Average Aerosol Optical Depth Values Research Articles

Analysis of characteristics and changes in three-dimensional spatial and temporal distribution of aerosol types in Central Asia

Atmospheric aerosol types and characteristics have regional and seasonal characteristics mainly due spatial and temporal differences in emission sources and diffuse transport conditions. We explored regional three-dimensional spatial and temporal distribution characteristics of aerosol types in Central Asia from daytime to nighttime by using long-term (2007–2021) CALIPSO lidar measurements. The three results are as follows: (1) Average aerosol optical depth (AOD) values during the 14 years were 0.44 and 0.47 during daytime and nighttime, respectively, with an overall decreasing trend, among which the AOD in spring in the southern border region and in winter in the northern border region showed high values, 0.66 and 0.31 during daytime and 0.69 and 0.33 during nighttime, respectively, and nighttime AOD values were higher than those of daytime, possibly due to the lower signal-to-noise ratio of the CALIPSO during the daytime than during the nighttime. (2) The primary representative aerosol type in the Taklamakan Desert region being pure sand and dust, and more apparent winter-polluted sand and dust exist along the northern slope of the Tianshan Mountains in Xinjiang in winter than in other areas. High-altitude soot mainly existed below 4 km and was primarily concentrated in northern Central Asia, with the highest values (0.016 and 0.003) in summer and winter, respectively, which may be due to different diffusion and transport conditions. (3) Dust aerosols in spring were mainly concentrated in the region of 2–6 km in the Taklamakan Desert area; pure dust particles in summer and fall lifted height diffusion and gradually moved to the northern border region; polluted dust was mainly in northern Xinjiang in fall and winter and spread to northern Central Asia; and the average top height of aerosols in the transmission process reached the top of the troposphere, and transmission height was higher than source area.

Propagation of NO2 originated in intense fires in the Paraná River Delta analyzed from satellite observations

Wildfires in the Paraná River Delta started to be a common situation in the year 2008 and during the first years of the 2020́s decade: 2020, 2021, 2022. These fires affected natural areas, primarily the islands within the delta, situated in front of Rosario city (32.95 °S, 60.67 °W, 25 meters above sea level (m.a.s.l.)), Argentina. They mostly occur during the period between June and September each year and are more intense when a strong La Niña event is present. The aim of this study is to examine the association between the propagation of high intensity nitrogen dioxide (NO2) plumes and the significant fire events that occurred in the Paraná River Delta from 6 to 17 September 2022. Satellite data of NO2 obtained from the TROPOspheric Monitoring Instrument (TROPOMI) on board the European Space Agency (ESA) Sentinel-5 Precursor satellite, air mass forward trajectories performed with The Hybrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT), Fire Radiative Power (FRP) data provided by Visible Infrared Imaging Radiometer Suite (VIIRS) on board The National Oceanic and Atmospheric Administration - 20 (NOAA-20) and Suomi National Polar-orbiting Partnership (S-NPP) satellites, Aerosol Optical Depth (AOD) from VIIRS S-NPP and Smoke Injection Height from Multi-Angle Implementation of Atmospheric Correction (MAIAC) Thermal Technique were employed. The trajectories followed by the air masses coming from the major fire sources locations nearby Rosario city and its surrounding area, were analyzed at altitudes of 20, 500, 1000, 1500 and 2000 m above ground level (AGL) in order to evaluate the impact of the NO2 clouds present in the atmosphere and carried by the winds, at different sites of Rosario and its adjacent region. The NO2 plumes has the potential to pose a significant health risk for this region, inhabited by an approximate population of one and a half million individuals. This risk is contingent upon the altitude where the highest levels of NO2 in the tropospheric column are found. Tropospheric vertical column densities (VCDs) of NO2 in the range of 4.68×1014 to 1.66×1016 molecules/cm2 were determined. The results indicate a robust correlation between elevated tropospheric NO2 VCD values and intense fires, as characterized by their FRP. Additionally, high tropospheric NO2 VCDs were observed to impact cities and towns located in close proximity to the fires. In particular, the unusually high tropospheric NO2 VCDs determined for the towns of Fighiera and Pueblo Esther, situated along the coast and near the Paraná River Delta, are noteworthy. This is uncommon considering they are small towns in rural areas that typically have good air quality. The results regarding FRP, provided by VIIRS on board NOAA-20 and S-NPP satellites, indicate that the fire characterization of hotspots during the considered period had a mean value in the range of 20.17-21.47 MW. On specific days (12, 13 and 16 September 2022), the cumulative (total) daily values were very high, ranging from 2000 to 10000 MW. Furthermore, on 12 and 13 September 2022, the smoke aerosols did not reach significant altitudes in the atmosphere, remaining within the range of 0 to 1500 m AGL. During the fire period, AOD values close to 1 were observed within the fire plume. Notably, Puerto San Martín (0.27), San Lorenzo (0.22), and Ibarlucea (0.20) recorded higher average AOD values compared to other sites. The remaining sites generally exhibited lower average AOD values, with a slight distinction between rural locations (Pueblo Esther: 0.14 and Fighiera: 0.14) and the city center of Rosario (0.09).

