Broadband Terahertz Pulses Research Articles

Achromatic prism-type wave plate for broadband terahertz pulses.

We demonstrated achromatic half- and quarter-wave plates for broadband terahertz pulses using phase retardation by internal total reflection. Prism-type wave plates realized ultra-broadband retardation stability up to 2.5THz, which was the limitation of our experimental setup. Novel aspects of our work were use of a 3λ/4 plate as a quarter-wave plate and a multistacked prism-type (MSP) wave plate for a large-aperture THz beam. Real-time polarization imaging of two crossed bunches of hairs was performed to show the efficiency of the MSP wave plate. We clearly observed polarization dependence of the hair direction.

Aeronautics composite material inspection with a terahertz time-domain spectroscopy system

The usability of pulsed broadband terahertz radiation for the inspection of composite materials from the aeronautics industry is investigated, with the goal of developing a mobile time-domain spectroscopy system that operates in reflection geometry. A wide range of samples based on glass and carbon fiber reinforced plastics with various types of defects is examined using an imaging system; the results are evaluated both in time and frequency domain. The conductivity of carbon fibers prevents penetration of the respective samples but also allows analysis of coatings from the reflected THz pulses. Glass fiber composites are, in principle, transparent for THz radiation, but commonly with significant absorption for wavelengths >1 THz . Depending on depth, matrix material, and size, defects like foreign material inserts, delaminations, or moisture contamination can be visualized. If a defect is not too deep in the sample, its location can be correctly identified from the delay between partial reflections at the surface and the defect itself.

Characterization of 700 μJ T rays generated during high-power laser solid interaction

Laser-produced solid density plasmas are well-known as table-top sources of electromagnetic radiation. Recent studies have shown that energetic broadband terahertz pulses (T rays) can also be generated from laser-driven compact ion accelerators. Here we report the measurement of record-breaking T-Ray pulses with energies no less than 0.7 mJ. The terahertz spectrum has been characterized for frequencies ranging from 0.1-133 THz. The dependence of T-Ray yield on incident laser energy is linear and shows no tendencies of saturation. The noncollinear emission pattern and the high yield reveal that the T rays are generated by the transient field at the rear surface of the solid target.

Generation of 0.3 mW high-power broadband terahertz pulses from GaP crystal pumped by negatively chirped femtosecond laser pulses

Based on optical rectification in a 3 mm GaP crystal with a femtosecond photonic crystal fiber amplifier as the pump source, a detailed experimental investigation on the influence of the chirp characteristics of the pump pulses on the THz wave generation efficiency is conducted. It is shown that a higher THz generation efficiency can be achieved using negatively chirped pulses rather than de-chirped pulses. In the chosen geometry, using 21 W pump pulses with a negative chirp of −2.3 × 10−3 ps2, broadband THz radiation with an average power of 0.3 mW is obtained, which is, to the best of our knowledge, the highest value reported so far for high-repetition-rate THz pulses generated by collinear optical rectification. The higher THz generation efficiency by negatively chirped pulses is explained by a pulse-narrowing mechanism in the nonlinear crystal.

A complementary study to “Hybrid hollow core fibers with embedded wires as THz waveguides” and “Two-wire terahertz fibers with porous dielectric support:” comment

In a recent paper, Anthony et al. [Opt. Express 21, 2903 (2013)] demonstrated broadband terahertz pulse propagation through the hollow core fibers with two embedded Indium wires. In another paper by A. Markov et al. [Opt. Express 21, 12728 (2013)], we proposed a plasmonic THz fiber featuring two metallic wires held in place by the porous dielectric cladding functioning as a mechanical support. Although the cross sections of the two waveguides look very similar, we were surprised to find that the guidance mechanisms for these two waveguides are quite different. In fact, waveguide considered by A. Markov et al. was guiding a plasmonic mode, while the waveguide presented by Anthony et al. was guiding a dielectric waveguide-like mode. Finally, we have realized that by reducing the waveguide dimensions by a factor of ~10-20 one can transition from the dielectric waveguide guidance as it is demonstrated by Anthony et al. to plasmonic guidance as reported in A. Markov et al. Therefore, we conclude that both waveguide are essentially identical, while their guidance mechanism changes as a function of the waveguide overall size.

