Cavity QED Research Articles

Cavity QED systems for steady-state sources of Wigner-negative light

We present a theoretical investigation of optical cavity quantum electrodynamics (cavity QED) systems, as described by the driven, open Jaynes–Cummings model and some of its variants, as potential sources of steady-state Wigner-negative light. We consider temporal modes in the continuous output field from the cavity and demonstrate pronounced negativity in their Wigner distributions for experimentally relevant parameter regimes. We consider models of both single and collective atomic spin systems, and find a rich structure of Wigner-distribution negativity as the spin size is varied. We also demonstrate an effective realization of all of the models considered using just a single 87Rb atom and based upon combinations of laser- and laser-plus-cavity-driven Raman transitions between magnetic sublevels in a single ground hyperfine state.

Electron-photon exchange-correlation approximation for quantum-electrodynamical density-functional theory

Quantum-electrodynamical density-functional theory (QEDFT) provides a promising avenue for exploring complex light-matter interactions in optical cavities for real materials. Similar to conventional density-functional theory, the Kohn-Sham formulation of QEDFT needs approximations for the generally unknown exchange-correlation functional. In addition to the usual electron-electron exchange-correlation potential, an approximation for the electron-photon exchange-correlation potential is needed. A recent electron-photon exchange functional [C. Schäfer , ], derived from the equation of motion of the nonrelativistic Pauli-Fierz Hamiltonian, shows robust performance in one-dimensional systems across weak- and strong-coupling regimes. Yet, its performance in reproducing electron densities in higher dimensions remains unexplored. Here we consider this QEDFT functional approximation from one- to three-dimensional finite systems and across weak to strong light-matter couplings. The electron-photon exchange approximation provides excellent results in the ultrastrong-coupling regime. However, to ensure accuracy also in the weak-coupling regime across higher dimensions, we introduce a computationally efficient renormalization factor for the electron-photon exchange functional, which accounts for part of the electron-photon correlation contribution. These findings extend the applicability of photon-exchange-based functionals to realistic cavity-matter systems, fostering the field of cavity QED (quantum-electrodynamics) materials engineering. Published by the American Physical Society 2024

High-efficiency all-optical switching based on broadband coherent perfect absorption in an atom-cavity system

We propose an ultrahigh-efficiency and broadband all-optical switching scheme based on coherent perfect absorption (CPA) in linear and nonlinear excitation regimes in a cavity quantum electrodynamics (CQED) system. Two separate atomic transitions are excited simultaneously by two signal fields coupled from two ends of an optical cavity under the collective strong coupling condition. Three polariton eigenstates are produced which can be tuned freely by varying system parameters. The output field intensities of multiple channels are zero when the CPA criterion is satisfied. However, destructive quantum interference can be induced by a free-space weak control laser when it is tuned to be resonant to the polariton state. As a consequence, the CQED system acts as a coherent perfect light absorber/transmitter as the control field is turned on/off the polariton resonances. In particular, the proposed scheme may be used to realize broadband multi-throw all-optical switching in the nonlinear excitation regime. The proposed scheme is useful for constructing all-optical routing, all-optical communication networks and various all-optical logic elements.

Engineering the Impact of Phonon Dephasing on the Coherence of a WSe_{2} Single-Photon Source via Cavity Quantum Electrodynamics.

Emitter dephasing is one of the key issues in the performance of solid-state single-photon sources. Among the various sources of dephasing, acoustic phonons play a central role in adding decoherence to the single-photon emission. Here, we demonstrate that it is possible to tune and engineer the coherence of photons emitted from a single WSe_{2} monolayer quantum dot via selectively coupling it to a spectral cavity resonance. We utilize an open cavity to demonstrate spectral enhancement, leveling, and suppression of the highly asymmetric phonon sideband, finding excellent agreement with a microscopic description of the exciton-phonon dephasing in a truly two-dimensional system. Moreover, the impact of cavity tuning on the dephasing is directly assessed via optical interferometry, which points out the capability to utilize light-matter coupling to steer and design dephasing and coherence of quantum emitters in atomically thin crystals.

