Autler-Townes Research Articles

Use of the 5P3/2→6P3/2 electric dipole forbidden transition in Rb as a non-perturbing probe of atom dynamics in an operating magneto-optical trap

Abstract Results of spectroscopy experiments using the $5P_{3/2} \to 6P_{3/2}$ electric dipole forbidden transition in cold rubidium atoms are presented. Production of this forbidden transition is detected by observing the emission of the $420 $ nm fluorescence photons that result from the decay of the $6P_{3/2} $ state into the ground state. The experiments are performed under the steady state operation conditions of a magneto-optical trap (MOT), and thus provide non-perturbing information on the atom-light system. The hyperfine structure of the $6P_{3/2}$ level is completely resolved, and the fluorescence peaks show the expected Autler-Townes (AT) splitting of the emission lines. This hyperfine structure is used to calibrate the frequency scale of all spectra recorded. A combination of this absolute frequency scale and an expression for the AT profile allows an absolute determination of the effective Rabi frequency and detuning of the MOT. The behavior of these AT doublets is studied as a function of frequency detuning and also as a function of the trapping light intensity.
The experiments also take full advantage of the strong polarization dependence of the relative intensities of the hyperfine fluorescence components.
This study results in a sensitive probe of the relative populations of the magnetic sublevel projections relative to the trapping magnetic field gradient.
An almost isotropic population distribution was found, but small deviations from isotropy could be determined with this electric dipole forbidden probe.

Simultaneously measuring microwave electric fields at different frequencies by Rydberg-atom-based electrometry with Zeeman-resolved Autler–Townes splitting

We provide the simultaneous traceable measurements of microwave electric fields at two different frequencies by the electromagnetically induced transparency (EIT) and Autler–Townes (AT) splitting. A static magnetic field working together with a linearly polarized probe and coupling light prepares Rydberg atoms in Zeeman sublevels with maximal |mJ| in an atomic vapor cell. Using the EIT-AT splitting of these two maximal |mJ| states, the microwave electric fields at two different frequencies are simultaneously measured, in which their frequency difference can be adjustable within the linear range of magnetic field-induced level shifts. The proposed method provides a promising prospect for calibrating multiple microwave frequencies simultaneously in the future.

Utilizing quantum coherence in Cs Rydberg atoms for high-sensitivity room-temperature terahertz detection: a theoretical exploration

In recent years, terahertz (THz) technology has made significant progress in numerous applications; however, the highly sensitive, room-temperature THz detectors are still rare, which is one of the bottlenecks in THz research. In this paper, we proposed a room-temperature electrometry method for THz detection by laser spectroscopy of cesium (Cs133) Rydberg atoms, and conducted a comprehensive investigation of the five-level system involving electromagnetically induced transparency (EIT), electromagnetically induced absorption (EIA), and Autler–Townes (AT) splitting in Cs133 cascades. By solving the Lindblad master equation, we found that the influence of the THz electric field, probe laser, dressing laser, and Rydberg laser on the ground state atomic population as well as the coherence between the ground state and the Rydberg state, plays a crucial role in the transformation and amplitude of the EIT and EIA signals. Temperature and the atomic vapor cell’s dimensions affect the number of Cs133 atoms involved in the detection, and ultimately determine the sensitivity. We predicted the proposed quantum coherence THz detection method has a remarkable sensitivity of as low as 10−9 V m−1 Hz−1/2. This research offers a valuable theoretical basis for implementing and optimizing quantum coherence effects based on Rydberg atoms for THz wave detection with high sensitivity and room-temperature operation.

Dynamically enhanced Autler–Townes splitting by orthogonal XUV fields

Abstract Based on numerical solutions of the time-dependent Schrödinger equation, we theoretically investigate the photoelectron spectrum of hydrogen atoms ionized by a pair of ultrashort, intense, and orthogonally polarized laser pulses with a relative time delay in a pump–probe configuration. The pump pulse resonantly excites electrons from the 1s and 2p levels, inducing Rabi oscillations. The resulting dynamically enhanced Autler–Townes (AT) splitting is observed in the photoelectron energy spectrum upon interaction with the second probe pulse. In contrast to the previous parallel-polarization scheme, the proposed orthogonal-polarization configuration enables the resolution of dynamically enhanced AT splitting over a considerably wider range of probe photon energies.