Simplified model for optical rectification of broadband terahertz pulses in lossy waveguides including a new generalized expression for the coherence length

We present a simplified coupled mode theory (CMT), suited for high losses, to describe ultra-broadband THz generation through optical rectification (OR) of fs infrared pulses in waveguides. We derive a new expression that incorporates loss effects into the coherence length for OR. The simplified approach reproduces the results of a computationally rigorous integral CMT that must be used for broadband THz generation. With the new model we perform a parametric study to establish the optimal conditions for OR in symmetric, five-layer, metal/cladding/core structures with electro optic polymer cores. We find conversion efficiencies as high as 35 × 10⁻⁴ W⁻¹ and bandwidths up to 20 THz when pumping at 1900 nm. We find that low-loss-cladding layers enhance the efficiency for phase-matched structures, increase the interaction length, and improve the stability of the efficiency with respect to variations in waveguide parameters.

Measuring TE1 mode Losses in Terahertz Parallel-Plate Waveguides

The parallel-plate waveguide (PPWG) has drawn considerable research interest [1–12], since it was first reported to support the undistorted propagation of broadband terahertz (THz) pulses. From that time, the transverse-electromagnetic (TEM) mode of the PPWG has been the popular choice for measurements due to its low loss, ease of quasi-optic coupling, and negligible dispersion as a result of the lack of a cutoff. Unlike the TEM mode, the lowest order transverse-electric (TE1) mode has a cutoff frequency, and thus this mode was largely unexplored in the THz regime until recently [13, 14]. This recent work showed that the cutoff frequency could be moved to lower frequencies to reduce the dispersion by increasing the plate separation, while matching the input beam size to the plate separation to realize dominantly single-mode propagation. This same work predicted the possibility of realizing ultra-low ohmic losses in the dB/km range by again utilizing the TE1 mode of this waveguide. These low ohmic losses could permit long-distance transport of THz radiation. However, with such long propagation distances a new concern arises: energy leakage out of the unconfined sides of the PPWG due to diffraction. In fact, this would be the dominant loss mechanism in the case under consideration, where the ohmic losses are virtually negligible. We addressed this diffraction problem in a recent article [15], where we showed that it is possible to inhibit diffraction losses for the TE1 mode by using a waveguide with slightly concave plates. Via a simple “bouncing plane wave” analysis, we demonstrated how to determine an ideal radius of curvature for the inner surfaces, for a waveguide operating at a given THz frequency. This is governed by a confocal condition, R 1⁄4 2bv .

Intense terahertz pulses from SLAC electron beams using coherent transition radiation

SLAC has two electron accelerators, the Linac Coherent Light Source (LCLS) and the Facility for Advanced Accelerator Experimental Tests (FACET), providing high-charge, high-peak-current, femtosecond electron bunches. These characteristics are ideal for generating intense broadband terahertz (THz) pulses via coherent transition radiation. For LCLS and FACET respectively, the THz pulse duration is typically 20 and 80 fs RMS and can be tuned via the electron bunch duration; emission spectra span 3-30 THz and 0.5 THz-5 THz; and the energy in a quasi-half-cycle THz pulse is 0.2 and 0.6 mJ. The peak electric field at a THz focus has reached 4.4 GV/m (0.44 V/Å) at LCLS. This paper presents measurements of the terahertz pulses and preliminary observations of nonlinear materials response.

Hybrid hollow core fibers with embedded wires as THz waveguides

We experimentally demonstrate broadband terahertz (THz) pulse propagation through hollow core fibers with two or four embedded Indium wires in a THz time-domain spectroscopy (THz-TDS) setup. The hybrid mode is guided in the air core region with power attenuation coefficients of 0.3 cm(-1) and 0.5 cm(-1) for the two-wire and four-wire configurations, respectively.

Intense broadband THz generation from femtosecond laser filamentation

Broadband and energetic terahertz (THz) pulses can be remotely generated in air through filamentation. We review such THz generation and detection in femtosecond Ti-sapphire laser induced remote filaments. New results are presented on the direct relationship between THz generation in a two color filament and induced N2 fluorescence through population trapping during molecular alignment and revival in air. This further supports the new technique of remote THz detection in air through the sensitive measurement of N2 fluorescence.

