Coherence Effects Research Articles

Spectrum‐Selective High‐Temperature Tolerant Thermal Emitter by Dual‐Coherence Enhanced Absorption for Solar Thermophotovoltaics

AbstractSolar thermophotovoltaics (STPV) receive considerable attention for the record high energy transfer efficiency beyond conventional photovoltaics systems, which requires a well‐designed structured absorber/emitter and high operating temperature. However, the inherent tradeoff between increased operation temperature and material/structure stability (especially for the thermal emitters) severely hinders the development of STPV. In this work, a new design is proposed for a step‐function‐like thermal emitter based on a two‐path (quasi) coherent perfect absorption effect, which is experimentally enabled by a few‐layer Si/Mo/AlN lamellar film on a Mo substrate through a sequential physical vapor deposition process. The as‐prepared lamellar emitter exhibits maximal emissivity of ≈97% for 1.4 µm with excellent thermal suppression down to 10% across 3.4–10 µm, the performance of which is well maintained up to 973 K. When employed in the established STPV system, the dual coherent enhanced absorption (DCEA) system contributes to an increase of 20% in the total system efficiency compared to the unimodal coherent perfect absorption counterpart. The design proposed in this study provides a new methodology for improving the efficiency of the STPV system and may have significant applications in improving thermal energy regulation for compact systems.

Significance of Energy Conservation in Coupled-Trajectory Approaches to Nonadiabatic Dynamics.

Through approximating electron-nuclear correlation terms in the exact factorization approach, trajectory-based methods have been derived and successfully applied to the dynamics of a variety of light-induced molecular processes, capturing quantum (de)coherence effects rigorously. These terms account for the coupling among the trajectories, recovering the nonlocal nature of quantum nuclear dynamics that is completely overlooked in traditional independent-trajectory algorithms. Nevertheless, some of the approximations introduced in the derivation of some of these methods do not conserve the total energy. We analyze energy conservation in the coupled-trajectory mixed quantum-classical (CTMQC) algorithm and explore the performance of a modified algorithm, CTMQC-E, where some of the terms are redefined to restore energy conservation. A set of molecular models is used as a test, namely, 2-cis-penta-2,4-dienimium cation, bis(methylene) adamantyl radical cation, butatriene cation, uracil radical cation, and neutral pyrazine.

Integrated Backward Second-Harmonic Generation through Optically Induced Quasi-Phase-Matching.

Quasi-phase-matching for efficient backward second-harmonic generation requires sub-μm poling periods, a nontrivial fabrication feat. For the first time, we report integrated first-order quasiphase-matched backward second-harmonic generation enabled by seeded all-optical poling. The self-organized grating inscription circumvents all fabrication challenges. We compare backward and forward processes and explain how grating period influences the conversion efficiency. These results showcase unique properties of the coherent photogalvanic effect and how it can bring new nonlinear functionalities to integrated photonics.

Skeletal muscle extracellular matrix structure under applied deformation observed using second harmonic generation microscopy

The mechanical and structural properties of passive skeletal muscle are important for musculoskeletal models in impact biomechanics, rehabilitation engineering and surgical simulation. Passive properties of skeletal muscle depend strongly on the architecture of the extracellular matrix (ECM), but the structure of ECM and its realignment under applied deformation remain poorly understood. We apply second harmonic generation (SHG) microscopy to study muscle ECM in intact muscle samples both under deformation and in the undeformed state. A method for regional relocation was developed, so that the same ECM segment could be viewed before and after applying deformations. Skeletal muscle ECM was viewed at multiple scales and in three states: undeformed, under compression and under tension. Results show that second harmonic generation microscopy provides substantial detail of skeletal muscle ECM over a wide range of length scales, especially the perimysium structure. We present images of individual portions of skeletal muscle ECM both undeformed and subjected to tensile/compressive deformation. We also present data showing the response of the perimysium to a partial thickness cut applied to a section under tensile deformation. Statement of significanceSecond Harmonic Generation (SHG) microscopy is an imaging technique which takes advantage of a non-linear and coherent frequency doubling optical effect that is present in a small number of biological molecules, primarily collagen Type I, II and myosin. Collagen I is the most abundant collagen type in skeletal muscle, making SHG a promising option for visualisation of the skeletal muscle extracellular matrix (ECM). SHG microscopy does not require fixing or staining. This short communication presents the application of SHG microscopy to skeletal muscle ECM to improve our understanding of how collagen fibres reorganise under applied tensile and compression, including microscopic observations of collagen fibre reorganisation for intact samples by using a method to re-identify specific regions in repeated deformation tests.