City-Scale Aerosol Loading Changes in the Sichuan Basin from 2001 to 2020 as Revealed by MODIS 1 km Aerosol Product

Long-term high-resolution monitoring of aerosol optical depth (AOD) is necessary to understand air pollution problems and climate change at regional to urban scales. Based on the 1 km AOD dataset retrieved by the MODIS Multi-Angle Implementation of Atmospheric Correction algorithm (MAIAC), the spatial-temporal evolutionary trends of AOD in the Sichuan Basin (SCB), Southwest China, and its 17 subordinate cities were analyzed from 2001 to 2020. In the past 20 years, the annual average AOD in SCB gradually decreased from south to north. The highest AOD of SCB in spring was 0.62, followed by an average AOD value of 0.60 in winter. At the city scale, Zigong, Neijiang, and Ziyang were identified as the three most polluted cities within the SCB. The average AOD in the SCB increased to 0.68 and 0.69 in February and March, respectively, and significantly decreased to 0.41 and 0.43 in June and July, respectively. The interannual AOD in the SCB presented an increasing trend from 2001 to 2010, with a range of 0.50 to 0.70, whereas it showed a decreasing trend from 2011 to 2020, with a range of 0.68 to 0.35. In spring, the annual average AOD at the district level showed significant high values from 2005 to 2012. In winter, the interannual AOD increased significantly, with high values concentrated in 2008, 2010, 2011, and 2013. The occurrence frequency of AOD in the SCB was mainly distributed between 0.2~0.5 and 1.5. There also was an increasing trend of AOD in the SCB from 2001 to 2008 and a decreasing trend from 2009 to 2020. The results of this study hold significance for further understanding the climatic characteristics and environmental effects of regional atmospheric aerosols.

HOTSPOT ANALYSIS AND COMPARISON BETWEEN SATELLITE-DERIVED AEROSOL OPTICAL DEPTH AND GROUND-BASED PARTICULATE MATTER MEASUREMENTS IN METRO MANILA

Abstract. Highly urbanized regions such as the Metro Manila area in the Philippines contribute to the deterioration of air quality through overpopulation, excessive vehicle emissions, and industrialization. However, the limited number of ground monitoring stations hinders the detailed estimation of the region’s overall air quality. Satellite-derived air pollutant concentrations have been used in several research studies as a substitute or supplementary to ground-based data due to their extensive spatial and temporal coverage. Using the aerosol optical depth (AOD) from the MODIS Multi-Angle Implementation of Atmospheric Correction (MAIAC) algorithm and ground measurements of coarse particulate matter (PM10), this study explores the comparison between satellite-derived and ground-based air pollutant concentrations measured from 2017 to 2020 through trend analysis of monthly average values per city. With 16 stations located in different cities, the monthly average values of AOD vs PM10 showed inconsistent results due to significant gaps in the ground data. Through optimized hotspot analysis, it was found that 7.24% of the Metro Manila region are considered hotspots using the MAIAC AOD values from 2017 to 2019 (pre-pandemic). From 2018 to 2020 (pandemic), 23.86% of Metro Manila are counted as hotspots. The AOD derived from satellite imagery and hotspot analysis can be used for future studies that focus on the development of models to predict ground pollutant values and the designation of non-attainment areas.

