Cloud Liquid Water Research Articles

Resolution dependence of southern Atlantic Ocean stratocumulus decks

AbstractOceanic stratocumulus decks of clouds are among the largest contributors to the Earth's radiation budget, covering around a fifth of the planet's surface and reflecting a large part of the incoming solar radiation. Unfortunately, these clouds are not well represented in modern climate models, resulting in one of the leading causes of uncertainty in climate change projections. This contribution analyses this issue from a novel perspective and sheds light on the mechanisms behind the misrepresentation and resolution dependence of these large clouds. The analysis is based on realistic week‐long simulations performed over a km oceanic domain. Four horizontal resolutions, between 4.4 and 0.55 km, are employed, resulting in a timely investigation, especially in light of the high resolutions employed by present and near‐future climate projections. Results show that the liquid cloud water, the main contributor to the simulated grid‐scale clouds, decreases with a power‐law decay as the resolution increases, whereas the water vapour, responsible for subgrid‐scale clouds, is much less affected by the grid spacing. The leading cause is identified as an imbalance between the rates of change of the advection and turbulence parametrisation terms. In order to verify this observation and provide a possible mitigation to the issue, a second set of simulations is performed where the turbulence parametrisation is tuned. The strategy proves to be successful, confirming the hypotheses and resulting not only in a resolution‐independent radiation budget but also cloud coverage.

Analysis of the Meteorological Conditions and Atmospheric Numerical Simulation of an Aircraft Icing Accident

With the rapid development of the general aviation industry in China, the influence of high-impact aeronautical weather events, such as aircraft icing, on flight safety has become more and more prominent. On 1 March 2021, an aircraft conducting weather modification operations crashed over Ji’an City, due to severe icing. Using multi-source meteorological observations and atmospheric numerical simulations, we analyzed the meteorological causes of this icing accident. The results indicate that a cold front formed in northwestern China and then moved southward, which is the main weather system in the icing area. Based on the icing index, we conducted an analysis of the temperature, relative humidity, cloud liquid water path, effective particle radius, and vertical flow field, it was found that aircraft icing occurred behind the ground front, where warm-moist airflows rose along the front to result in a rapid increase of water vapor in 600–500 hPa. The increase of water vapor, in conjunction with low temperature, led to the formation of a cold stratiform cloud system. In this cloud system, there were a large number of large cloud droplets. In addition, the frontal inversion increased the atmospheric stability, allowing cloud droplets to accumulate in the low-temperature region and forming meteorological conditions conducive to icing. The Weather Research and Forecasting model was employed to provide a detailed description of the formation process of the atmospheric conditions conducive to icing, such as the uplifting motion along the front and supercooled water. Based on a real case, we investigated the formation process of icing-inducing meteorological conditions under the influence of a front in detail in this study and verified the capability of a numerical model to simulate the meteorological environment of frontal icing, in order to provide a valuable reference for meteorological early warnings and forecasts for general aviation.

Supercooled Water Cloud Detection From Polarized Multi‐Angle Imager Data Using 1.37 μm Water Vapor Polarized Channel

AbstractDetecting supercooled water clouds (SWCs) is essential for enhancing artificial rainfall, preventing aircraft ice accretion, and developing a better understanding of radiative energy balance. The 1.37 μm channel, known as strong water vapor absorbing, was made polarized in the polarized multi‐angle imager (PMAI) onboard FengYun‐3G satellite. The infight data shown that the new 1.37 μm polarized channel could be used to detect SWCs. The cloudbow is observed around the 140° scattering angle in the 1.37 μm polarization image, with a maximum polarization reflectance of approximately 0.04–0.06. The indicated water clouds with spherical particles in the high‐level altitude could be SWCs. Then, the SWCs detected by 1.37 μm polarized channel is verified using polarized reflectance of other channels, the reflectance difference of channels, and thermal infrared bright temperature. The presence of cloudbow in 1.03 and 1.64 μm channels indicate liquid water cloud. The reflectance difference between 1.03 and 1.64 μm of SWCs agree with characteristic of water cloud. The thermal infrared channels from the imager on the same platform indicate cold cloud with the brightness temperature far below 273.16 K. Therefore, the only use of 1.37 μm polarized channel could perform the identification of SWCs. PMAI provides a powerful tool for monitoring supercooled water clouds.

