Circular Rydberg Atoms Research Articles

Towards Quantum Simulation with Circular Rydberg Atoms

The main objective of quantum simulation is an in-depth understanding of many-body physics. It is important for fundamental issues (quantum phase transitions, transport, . . . ) and for the development of innovative materials. Analytic approaches to many-body systems are limited and the huge size of their Hilbert space makes numerical simulations on classical computers intractable. A quantum simulator avoids these limitations by transcribing the system of interest into another, with the same dynamics but with interaction parameters under control and with experimental access to all relevant observables. Quantum simulation of spin systems is being explored with trapped ions, neutral atoms and superconducting devices. We propose here a new paradigm for quantum simulation of spin-1/2 arrays providing unprecedented flexibility and allowing one to explore domains beyond the reach of other platforms. It is based on laser-trapped circular Rydberg atoms. Their long intrinsic lifetimes combined with the inhibition of their microwave spontaneous emission and their low sensitivity to collisions and photoionization make trapping lifetimes in the minute range realistic with state-of-the-art techniques. Ultra-cold defect-free circular atom chains can be prepared by a variant of the evaporative cooling method. This method also leads to the individual detection of arbitrary spin observables. The proposed simulator realizes an XXZ spin-1/2 Hamiltonian with nearest-neighbor couplings ranging from a few to tens of kHz. All the model parameters can be tuned at will, making a large range of simulations accessible. The system evolution can be followed over times in the range of seconds, long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization, disorder or Floquet time crystals. This platform presents unrivaled features for quantum simulation.

Measuring the Rydberg constant using circular Rydberg atoms in an intensity-modulated optical lattice

A method for performing a precision measurement of the Rydberg constant, $R_{\infty}$, using cold circular Rydberg atoms is proposed. These states have long lifetimes, as well as negligible quantum-electrodynamics (QED) and no nuclear-overlap corrections. Due to these advantages, the measurement can help solve the "proton radius puzzle" [Bernauer, Pohl, Sci. Am. 310, 32 (2014)]. The atoms are trapped using a Rydberg-atom optical lattice, and transitions are driven using a recently-demonstrated lattice-modulation technique to perform Doppler-free spectroscopy. The circular-state transition frequency yields $R_{\infty}$. Laser wavelengths and beam geometries are selected such that the lattice-induced transition shift is minimized. The selected transitions have no first-order Zeeman and Stark corrections, leaving only manageable second-order Zeeman and Stark shifts. For Rb, the projected relative uncertainty of $R_{\infty}$ in a measurement under the presence of the Earth's gravity is $10^{-11}$, with the main contribution coming from the residual lattice shift. This could be reduced in a future micro-gravity implementation. The next-important systematic arises from the Rb$^+$ polarizability (relative-uncertainty contribution of $\approx 3 \times10^{-12}$).

Measurement of a microwave field amplitude beyond the standard quantum limit

We report a quantum measurement beyond the standard quantum limit (SQL) for the amplitude of a small displacement acting on a cavity field. This measurement uses as resource an entangled mesoscopic state, prepared by the resonant interaction of a circular Rydberg atom with a field stored in a superconducting cavity. We analyse the measurement process in terms of Fisher information and prove that it is, in principle, optimal. The achieved experimental precision, 2.4 dB below the SQL, is well understood in terms of experimental imperfections.This method could be transposed to other systems, particularly to circuit QED, for the precise measurements of weak forces acting on oscillators.

One-cavity scheme enabling to implement delayed choice for entanglement swapping in cavity QED

In this paper we present a simplified scheme to implement entanglement swapping in the context of cavity QED. The scheme presented here has the advantage of being much simpler than those presented previously, and can easily be adapted to perform the delayed choice for entanglement swapping, thus enabling one to also demonstrate time-like entanglement in the cavity QED domain. In contrast to previous schemes, our proposal uses just one high-Q cavity, besides the usual circular Rydberg atoms, Ramsey zones and selective atomic state detectors. The simplicity of our scheme makes it feasible with current QED technology, making it attractive from the experimental point of view for demonstrating entanglement swapping both in the conventional and in the delayed choice manner.

Trapped quantum light

Matter-field interaction finds its simplest implementation in Cavity Quantum Electrodynamics (CQED). A single two-level atom is coupled to a few photons stored in a single mode of a high-quality resonator. In the strong-coupling regime, the coherent atom-field interaction overwhelms dissipative processes. This situation illustrates the basic quantum postulates. It is also ideal for the exploration of the quantum-classical boundary and for the realization of quantum information protocols. We briefly describe the general frame of CQED. We illustrate its fundamental interest by discussing two recent experiments, performed with circular Rydberg atoms and superconducting millimeter-wave cavities.