Aerosol Optical Depth Spatial and Temporal Variability Using Satellite Data Over Indian Major Cities

Introduction: The study’s main aim is to investigate the long-term variation of Aerosol Optical Depth (AOD). It also aims to show the relationship between meteorological parameters. This study evaluates long-term (2010 to 2021) special and temporal changes over major Indian regions using satellite-based data from NASA’s Terra Satellite.
 Materials and Methods: This study was carried out during 2010-2021 using MODIS data for long-term analysis. Variation of AOD with meteorological parameters was also performed to show the impact of these parameters (Temperature and Relative Humidity) on AOD by the MERRA-II model.
 Results: Based on Terra AOD data, in all the studied regions, especially the eastern region (Kolkata), the mean AOD was high (0.9-1.2). In the western region (Mumbai, Ahmedabad, and Surat), the mean AOD was low to moderate during all seasons. Furthermore, the impact of meteorological parameters on AOD shows significant variation in average annual AOD in Kolkata (0.70 ± 0.09), while other regions reported lower than average AOD values during the study period. Mumbai and Surat had average AODs (0.44 ± 0.13), (0.45 ± 0.14), while Ahmedabad and Jaipur reported average AOD of 0.45 ± 0.14 and 0.23 ± 0.11 during the study period, respectively.
 Conclusion: Generally, AOD values vary from season to season due to aerosol’s optical and microphysical properties being affected by meteorological conditions and surface albedo. This study examined the spatial and temporal distribution of AOD over five major Indian cities.

Spatiotemporal Variation and Influencing Factors of AOD in the North China Plain

A better knowledge of the spatial and temporal variation in atmospheric aerosol and its influencing factors is of great significance to controlling atmospheric pollution and improving the atmospheric environment. First, the visible infrared imaging radiometer suite (VIIRS) intermediate product (IP) aerosol optical depth (AOD) data from 2013 to 2019 were used to analyze the temporal and spatial variation in AOD in the North China Plain. Secondly, SO2, NO2, PM2.5, meteorological data, NDVI, DEM, GDP, and POPU were selected as influencing factors, and the linkage models between AOD and its influencing factors were established based on the XGBoost model for each of the five representative cities in the North China Plain to quantitatively estimate and reveal the contribution of various influencing factors behind the temporal and spatial distribution in AOD. The results showed that in terms of spatial distribution, the AOD of the North China Plain was bounded by the Taihang Mountains, showing a pattern of high AOD in the southeast and low AOD in the northwest. In terms of temporal changes, the annual average value of AOD in the five cities showed an overall decreasing trend, and the monthly average value of AOD first increased and then decreased, with the highest value appearing in July and the lowest value in December. In addition, the AOD estimation model established in this paper for the five cities in North China had high accuracy, with R2 ranging from 0.60 to 0.67. Among the factors influencing AOD in the North China Plain, NO2 and SO2 were the most influential factors contributing to AOD in the five cities. In addition, PM2.5 was another important pollutant emission factor. In terms of meteorological factors, temperature (T), relative humidity (RH), wind speed (WS), and wind direction (WD) were the other four important influencing factors. There were both commonalities and differences in the rankings of the contribution and importance of AOD influencing factors in the five representative cities in North China.

Wildfire smoke injection heights in China based on multi-angle imaging spectroradiometer (MISR) observations

Smoke injection height is a key driving factor for plume transport, which determines the lifetime of smoke aerosol in the atmosphere, transport path and diffusion along with the wind, and impacts on atmospheric environment. In this study, raw data obtained from the latest multi-angle imaging spectroradiometer (MISR) plume height project was extracted and analzyed. The variation of smoke injection heights of wildfire in China was investigated with statistical analysis methods. The effects of fire characteristics (combustion biomass type and fire radiative power) on the smoke injection height were explored. Meanwhile, the influence of smoke injection heights on the atmospheric environment was discussed based on the proportion of higher injection height plumes and the value of smoke aerosol optical depth (AOD). The results showed that smoke injection heights from wildfire ranged from 345 to 7719 m, with 57.1% of which ranging from 500 to 1000 m. Except for an abnormally high value of smoke injection height from a large grassland fire, the rest of smoke injection heights were lower than 3000 m. The biomass type for combustion was an important factor affecting smoke injection heights. The injection heights of the plume caused by forest fire were the highest and had the greatest variability. Smoke injection heights increased with the fire radiation power, but with obvious dispersion (R2=0.19). By setting a simple threshold, the proportion of higher injection plumes which might cause long-distance transportation of air pollutants in China was 10.5%. Combined with the analysis of smoke AOD, it was found that the average smoke injection height from cropland burning was the lowest, but their smoke caused the highest regional air pollution. In contrast, although forest fires could produce the highest smoke injection height, their smoke had a lower average value of AOD, which indicated a relatively weak impact of forest fires on regional air quality.