Multi‐Layer Cloud Detection and Distributions Over the Asia–Pacific Region Based on Geostationary Satellite Imagers

AbstractA large portion of cloud scenes over the globe shows multiple layers composed of different phases, in general with ice clouds on the top and liquid water clouds beneath. Such multi‐layer (ML) clouds constitute major challenges in cloud observations and weather and climate modeling. This study improved a threshold algorithm for detecting ice‐over‐water ML clouds using geostationary satellites. Optimal thresholds were established for the spectral characteristics of the Advanced Himawari Imager (AHI) and the Advanced Geostationary Radiation Imager (AGRI), accounting for differences between land and ocean surfaces. Validation with collocated space radar and lidar measurements indicated the identification accuracies of approximately 82% over the land and 76% over the ocean. Annual distributions of ML clouds inferred by AHI and AGRI exhibited strong similarity. Furthermore, 6 years of hourly observations revealed distinct monthly and daily variations in ice‐over‐water clouds over the Asia–Pacific region. The ML cloud monthly variations were similar to those of the seasonal convection cycle, with occurrence frequencies over the typical regions higher in summer (maximum ∼27%) and lower (minimum 6%–10%) in winter. Regarding daily variations, ice‐over‐water clouds occurred more frequently around local noon over most of the six time zones (from UTC + 06 to UTC + 11) throughout all seasons. The refined spatiotemporal distribution of ML clouds, particularly the daily variations, is possible to improve our understanding of cloud vertical distributions and radiative effects, and has the potential to promote subsequent validation and parameterization of cloud overlapping in global climate modeling.

The Ensemble Tangent Linear Model Applied to a Cloud Physics Parameterization

Abstract An Ensemble Tangent Linear Model (ETLM) is applied to a cloud physics scheme used in the Navy Global Environmental Model (NAVGEM). The ensemble is created using 3-hour forecasts from the Ensemble Transform method used in the NAVGEM data assimilation system. The model states are saved before and after applying the cloud physics parameterization (which includes condensation/evaporation of cloud ice and cloud liquid water and stratiform precipitation), and these states are used to construct linearized model tendencies for temperature, specific humidity, cloud liquid water, and cloud ice water. We examine separately the application of the ETLM to cloud physics components that are explicitly local versus non-local. For the local components, an ETLM is built using a single grid point. ETLMs from 50 to 1000 members are tested, and skillful forecasts can be obtained for both local and non-local physics even with a moderate sized ensemble (e.g., 100 members). At 1000 members, the globally-averaged forecast error reductions (relative to persistence errors) are ∼40% for temperature, water vapor, and cloud liquid water and ∼30% for cloud ice. When initial perturbations are reduced by a factor of 0.1, the error reductions increase to ∼65% for all variables. For physics with non-local components (stratiform precipitation) the covariances that comprise the ETLM are localized with a Schur product matrix using a Gaussian localization shape with tunable length. The optimal lengths increased with ensemble size from ∼2-3 km for 50 members to ∼10 km for 1000 members. ETLMs for “all cloud physics” are also constructed and evaluated.