Strong coupling between plasmonic nanocavity gold nanorods and quantum dots emitter

The discovery of hybrid states in strong coupling interaction has gained growing attention in cavity-quantum electrodynamics research owing to its fundamental directives and potential in advanced optical applications. The ultra-confined mode volume of plasmonic cavity gold nanorods (AuNRs), particularly at the nanorod tip “hotspot” provides a large coupling strength, a prerequisite for a coherent energy exchange in the strong coupling regime. Here, we reported a remarkable Rabi splitting of ∼231 meV between gold nanorods longitudinal localized surface plasmon resonance (LLSPR) mode and quantum dots (QDs) at ambient conditions, monitored by dielectric medium tuning. Numerical simulations confirmed the result, displaying absorption spectral splitting.

Nonreciprocal Superradiant Phase Transitions and Multicriticality in a Cavity QED System.

We demonstrate the emergence of nonreciprocal superradiant phase transitions and novel multicriticality in a cavity quantum electrodynamics system, where a two-level atom interacts with two counterpropagating modes of a whispering-gallery-mode microcavity. The cavity rotates at a certain angular velocity and is directionally squeezed by a unidirectional parametric pumping χ^{(2)} nonlinearity. The combination of cavity rotation and directional squeezing leads to nonreciprocal first- and second-order superradiant phase transitions. These transitions do not require ultrastrong atom-field couplings and can be easily controlled by the external pump field. Through a full quantum description of the system Hamiltonian, we identify two types of multicritical points in the phase diagram, both of which exhibit controllable nonreciprocity. These results open a new door for all-optical manipulation of superradiant transitions and multicritical behaviors in light-matter systems, with potential applications in engineering various integrated nonreciprocal quantum devices.

High-fidelity single logical qubit encoding scheme assisted by single-sided quantum dot-cavity systems.

We present an encoding scheme of a single logical qubit with single-sided quantum dot (QD)-cavity systems, which is immune to the collective decoherence. By adjusting the Purcell factor to satisfy the balanced reflection condition, the detrimental effects of unbalanced reflection between the coupled and uncoupled QD-cavity systems can be effectively suppressed. Furthermore, the fidelity of each step can be increased to unity regardless of the strong coupling regime and the weak coupling regime of cavity quantum electrodynamics (QED) with the assistance of waveform correctors. The scheme requires QD-cavity systems and simple linear optical elements, which can be implemented with the currently experimental techniques.

Quantum catalysis in cavity quantum electrodynamics

Catalysis plays a key role in many scientific areas, most notably in chemistry and biology. Here we present a catalytic process in a paradigmatic quantum optics setup, namely the Jaynes-Cummings model, where an atom interacts with an optical cavity. The atom plays the role of the catalyst, and it allows for the deterministic generation of nonclassical light in the cavity. Considering a cavity prepared in a “classical” coherent state, and choosing appropriately the atomic state and the interaction time, we obtain an evolution with the following properties. First, the state of the cavity has been modified, and it now features nonclassicality, as witnessed by sub-Poissonian statistics or Wigner negativity. Second, the process is catalytic in the sense that the atom is deterministically returned to its initial state exactly, and it can be reused multiple times. What is more, we also show that our findings are robust under dissipation and can be applied to scenarios featuring cavity loss and atomic decay. Finally, we investigate the mechanism of this catalytic process, in particular highlighting the key role of correlations and quantum coherence. Published by the American Physical Society 2024

Opto-RF transduction in Er3+:CaWO4

We use an erbium doped CaWO4 crystal as a resonant transducer between the RF and optical domains at 12 GHz and 1532 nm respectively. We employ a RF resonator to enhance the spin coupling but keep a single-pass (non-resonant) optical setup. The overall efficiency is low but we carefully characterize the transduction process and show that the performance can be described by two different metrics that we define and distinguish: the electro-optics and the quantum efficiencies. We reach an electro-optics efficiency of -84 dB for 15.7 dBm RF power. The corresponding quantum efficiency is -142 dB for 0.4 dBm optical power. We develop the Schrödinger-Maxwell formalism, well-known to describe light-matter interactions in atomic systems, in order to model the conversion process. We explicitly make the connection with the cavity quantum electrodynamics (cavity QED) approach that are generally used to describe quantum transduction.

