Soil curling caused by drying is a common phenomenon in nature, and it can vary depending on different atmospheric effects. To investigate the coupled effects of temperature and relative humidity on soil curling, a sequence of desiccation experiments were performed by using elongated strip soil samples in the laboratory. The soil curling process is divided into five stages: vertical settlement stage, lateral contraction stage, concave-up curling stage, curling recovery stage and convex-up curling stage. In this study, the soil evaporation characteristic and curvature curves are obtained under different temperature and relative humidity conditions. The findings revealed that a lower relative humidity results in a higher evaporation rate and a smaller maximum concave-up curling curvature for soil samples. Additionally, as the temperature increased, the water content associated with concave curling decreased. The maximum concave-up curling curvature was determined by the transition from the appearance of concave-up curling to the maximum curvature of concave-up curling. Under the coupled effect of temperature and relative humidity, all the water content associated with the occurrence of concave-up curling, maximum concave-up and convex-up curling appearance are reduced with increasing temperature and decreasing relative humidity. As the temperature ranged from 20 °C to 40 °C, the maximum concave-up curling curvature initially decreased and then increased. Conversely, the maximum concave-up curling curvature increased within the relative humidity range of 30% to 45%.