Evolution of quantum resources in quantum-walk-based search algorithm

Quantum walk is fundamental to designing many quantum algorithms. Here we consider the effects of quantum coherence and quantum entanglement for the quantum walk search on the complete bipartite graph. First, we numerically show the complementary relationship between the success probability and the two quantum resources (quantum coherence and quantum entanglement). We also provide theoretical analysis in the asymptotic scenarios. At last, we discuss the role played by generalized depolarizing noises and find that it would influence the dynamics of success probability and quantum coherence sharply, which is demonstrated by theoretical derivation and numerical simulation.

Broadband quasi-perfect sound absorption by a metasurface with coupled resonators at both low- and high-amplitude excitations

This study presents an acoustic metasurface (AM) consisting of coupled Helmholtz resonators with extended necks (HRENs) to effectively absorb broadband sound waves at both low and high amplitudes. A nonlinear acoustic model is proposed to characterize the AM performance based on the equivalent medium theory and the transfer matrix method. The nonlinear effects due to the high-amplitude excitation are considered by a velocity-dependence equivalent density of the air in the neck. The acoustic characteristics of an AM with two coupled HREN units at the sound pressure level (SPL) ranging from 100dB to 140dB are analytically, numerically, and experimentally investigated. Results from the three approaches show good agreement. The AM achieves quasi-perfect absorption (absorption coefficient α>0.9) in a wide range of SPL, while each HREN unit alone only performs well at around 130dB. The superior absorption performance of the AM at relatively low-amplitude excitation originates from the coherent coupling effects between adjacent units. With the increase of the sound level, the coupling effects tend to deteriorate; fortunately, the sound-vortex conversions occur, contributing to additional acoustic dissipation and thereby sustaining the quasi-perfect absorption capability. Based on the absorption mechanisms, a broadband AM with multiple coupled resonators is designed and manufactured. The measured averaged absorption coefficient of the AM is larger than 0.91 at the SPL below 140 dB (α>0.97 at 100dB) within [700,1100]Hz, and the compact thickness is of 1/18 wavelength at the lowest operating frequency. The findings in this study offer a promising approach to achieve highly efficient broadband sound absorption in a wide-ranging noise level, which holds great potentials in practical applications for noise control.

Experimental signature of initial quantum coherence on entropy production

We report on the experimental quantification of the contribution to non-equilibrium entropy production stemming from the quantum coherence content in the initial state of a qubit exposed to both coherent driving and dissipation. Our experimental demonstration builds on the exquisite experimental control of the spin state of a nitrogen-vacancy defect in diamond and is underpinned, theoretically, by the formulation of a generalized fluctuation theorem designed to track the effects of quantum coherence. Our results provide significant evidence of the possibility to pinpoint the genuinely quantum mechanical contributions to the thermodynamics of non-equilibrium quantum processes in an open quantum systems scenario.

Operating mode dependent energy transfer efficiency in a quantum well waveguide

In this paper, we delve into the intricate interplay between optical fields with varying relative phases in a closed-loop configuration semiconductor quantum well waveguide with four distinct energy levels, and how it impacts the Fraunhofer diffraction patterns obtained via four-wave mixing. By harnessing a strong control field, a standing wave driving field, and two weak probe and signal fields, we drive the waveguide to generate these patterns with maximum efficiency. To achieve this, we consider three distinct light-matter interaction scenarios, where the system is first set up in either a lower electromagnetically induced transparency or a coherent population trapping state, followed by a final state that enables electron spin coherence (ESC) induction. Our results reveal that the efficiency of Fraunhofer diffraction in the quantum well waveguide can be enhanced significantly under specific parameter regimes via the spin coherence effect. Further investigation of the light-matter interaction in the ESC zone, where only one of the control fields is a standing wave field, demonstrates that spin coherence facilitates more efficient transfer of energy from the probe light to the third and fourth orders, highlighting its crucial role in shaping the diffraction patterns.