Limitations in design and applications of ultra-small mode volume photonic crystals

Ultra-small mode volume nanophotonic crystal cavities have been proposed as powerful tools for increasing coupling rates in cavity quantum electrodynamics systems. However, their adoption in quantum information applications remains elusive. In this work, we investigate possible reasons why, and analyze the impact of different low mode volume resonator design choices on their utility in quantum optics experiments. We analyze band structure features and loss rates of low mode volume bowtie cavities in diamond and demonstrate independent design control over cavity-emitter coupling strength and loss rates. Further, using silicon vacancy centers in diamond as exemplary emitters, we investigate the influence of placement imprecision. We find that the benefit on photon collection efficiency and indistinguishability is limited, while the fabrication complexity of ultra-small cavity designs increases substantially compared to conventional photonic crystals. We conclude that ultra-small mode volume designs are primarily of interest for dispersive spin-photon interactions, which are of great interest for future quantum networks.

Band gap engineering and controlling transport properties of single photons in periodic and disordered Jaynes–Cummings arrays

We theoretically study the single-photon transport properties in periodic and position-disordered Jaynes–Cummings (or JC) arrays of waveguide-coupled microtoroidal ring resonators, each interacting with a single two-level quantum emitter. Employing the real-space formalism of quantum optics, we focus on various parameter regimes of cavity quantum electrodynamics (cQED) to gain better control of single-photon propagation in such a many-body quantum optical setting. As for some of the key findings, we observe that the periodic setting leads to the formation of the band structure in the photon transmission spectra, which is most evident in the strong coupling regime of cQED. However, under resonant conditions with no losses, the application of Bloch’s theorem indicates that the width of forbidden gaps can be altered by tuning the emitter-cavity coupling to small values. Moreover, in the disordered case, we find that the single-photon transmission curves show the disappearance of band formation. However, spectral features originating from cQED interactions observed for the single atom-cavity problem remain robust against weak-disordered conditions. The results of this work may find application in the study of quantum many-body effects in the optical domain as well as in different areas of quantum computation and quantum networking.

Reconciling quantum and classical spectral theories of ultrastrong coupling: role of cavity bath coupling and gauge corrections

Cavity quantum-electrodynamics (QED) is a rich area of optical physics, where extreme light–matter coupling can give rise to ultrastrong coupling. The ultrastrong coupling regime presents some fascinating uniquely quantum mechanical effects, such as ground state virtual photons and vacuum squeezing. Focusing on the widely adopted Hopfield model with cavity dissipation, we show how the linear spectrum of an ultrastrong coupled cavity and a dipole can be described either classically or quantum mechanically, but only when the quantum model includes (i) corrections to maintain gauge invariance, and (ii) a specific type of cavity bath coupling, which has so far not been identified. We also show the impact of this bath model on the quantum Rabi model, which has no classical analog in ultrastrong coupling. These results can be used to guide emerging experiments and significantly impact current models and interpretations of ultrastrong coupling between light and matter.

Dispersive nonreciprocity between a qubit and a cavity.

The dispersive interaction between a qubit and a cavity is ubiquitous in circuit and cavity quantum electrodynamics. It describes the frequency shift of one quantum mode in response to excitations in the other and, in closed systems, is necessarily bidirectional, i.e., reciprocal. Here, we present an experimental study of a nonreciprocal dispersive-type interaction between a transmon qubit and a superconducting cavity, arising from a common coupling to dissipative intermediary modes with broken time reversal symmetry. We characterize the qubit-cavity dynamics, including asymmetric frequency pulls and photon shot noise dephasing, under varying degrees of nonreciprocity by tuning the magnetic field bias of a ferrite component in situ. We introduce a general master equation model for nonreciprocal interactions in the dispersive regime, providing a compact description of the observed qubit-cavity dynamics agnostic to the intermediary system. Our result provides an example of quantum nonreciprocal phenomena beyond the typical paradigms of non-Hermitian Hamiltonians and cascaded systems.