Using Lidar and Historical Similar Meteorological Fields to Evaluate the Impact of Anthropogenic Control on Dust Weather During COVID-19

Asian dust can be transported at least one full circuit around the globe. During the transportation, dust can interact with local air-borne dust and pollutants, and has a profound impact on the environment. A novel coronavirus (COVID-19) has been affecting human activities worldwide since early 2020. The Chinese government has implemented emergency control measures. Since April 2020, control measures to reduce anthropogenic emissions have been gradually reduced. The optical properties of aerosols during the dust transport were affected by meteorological conditions, local environmental conditions and human activities. Therefore, two dust weather processes in March 2018 and March 2020 were screened under similar meteorological fields and transportation paths, which were mainly affected by human activities. Based on lidar data, in East China, compared with 2018, the average aerosol optical depth (AOD) of all types of aerosols at 0–4 km in 2020 decreased by 55.48%, while the AOD of dust aerosols decreased by 43.59%. The average particle depolarization ratio and color ratio decreased by 40.33 and 10.56% respectively. Due to the reduction of anthropogenic emissions in China (detected by lidar), the concentration of surface PM2.5 decreased by 57.47%. This indicated that due to the decrease in human activities caused by COVID-19 control measures, the optical properties of aerosols were significantly reduced during dust weather process in eastern China. However, in the Pacific region, compared with 2018, the AOD values of 0–1 km layer and 1–6 km layer in 2020 increased by 56.4% and decreased by 29.2% respectively. The difference between the two contributions of dust aerosols was very small. Meanwhile, compared with 2018, China’s near surface pollutants decreased significantly in 2020, indicating that the near surface AOD of the Pacific in 2020 was mainly contributed by local pollutants. This study was of great significance to the study of long-range and cross regional transport of pollutants.

Spatio-temporal changes of AOD in Xinjiang of China from 2000 to 2019: Which factor is more influential, natural factor or human factor?

Aerosol optical depth (AOD), which represents the optical attenuation, poses a major threat to the production activity, air quality, human health and regional sustainable development of arid and semi-arid areas. To some degree, AOD shows areal air pollution level and possesses obvious spatio-temporal characteristics. However, long-time sequences and detailed AOD information can not be provided due to currently limited monitoring technology. In this paper, a daily AOD product, MODIS-based Multi-angle Implementation of Atmospheric Correction (MAIAC), is deployed to analyze the spatio-temporal characteristics in Xinjiang Uygur Autonomous Region from 2000 to 2019. In addition, the importance of influencing factors for AOD is calculated through Random Forest (RF) Model and the propagation trajectories of pollutants are simulated through Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) Model. Spatio distribution of AOD presents a tendency that AOD value in northern Xinjiang is low while the value in southern Xinjiang is high. Regions with high AOD values are mainly concentrated in Tarim Basin. AOD in southern Xinjiang is the highest, followed by that in eastern Xinjiang and AOD value in northern Xinjiang is the lowest. Seasonal variation of AOD is significant: Spring (0.309) > summer (0.200) > autumn (0.161) > winter (0.158). Average AOD value in Xinjiang is 0.196. AOD appears wavy from 2000 to 2014 with its low inflection point (0.157) appearing in 2005, and then increases, reaching its peak in 2014 (0.223). The obvious downward tendency after 2014 shows that the use of coal to natural gas (NG) conversion project improves the conditions of local environment. According to RF Model, NG contributes most to AOD. HYSPLIT Model reveals that aerosol in southern Xinjiang is related to the short-distant carriage of dust aerosol from the Taklimakan Desert. Aerosol there can affect Inner Mongolia through long-distant transport. Blocked by the Tianshan Mountains, fine dust particles can not cross the Tianshan Mountains to become a factor contributing to AOD in northern Xinjiang.

Spatial and temporal variation of aerosol optical depths over six major cities in Bangladesh

The Aerosol Optical Depth (AOD) is a crucial parameter for assessing aerosol content and determining the level of air pollution. In this study, we represent almost seven years' aerosol optical behavioral patterns of six major cities in Bangladesh with emphasis on trends, seasonal variations, sources characterization, comparison between ground (AERONET) and satellite (MODIS Terra and Aqua) measurements, and relation with particulate matter (PM). High AOD values (>0.70) were obtained in most of the western parts of the country in all seasons. Decreasing patterns were observed from northwest to southeast. Average values of AOD for Dhaka, Chattagram, Rajshahi, Khulna, Barishal, and Sylhet were 0.71 ± 0.08, 0.50 ± 0.08, 0.78 ± 0.06, 0.72 ± 0.14, 0.64 ± 0.08, 0.60 ± 0.07 (Terra), and 0.59 ± 0.07, 0.48 ± 0.05, 0.69 ± 0.08, 0.64 ± 0.12, 0.56 ± 0.05, 0.56 ± 0.07 (Aqua), respectively. AERONET AODs at 870, 500, and 340 nm, and Ångström Exponent (AE440–870) values for Dhaka city were 0.40, 0.78, 1.06, and 1.18, respectively. Mean Absolute Error (MAE), Root Mean Square Error (RMSE), and Correlation coefficient (r) values were 0.23, 0.30, 0.64 (Terra) and 0.12, 0.29, 0.76 (Aqua), respectively. Both PM2.5 and PM10 were well correlated with all AODs but weakly correlated with AE. AODs, AE, and PM were negatively associated with meteorological variables such as rainfall, relative humidity, wind speed, and temperature. Anthropogenic and biomass burning aerosols were dominated in all four seasons, but dust and mixed type aerosols were only dominated in pre-monsoon and monsoon seasons. This research would help researchers further know the nature of atmospheric aerosols and how they affect seasonal patterns.