Analysis of a controlled phase gate using circular Rydberg states

We propose and analyze the implementation of a two qubit quantum gate using circular Rydberg states with maximum orbital angular momentum. The intrinsic quantum gate error is limited by the finite Rydberg lifetime and finite Rydberg blockade shift. Circular states have much longer radiative lifetimes than low orbital angular momentum states and are therefore candidates for high fidelity gate operations. We analyze the dipole-dipole interaction of two circular state Rydberg atoms and present numerical simulations of quantum process tomography to find the intrinsic fidelity of a Rydberg blockade controlled phase gate. Our analysis shows that the intrinsic gate error can be less than $9 \times10^{-6}$ for circular Cs atoms in a cryogenic environment.

Production and trapping of cold circular Rydberg atoms

Cold circular Rydberg atoms are produced and magnetically trapped. The trap is characterized by direct spatial imaging of ion distributions, ion counting, and state-selective field ionization. At room temperature, we observe about 70% of the trapped atoms remaining after 6 ms. We measure a trap oscillation frequency increase of the circular Rydberg atom trap relative to the ground-state atom trap due to the larger magnetic moment of the circular Rydberg atoms. Simulations of the center-of-mass and internal-state evolution of circular states in our magnetic trap are performed and results are in good agreement with experimental observations.

Field Locked to a Fock State by Quantum Feedback with Single Photon Corrections

Fock states with photon numbers n up to 7 are prepared on demand in a microwave superconducting cavity by a quantum feedback procedure that reverses decoherence-induced quantum jumps. Circular Rydberg atoms are used as quantum nondemolition sensors or as single-photon emitter or absorber actuators. The quantum nature of these actuators matches the correction of single-photon quantum jumps due to relaxation. The flexibility of this method is suited to the generation of arbitrary sequences of Fock states.

Interaction-induced stabilization of circular Rydberg atoms

We discuss a candidate solution for the controlled trapping and manipulation of two individual Rydberg atoms by means of a magnetic Ioffe-Pritchard trap that is superimposed by a constant electric field. In such a trap Rydberg atoms experience a permanent electric dipole moment that can be of the order of several hundred Debye. The interplay of electric dipolar repulsion and three dimensional magnetic confinement leads to a well controllable equilibrium configuration with tunable trap frequency and atomic distance. We thoroughly investigate the trapping potentials and analyze the interaction-induced stabilization of two such trapped Rydberg atoms. Possible limitations and collapse scenarios are discussed.

Stabilization of circular Rydberg atoms by circularly polarized infrared laser fields

The ionization dynamics of circular Rydberg states in strong circularly polarized infrared (800 nm) laser fields is studied by means of numerical simulations with the time-dependent Schr\odinger equation. We find that at certain intensities, related to the radius of the Rydberg states, atomic stabilization sets in, and the ionization probability decreases as the intensity is further increased. Moreover, there is a strong dependence of the ionization probability on the rotational direction of the applied laser field, which can be understood from a simple classical analogy.

Quantum Incompressibility of a Falling Rydberg Atom, and a Gravitationally-Induced Charge Separation Effect in Superconducting Systems

Freely falling point-like objects converge toward the center of the Earth. Hence the gravitational field of the Earth is inhomogeneous, and possesses a tidal component. The free fall of an extended quantum mechanical object such as a hydrogen atom prepared in a high principal-quantum-number state, i.e. a circular Rydberg atom, is predicted to fall more slowly than a classical point-like object, when both objects are dropped from the same height above the Earth’s surface. This indicates that, apart from transitions between quantum states, the atom exhibits a kind of quantum mechanical incompressibility during free fall in inhomogeneous, tidal gravitational fields like those of the Earth.A superconducting ring-like system with a persistent current circulating around it behaves like the circular Rydberg atom during free fall. Like the electronic wavefunction of the freely falling atom, the Cooper-pair wavefunction is quantum mechanically incompressible. The ions in the lattice of the superconductor, however, are not incompressible, since they do not possess a globally coherent quantum phase. The resulting difference during free fall in the response of the nonlocalizable Cooper pairs of electrons and the localizable ions to inhomogeneous gravitational fields is predicted to lead to a charge separation effect, which in turn leads to a large Coulomb force that opposes the convergence caused by the tidal gravitational force on the superconducting system.A “Cavendish-like” experiment is proposed for observing the charge separation effect induced by inhomogeneous gravitational fields in a superconducting circuit. The charge separation effect is determined to be limited by a pair-breaking process that occurs when low frequency gravitational perturbations are present.

Interatom intrashell blockade

We demonstrate a feature of the Rydberg blockade mechanism which occurs between two initially excited circular Rydberg atoms. When both atoms are exposed to weak time-dependent electric fields, it is shown that the intrashell dynamics of each atom is strongly modified by the presence of the other. Three characteristic dynamical regimes are identified with separating radii which both scale linearly with principal quantum number $n$ for otherwise constant field parameters. A region of conditional entangled electron dynamics is separated from the outer asymptotic region of independent atom dynamics through a conditional radius, ${R}_{c}$. An inner region, where both atoms becomes locked in their initial state, is again separated from the conditional region by a smaller blocking radius, ${R}_{b}$.