Polarization sensitive terahertz imaging: detection of birefringence and optical axis

We present a practicable way to take advantage of the spectral information contained in a broadband terahertz pulse for the determination of birefringence and orientation of the optical axis in a glass fiber reinforced polymer with a single measurement. Our setup employs circularly polarized terahertz waves and a polarization-sensitive detector to measure both components of the electromagnetic field simultaneously. The anisotropic optical parameters are obtained from an analysis of the phase and frequency resolved components of the terahertz field. This method shows a high tolerance against the skew of the detection axes and is also independent of a reference measurement.

Oxidation kinetics of nanoscale copper films studied by terahertz transmission spectroscopy

Terahertz (THz) transmission spectroscopy is used to measure the oxidation kinetics of copper thin films evaporated on silicon substrates. The transmission of broadband THz pulses from 1 to 7 THz through the copper film is measured while it gets oxidized at an elevated temperature in ambient air. The change in the transmitted THz electric field is correlated with the growth of the cuprous oxide layer and the decrease in thickness of the copper layer. Oxidation curves were obtained for heating temperatures of 120–150 °C and were found to follow a parabolic rate law. Using the Arrhenius equation, we calculate an activation energy for diffusion of 0.55 eV. By measuring the THz transmission through unoxidized copper layers of several thicknesses, we also measured the optical properties of thin copper films around the percolation threshold thickness of 7 nm. Around the percolation transition, the optical properties of freshly deposited copper thin films are very different from that of copper layers of the same thickness remaining after partial oxidation of thick copper films.

Efficient measurement of broadband terahertz optical activity

We report a method to determine the four Stokes parameters of each spectral component in a broadband terahertz (THz) pulse by using a continuously rotating analyzer and a standard THz time domain spectroscopy (THz-TDS) instrument. A complete characterization of the polarization state at each frequency is obtained through a single time-domain measurement. Our method requires no specialized THz emitters or detectors; it is, therefore, perfectly general and suitable for any existing THz-TDS apparatus.

Photocarriers dynamics in silicon wafer studied with optical-pump terahertz-probe spectroscopy

Optical pump-terahertz probe spectroscopy is employed to investigate the optical characteristics of silicon wafer. The wafer surface undergoes a phase transition from insulator to metal for terahertz wave with increasing pump fluence. The real part of the pump-induced conductivity shows strong frequency dependence, which can be well described with Drude–Smith model. Our results also demonstrate that the photoexcited Si layer acts as a broadband terahertz pulse antireflection coating with proper pump fluence. In addition, it is observed that the terahertz pulse apparently arrives at the detector earlier when silicon is optically excited.

The THz Radiation Source at the SPARC Facility

The interest for Terahertz (THz) radiation is rapidly growing, both as it is a powerful tool for investigating the behavior of matter at low energy, and as it allows for a number of possible spectroscopic applications spanning from medical science to security. The linac-driven THz source at the SPARC facility can deliver broadband THz pulses with femtosecond shaping and can be used for electron beam diagnostics to fully reconstruct the longitudinal charge distribution. Beyond this application, the possibility to store much more energy in a single THz pulse than table-top sources renders the SPARC THz source very interesting for a spectroscopic use. In addition, taking advantage from electron beam manipulation techniques, high power, narrow-band THz radiation can be also generated. Those source characteristics provide a unique chance to realize THz-pump/THz-probe spectroscopy, a technique practically unexplored up to now.

Terahertz probe for spectroscopy of sub-wavelength objects

A system of two probes is designed for terahertz (THz) time-domain spectroscopy of sub-wavelength size objects. A twin-needle probe confines broadband THz pulses spatially by means of surface plasmon waves to a sub-wavelength spot smaller than 10 microns. The confined pulses are detected within the near-field zone of the twin-needle probe by a sub-wavelength aperture probe. The system allows THz spectroscopy to be applied to single micrometer-size objects in the 1-2.5THz region.

Surface Plasmon Resonant THz Wave Transmission on Carbon Nanotube Film

The properties of the terahertz resonant surface plasmons wave on the carbon nanotube film and dielectric interface have been investigated. As a first step towards engineering terahertz SPPs-like surface modes, we present a computer experiment to demonstrate that the carbon nanotube film surface can also be employed to concentrate and guide the terahertz SPPs wave. The carbon nanotube film is modeled in an experimentally realizable geometry. It is shown that a unique electromagnetic surface mode in terahertz region can be supported along the carbon nanotube film/dielectric interface when the free-space broadband terahertz pulse is incident on the carbon nanotube film with subwavelength gratings. Comparing with noble metals, plasmonic nano-structure materials based on carbon nanotube film offer a potentially more versatile approach to engineering tightly confined surface modes in the THz regime.