Optical characterization of a fiber Fabry-Perot cavity: precision measurement of intra-cavity loss, transmittance, and reflectance

We propose and demonstrate a method for characterizing the individual mirror parameters of a fiber Fabry–Perot cavity (FFPC). By measuring the reflection and transmission spectra of the FFPC with an incident laser propagating from the two mirrors of the FFPC and considering several normal or unique losses, the transmittance, reflectance, and intra-cavity loss of the individual mirrors can be determined. Due to the intrinsic limitation of cavity length, traditional powerful methods, such as the cavity ring-down technique, are not applicable to FFPCs for characterizing the parameters of individual mirrors. This scheme provides a dependable method for assessing FFPC mirrors and provides a significant capability for the implementation of strong-coupling cavity quantum electrodynamics based on FFPCs.

Integrated Fabry–Perot Cavities: A Quantum Leap in Technology

Integrated Fabry–Perot cavities (IFPCs), often referred to as nanobeams due to their form factor and size, have profoundly modified the landscape of integrated photonics as a new building block for classical and quantum engineering. In this entry, the main properties of IFPCs will be summarized from the classical and quantum point of view. The classical will provide some of the main results obtained in the last decade, whereas the quantum point of view will explore cavity quantum electrodynamics (CQED), which promises to revolutionize the future “quantum internet”.

Microscopic theory of exciton-polariton model involving multiple molecules: Macroscopic quantum electrodynamics formulation and essence of direct intermolecular interactions.

Cavity quantum electrodynamics (CQED) and its extensions are widely used for the description of exciton-polariton systems. However, the exciton-polariton models based on CQED vary greatly within different contexts. One of the most significant discrepancies among these CQED models is whether one should include direct intermolecular interactions in the CQED Hamiltonian. To answer this question, in this article, we derive an effective dissipative CQED model including free-space dipole-dipole interactions (CQED-DDI) from a microscopic Hamiltonian based on macroscopic quantum electrodynamics. Dissipative CQED-DDI successfully captures the nature of vacuum fluctuations in dielectric media and separates them into free-space effects and dielectric-induced effects. The former include spontaneous emissions, dephasings, and dipole-dipole interactions in free space; the latter include exciton-polariton interactions and photonic losses due to dielectric media. We apply dissipative CQED-DDI to investigate the exciton-polariton dynamics (the population dynamics of molecules above a plasmonic surface) and compare the results with those based on the methods proposed by several previous studies. We find that direct intermolecular interactions are a crucial element when employing CQED-like models to study exciton-polariton systems involving multiple molecules.

Photonic quantum metrology with variational quantum optical nonlinearities

Photonic quantum metrology harnesses quantum states of light, such as NOON or twin-Fock states, to measure unknown parameters beyond classical precision limits. Current protocols suffer from two severe limitations that preclude their scalability: the exponential decrease in fidelities (or probabilities) when generating states with large photon numbers due to gate errors and the increased sensitivity of such states to noise. Here, we develop a deterministic protocol combining quantum optical nonlinearities and variational quantum algorithms that provides a substantial improvement on both fronts. First, we show how the variational protocol can generate metrologically relevant states with a small number of operations which do not significantly depend on photon number, resulting in exponential improvements in fidelities when gate errors are considered. Second, we show that such states offer a better robustness to noise compared to other states in the literature. Since our protocol harnesses interactions already appearing in state-of-the-art setups, such as cavity QED, we expect that it will lead to more scalable photonic quantum metrology in the near future. Published by the American Physical Society 2024

Quantum computing simulation of a mixed spin-boson Hamiltonian and its performance for a cavity quantum electrodynamics problem

Quantum computing simulation of a mixed spin-boson Hamiltonian and its performance for a cavity quantum electrodynamics problem

Phase-engineered photon correlations in weakly coupled nanofiber cavity QED

Phase-engineered photon correlations in weakly coupled nanofiber cavity QED

Reciprocal asymptotically decoupled Hamiltonian for cavity quantum electrodynamics

Reciprocal asymptotically decoupled Hamiltonian for cavity quantum electrodynamics