Spatiotemporal Distribution of Aerosol Optical Depth Based on Landsat Data in the Hinterland of the Guanzhong Basin and Its Relationship with Urbanization

Aerosol optical depth (AOD) is one of the most fundamental optical properties of aerosols that characterizes the attenuation of light by aerosols and is an indicator of regional air pollution. Based on the blue band surface reflectance database from the MOD09A1 products for the period 2000-2019 and the ASTER spectral database, AOD was estimated from Landsat TM/OLI data using the deep blue algorithm (DB). Multi-year average/annual average and seasonal AOD values for the period 2000-2019 were then calculated to analyze the spatial characteristics and temporal variations of AOD using the empirical orthogonal function method (EOF). Furthermore, the impacts of urbanization on the spatio-temporal distribution of AOD were analyzed. The obtained results are summarized as follows:① The multi-year average AOD spatial distribution in the hinterland of the Guanzhong Basin was significantly affected by topography and human activities, with higher AOD values and variationsin areas of low altitude and high-intensity human activities compared to the surrounding mountains. Thus, changes in AOD in the study area are mainly affected by anthropogenic factors. AOD also showed significant seasonal variations, whereby spring (0.34) > summer (0.33) > autumn (0.23) > winter (0.12), and the largest regional differences occurred in summer; ② The annual average AOD (from 2000-2019) showed the trend of "increase-decrease-increase", and reached a maximum in 2005, with the high AOD area gradually moving to the south. The distribution of AOD values in spring and summer was relatively discrete, while it is in a low-value agglomeration state in winter; ③ Three main AOD spatial distribution modes were identified based on the EOF, which had cumulative contribution rate of 83.0%. The spatial distribution trend of AOD showed regional consistency, with feature vectors consistent with the altitude, thus reflecting the difference of AOD at different altitudes. Taking the Qinling Mountains as the dividing line, the AOD presented the "north-south" pattern, AOD showed a "north-south" pattern, reflecting the uniqueness of the regional development in the Guanzhong Basin compared to the southern Qinling Mountains. The "southeast-northwest" distribution pattern indicated that the AOD presented a reverse change trend between urban and non-urban; and ④ The results of correlation analysis between the AOD and urbanization revealed a positive correlation with permanent population density (R2=0.707, P<0.05), impervious surface density (R2=0.377, P<0.05), and industrial POI density (R2=0.727, P<0.5). These results are significant for improving the monitoring of air quality in the Guanzhong Basin and for the construction of an urban ecological environment.

SNOW ALBEDO REDUCTION IN CENTRAL ANDES BY ATMOSPHERIC AEROSOLS: CASE STUDY ON THE TUNUYÁN BASIN (ARGENTINA)

Abstract. Changes in snow albedo (SA) on several basins of the central Andes of Argentina are associated with the possible deposition of light-absorbing particles (LAP) in the austral spring. To demonstrate this possibility, we correlate SA with daily data of snow cover (SC), aerosol optical depth (AOD) and land surface temperature (LST) available from the Moderate-Resolution Imaging Spectroradiometer (MODIS) on board NASA Terra satellite during 2000–2016, and other derived parameters such as days after albedo (DAS) and snow precipitation (SP) from the Tropical Rainfall Measuring Mission (TRMM). We used satellite pixels with 100% snow cover to obtain monthly average value of SA, LST, AOD, DAS and SP performing multiple regression analysis. Further, we analysed biomass burning emissions in northern Argentina using MODIS products MCD64 collection C6 as possible source for snow pollution. Aerosol deposition and trajectories were analysed using WRF-Chem atmospheric numerical prediction model, with inventories of regional anthropogenic emissions of own elaboration (lat. 0.025° × long. 0.025°) and the estimation of open burning emissions from the FINN global inventory (Fire INventory from NCAR).