Cloud water adjustments to aerosol perturbations are buffered by solar heating in non-precipitating marine stratocumuli

Abstract. Marine low-level clouds are key to the Earth's energy budget due to their expansive coverage over global oceans and their high reflectance of incoming solar radiation. Their responses to anthropogenic aerosol perturbations remain the largest source of uncertainty in estimating the anthropogenic radiative forcing of climate. A major challenge is the quantification of the cloud water response to aerosol perturbations. In particular, the presence of feedbacks through microphysical, dynamical, and thermodynamical pathways at various spatial and temporal scales could augment or weaken the response. Central to this problem is the temporal evolution in cloud adjustment, governed by entangled feedback mechanisms. We apply an innovative conditional Monte Carlo subsampling approach to a large ensemble of diurnal large-eddy simulation of non-precipitating marine stratocumulus to study the role of solar heating in governing the evolution in the relationship between droplet number and cloud water. We find a persistent negative trend in this relationship at night, confirming that the role of microphysically enhanced cloud-top entrainment. After sunrise, the evolution in this relationship appears buffered and converges to ∼-0.2 in the late afternoon. This buffering effect is attributed to a strong dependence of cloud-layer shortwave absorption on cloud liquid water path. These diurnal cycle characteristics further demonstrate a tight connection between cloud brightening potential and the relationship between cloud water and droplet number at sunrise, which has implications for the impact of the timing of advertent aerosol perturbations.

Evaluation of the Surface Downward Longwave Radiation Estimation Models over Land Surface

Surface downward longwave radiation (SDLR) is crucial for maintaining the global radiative budget balance. Due to their ease of practicality, SDLR parameterization models are widely used, making their objective evaluation essential. In this study, against comprehensive ground measurements collected from more than 300 globally distributed sites, four SDLR parameterization models, including three popular existing ones and a newly proposed model, were evaluated under clear- and cloudy-sky conditions at hourly (daytime and nighttime) and daily scales, respectively. The validation results indicated that the new model, namely the Peng model, originally proposed for SDLR estimation at the sea surface and applied for the first time to the land surface, outperformed all three existing models in nearly all cases, especially under cloudy-sky conditions. Moreover, the Peng model demonstrated robustness across various land cover types, elevation zones, and seasons. All four SDLR models outperformed the Global Land Surface Satellite product from Advanced Very High-Resolution Radiometer Data (GLASS-AVHRR), ERA5, and CERES_SYN1de-g_Ed4A products. The Peng model achieved the highest accuracy, with validated RMSE values of 13.552 and 14.055 W/m2 and biases of −0.25 and −0.025 W/m2 under clear- and cloudy-sky conditions at daily scale, respectively. Its superior performance can be attributed to the inclusion of two cloud parameters, total column cloud liquid water and ice water, besides the cloud fraction. However, the optimal combination of these three parameters may vary depending on specific cases. In addition, all SDLR models require improvements for wetlands, bare soil, ice-covered surfaces, and high-elevation regions. Overall, the Peng model demonstrates significant potential for widespread use in SDLR estimation for both land and sea surfaces.

Novel method for inversion of microphysical properties of clouds using Raman lidar data

Aerosol–cloud–precipitation interactions are important in the balance of Earth’s radiation budget. To further explore the relationship between clouds and precipitation, and to improve operational weather modification, it is necessary to study the microphysical parameters of liquid water clouds. Here, an inversion method that uses a back propagation (BP) neural network based on a genetic algorithm (GA), namely a GABP, is proposed to invert cloud microphysical parameters using ground-based dual-field-of-view (FOV) Raman lidar data. To verify the feasibility of the method, long-term continuous observations were conducted in the Liupan Mountains (China). Results revealed that the proposed inversion method using the GABP is feasible for retrieving the liquid water content (LWC) and the cloud droplet effective radius after training a large number of data measured simultaneously by the Raman lidar and a microwave radiometer. When inverting LWC, the root mean square error (RMSE) of the GABP algorithm was found in the range 0–0.005, whereas the RMSE of the BP algorithm fluctuated in the range 0–0.01. It was evident that the GABP algorithm yields better inversion results and finer detail. When maintaining other variables and comparing the inversion results of signals in the inner and outer FOVs, the RMSE of the inner FOV signal was within 0.005 at near-ground heights (i.e., <2 km), whereas the outer FOV signal exceeded 0.005 at certain heights. This study developed a feasible solution for detecting characteristic cloud microphysical parameters using a Raman lidar, which could be used to study aerosol–cloud–precipitation interactions, and thereby have considerable practical importance for improving artificial rainfall operations.