Competition of multiphoton ionization pathways in lithium

We study the three-photon ionization of atomic lithium by intense, short light pulses, via numerically solving the time-dependent Schrödinger equation. Two-photon Rabi oscillations are induced between the 2s and 4s states, which are damped due to single-photon ionization to the p continuum. Developing a minimal three-level model, we analyze the spectral features of the Autler–Townes (AT) doublet that is formed upon the resonant coupling with the laser pulse. Furthermore, we show that this 2s→→4s→p continuum pathway is the dominant process, if the duration of the laser pulse exceeds a certain value. For shorter pulses, ionization through the 2p state ( 2s→2p→4d→f continuum ) gradually becomes the dominant process, provided that the pulse is strong enough to induce several Rabi floppings. Here, we trace the competition of these ionization pathways by observing the structural changes in the shape of the AT doublet.

Microwave electrometry with Rydberg atoms in a vapor cell using microwave amplitude modulation

We have theoretically and experimentally studied the dispersive signal of the Rydberg atomic electromagnetically-induced transparency (EIT) Autler–Townes (AT) splitting spectra obtained using amplitude modulation of the microwave (MW) electric field. In addition to the two zero-crossing points interval Δf zeros, the dispersion signal has two positive maxima with an interval defined as the shoulder interval Δf sho, which is theoretically expected to be used to measure a much weaker MW electric field. The relationship of the MW field strength E MW and Δf sho is experimentally studied at the MW frequencies of 31.6 GHz and 9.2 GHz respectively. The results show that Δf sho can be used to characterize the much weaker E MW than that of Δf zeros and the traditional EIT–AT splitting interval Δf m; the minimum E MW measured by Δf sho is about 30 times smaller than that by Δf m. As an example, the minimum E MW at 9.2 GHz that can be characterized by Δf sho is 0.056 mV/cm, which is the minimum value characterized by the frequency interval using a vapor cell without adding any auxiliary fields. The proposed method can improve the weak limit and sensitivity of E MW measured by the spectral frequency interval, which is important in the direct measurement of weak E MW.

Magnetic-field-induced splitting of Rydberg Electromagnetically Induced Transparency and Autler-Townes spectra in 87Rb vapor cell.

We theoretically and experimentally investigate the Rydberg electromagnetically induced transparency (EIT) and Autler-Townes (AT) splitting of 87Rb vapor under the combined influence of a magnetic field and a microwave field. In the presence of static magnetic field, the effect of the microwave field leads to the dressing and splitting of each mF state, resulting in multiple spectral peaks in the EIT-AT spectrum. A simplified analytical formula was developed to explain the EIT-AT spectrum in a static magnetic field, and the theoretical calculations agree qualitatively with experimental results. The Rydberg atom microwave electric field sensor performance was enhanced by making use of the splitting interval between the two maximum absolute mF states separated by the static magnetic field, which was attributed to the stronger Clebsch-Gordon coefficients between the extreme mF states and the frequency detuning of the microwave electric field under the static magnetic field. The traceable measurement limit of weak electric field by EIT-AT splitting method was extended by an order of magnitude, which is promising for precise microwave electric field measurement.

Extending bandwidth sensitivity of Rydberg-atom-based microwave electrometry using an auxiliary microwave field

We demonstrate the use of an auxiliary microwave field to extend the bandwidth sensitivity of Rydberg-atom-based microwave electrometry. Electromagnetically induced transparency (EIT) and Autler-Townes (AT) splitting in Rydberg atom microwave electrometry provide advantageous sensitivity for the resonant detection of microwave (MW) fields because the Stark shift of the target Rydberg state takes the linear form of AT splitting. However, the sensitivity is reduced by several orders of magnitude for detuned MW fields because the Stark shift of the target Rydberg state depends on a weak nonlinear effect. We show that the auxiliary microwave field with appropriate Rabi frequency or detuning could shift the atomic energy levels to bring a particular Rydberg-Rydberg transition of interest for microwave sensing into resonance with the target microwave field. Using the atomic superheterodyne method, we verified the general method that regulates Rydberg energy levels using an auxiliary microwave field. The experimental results of this study confirm that this technique works efficiently for detecting microwave fields detuned by up to 100 MHz from resonance with the field-free Rydberg-Rydberg transition used for sensing. The measurement sensitivity of the detuned target field is increased by a factor of 10 compared with that achieved without the application of the auxiliary dressing field.