Comparison of MODIS- and CALIPSO-Derived Temporal Aerosol Optical Depth over Yellow River Basin (China) from 2007 to 2015

In this study, Collection 6.1 (C6.1) of different aerosol optical depth (AOD) products of different spatial resolutions were used from the aqua moderate resolution imaging spectroradiometer (MODIS) including dark target (DT), deep blue (DB), deep blue (DB), and DT-DB (DTB). These products were compared with cloud-aerosol lidar, and infrared pathfinder satellite observation (CALIPSO) AOD retrievals over the Yellow River Basin (YERB), China from 2003 to 2017. The YERB was divided into three sub-regions, namely YERB1 (the mountainous terrain in the upper reaches of the YERB), YERB2 (the Loess Plateau region in the middle reaches of the YERB), and YERB3 (the plain region downstream of the YERB). Errors and agreement between MODIS and CALIPSO data were reported using Pearson’s correlation (R) and relative mean bias (RMB). Results showed that the CALIPSO whole layers AOD (AODS) were better matched with MODIS AOD than the CALIPSO lowest layer AOD (AOD1). The time series of AOD shows higher values in spring and summer, and a small difference in AOD products was observed in autumn. The overall average value of CALIPSO AOD and MODIS AOD both fitted the order: YERB3 > YERB2 > YERB1. The CALIPSO AOD retrievals have the best consistency with the DTB10K and the lowest consistency with DT3K. Overall, the regional distributions of the CALIPSO AOD and MODIS AOD are significantly different over the YERB, and the difference is closely related to the season, region, and topography. This study can help researchers understand the difference of aerosol temporal and spatial distribution utilizing different satellite products over YERB, and also can provide data and technical support for the government in atmospheric environmental governance over YERB.

Seasonal variation in particle contribution and aerosol types in Shanghai based on satellite data from MODIS and CALIOP

Although the concentration of atmospheric particulate matter in Shanghai has declined in recent years, aerosols remain one of the major pollutants affecting air quality. Herein, spatio-seasonal variation in aerosol optical properties and aerosol types were studied over a 10-year period (2006–2015) in Shanghai, China, using satellite data from Moderate Resolution Imaging Spectroradiometer (MODIS) and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The average aerosol optical depth values for central urban and suburban areas of Shanghai were between 0.9 and 1.0. Clear seasonal variation in aerosol concentrations occurred, causing strongest attenuation in summer and weakest attenuation in autumn. Polluted dust, polluted continental (urban/industrial) and smoke aerosols were the main aerosol types. Desert dust aerosols occurred in the Shanghai area at higher altitudes (greater than 3 km) in spring, related to dusty weather in the north; while in winter, smoke aerosols occurred at high altitudes, related to haze pollution in the north. The aerosols detected in autumn were mainly from local sources, comprising polluted dust, polluted continental, and smoke aerosols. Aerosols in Shanghai clearly reflect both local and regional sources at different times.

Assessment of absorbing aerosols on austral spring snow albedo reduction by several basins in the Central Andes of Chile from daily satellite observations (2000–2016) and a case study with the WRF-Chem model

Changes in snow albedo (SA) on the Limari, Choapa, Aconcagua and Maipo basins of the Central Andes of Chile (CAC) are associated with the possible deposition of light-absorbing particles in the austral spring. We correlate SA with daily data of snow cover, aerosol optical depth (AOD) and land surface temperature (LST) available from the Moderate Resolution Imaging Spectroradiometer (MODIS) onboard the NASA Terra satellite between 2000 and 2016, and other derived parameters such as days after albedo (DAS) and snow precipitation (SP). We used satellite pixels with 100% snow cover to obtain monthly average value of SA, LST, AOD, DAS and SP from September to November performing multiple regression analysis. We show that in Maipo, after considering LST, AOD represents an important role in changes induced to SA. The multiple regression model illustrates that AOD increases can reduce the SA during spring months by 13.59, 0.01, 0.77 and 3.8% in Limari, Choapa, Aconcagua and Maipo, respectively. In addition, we used a numerical prediction Weather Research and Forecasting model coupled with Chemistry (WRF-Chem), showing that the black carbon distribution and average daily AOD are associated with the SA decrease of 0.15 in the Maipo basin between September 29 and 30, 2016. The WRF-Chem output showed aerosols are transported mainly with dominating westerly winds to the Limari and Maipo basins. Our results further suggest that SA decrease due to AOD may be originated in the largest industrial and urban areas in Chile, producing a negative impact on the hydrological resource, generated in the CAC.

