Chirped Pulse Research Articles

Chirped fiber Bragg gratings directly inscribed by a femtosecond laser in an ytterbium-doped fiber for spectrum recovery, loss compensation and effective use in a CPA scheme

Point-by-point femtosecond laser inscribed chirped Bragg gratings are good candidates for use in fiber chirped pulse amplification systems due to the high flexibility of their dispersion properties, low cost, and no length limitation. However, such gratings have two significant drawbacks: high losses and distortions of the short-wavelength part of the spectrum when operating in the normal group velocity dispersion mode. We propose a novel approach based on writing such gratings in a highly doped active fiber, which allows us to correct both shortcomings. We have also demonstrated, for the first time to our knowledge, a successful use of such gratings as stretchers in a fiber chirped pulse amplification system.

44-fs, 1-MHz, 70-µJ Yb-doped fiber laser system for high harmonic generation

We report the development of a robust Yb-doped fiber laser system based on chirped-pulse amplification (CPA), generating 44-fs laser pulses with up to 70-µJ pulse energy at a 1-MHz repetition rate. It consists of a Yb-doped nonlinear polarization evolution (NPE) mode-locked fiber oscillator, a chirped fiber Bragg grating (CFBG) stretcher, a wave-shaper for manipulating the spectrum of the signal, cascaded fiber amplifiers, and two compression units. The output pulse duration of 44 fs for efficient high harmonic generation (HHG) was achieved by a multi-pass multi-plate Herriott-type non-linear compression unit.

Suppression of Kerr-induced satellites in multi-pulse CPA

Amplification of bursts of ultrashort pulses is very challenging when the intraburst repetition frequency reaches the THz range, corresponding to (sub)-ps intervals between consecutive pulses. Periodic interference significantly modifies conditions for chirped pulse amplification (CPA), leading to temporal and spectral distortions during CPA due to optical Kerr nonlinearity. Multi-pulse chirped amplification to mJ energies may lead to a pronounced degradation of burst fidelity and the appearance of periodic temporal satellites after de-chirping the amplified waveform. We study, experimentally and numerically, the limitations of THz burst-mode CPA caused by self- and cross-phase modulation. A number of practical recipes to suppress nonlinear distortions and improve energy scaling by optimizing burst parameters and applying modulation techniques are presented.

Wideband FMCW radar for long-distance target detection based on photonic chirp pulse stitching.

Current wideband frequency-modulated continuous-wave (FMCW) radar fails in detecting long-distance target, since only the target whose echo is temporally close to the reference linear frequency modulation (LFM) chirp can be detected. We propose a long-distance target detection method for the wideband FMCW radar based on photonic chirp pulse stitching. The stitching photonic chirp pulse that is generated through optical up- and downconversion of the LFM is employed as local signal for the de-chirping process instead of the LFM itself, as currently used. By adjusting the transmitting signal period, a theoretically arbitrarily large detection distance can be obtained with the proposed method. Experiments obtain high-resolution range profiles for two targets located at 1.44 km and 14.5 km, respectively, proving the feasibility of the proposed scheme.

Efficient temporal compression of 10-µJ pulses in periodic layered Kerr media.

Pulse compression based on periodic layered Kerr media has been demonstrated as an effective technique for femtosecond pulses with energies around 100 µJ or more. We report such a compressor designed for pulses in the 10-µJ range, which is valuable for many applications. Pulses from a fiber chirped-pulse amplifier are compressed from 300 fs to as short as 60 fs, with good pulse and beam quality. The compressor is a simple and efficient way to extend the performance of common Yb-based sources of pulses with microjoule energies.

High-efficiency Yb:YAG thin-disk chirped pulse amplifier delivering 884-femtosecond laser with tunable repetition rates and high stability

We experimentally demonstrated a compact, highly efficient, stable, chirped pulse amplification (CPA) thin-disk regenerative system with a tunable repetition rate. The laser head consists of a 9 at. % Yb:YAG thin-disk with a diameter of 8.8 mm and a thickness of 150 μm, is designed for a 48-pump pass configuration. In CPA-based regenerative amplifier configuration, a maximal output power of 85 W at 500 kHz is achieved with a conversion efficiency of 53.1 %. This corresponds to a pulse energy of 170 μJ. To the best of our knowledge, this is the highest conversion efficiency in CPA thin-disk regenerative amplifiers. The pulse width is compressed to 884 fs with a pair of grating, resulting in a peak power of 192 MW. At 85 W, a near diffraction limit beam quality factor M2 of 1.40 is measured, which is essential in precision applications. In addition, remarkable long-term power stability is confirmed with a root-mean-square (RMS) fluctuation of 0.12 % over a 24-hour duration. The reported femtosecond amplifier is believed to be a promising tool for various applications such as extreme manufacturing, terahertz spectroscopy, etc.