In situ observations of supercooled liquid water clouds over Dome C, Antarctica, by balloon-borne sondes

Abstract. Clouds in Antarctica are key elements that affect radiative forcing and thus Antarctic climate evolution. Although the vast majority of clouds are composed of ice crystals, a non-negligible fraction constitutes supercooled liquid water (SLW; water held in liquid form below 0 °C). Numerical weather prediction models have great difficulty in forecasting SLW clouds over Antarctica, favouring ice at the expense of liquid water and therefore incorrectly estimating the cloud radiative forcing. Remote-sensing observations of SLW clouds have been carried out for several years at Concordia Station (75° S, 123° E; 3233 m above mean sea level), combining active lidar measurements (SLW cloud detection) and passive HAMSTRAD microwave measurements (liquid water path, LWP). The present project aimed at in situ observations of SLW clouds using sondes developed by the company Anasphere, specifically designed for SLW content (SLWC) measurements. These SLWC sondes were coupled to standard meteorological pressure–temperature–humidity sondes from Vaisala and released under meteorological balloons. During the 2021–2022 summer campaign, 15 launches were made, of which 7 were scientifically exploitable above a height of 400 m above ground level, a threshold height imposed by the time the SLWC sonde takes to stabilize after launch. The three main outcomes from our analyses are as follows: (a) the first in situ observations so far of SLW clouds in Antarctica with SLWC sondes; (b) on average, the consistency of SLW cloud heights as observed by in situ sondes and remote-sensing lidar; and (c) the liquid water path (vertically integrated SLWC) deduced by the sondes being generally equal to or greater than the LWP remotely sensed by HAMSTRAD. In general, the SLW clouds were observed in a layer close to saturation (U &gt; 80 %) or saturated (U ∼ 100 %–105 %) just below or at the lowermost part of the entrainment zone, or capping inversion zone, which exists at the top of the planetary boundary layer and is characterized by an inflection point in the potential temperature vertical profile. Our results are consistent with the theoretical view that SLW clouds form and remain at the top of the planetary boundary layer.

Effect of microphysics scheme and data assimilation on hydrometeor and radiative flux simulations in the Arctic.

Although clouds are a major factor influencing atmospheric environments in the Arctic, numerical simulations of Arctic clouds are uncertain. In this study, the effects of microphysics scheme and data assimilation (DA) on the simulation of clouds, hydrometeors and radiative fluxes in the Arctic were investigated using the polar weather research and forecasting (WRF) model and three-dimensional variational DA. Compared with the WRF 5-class (WSM5) microphysics scheme, when the Morrison double-moment (Morrison) scheme was used, the simulated amount of cloud ice water decreased by approximately 68%. In contrast, the amount of water vapour, cloud liquid water, snow and rain in the atmosphere increased. With DA, the amount of water vapour increased, leading to increased hydrometeors. The cloud liquid water increased in the middle and low atmospheres when Morrison was used, whereas it increased in the low atmosphere when DA was used. The increase in cloud liquid water by using Morrison resulted in a decrease in the downward short-wave radiative flux at the surface, whereas using DA increased the downward long-wave radiative flux. Changing the microphysics scheme induced redistribution of the region and amounts of hydrometeors, whereas DA induced an increase in hydrometeors in specific regions by adding observation information to the model states.

