000 cm−1).

Coherent propagation and amplification of intense laser pulses in hexagonal multicore fibers.

Propagation and amplification of intense coherent laser pulses in a multicore fiber of 24 weakly coupled cores arranged in the form of seven close-packed hexagons were studied. Exact stable analytical solutions are found for the out-of-phase mode, which describes the coherent propagation of wave beams and temporal soliton solutions in such fibers. Their stability is demonstrated. The analytical results are confirmed by the direct numerical simulation of the wave equation.

THE INFLUENCE OF STATISTICAL CHARACTERISTICS OF THE FLUCTUATIONS OF THE RADIATION SIGNAL INITIAL PHASES ON THE ACCURACY OF THE MEASUREMENT AERODYNAMIC OBJECT RADIAL VELOCITY

The article deals with the estimation of radial velocity when using a coherent packet of radio pulses regarding the case of the presence of correlated fluctuations of the initial phases in the reflected from the aerodynamic object pulses. The subject of the research is the accuracy of measuring the frequency of the received packet for the case of concerted processing without taking into account the phase fluctuations of its radio pulses. The purpose is a numerical analysis of the influence of the statistical characteristics of the fluctuations of the received pack’s initial phases on the decrease in the accuracy of measuring the radial velocity of the aerodynamic object. The task : to estimate the possible values of fluctuation constituent middling quadratic error of measuring of radial speed of aerodynamic object. Consideration is given to the assumption that an additive mixture of deflected signal and uncorrelated Gaussian noise is input to the radar receiver. It is considered that the phase fluctuations of the received packet are distributed according to the normal law with zero mean, and the correlation of phase fluctuations with the increase of the interval between the packet radio pulses decreases according to the alternating law. Methods used: methods of probability theory and mathematical statistics. The following results are obtained: the accuracy of frequency measurement of the pack had been estimated in the presence of correlated phase fluctuations of its radio pulses. Conclusions . The results indicate that for modern radars in the conditions of regular measurement the accuracy of estimating the frequency of the packet of radio pulses is much more influenced by the statistical characteristics of the phase fluctuation than the signal-to-noise ratio. Due to the phase fluctuations of the radio pulses of the received packet, the mean-square error (MSE) of radial velocity measurement of the aerodynamic object is able to exceed the values determined by the requirements for coherent pulse radar.

Generation of High-Frequency Radiation in the Conditions of Superradiance of Particles with a Constant Dipole Moment

A localized ensemble of identical particles with a constant dipole moment generates during superradiance a coherent pulse of low-frequency radiation, the pulse shape depending significantly on the number of particles in the ensemble. In particular, low-frequency radiation pulse is transformed from one-hump to two-hump shape in a narrow range of variation of ensemble parameters.

Robust entanglement distribution via telecom fibre assisted by an asynchronous counter-propagating laser light

Distributing entangled photon pairs over noisy channels is an important task for various quantum information protocols. Encoding an entangled state in a decoherence-free subspace (DFS) formed by multiple photons is a promising way to circumvent the phase fluctuations and polarisation rotations in optical fibres. Recently, it has been shown that the use of a counter-propagating coherent light as an ancillary photon enables us to faithfully distribute entangled photon with success probability proportional to the transmittance of the optical fibres. Several proof-of-principle experiments have been demonstrated, in which entangled photon pairs from a sender side and the ancillary photon from a receiver side originate from the same laser source. In addition, bulk optics have been used to mimic the noises in optical fibres. Here, we demonstrate a DFS-based entanglement distribution over 1 km optical fibre using DFS formed by using fully independent light sources at the telecom band, and obtain a high-fidelity entangled state. This shows that the DFS-based scheme protects the entanglement against collective noise in 1 km optical fibre. In the experiment, we utilise an interference between asynchronous photons from continuous wave pumped spontaneous parametric down conversion (SPDC) and mode-locked coherent light pulse. After performing spectral and temporal filtering, the SPDC photons and light pulse are spectrally indistinguishable. This property allows us to observe high-visibility interference without performing active synchronisation between fully independent sources.

Enhanced spectral broadening in an optical parametric oscillator based on a PPLN crystal.

We report a chirped-pulse optical parametric oscillator (OPO) generating light pulses with an instantaneous-bandwidth much wider than the parametric gain-bandwidth of nonlinear crystals. Our numerical simulations show that a relatively high residual second-order-dispersion within the OPO cavity is required in order to achieve the maximum signal-bandwidth from an OPO system. Based on this principle, we constructed an OPO using a 3-mm-long PPLN crystal, which produced a signal wave with an instantaneous-bandwidth of 20 THz (at -20 dB) covering 1447-1600 nm, roughly twice as much as the phase-matching bandwidth of the nonlinear crystal. This scheme represents a promising technical route for generating high-repetition-rate, ultrashort optical pulses with a wide bandwidth at various wavelengths, which may benefit many applications, including optical coherence tomography, pulse synthesis and spectroscopy.

Surface processing of PMMA and metal nano-particle resist by sub-micrometer focusing of coherent extreme ultraviolet high-order harmonics pulses.

We demonstrate sub-micrometer processing of two kinds of thin films, polymethyl methacrylate (PMMA) and metal nano-particle resist, by focusing high-order harmonics of near-IR femtosecond laser pulses in the extreme ultraviolet (XUV) wavelength region (27.2-34.3 nm) on the thin film samples using an ellipsoidal focusing mirror. The ablation threshold fluences for the PMMA sample and the metal nano-particle resist per XUV pulse obtained by the accumulation of 200 XUV pulses were determined to be 0.42mJ/cm2 and 0.17mJ/cm2, respectively. The diameters (FWHM) of a hole created by the ablation on the PMMA film at the focus were 0.67 µm and 0.44 µm along the horizontal direction and the vertical direction, respectively. The fluence dependence of the Raman microscope spectra of the processed holes on the PMMA sample showed that the chemical modification, in which C=C double bonds are formed associated with the scission of the PMMA polymer chains, is achieved by the irradiation of the XUV pulses.