Growth, optical and thermal properties of YbxSm1-xCa4O(BO3)3 crystals

YbxSm1-xCOB (x = 0.1, 0.2) crystals were grown by the Bridgman method for the first time. The purpose of this paper is to evaluate the application prospect of Yb:SmCOB crystal in quasi-parametric chirped pulse amplification (QPCPA) and frequency-doubling laser. The phase structure, thermal properties and optical properties of Yb:SmCOB were studied, and the density of states of SmCOB crystal was calculated by first-principles. The effective segregation coefficient Keff of Yb0.1Sm0.9COB and Yb0.2Sm0.8COB crystals are 0.89 and 0.88, respectively. The thermal diffusivity and thermal conductivity of Yb:SmCOB decrease with increasing temperature. The specific heat increases with the increase of temperature and eventually tends to be constant. The specific heat of Yb:SmCOB crystal is greater than 0.70 J/(g·K) at room temperature. The transmittance of Yb:SmCOB crystal reaches 87 % in the range of 500 ∼ 900 nm. With the increase of Yb3+ doping concentration, the UV absorption cut-off edge is red shifted. The frequency doubling emission peak of Yb:SmCOB crystal at 490 nm was measured by 980 nm laser. Yb:SmCOB has the characteristics of high transmittance and high specific heat, and has application potential in laser frequency doubling and QPCPA.

Ultrafast 550-W average-power thin-disk laser oscillator

SESAM modelocked oscillators are interesting for applications in strong-field physics such as high-harmonic generation and attosecond science at high repetition rates or frequency combs in the ultraviolet. Here we present a SESAM modelocked ultrafast thin-disk laser oscillator providing 550W of average output power with 852fs pulses at 5.5MHz repetition rate. To reach this significant power scaling, a replicating cavity design for modelocked oscillators is utilized. The oscillator delivers 103 MW of peak power with a pulse energy of 100 µJ at a beam quality of M2<1.2, with a high optical-to-optical efficiency of 35%. The advances in SESAM design and manufacturing that enabled this result are discussed, as well as practical challenges when scaling oscillators to the kW-class. When combined with established pulse compression technologies, this oscillator can enable simpler systems by avoiding the complexity of chirped pulse amplifier chains. Additionally, high power oscillators support a much lower noise floor due to the reduced influence of shot noise, which may provide a route to more sensitive pump-probe measurements.

Mid-infrared optical parametric chirped-pulse amplifier at 50 W and 38 fs pumped by a high-power Yb-InnoSlab platform

High-power Yb:InnoSlab lasers are proliferating into multiple modern application areas of laser physics ranging from plasma physics and nanolithography to driving optical parametric amplifiers for high-harmonic generation and attosecond science. Here, we present, the layout, design and first results of an optical parametric chirped-pulse amplifier system pumped by a kW-level average power Yb-InnoSlab laser. We describe the layout and concepts of the pump lasers, with particular attention to the specific design principles required for our application. In the current configuration, the pump laser delivers up to 933 W, 18.7 mJ, 1.2 ps pulses at 50 kHz repetition rate. In a first attempt this has generated above 70 W average power at 2 μm via parametric amplification. Chirped-mirror compression resulted in mJ-level pulses at 50 W and 38-fs pulse duration (5.7 cycles at 2 μm).

Multiwavelength highly transient stimulated Raman scattering on dual Raman modes in Sr(MoO4)0.8(WO4)0.2 and Sr(MoO4)0.4(WO4)0.6.