Coherence effects on the interference colors of soap films

Acquiring the thickness field of a soap film from interference colors requires an accurate relationship between color and film thickness. Throughout the literature, an interference relation derived using monochromatic waves is widely used to calculate the colors of soap films illuminated by light sources with significant frequency bandwidths by applying the relation at a number of discrete wavelengths in the source, which assumes that the interfering waves are perfectly coherent. However, since the coherence between waves is expected to decrease with increasing film thickness, it is poorly understood when interference relations derived using monochromatic waves can be applied. In this study, an interference relation incorporating the coherence between interfering waves is derived. The effects of coherence on the interference colors of soap films are then studied by comparing the colors computed using each of these two interference relations for light sources with different frequency bandwidths. As the frequency bandwidth of the light source increases, the difference in the colors computed using each interference relation increases, which implies that the accuracy of the method involving the monochromatic relation decreases with increasing frequency bandwidth of the source. The findings of this study will allow for more accurate measurements of the thickness of soap films from their interference colors.

Experimental quantum imaging distillation with undetected light.

Imaging based on the induced coherence effect makes use of photon pairs to obtain information of an object without detecting the light that probes it. While one photon illuminates the object, only its partner is detected, so no measurement of coincidence events is needed. The sought-after object's information is revealed, observing a certain interference pattern on the detected photon. Here, we demonstrate experimentally that this imaging technique can be made resilient to noise. We introduce an imaging distillation approach based on the interferometric modulation of the signal of interest. We show that our scheme can generate a high-quality image of an object even against noise levels up to 250 times the actual signal of interest. We also include a detailed theoretical explanation of our findings.

Effect of noise-induced quantum coherence in the intermediate band solar cells

It has been shown that quantum coherence induced by incoherent light can increase the efficiency of solar cells. Here we evaluate the effect of such coherence in the intermediate band solar cells (IBSC). We first examine a six-level quantum IBSC model and demonstrate by simulation that the maximum output power in a solar cell with a quantum structure increases more than 16 percent in the case of coherence existence. We then propose an IBSC model which can absorb continuous spectra of sunlight and show that the quantum coherence can increase the output power of the cell. For instance, calculations indicate that the coherence makes an increase of about 31% in the maximum output power of a cell that the width of the conduction and intermediate bands are 100 and 10 meV, respectively. Also, our calculations show that the quantum coherence effect is still observed in increasing the solar cell power by expanding the width of the conduction band, although the output power is reduced due to an increase in thermalization loss. However, expanding the width of the intermediate band reduces the coherence effect.

Multiple electron spin resonance echoes observed for paramagnetic defects in diamond at room temperature

Magnetic resonance offers an invaluable testbed for observing and studying the fundamental concepts of quantum cavity interactions with two-level systems in the microwave regime. Typically, these experiments are conducted at low cryogenic temperatures, utilizing spin systems embedded within a high-quality (Q-factor) superconducting cavity. Recent studies indicate that under these conditions, especially in a high-cooperativity regime with strong collective coupling between an electron spin system and a microwave cavity, multiple spin echoes can be detected. These echoes are interpreted as manifestations of coherent quantum effects. To put it simply, photons within the cavity can excite the spin system, which subsequently can stimulate the cavity, creating a feedback loop. In our research, we demonstrate that a specially designed moderate-Q cavity, paired with diamond crystals rich in nitrogen vacancy (NV) centers, allows us to observe such nonlinear quantum phenomena, even at ambient temperatures. Crucially, our experimental design necessitates amplifying the net number of spins for a specific, limited spin concentration. This is achieved by lowering the spins' thermodynamic temperature (as opposed to their physical temperature) to a few kelvins. Notably, we find that maintaining high cooperativity or strong coupling is not essential for these observations. The potential to observe significant microwave cavity quantum effects at room temperature could be useful for future applications, such as quantum memories and quantum sensing.

Broadband low-frequency sound-absorbing metastructure based on an impedance-matching coiled-up cavity with continuously variable cross section

Proposed here is a metastructure based on a micro-perforated panel and an impedance-matching coiled-up cavity with continuously variable cross section, which achieves perfect absorption with a resonant frequency of 496 Hz and an absolute bandwidth (α ≥ 0.5) of 468 Hz. The structure thickness is ca. 1/13 of the operating wavelength λ in the deep subwavelength range. A relative bandwidth of 84.04%–111.67% is achieved through parametric studies. Physically, the continuous variation of the cavity cross section through which sound waves enter weakens the acoustic reflections generated by cross-sectional abruptness and enhances the impedance matching with the air. Furthermore, particle swarm optimization is coupled with a theoretical model to tailor the metastructure to realize the maximum absorption coefficient in the defined frequency range. It is shown theoretically that coherent coupling “weak resonance”—in which each unit individually exhibits imperfect absorption peaks—significantly improves the absorption performance in a broad frequency band through the coherent coupling effect. Finally, a hybrid metastructure using a parallel coupling sample is fabricated, and its acoustic properties are measured in an impedance tube. The average absorption coefficient of this metastructure is 0.934 in the quasi-perfect band (α > 0.9) from 400 to 650 Hz, and the thickness is only ca. λ/15. The unique innovation of a cavity with continuously variable cross section provides new ideas for designing broadband low-frequency sound-absorbing metastructures.