Aerosol optical depth climatology over Central Asian countries based on Aqua-MODIS Collection 6.1 data: Aerosol variations and sources

The aim of this study is to explore the aerosol optical depth (AOD) – an indicator of air quality, based on satellite data over Central Asia. Due to limited studies and lack of knowledge regarding AOD variations over this region, five countries (Kazakhstan, Kyrgyzstan, Tajikistan, Turkmenistan, and Uzbekistan) and fifteen sites including the capital cities were selected for the analysis. Long-term Aqua-MODIS Collection 6.1 Deep Blue (DB) AOD observations at 10 km spatial resolution were obtained for 2002–2017 and the Ångström exponent (AE) was calculated using spectral AOD observations. AOD and AE were explored based on seasonal and inter-annual scale. The relationship between aerosol loading and economic indicator (gross domestic product) was also analyzed. Highest frequencies of low AOD and high AE were observed in all countries. Average AOD (AE) values during the study period were 0.17 ± 0.09 (1.29 ± 0.17) for Kazakhstan, 0.11 ± 0.13 (1.41 ± 0.13) for Kyrgyzstan, 0.17 ± 0.14 (1.36 ± 0.18) for Tajikistan, 0.20 ± 0.10 (1.10 ± 0.28) for Turkmenistan, and 0.18 ± 0.09 (1.18 ± 0.24) for Uzbekistan. Summer season experienced highest aerosol loading over Kazakhstan, Tajikistan, and Uzbekistan, whereas spring season experienced highest aerosol loading over Kyrgyzstan and Turkmenistan possibly due to the influence of less precipitation and dust from the arid regions. All fifteen cities selected in this study exhibited increasing aerosol load. Aerosol types based on the relationship between AOD and AE were investigated, results suggested the clean continental aerosol as a major aerosol type over the region, whereas the contribution of mixed aerosols was observed during spring and summer seasons. This study suggests for establishment of ground-based aerosol monitoring stations network and inclusions of modeling works to understand the complex nature of aerosol over this vast landmass.

Spatial analysis of aerosol optical depth obtained by air quality modelling and SEVIRI satellite observations over Portugal

The aim of this work is to explore the aerosol optical depth (AOD) data provided by different sources, namely satellite observations, air quality modelling and Aerosol Robotic Network (AERONET) observations, in order to improve characterisation of aerosol spatial distribution and to assess the contribution of the dust events on AOD over Portugal. Thus, the spatial and temporal variations of the AOD data were analysed for May 2011 taking into account the occurrence of mineral dust events. Satellite data obtained by Spinning Enhanced Visible and Infra-Red Imager (SEVIRI) instrument and air quality modelling results from the Comprehensive Air Quality Model (CAMx) over Portugal were explored. In this work, AOD values with a temporal resolution of 15 min were obtained from SEVIRI. Additionally, 3D data with 23 vertical layers for each aerosol constituent, size distribution and chemical composition were obtained from the modelling approach and used to compute the AOD at 550 nm by integrating of aerosol extinction coefficient (Qext) over the total atmospheric column. Despite the outbreaks of mineral dust occurring during this period, the overall contribution of organic carbon (OC), black carbon (BC) and sulphate (SO 4 ) compounds to the monthly average AOD values estimated by the model is very important achieving 95% mainly located in the northern part of the studied region. The model outputs and SEVIRI data were validated with AERONET observations presenting correlation coefficients of 0.71 and 0.68 respectively. Three different modes of aerosol were classified based on Ångström coefficient versus AOD and distinguishing between the dominance of fine and coarse aerosol fractions. The analysis implemented reveal that intercomparison of satellite observations with air quality modelling contribute to better understanding of the discrepancies presented in spatial pattern of AOD. • AOD data from satellite observations and air quality modelling were used. • Spatial and temporal variations of the AOD data were investigated. • Better correlation between modelling results and AERONET observations was obtained. • Satellite data and modelling results are in agreement but with different absolute values. • Analysis for observation points and for all domain provided different conclusions.

Observation of optical properties and sources of aerosols at Buddha's birthplace, Lumbini, Nepal: environmental implications.