Quantifying Changes in the Arctic Shortwave Cloud Radiative Effects

AbstractThe shortwave cloud radiative effect (SWCRE) is important for the Arctic surface radiation budget and is a major source of inter‐model spread in simulating Arctic climate. To better understand the individual contributions of various radiative processes to changes in SWCRE, we extend the existing Approximate Partial Radiative Perturbation (APRP) method by adding the absorptivity for the upward beam, considering differences in reflectivity between upward and downward beams, and analyzing the cloud masking effect resulting from changes in surface albedo. Using data from CMIP model experiments, the study decomposes the SWCRE over the Arctic surface and analyzes inter‐model differences in quadrupled CO2 simulations. The study accounts for the influence of surface albedo, cloud amount, and cloud microphysics in the response of SWCRE to Arctic warming. In the sunlit season, CMIP models exhibit a strong, negative SWCRE with a large inter‐model spread. Arctic clouds dampen the surface albedo feedback by reflecting incoming solar radiation and further decrease the shortwave radiation reflected by surface, a fraction of which is scattered back to the surface by clouds. Specifically, this accounts for the majority of the inter‐model spread in SWCRE. In addition, increased (decreased) cloud amount and cloud liquid water reduce (increase) incoming shortwave fluxes at the surface, but they are found to be not critical to the Arctic surface radiation budget and its inter‐model variation. Overall, the extended APRP method offers a useful tool for analyzing the complex interactions between clouds and radiative processes, accurately decomposes the individual SWCRE responses at the Arctic surface.

Significance of anthropogenic black carbon in modulating atmospheric and cloud properties through aerosol-radiation interaction during a winter-time fog-haze

The present study investigated the aerosol-radiation-cloud interaction of anthropogenic black carbon (BC) during a severe fog-haze event by utilizing WRF-Chem, multi-satellite and in-situ observations, reanalyses datasets, and HYSPLIT model. The WRF-Chem model adequately captured the regional distribution of aerosol, cloud, and meteorological variables over the study domain. The maximum BC surface concentration (≥7 μg m−3) was predominantly evident over densely populated central and lower Indo-Gangetic Plain (IGP) regions. Although smoke aerosols usually persisted within 4 km above the surface at daylight hours, they reached as high as 6 km during nighttime, specifically over the central IGP regions. The heavily influenced areas by BC aerosols expanded to almost the entire landmass and the continental outflow region upon doubling the anthropogenic emission. The geographical distribution of maximum perturbations in net shortwave radiation flux at the surface closely matched the spatial patterns of the highest BC concentration, indicating a crucial role of BC in directly preventing the incoming sunlight from reaching the surface. Consequently, the reduced solar radiation at the ground might result in substantial surface cooling (between −0.3 and −0.5 °C), eventually prohibiting surface evapotranspiration and diminishing the outgoing sensible and latent heat fluxes. Also, more amplified cooling in the polluted atmosphere can prevent further development of the planetary boundary layer (PBL), increasing particle entrapment near the surface via an ‘aerosol-radiation-PBL’ feedback loop. However, the most striking contrast between the two scenarios (typical and polluted) was the prolonged and intensified warming (0.5–0.8 °C) in the mid-troposphere, causing a remarkable drop in moisture (more than two to three times) and hence burn-off of liquid cloud droplets due to the semi-direct effect of increased BC aerosols. The intense mid-tropospheric heating could remarkably enhance the updraft velocity, supporting the vertical transport of the additional moisture to higher altitudes, forming more ice clouds at night. Therefore, the current study highlighted the urgency of mitigating anthropogenic BC emissions in highly polluted regions since increased emissions could considerably worsen severe fog-haze conditions and influence both liquid water and ice clouds, depending on the atmospheric conditions.

Precipitation and cloud Parameters's characteristics of stratus in summer in Ningxia, eastern of northwest China

Stratus is the main artificial seeding target for weather modification in Ningxia. Meteorological satellites can detect macro and microcosmic physical parameters of large-scale stratus. Researching precipitation and cloud parameter characteristics of stratus can provide scientific and technological support for understanding the development and evolution of stratus to identify seeding conditions and effects. Eight typical stratus precipitation events of the summers of 2016–2021 of Ningxia were selected, using the nine point average method, that matched characteristic cloud parameters retrieved by FY-2G satellite with precipitation classification data of 25 national meteorological observation stations in Ningxia. These stratus precipitation characteristics were correlated with cloud parameters. The results indicate that precipitation decreased rapidly from the southeast to the northwest of Ningxia. In the synoptic background of precipitation, the cloud top height, super-cooled layer thickness, cloud optical thickness, cloud particle effective radius, and cloud liquid water content were all larger than those in the synoptic background of no precipitation. The spatial distribution feature manifests as gradually increased from southeast to northwest. The cloud top temperature and cloud blackbody temperature were smaller than those in the synoptic background of no precipitation. The cloud top temperature was near the cloud “seeding temperature window”, and the depth of the super-cooled layer was thick. This was in line with the “Seeder-Feeder” structure characteristic of cold stratus.

Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation

Abstract. The Weather Research Forecasting (WRF) version 4.3 model is configured within a Lagrangian framework to quantify the impact of aerosols on evolving cloud fields. Kilometer-scale simulations utilizing meteorological boundary conditions are based on 10 case study days offering diverse meteorology during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA). Measurements from aircraft, the ground-based Atmosphere Radiation Measurement (ARM) site at Graciosa Island in the Azores, and A-Train and geostationary satellites are utilized for validation, demonstrating good agreement with the WRF-simulated cloud and aerosol properties. Higher aerosol concentration leads to suppressed drizzle and increased cloud water content in all case study days. These changes lead to larger radiative cooling rates at cloud top, enhanced vertical velocity variance, and increased vertical and horizontal wind speed near the base of the lower-tropospheric inversion. As a result, marine cloud cell area expands, narrowing the gap between shallow clouds and increasing cloud optical thickness, liquid water content, and the top-of-atmosphere outgoing shortwave flux. While similar aerosol effects are observed in lightly to non-raining clouds, they tend to be smaller by comparison. These simulations show a relationship between cloud cell area expansion and the radiative adjustments caused by liquid water path and cloud fraction changes. The adjustments are positive and scale as 74 % and 51 %, respectively, relative to the Twomey effect. While higher-resolution large-eddy simulations may provide improved representation of cloud-top mixing processes, these results emphasize the importance of addressing mesoscale cloud-state transitions in the quantification of aerosol radiative forcing that cannot be attained from traditional climate models.

On the retrieval of cloud optical thickness from spectral radiances - A sensitivity study with high albedo surfaces

Measurements of spectral zenith radiance in the 320–950 nm wavelength range have been carried out since 2021 at the Thule High Arctic Atmospheric Observatory (THAAO, https://www.thuleatmos-it.it/, 76.5° N, 68.8° W, 225 m a.s.l) located in Pituffik, northern Greenland. This study evaluates whether such observations could provide, in principle, scientifically meaningful cloud optical depth (τ) estimates, what would be the limitations, which are the necessary auxiliary measurements, and which radiance wavelengths would be better suited for the goal. Although clouds play a critical role in the Arctic, a climatology of τ in high albedo conditions is particularly difficult to obtain. THAAO might have the instrument capabilities to provide such a long-term dataset. We use a radiative transfer package to simulate visible spectra with different cloud and surface conditions, assuming homogeneous overcast sky and liquid water clouds of fixed geometrical thickness. Simulations are run to reproduce typical conditions encountered at THAAO when measurements are carried out. We find that the assumption of a broadband albedo instead of a spectrally-resolved one is the source of the largest uncertainties. Tests on size and phase of cloud particles showed that a 50% uncertainty in reff leads to a ∼10% error in τ, and that a 10% contamination of ice crystals in a low-level liquid water cloud leads to an error in τ estimates of less than 5%. All the tests showed that the most critical τ range is between the thin and thick cloud regimes (τ ∼ 7–15), where the retrievals can be less reliable. Otherwise, tests suggest that in the environmental conditions that characterize late spring and summer at THAAO, and given the observatory measurements capabilities, estimates of τ for low-level clouds could be accurately retrieved both in high and low surface albedo conditions by means of zenith radiance measurements in the UV-Vis-NIR range.