Autler–Townes splitting in the trap-loss fluorescence spectroscopy due to single-step direct Rydberg excitation of cesium cold atomic ensemble

We experimentally investigate trap-loss spectra of the cesium 6S1/2(F = 4) → 71P3/2 Rydberg transition by combining the cesium atomic magneto-optical trap with the narrow-linewidth, continuously tunable 318.6 nm ultraviolet laser. Specifically, the atoms in the magneto-optical trap are excited to the Rydberg state due to the ultraviolet laser single-step Rydberg excitation, which leads to the reduction of atomic fluorescence. Based on the trap-loss spectroscopy technology, the Autler–Townes (AT) splitting due to a strong cooling laser is observed, and the parameter dependence of the AT splitting interval of trap-loss spectroscopy is investigated. The effective temperature of cold atoms is measured by using simplified time-of-flight fluorescence imaging. In addition, closed-loop feedback power stabilization of 318.6 nm ultraviolet laser is carried out. This lays the foundation for further experimental research related to the Rydberg atoms using ultraviolet lasers, which is of great significance for the development of quantum computing and quantum information.

Atomic mixer based on phase control without ac Zeeman shift

Atom-based mixers have been shown to be very useful in performing the absolute measurement of the magnitude of a radio-frequency (rf) field by using Autler-Townes (AT) splitting. However, there has been less success in measuring the phase of a rf field with the AT splitting in a magnetic-resonance system. The phase of the rf magnetic field plays a very important role in imaging applications. Here, we design an atomic mixer for measuring the phase of the rf field by detecting the transmission spectra of a laser-detected magnetic-resonance system based on the interference between Raman and cascade two-photon processes for ${F}_{g}=4$ of the ${D}_{1}$ line of cesium atoms. A scheme of measuring the rf phase can be realized with the elimination of the ac Zeeman shift of the system by adjusting the amplitude ratio of a transverse fundamental-wave field and its third-harmonic field. Theoretical and experimental results show that the scheme with cancellation of the ac Zeeman shift is superior in linear measurement of the longitudinal rf component. Our results provide schemes for a magnetic sensor based on quantum interference of nonlinear processes for the absolute measurement of the relative phase of rf fields.

Effect of nonresonant states in near-resonant two-photon ionization of hydrogen

By numerically solving the three-dimensional time-dependent Schr\"odinger equation, two-photon ionization of hydrogen is investigated at the near-resonant frequencies of the $1s\text{\ensuremath{-}}2p$ transition. Due to the Rabi oscillations between the $1s$ and $2p$ states, the photoelectron energy spectra exhibit the Autler-Townes (AT) doublets and we focus on the energy spacing and the asymmetry of the doublets. Our results show that the laser frequency for the minimum energy spacing of AT doublets locates at the resonant frequency of the ac-stark-shifted states, while the symmetry of the AT doublets is affected both by the ac-stark shift and the nonresonant ionization pathway. Developing the minimal three-state model including all of the nonresonant (nonessential) states, the effects of the ac-stark shift and the nonresonant ionization pathway on the AT doublets due to the nonresonant states are identified. Furthermore, due to the nonresonant ionization pathway, the photoelectron angular distributions are distinctly different for the lower- and higher-energy peaks in the AT doublets and these angular distributions sensitively depend on the laser intensity and pulse duration. These results are well reproduced by our minimal three-state model.

Discerning the transition from electromagnetically induced transparency to Autler–Townes splitting using the decaying dressed state formalism

We use biorthogonal basis consisting of the ‘right’ and ‘left’ eigenvectors of the effective non-Hermitian Hamiltonian of a three-level system driven by a bi-chromatic field, and resolve the probe absorption spectrum into components corresponding to the decaying dressed states of the system. It is observed that the spectrum primarily consists of three components and two of them undergo dramatic changes when the control field Rabi frequency is changed from the low to high field regime. Based on the symmetry properties of a combination of these components, a parameter internal to the dynamics of the system is defined and is used to distinguish between electromagnetically induced transparency (EIT) and Autler–Townes (AT) splitting, and the threshold for transition between them in an objective manner. The formulation is further extended to the resonance fluorescence spectrum on the probe transition in the EIT and AT regimes.