A sensory-motor decoder that transforms neural responses in extrastriate area MT into smooth pursuit eye movements.

Visual motion drives smooth pursuit eye movements through a sensory-motor decoder that uses multiple parallel neural pathways to transform the population response in extrastriate area MT into movement. We evaluated the decoder by challenging pursuit in monkeys with reduced motion reliability created by reducing coherence of motion in patches of dots. Our strategy was to determine how reduced dot coherence changes the population response in MT. We then predicted the properties of a decoder that transforms the MT population response into dot coherence-induced deficits in the initiation of pursuit and steady-state tracking. During pursuit initiation, decreased dot coherence reduces MT population response amplitude without changing the preferred speed at its peak. The successful decoder reproduces the measured eye movements by multiplication of 1) the estimate of target speed from the peak of the population response with 2) visual-motor gain based on the amplitude of the population response. During steady-state tracking, the decoder that worked for pursuit initiation failed to reproduce the paradox that steady-state eye speeds do not accelerate to the target speed despite persistent image motion. It predicted eye acceleration to target speed even when monkeys' eye speeds were steady at well below the target speed. To account for the effect of dot coherence on steady-state eye speed, we postulate that the decoder uses sensory-motor gain to modulate the eye velocity positive feedback that normally sustains perfect steady-state tracking. Then, poor steady-state tracking persists because of balance between eye deceleration caused by low positive feedback gain and acceleration driven by MT.NEW & NOTEWORTHY By challenging a sensory-motor system with degraded sensory stimuli, we reveal how the sensory-motor decoder transforms the population response in extrastriate area MT into commands for the initiation and steady-state behavior of smooth pursuit eye movements. Conclusions are based on measuring population responses in MT for multiple target speeds and different levels of motion reliability and evaluating a decoder with a biologically motivated architecture to determine the decoder properties that create the measured eye movements.

Multivariate prediction of cognitive performance from the sleep electroencephalogram

Human cognitive performance is a key function whose biological foundations have been partially revealed by genetic and brain imaging studies. The sleep electroencephalogram (EEG) is tightly linked to structural and functional features of the central nervous system and serves as another promising biomarker. We used data from MrOS, a large cohort of older men and cross-validated regularized regression to link sleep EEG features to cognitive performance in cross-sectional analyses. In independent validation samples 2.5–10% of variance in cognitive performance can be accounted for by sleep EEG features, depending on the covariates used. Demographic characteristics account for more covariance between sleep EEG and cognition than health variables, and consequently reduce this association by a greater degree, but even with the strictest covariate sets a statistically significant association is present. Sigma power in NREM and beta power in REM sleep were associated with better cognitive performance, while theta power in REM sleep was associated with worse performance, with no substantial effect of coherence and other sleep EEG metrics. Our findings show that cognitive performance is associated with the sleep EEG (r = 0.283), with the strongest effect ascribed to spindle-frequency activity. This association becomes weaker after adjusting for demographic (r = 0.186) and health variables (r = 0.155), but its resilience to covariate inclusion suggest that it also partially reflects trait-like differences in cognitive ability.

Addressing the hydrogen entrapment in Al2024 alloys using scanning transmission electron microscopy and density functional theory

The effect of precipitate coherency in an aged aluminum (Al) 2024 alloy is investigated using scanning transmission electron microscopy (STEM) and density functional theory (DFT) methods. The focus of the study is on understanding the effects of hydrogen (H2) entrapment in the alloy, which leads to the degradation of its corrosion resistance. We employed STEM to analyze the structure and strain properties of the alloy at high spatial resolution. This has been achieved by applying the geometrical phase analysis (GPA) to the acquired HRSTEM images. The determination of strain field around the precipitates was utilized to gauge the degree of coherency at the interface of the precipitates with Al matrix. We also applied density functional theory (DFT) simulations to investigate the interfacial energy at the interfaces of the precipitates with the Al matrix. The obtained results of the DFT simulations showed that the interfacial energy at the semi-coherent precipitates was determined to be 0.06 eV per atom, which was higher compared to the coherent precipitates. Our findings suggest that the semi-coherent precipitates have a less stable interface with the Al matrix. Furthermore, the study revealed that the H2 entrapped at the semi-coherent precipitate regions exhibits a binding energy which is 3.2 eV lower than that of the coherent precipitates. This implies that hydrogen binds more strongly at the semi-coherent precipitate cites, which enhances the process of the alloy embrittlement.