Effects of aerosols on the lifecycle of a mesoscale cloud cluster over the Indian peninsula: A numerical study with a bin-based cloud microphysics scheme

The effects of aerosols (i.e., CCN) on the lifecycle of a well-documented mesoscale cloud cluster (CC) over the Indian peninsula are investigated in this study. The WRF model coupled with a sophisticated spectral bin microphysics scheme is employed to simulate the observed cloud system under various CCN scenarios. The CCN sensitivity experiments were carried out using three different background CCN concentrations (250, 1000, and 3000 cm−3). The prevailing environment featured a relatively dry mid-level. The introduction of more aerosols weakened the convection and moistened the upper troposphere in the initiation and mature phases. The major impacts of the enhanced aerosols include the dissipation of shallow clouds, a decrease in the number of convective cells and their overall coverage, enhanced convective organization in the early phase(s) of the lifecycle, enhancement of the cloud-free area, etc. The key microphysical changes due to enhanced aerosols are the increase in cloud liquid water, presence of numerous smaller cloud droplets, enhancement of condensation and evaporation, formation of smaller ice crystals, reduced snow mass and reduction in the aggregation process, high graupel mass and number and a reduction in graupel size, fewer raindrops with slight enhancement in raindrop size, etc. Cloud growth is significantly limited in the high aerosol scenarios due to large evaporation favored by a relatively dry environment and no invigoration effect is noted. A significant reduction in the rainfall (and associated rainfall-type) from isolated convective cores is noted due to high aerosols, especially in the initiation and mature phases. The eventual impact on the surface precipitation is a decrease in overall rainfall in the enhanced aerosol scenarios, with suppression of heavy rain. The study indicates that in a dry environment, the microphysical changes in various CCN scenarios cumulatively lead to macrophysical changes, which are found to be the primary controller of the overall surface rainfall associated with the CC.

Impact of Aerosols on the Macrophysical and Microphysical Characteristics of Ice-Phase and Mixed-Phase Clouds over the Tibetan Plateau

Using CloudSat/CALIPSO satellite data and ERA5 reanalysis data from 2006 to 2010, the effects of aerosols on ice- and mixed-phase, single-layer, non-precipitating clouds over the Tibetan Plateau during nighttime in the MAM (March to May), JJA (June to August), SON (September to November), and DJF (December to February) seasons were examined. The results indicated the following: (1) The macrophysical and microphysical characteristics of ice- and mixed-phase clouds exhibit a nonlinear trend with increasing aerosol optical depth (AOD). When the logarithm of AOD (lnAOD) was ≤−4.0, with increasing AOD during MAM and JJA nights, the cloud thickness and ice particle effective radius of ice-phase clouds and mixed-phase clouds, the ice water path and ice particle number concentration of ice-phase clouds, and the liquid water path and cloud fraction of mixed-phase clouds all decreased; during SON and DJF nights, the cloud thickness of ice-phase clouds, cloud top height, liquid droplet number concentration, and liquid water path of mixed-phase clouds all decreased. When the lnAOD was &gt;−4.0, with increasing AOD during MAM and JJA nights, the cloud top height, cloud base height, cloud fraction, and ice particle number concentration of ice-phase clouds, and the ice water path of mixed-phase clouds all increased; during SON and DJF nights, the cloud fraction of mixed-phase clouds and the ice water path of ice-phase clouds all increased. (2) Under the condition of excluding meteorological factors, including the U-component of wind, V-component of wind, pressure vertical velocity, temperature, and relative humidity at the atmospheric pressure heights near the average cloud top height, within the cloud, and the average cloud base height, as well as precipitable water vapor, convective available potential energy, and surface pressure. During MAM and JJA nights. When the lnAOD was ≤−4.0, an increase in aerosols may have led to a decrease in the thickness of ice and mixed-phase cloud layers, as well as a reduction in cloud water path values. In contrast, when the lnAOD was &gt;−4.0, an increase in aerosols may contribute to elevated cloud base and cloud top heights for ice-phase clouds. During SON and DJF nights, changes in various cloud characteristics may be influenced by both aerosols and meteorological factors.