Sensitivity enhancement of far-detuned RF field sensing based on Rydberg atoms dressed by a near-resonant RF field.

Rydberg-atom electrometers promise traceable standards for RF electrometry by enabling stable and uniform measurement. In this Letter, we propose an approach to increase the sensitivity of the Rydberg-atom electrometer for far-detuned RF field sensing. The key physical mechanism is the addition of a new ingredient-a local RF field near-resonant with a Rydberg transition-so that the far-detuned field can be detected by the shift of an Autler-Townes (AT) splitting peak, which can be dozens of times larger than the AC Stark shift of the electromagnetic induced transparency (EIT) signal without the near-resonant field. The method enables us to measure far-detuned fields with higher sensitivities, including sub-GHz RF fields (even DC electric fields) which are rarely involved in the existing sensitivity enhancement methods.

Bright and dark Autler–Townes states in the atomic Rydberg multilevel spectroscopy

We investigated the Autler–Townes (AT) splitting produced by microwave (mw) transitions between atomic Rydberg states explored by optical spectroscopy from the ground electronic state. The laser-atom Hamiltonian describing the double irradiation of such a multilevel system is analysed on the basis of the Morris–Shore transformation. The application of this transformation to the mw-dressed atomic system allows the identification of bright, dark, and spectator states associated with different configurations of atomic states and mw polarisations. We derived synthetic spectra that show the main features of Rydberg spectroscopy. Complex AT spectra are obtained in a regime of strong mw dressing, where a hybridisation of the Rydberg fine structure states is produced by the driving.

Angular shift of Autler–Townes doublet from multi-photon ionization of molecules by circularly polarized laser pulses

We theoretically study the Autler–Townes (AT) splitting of a molecule in a circularly polarized laser pulse by solving the time-dependent Schrödinger equation. We find that the AT doublet in the photoelectron momentum distribution reveals different angular shifts with respect to the molecular axis direction. Using an improved strong-field approximation method, we reproduce the difference of the angular shifts for the AT doublet, which originates from the interference of the electron wave packets released from the ground and excited states of the molecule. By tracing the time evolution of the electron density distribution along the molecular axis, we find that electron delocalization on the two nuclei of the molecule plays a significant role in the formation of photoelectron angular distribution for the AT doublet, which corresponds to a phase jump of π for the phase difference between the ground and excited states.

Autler-Townes splitting of three-photon excitation of cesium cold Rydberg gases.

We demonstrate the three-photon Autler-Townes (AT) spectroscopy in a cold cesium Rydberg four-level atom by detecting the field ionized Rydberg population. The ground state |6S1/2〉, two intermediate states |6P3/2〉 and |7S1/2〉 and Rydberg state |60P3/2〉 form a cascade four-level atomic system. The three-photon AT spectra and AT splittings are characterized by the Rabi frequency Ω852 and Ω1470 and detuning δ852 of the coupling lasers. Due to the interaction of two coupling lasers with the atoms, the AT spectrum has three peaks denoted with the letters A, B and C. Positions of the peaks and relative AT splittings, γAB and γBC, strongly depend on two coupling lasers. The dependence of the AT splitting, γAB and γBC, on the coupling laser detuning, δ852, and Rabi frequency, Ω852 and Ω1470 are investigated. It is found that the AT splitting γAB mainly comes from the first photon coupling, whereas the γBC mainly comes from the second photon coupling with the atom. The three-photon AT spectra and relevant AT splittings are simulated with the four-level density matrix equation and show good agreement with the theoretical simulations considering the spectral line broadening. Our work is of great significance both for further understanding the interaction between the laser and the atom, and for the application of the Rydberg atom based field measurement.