Scalable Microstructured Photoconductive Terahertz Emitters

The development of scalable emitters for pulsed broadband terahertz (THz) radiation is reviewed. Their large active area in the 1 – 100 mm2 range allows for using the full power of state-of-the-art femtosecond lasers for excitation of charge carriers. Large fields for acceleration of the photogenerated carriers are achieved at moderate voltages by interdigitated electrodes. This results in efficient emission of single-cycle THz waves. THz field amplitudes in the range of 300 V/cm and 17 kV/cm are reached for excitation with 10 nJ pulses from Ti:sapphire oscillators and for excitation with 5 μJ pulses from amplified lasers, respectively. The corresponding efficiencies for conversion of near-infrared to THz radiation are 2.5 × 10-4 (oscillator excitation) and 2 × 10-3 (amplifier excitation). In this article the principle of operation of scalable emitters is explained and different technical realizations are described. We demonstrate that the scalable concept provides freedom for designing optimized antenna patterns for different polarization modes. In particular emitters for linearly, radially and azimuthally polarized radiation are discussed. The success story of photoconductive THz emitters is closely linked to the development of mode-locked Ti:sapphire lasers. GaAs is an ideal photoconductive material for THz emitters excited with Ti:sapphire lasers, which are widely used in research laboratories. For many applications, especially in industrial environments, however, fiber-based lasers are strongly preferred due to their lower cost, compactness and extremely stable operation. Designing photoconductive emitters on InGaAs materials, which have a low enough energy gap for excitation with fiber lasers, is challenging due to the electrical properties of the materials. We discuss why the challenges are even larger for microstructured THz emitters as compared to conventional photoconductive antennas and present first results of emitters suitable for excitation with ytterbium-based fiber lasers. Furthermore an alternative concept, namely the lateral photo-Dember emitter, is presented. Due to the strong THz output scalable emitters are well suited for THz systems with fast data acquisition. Here the application of scalable emitters in THz spectrometers without mechanical delay stages, providing THz spectra with 1 GHz spectral resolution and a signal-to-noise ratio of 37 dB within 1 s, is presented. Finally a few highlight experiments with radiation from scalable THz emitters are reviewed. This includes a brief discussion of near-field microscopy experiments as well as an overview over gain studies of quantum-cascade lasers.

Probing structure and phase-transitions in molecular crystals by terahertz time-domain spectroscopy

Abstract Since the introduction of ultra-fast laser techniques for the generation and detection of broadband terahertz pulses, terahertz time-domain spectroscopy has become a versatile tool for vibrational spectroscopy of molecular systems in the far-infrared. Due to their highly collective and delocalized character vibrational modes in this part of the spectrum are highly sensitive to molecular structure and arrangement within a molecular crystal. Here we utilize this sensitivity to differentiate between the enantiopure amino acid l -cysteine and its racemic crystalline dl -form. Using terahertz time-domain spectroscopy we are able to observe temperature induced solid-state phase transitions in polycrystalline dl -cysteine, as well as in polycrystalline benzoic acid. The dynamics of the transitions is studied by tracing the temperature dependency of spectral features that are assigned to certain conformational phases.

Half Cycle Terahertz Pulse Generation by Prism-Coupled Cherenkov Phase-Matching Method

Nonlinear optical terahertz wave generation is a promising method for realizing a practical source with wide frequency range and high peak power. Unfortunately, many nonlinear crystals have a strong absorption in the terahertz frequency region. This limits efficient and widely tunable terahertz wave generation. The Cherenkov phase-matching method is one of the most promising techniques for overcoming these problems. We propose a prism-coupled Cherenkov phase-matching method, in which a prism with a suitable refractive index at terahertz frequencies is coupled to a nonlinear crystal. We demonstrate prism-coupled Cherenkov phase-matching terahertz generation using the DAST and LiNbO3 crystals. With a DAST crystal, we obtain a spectral flat tunability up to 10 THz by difference frequency generation. With a LiNbO3 crystal, we observe a spectral flat broadband terahertz pulse generation up to 5 THz pumped by a femto second fiber laser. The obtained temporal waveform is an ideal half cycle pulse suitable for reflection terahertz tomography.