How Cloud Droplet Number Concentration Impacts Liquid Water Path and Precipitation in Marine Stratocumulus Clouds—A Satellite-Based Analysis Using Explainable Machine Learning

Aerosol–cloud–precipitation interactions (ACI) are a known major cause of uncertainties in simulations of the future climate. An improved understanding of the in-cloud processes accompanying ACI could help in advancing their implementation in global climate models. This is especially the case for marine stratocumulus clouds, which constitute the most common cloud type globally. In this work, a dataset composed of satellite observations and reanalysis data is used in explainable machine learning models to analyze the relationship between the cloud droplet number concentration (Nd), cloud liquid water path (LWP), and the fraction of precipitating clouds (PF) in five distinct marine stratocumulus regions. This framework makes use of Shapley additive explanation (SHAP) values, allowing to isolate the impact of Nd from other confounding factors, which proved to be very difficult in previous satellite-based studies. All regions display a decrease of PF and an increase in LWP with increasing Nd, despite marked inter-regional differences in the distribution of Nd. Polluted (high Nd) conditions are characterized by an increase of 12 gm−2 in LWP and a decrease of 0.13 in PF on average when compared to pristine (low Nd) conditions. The negative Nd–PF relationship is stronger in high LWP conditions, while the positive Nd–LWP relationship is amplified in precipitating clouds. These findings indicate that precipitation suppression plays an important role in MSC adjusting to aerosol-driven perturbations in Nd.

A Regionally Refined and Mass‐Consistent Atmospheric and Hydrological De‐Aliasing Product for GRACE, GRACE‐FO and Future Gravity Missions

AbstractDe‐aliasing products are used in the estimation process of satellite‐based gravity field computation to reduce errors from high‐frequency mass variations that alias into monthly gravity fields. The latest official product is AOD1B RL07 and describes non‐tidal atmosphere and oceanic mass variations at 3‐hourly resolution. However, the model‐based de‐aliasing products are inevitably incomplete and prone to temporally and spatially correlated errors that substantially contribute to errors in the estimated gravity fields. Here, we investigate possible enhancement of current de‐aliasing products by nesting a regional high‐resolution atmospheric reanalysis over Europe into a global reanalysis. As further novelty we include almost mass consistent terrestrial water storage variability from a regional hydrological model nested into a global model as additional component of the de‐aliasing product. While we find in agreement with earlier studies only minor contributions from increasing the temporal resolution beyond 3‐hourly data, our investigations suggest that contributions from continental hydrology and from regional non‐hydrostatic atmospheric modeling to sub‐monthly mass variations could be relevant already for gravity fields estimated from current gravity missions. Moreover, in the context of extreme events, we find regionally contributions from additional moisture fields, such as cloud liquid water, in the order of a few mm over Europe. We suggest this needs to be taken into account when preparing data analysis schemes for future space gravimetric missions.

Using Satellite and ARM Observations to Evaluate Cold Air Outbreak Cloud Transitions in E3SM Global Storm‐Resolving Simulations

AbstractThis study examines marine boundary layer cloud regime transition during a cold air outbreak (CAO) over the Norwegian Sea, simulated by a global storm‐resolving model (GSRM) known as the Simple Cloud‐Resolving Energy Exascale Earth System Model Atmosphere Model (SCREAM). By selecting observational references based on a combination of large‐scale conditions rather than strict time‐matched comparisons, this study finds that SCREAM qualitatively captures the CAO cloud transition, including boundary layer growth, cloud mesoscale structure, and phase partitioning. SCREAM also accurately locates the greatest ice and liquid in the mesoscale updrafts, however, underestimates supercooled liquid water in cumulus clouds. The model evaluation approach adopted by this study takes advantages of the existing computational‐expensive global simulations of GSRM and the available observations to understand model performance and can be applied to assessments of other cloud regimes in different regions. Such practice provides valuable guidance on the future effort to correct and improve biased model behaviors.