The effect of the Doppler mismatch in microwave electrometry using Rydberg electromagnetically induced transparency and Autler–Townes splitting

We have systematically investigated the influence of the gas temperature (T), the Rabi frequencies of the probe laser (Ωp), the coupling laser (Ωc) and the radio-frequency (RF) (ΩRF) on the Rydberg electromagnetically induced transparency (EIT) and Autler–Townes (AT) splitting (Δf) by defining a general Doppler mismatch factor D g = ΩRF/Δf in the Rydberg atom-based microwave electrometry. The effect of T on D g is studied in detail from 0 to 1000 K, the results show that D g is insensitive to T when T < 10 μK or T > 10 K, while D g changes significantly with 10 K . Then the effects of Ωp, Ωc and ΩRF on factor D g at T = 300 K (typical room temperature) and T = 10 μK (typical temperature of cold atom by laser cooling) are studied in detail, respectively. The results show that the linewidth of Rydberg EIT (ΓEIT) can be used as a key parameter to characterize the dependence of D g on Ωp and Ωc in both cases. D g is insensitive to T, Ωp and Ωc when ΩRF > 3ΓEIT which means that ΓEIT determines the lower limit of the linear region of the RF electric field strength measured by EIT–AT splitting. More interesting, the range where D g is insensitive to Ωp and Ωc can be greatly expanded by lowering the gas temperature to 10 μK. The ranges of parameters where D g is insensitive to T, Ωp, Ωc and ΩRF are given, and such relationship can be easily scaled to other atomic systems. The results can help the selection of various parameters in the experiments and specific applications to ensure the accuracy of measuring the RF electric field.

Microwave two-photon spectroscopy of cesium Rydberg atoms

We present a two-photon microwave spectra of cesium Rydberg atoms in the room-temperature vapor cell. The three-level atom including a ground state 6S1/2 (F = 4), an excited state 6P3/2 (F′ = 5) and Rydberg state consists of Rydberg electromagnetically induced transparency (Rydberg-EIT), that is employed to detect the microwave two-photon spectra. The microwave field with frequency ν DD = 11.42865 GHz couples the transition of Rydberg energy level |68D5/2〉 → |69D5/2〉, measured two-photon spectra display a rich of information including the microwave ac Stark shifts and two-photon Autler-Townes (AT) splitting. In the strong microwave field, the two-photon spectroscopy shows the state mixture between |68D5/2〉 and |68D3/2〉 Stark lines. The microwave two-photon spectra of the |69S1/2〉 → |70S1/2〉 transition coupled with frequency ν SS = 11.73503 GHz are also presented. The Floquet theory is employed to simulate the two-photon microwave spectra, showing the good agreement with the measurements. The work suggests the new method that may be used to investigate the multi-photon field-atom interaction and as an atom-based technique for precision field measurements.

Pole analysis of EIT-AT spectrum with Rydberg atoms.

We investigate the electromagnetically induced transparency (EIT) and Autler Townes (AT) splitting spectrum with a four-level Rydberg atom by pole analysis of the probe coherence. A pair of poles corresponding to the two peaks of the spectral splitting is observed. The spectral split or the pole positions are affected by the microwave intensity (MW) and the detuning between the probe and the coupling laser. In the absence of any detuning, the two poles coincide and separate again on the imaginary axis of the complex detuning plane at weak MW field. The two poles do not coincide when the probe (coupling) laser is detuned for scanning the coupling (probe) laser frequency. However, under finite detuning, the two poles approach the nearest distance in the absence of any splitting and are separated again in the direction parallel to the imaginary axis. The spectral analysis of the poles provides an alternate way to establish the relationship between the splitting and the intensity of MW, which may play a role in the application of atomic-based MW measurements.

Continuous radio-frequency electric-field detection through adjacent Rydberg resonance tuning

We demonstrate the use of multiple atomic-level Rydberg-atom schemes for continuous frequency detection of radio-frequency (RF) fields. Resonant detection of RF fields by electromagnetically induced transparency and Autler-Townes (AT) splitting in Rydberg atoms is typically limited to frequencies within the narrow bandwidth of a Rydberg transition. By applying a second field resonant with an adjacent Rydberg transition, far-detuned fields can be detected through a two-photon resonance AT splitting. This two-photon AT splitting method is several orders of magnitude more sensitive than off-resonant detection using the Stark shift. We present the results of various experimental configurations and a theoretical analysis to illustrate the effectiveness of this multiple level scheme. These results show that this approach allows for the detection of frequencies in a continuous band between resonances with adjacent Rydberg states.