For the first time to our knowledge, multiwavelength, highly transient, single-pass stimulated Raman scattering with a low wavelength spacing on dual (stretching and bending) Raman modes in Sr(MoO4)0.8(WO4)0.2 and Sr(MoO4)0.4(WO4)0.6 solid solutions in a range of 1000-1300 nm (transparence window of biological tissue) under ultrafast chirped pulse laser pumping is comparatively investigated in the interests of multicolor two-photon imaging of a living tissue. For both the solid solutions, the optimum range (1-5 ps) of chirped pump pulse durations for multiwavelength Raman conversion on dual Raman modes was wider than for SrMoO4 (2-3 ps) due to the higher integral cross section of the bending Raman mode. Higher efficient SRS conversion took place at negative chirping of the pump pulse with its stretching from 0.25 ps up to 5 ps due to the compensation of a positive chirp caused by nonlinear phase modulation with total Raman conversion efficiency of up to 36% for Sr(MoO4)0.8(WO4)0.2 and 49% for Sr(MoO4)0.4(WO4)0.6. The highest number (five) of Stokes components in the desired range (1000-1300 nm) was observed in the optimum Sr(MoO4)0.4(WO4)0.6 solid solution, which has the Raman modes with comparable intensities.

Effect of laser chirping on third harmonic generation in anharmonic clusters with ripple on cluster density

A proposed model delves into the resonant enhancement of third harmonic generation (THG) by a short-pulse laser inside nanoclustered plasma under the influence of density ripple. An intense chirped laser pulse incident on a clustered plasma of argon gas displaces the electrons of the medium and produces a restoring force. This force is considered to vary nonlinearly with electron displacement, leading to the anharmonic response of the electron clouds of the cluster. The nonlinear current at the third harmonic frequency arises from the perturbation of the electron density of the cluster by the ponderomotive force exerted on them by the incident laser pulse. Applying ripple in cluster density and electron density of surrounding plasma enables the phase-matching criteria for THG to be satisfied, which leads to enhanced harmonic output. An anharmonic structure of clusters exhibits strong optical nonlinearities, resulting in the plasmon resonance broadening and producing harmonics with greater efficiency. Numerical analysis shows that the chirp parameter of the laser pulse and ripple on cluster density enhance system nonlinearity causing the generation of a third harmonic of enhanced amplitude. The study explores how different factors such as laser intensity, cluster size, ripple parameter, chirp parameter, and electron excursion influence the efficiency of THG.

1 kHz, 10 mJ, sub-200 fs regenerative amplifier utilizing a dual-crystal configuration of Yb:CaGdAlO4 featuring exceptional beam quality

In order to boost the energy of the femtosecond regenerative amplifier (RA), we adopt the chirped pulse amplification technique to stretch the seed pulses through the Martinez stretcher and inject them into our specially designed dual-crystal regenerative cavity based on the Yb:CaGdAlO4 (Yb:CGA) crystals. To avoid damaging the component coating, we meticulously regulate the size of the cavity mode on the surface of each component within the cavity to ensure that the energy density remains below the damage threshold. The final output of 11.3 mJ pulse energy was obtained at a 1 kHz repetition rate with a power stability of 0.35% over 1 hour, which is the highest energy we know of for the regenerative output of Yb:CGA crystals. Additionally, leveraging the wide gain spectrum of the Yb:CGA crystal, we achieve a spectrum full width at half maximum (FWHM) of 9 nm along with a compressed pulse duration of 198 fs. The combination of the dual-crystal setup, superior thermal properties of the Yb:CGA crystals, quasi-continuous wave pumping approach, and the thermal-insensitive design of the regenerative cavity effectively minimize the thermal impact on the crystals. The output beam exhibits near-diffraction-limited performance, with an M2 value of only 1.05 × 1.06.

The Study on the Nonlinear Effects of Soliton in Optical Fibre

Abstract: In optical fibres, the chirps generated by GVD and SPM, which both limit the system's performance when operating independently, balance each other out to produce soliton formation. To comprehend how such a balance is possible, we shall study the nonlinear optical effects and the dispersion-induced pulse broadening. If an optical pulse is not adequately chirped before it propagates inside an optical fibre, the GVD broadens the pulse. More specifically, an early stage of transmission compresses a chirped pulse whenever β2 and the chirp parameter C have opposite signs and β2C is negative. The optical pulse chirps due to SPM, ensuring that C > 0. If β2 < 0, it is easy to meet the criteria β2C < 0. Moreover, because the SPM-induced chirp depends on power, it is possible that in some situations, SPM and GVD could cooperate to the extent that the SPM-induced chirp is precisely the right amount to cancel out the pulse broadening caused by GVD. Here, an optical pulse propagates distortion-free as a soliton [27].