Highly excited Rydberg electron as a spectator to an ion-molecule reaction

We have theoretically studied the conditions of the behavior of a high Rydberg electron as a spectator to an ion-molecule reaction in high Rydberg neutral collisions. Adoption of a circular high Rydberg atom in the initial channel of the high Rydberg neutral collisions ensures the behavior of the high Rydberg electron as the spectator to interaction between an ion core of the high Rydberg atom and an incoming neutral species; i.e., the ion-molecule reaction. This theoretical consideration leads to equivalence between the high Rydberg neutral collision and the ion-molecule reaction with high accuracy. This equivalence gives us a possibility of probing the ion-molecule reaction at low energies without space-charge effects encountered in ion-beam experiments.

The quantum Zeno effect and quantum feedback in cavity QED

We explore experimentally the fundamental projective properties of a quantum measurement and their application in the control of a system's evolution. We perform quantum non-demolition (QND) photon counting on a microwave field trapped in a very-high-Q superconducting cavity, employing circular Rydberg atoms as non-absorbing probes of light. By repeated measurement of the cavity field we demonstrated the freeze of its initially coherent evolution, illustrating the back action of the photon number measurement on the field's phase. On the contrary, by utilizing a weak QND measurement in combination with the control injection of coherent pulses, we plan to force the field to deterministically evolve towards any target photon-number state. This quantum feedback procedure will enable us to prepare and protect photon-number states against decoherence.

Protocol and quantum circuit for implementing the N-bit discrete quantum Fourier transform in cavity QED

We present a simple protocol and quantum circuit for efficient implementation of the N-bit discrete quantum Fourier transform by using two-qubit controlled-NOT gate and SWCZ gate that is a combination of -SWAP and controlled-Z gates in cavity quantum electrodynamics. In this protocol long-lived electronic states in circular Rydberg atoms are used as quantum bits and the one-bit and two-bit quantum gate operations required for implementing the discrete quantum Fourier transform in the quantum circuit can be easily achieved with atom–microwave resonant interaction and atom–cavity interaction occurring only between two nearest-neighbour atoms. We present the detailed experimental procedure and analyse the experimental feasibility.

Manipulating and probing microwave fields in a cavity by quantum non-demolition photon counting

We perform quantum non-demolition (QND) photon counting on a microwave field trapped in a very high Q superconducting cavity, employing circular Rydberg atoms as non-absorbing light probes. Beyond realizing fundamental tests of quantum measurement theory, we use this QND method to prepare non-classical Fock and Schrödinger cat states of the field and to reconstruct their Wigner functions. Monitoring the evolution of these functions provides a direct observation of the decoherence process. Quantum feedback procedures will enable us to steer the field towards target states and to protect them against decoherence.

Freezing Coherent Field Growth in a Cavity by the Quantum Zeno Effect

We have frozen the coherent evolution of a field in a cavity by repeated measurements of its photon number. We use circular Rydberg atoms dispersively coupled to the cavity mode for an absorption-free photon counting. These measurements inhibit the growth of a field injected in the cavity by a classical source. This manifestation of the quantum Zeno effect illustrates the backaction of the photon number determination onto the field phase. The residual growth of the field can be seen as a random walk of its amplitude in the two-dimensional phase space. This experiment sheds light onto the measurement process and opens perspectives for active quantum feedback.

A cavity-QED scheme for Heisenberg-limited interferometry

We propose a Ramsey interferometry experiment using an entangled state of N atoms to approach the Heisenberg limit for the estimation of an atomic phase shift if the atom number parity is perfectly determined. In a more realistic situation, due to statistical fluctuations of the atom source and the finite detection efficiency, the parity is unknown. We then achieve about half the Heisenberg limit. The scheme involves an ensemble of circular Rydberg atoms which dispersively interact successively with two initially empty microwave cavities. The scheme does not require very high-Q cavities. An experimental realization with about ten entangled Rydberg atoms is achievable with a state of art apparatus.

Entanglement and decoherence ofNatoms and a mesoscopic field in a cavity

We investigate the behavior of N atoms resonantly coupled to a single electromagnetic field mode sustained by a high quality cavity, containing a mesoscopic coherent field. We show with a simple effective hamiltonian model that the strong coupling between the cavity and the atoms produces an atom-field entangled state, involving N+1 nearly-coherent components slowly rotating at different paces in the phase plane. The periodic overlap of these components results in a complex collapse and revival pattern for the Rabi oscillation. We study the influence of decoherence due to the finite cavity quality factor. We propose a simple analytical model, based on the Monte Carlo approach to relaxation. We compare its predictions with exact calculations and show that these interesting effects could realistically be observed on a two or three atoms sample in a 15 photons field with circular Rydberg atoms and superconducting cavities.

Probing a quantum field in a photon box

Einstein often performed thought experiments with ‘photon boxes’, storing fields for unlimited times. This is yet but a dream. We can nevertheless store quantum microwave fields in superconducting cavities for billions of periods. Using circular Rydberg atoms, it is possible to probe in a very detailed way the quantum state of these trapped fields. Cavity quantum electrodynamics tools can be used for a direct determination of the Husimi Q and Wigner quasi-probability distributions. They provide a very direct insight into the classical or non-classical nature of the field.