Childhood maltreatment predicts maternal sensitivity to distress: Negative attributions during the transition to parenthood.

Childhood maltreatment is a predictor of subsequent parenting behaviors; however, the mechanisms explaining this association have been understudied. The present study examined the indirect effect of childhood maltreatment on maternal sensitivity to distress via (a) emotion regulation difficulties, (b) negative attributions about infant crying, (c) minimizing attributions about infant crying, and (d) situational attributions about infant crying. The sample included 259 primiparous mothers (131 Black and 128 White) and their 6-month-old infants (52% female). Mothers retrospectively reported on their childhood history of maltreatment when their infants were about 2 years old. Emotion regulation difficulties and causal attributions about infant crying were assessed prenatally. Maternal sensitivity to distress was rated during three distress-eliciting tasks when children were 6 months old. Results from the structural equation model demonstrated that maternal childhood maltreatment was significantly positively associated with negative attributions about infant crying but not with emotion regulation difficulties, minimizing attributions, or situational attributions about crying. Furthermore, negative attributions about crying were associated with lower sensitivity to distress, and there was an indirect effect of childhood maltreatment on sensitivity to distress via negative attributions about infant distress. These effects were significant above and beyond the effects of coherence of mind, concurrent depressive symptoms, infant affect, maternal age, race, education, marital status, and income-to-needs ratio. The results suggest that altering negative attributions about infant crying may be an important area to intervene during the prenatal period to reduce continuity in maladaptive parenting across generations. (PsycInfo Database Record (c) 2023 APA, all rights reserved).

Multi-species thermalization cascade of energetic particles in the early universe

Heavy long-lived particles are abundant in BSM physics and will, under generic circumstances, get to dominate the energy density of the universe. The resulting matter dominated era has to end through the decay of the heavy matter component particles of mass M, and before the universe cools down to a temperature of a few MeV, in order not to upset the successful predictions of Big Bang Nucleosynthesis. The process of thermalization of their decay products, of initial energy ∼ M/2, into a thermal bath of temperature T primarily involves near-collinear splittings of energetic particles into two particles with lower energy. The correct treatment of these processes requires the inclusion of coherence effects which suppress the splitting rate. We write down and numerically solve the resulting coupled Boltzmann equations including all gauge bosons and fermions of the unbroken phase of the Standard Model (SM). We then comment on the dependence of the nonthermal spectra on the ratio M/T, as well as on the matter decay rate and branching ratios into various SM particles.

The amplification effect of river valley topography on the seismic response of a tunnel near a valley: simulated using the boundary element method

Many tunnels are inevitably built in or near valley terrains, which greatly amplifies the seismic response of the tunnel. This paper considers the interaction between the valley terrain and tunnels, proposes a high-precision indirect boundary element method (IBEM) for simulation, and verifies the correctness of the method. The impact of factors such as incident-wave type, incident-wave frequency, and distance between the tunnel and the valley on the seismic response of the tunnel is then analysed in detail. The numerical analysis demonstrates that the stress of the tunnel can be approximately doubled when the distance between the river valley and the tunnel is 10 m due to the scattering and coherence effects of seismic waves. However, when this distance is greater than 50 m, the presence of river valleys has little effect on the stress of the tunnel. The stress at the right shoulder of the tunnel and the displacement amplification effect on the valley slope is significant compared to other areas. The findings of this study provide theoretical guidance for the seismic fortification and disaster avoidance of tunnel structures near river valleys.

Broadband ptychography using curved wavefront illumination.

We examine the interplay between spectral bandwidth and illumination curvature in ptychography. By tailoring the divergence of the illumination, broader spectral bandwidths can be tolerated without requiring algorithmic modifications to the forward model. In particular, a strong wavefront curvature transitions a far-field diffraction geometry to an effectively near-field one, which is less affected by temporal coherence effects. The relaxed temporal coherence requirements allow for leveraging wider spectral bandwidths and larger illumination spots. Our findings open up new avenues towards utilizing pink and broadband beams for increased flux and throughput at both synchrotron facilities and lab-scale beamlines.