Unveiling Ultrafast-Weak-Field Coherent Control of Indirect Dissociation Reactions.

Coherent control of molecular photodissociation through one-photon transitions has become a topic of interest in physical chemistry. Previous studies have shown that modulating the spectral phase of a single ultrafast laser pulse while keeping its spectral amplitude constant does not affect the dissociation yield of reactions originating from a pure eigenstate of the ground electronic state. Here, we explore the indirect photodissociation reaction of NaI molecules using theoretical and numerical methods. Our findings show that, in contrast to the outcomes achieved with negatively chirped pulses, time-dependent population of the eigenstates of the excited adiabatic potential induced by positively chirped laser pulses, acting as intermediates in the reaction, cannot be periodically restored to that caused by the unchirped pulse. This gives rise to an intriguing phenomenon: the sign of the pulse's chirp rate influences the distribution of dissociation fragments in coordinate and momentum space over extended periods. This work highlights the potential of using spectral-phase modulated pulses to manipulate indirect photodissociation reactions, offering a way to modify the transient photofragment distributions by controlling reaction intermediates.

Generation and Evaluation of an Efficient Femtosecond Green Laser.

We demonstrate femtosecond ultra-stable green laser generation by an ytterbium-doped polarization-maintaining fiber laser with a 2.4 mm long lithium triborate (LBO) crystal. We generated 5.6 W of femtosecond green light at 520 nm for a fundamental power of 12 W, which corresponds to a conversion efficiency of 46.7%. The fiber chirped-pulse amplifier, which has an environmentally immune front end, delivered 170 fs pulses at a 75 MHz repetition rate centered at 1040 nm. According to the dispersion of the optical material in a double-frequency setup, the introduced dispersion had a negligible effect for the green laser, and the pulse duration of the generated green laser was calculated to be 171 fs, resulting in an excellent power stability, with fluctuation as low as 0.16% of the generated green light. This system could be of great interest in ultrafast optical and photobiology research.

Watt-level ultra-flat wideband supercontinuum generation in GeO2 fiber by femtosecond pulse

The high-power ultra-flat supercontinuum (SC) sources play an important role in various fields. In this letter, we experimentally demonstrated an all-fiber, high-power, ultra-flat SC source in GeO2 highly nonlinear fiber (HNLF) pumped by a femtosecond fiber laser system. The system is mode-locked by a semiconductor saturable absorber mirror with an all-polarization-maintaining (PM) structure. Based on the technology of chirped pulse amplification, a maximum power of 3.12 W was realized with a repetition rate of 80 MHz at 1.56 μm, and the pulse duration was compressed to 124 fs in a segment of PM single-mode fiber. Furthermore, by optimizing the length of the HNLF, a wideband SC spectrum of nearly 700 nm was obtained at10 dB with a maximum power of 1.82 W, and the flatness of the spectrum was better than 5 dB in the range of 1600–2200 nm. We observed that the pulse evolved into a noise-like pulse with a narrowest pulse duration of 62 fs. Thanks to the all-PM structure of the fiber laser, the long-term stability of SC power was manifested with a relative fluctuation as low as 0.53 % over 6 h.

Plasma-grating-based laser pulse compressor.

To avoid damage in high-power laser systems, a chirped plasma-based grating is proposed for compressing laser pulses that have been previously stretched and amplified. This chirped grating is generated through the interaction of chirped pump laser pulses in a plasma slab. Particle-in-cell (PIC) simulations demonstrate that the grating exists for a duration sufficient to be utilized in the final chirped pulse amplification (CPA) stage. The generation of the grating is quite flexible, as several parameters can be adjusted, such as plasma density, chirp, length, and intensity of the pump laser. To begin, the structure of the grating is analyzed in terms of ponderomotive effects of the pump laser pulses. The primary application of the chirped plasma-based grating lies in compressing laser pulses to large amplitudes and short durations after they have been stretched and amplified beforehand. The compression factor is explored in connection with potential grating parameters. Reflectivity and effective bandwidth of chirped plasma gratings are parameters to be optimized. However, the grating spectral bandwidth can only be increased at the expense of reflectivity. The PIC results are made understandable through model calculations based on coupled mode equations.