For the first time, aerosol optical properties are measured over Lumbini, Nepal, with CIMEL sunphotometer of the Aerosol Robotic Network (AERONET) program. Lumbini is a sacred place as the birthplace of Lord Buddha, and thus a UNESCO world heritage site, located near the northern edge of the central Indo-Gangetic Plains (IGP) and before the Himalayan foothills (and Himalayas) to its north. Average aerosol optical depth (AOD) is found to be 0.64 ± 0.38 (0.06-3.28) over the sampling period (January 2013-December 2014), with the highest seasonal AOD during the post-monsoon season (0.72 ± 0.44). More than 80% of the daily averaged AOD values, during the monitoring period, are above 0.3, indicating polluted conditions in the region. The levels of aerosol load observed over Lumbini are comparable to those observed at several heavily polluted sites in the IGP. Based on the relationship between AOD and Ångstrom exponent (α), anthropogenic, biomass burning, and mixed aerosols are found to be the most prevalent aerosol types. The aerosol volume-size distribution is bi-modal during all four seasons with modes centered at 0.1-0.3 and 3-4μm. For both fine and coarse modes, the highest volumetric concentration of ~ 0.08μm-3μm-2 is observed during the post-monsoon and pre-monsoon seasons. As revealed by the single-scattering albedo (SSA), asymmetry parameter (AP), and refractive index (RI) analyses, aerosol loading over Lumbini is dominated by absorbing, urban-industrial, and biomass burning aerosols.

Generalization of Results of Atmospheric Aerosol Optical Depth Measurements on Spitsbergen Archipelago in 2011–2016

We discuss the results of spectral measurements of aerosol optical depth (AOD) of the atmosphere, carried out in warm periods of 2011–2016 in the Arctic settlement Barentsburg (Spitsbergen Archipelago). The statistical characteristics of seasonal and interannual variations in atmospheric AOD in the wavelength range of 0.34–2.14 μm are presented. The average AOD (0.5 μm) over the six-year period of observations had been 0.086, and, in particular, the fine mode AOD component had been 0.062 and the coarse mode AOD component had been 0.024. It is shown that the seasonal variations were best manifested in the decrease of modal (most probable) values of fine mode AOD component from 0.055 in spring to 0.025 in autumn. As compared to the preceding (pre-2011) period, we noted a closer convergence in the average AOD values between spring and summer, primarily due to a decrease in the content of fine mode aerosol in spring and its increase in summer. The summertime AOD growth is most likely due to episodic outflows of smoke aerosol from boreal zones of Eurasia and North America.

The aerosol optical properties and PM2.5 components over the world's largest industrial zone in Tangshan, North China

To achieve an in-depth understanding of the aerosol optical properties in the highly-industrial region of Tangshan, we provided systematic aerosol optical properties analysis in this largest industrial zone for the first time. The aerosol optical datasets (2013.05–2015.04) and chemical component data of PM2.5 (2014–2015) obtained from the Tangshan site of the campaign on atmospheric aerosol research (CARE-China) network were analyzed. The results showed that the Tangshan region was seriously affected by fine-mode industrial aerosols all year, which would promote the accumulation of pollutants and influence the atmospheric circulation through changing the vertical temperature gradient. The annual average aerosol optical depth (AOD) and Ångstrӧm exponent (α) were 0.80±0.26 and 1.05±0.10, respectively. The aerosol optical properties revealed significant seasonal characteristics. The maximum seasonal average AOD (1.03±0.62) and α (1.12±0.19) accompanied the highest seasonal secondary inorganic aerosol concentrations (SIA: SO42−,NO3−,NH4+), 53.33μg/m3, occurred in summer, and this phenomenon was attributed to the photochemical reactions favored by the high temperature and humidity. During the spring, frequent dust events led to the maximum Ca2+ concentration of 6.57μg/m3 and the lowest seasonal α of 0.98±0.31. Coal was used for generating heat in winter, resulting in the highest levels of pollutant emissions (Cl−, Elemental carbon (EC) and organic carbon (OC)). The aerosol type classifications showed that the industrial aerosols were the main controls in the summer and fall, representing 56%–58% of the total aerosols. While for spring and winter, mixed aerosols represented 53%–54% of the total aerosols. Hygroscopic growth effect of aerosols existed all year, which could enhance the negative radiative forcing and eventually cool the earth-atmosphere system. The classification Wing for Tangshan data showed high AOD values (>0.70) were mainly clustered in the fine-mode growth wing and coarse-mode. Of these values, summer showed a dense AOD distribution and the highest magnitude of fine-mode AODs, with a corresponding fine particle fraction of η~90% and an Rf ~0.20μm. In addition, spring showed the most coarse-mode aerosols.