Bridgman growth and characterizations of nonlinear optical crystal La3Ga5.5Nb0.5O14

La3Ga5.5Nb0.5O14 (LGN) crystal is a promising material for optical parametric chirped-pulse amplification (OPCPA) with high laser damage threshold and wide transmission range which is able to achieve high peak power laser. LGN with a diameter of 25 mm was successfully grown by the vertical Bridgman method for the first time and a series of characterizations were performed. The 1.7 µm absorption peak in transmittance spectra of LGN crystal which was caused by the Czochralski technique can be effectively eliminated by the vertical Bridgman method. LGN crystal possesses a high transmittance of 81.3 % in the range of 0.294 ∼ 7.500 μm. The experimental optical band gap of LGN is 4.16 eV which is positively correlated with laser damage threshold. The experimental laser damage threshold of LGN was determined to 1.416 GW/cm2 by Nd:YAG. The outstanding thermal properties of LGN indicate that it possesses thermal stability in high energy laser field. This work demonstrates that LGN crystal holds great potential for OPCPA applications and the vertical Bridgman method is proved to be a effective and excellent technique to grow high quality LGN crystal.

A Review of an Investigation of the Ultrafast Laser Processing of Brittle and Hard Materials.

Ultrafast laser technology has moved from ultrafast to ultra-strong due to the development of chirped pulse amplification technology. Ultrafast laser technology, such as femtosecond lasers and picosecond lasers, has quickly become a flexible tool for processing brittle and hard materials and complex micro-components, which are widely used in and developed for medical, aerospace, semiconductor applications and so on. However, the mechanisms of the interaction between an ultrafast laser and brittle and hard materials are still unclear. Meanwhile, the ultrafast laser processing of these materials is still a challenge. Additionally, highly efficient and high-precision manufacturing using ultrafast lasers needs to be developed. This review is focused on the common challenges and current status of the ultrafast laser processing of brittle and hard materials, such as nickel-based superalloys, thermal barrier ceramics, diamond, silicon dioxide, and silicon carbide composites. Firstly, different materials are distinguished according to their bandgap width, thermal conductivity and other characteristics in order to reveal the absorption mechanism of the laser energy during the ultrafast laser processing of brittle and hard materials. Secondly, the mechanism of laser energy transfer and transformation is investigated by analyzing the interaction between the photons and the electrons and ions in laser-induced plasma, as well as the interaction with the continuum of the materials. Thirdly, the relationship between key parameters and ultrafast laser processing quality is discussed. Finally, the methods for achieving highly efficient and high-precision manufacturing of complex three-dimensional micro-components are explored in detail.

A Tale of Two Tails: Rotational Spectroscopy of N-Ethyl Maleimide and N-Ethyl Succinimide.

Broadband microwave spectra of N-ethyl maleimide (NEM) and N-ethyl succinimide (NES) have been recorded using chirped pulse Fourier transform microwave spectroscopy in the Ka-band (26.5-40 GHz). The spectra for both molecules were fit to a Watson A-reduced Hamiltonian in the Ir representation to obtain best fit experimental rotational constants (NEM: A0 = 2143.1988(29), B0 = 1868.7333(22), C0 = 1082.98458(36); NES: A0 = 2061.47756(14), B0 = 1791.73517(12), C0 = 1050.31263(11)), centrifugal distortion constants, and nuclear quadrupole coupling constants. While the heavy atoms of the five-membered ring of both molecules are planar, the ethyl chain has its terminal methyl group perpendicular to the ring. Along the relaxed potential energy curve for the ethyl dihedral angle (θ1 = C(6)-C(5)-N-C(4)), the ethyl group experiences significant steric strain when it is in the plane of the ring, associated with the interaction of the ethyl group with the two carbonyl oxygens. This leads to calculated barriers of θ1 = 1469 cm-1 and θ1 = 1680 cm-1 in N-ethyl maleimide and N-ethyl succinimide, respectively.