Attenuated Backscatter Coefficient Research Articles

Three-dimensional reconstruction of aerosols based on spectral radiance matching

This paper evaluates a three-dimensional scene construction algorithm that assigns CALIPSO-observed profiles to receiving pixels in MODIS imagery through spectral radiance matching (SRM), so that a limited number of vertically resolved aerosol observations can be expanded into a regionally continuous three-dimensional aerosol structure. The SRM algorithm was tested using moderate resolution imaging spectro-radiometer (MODIS) and cloud-aerosol lidar and infrared pathfinder satellite observation (CALIPSO) data for the period of April 10–25, 2015. First, the spectral radiance channel and the surface reflectance channel were selected for combination tests to select the best channel combination 01-04-07-26 for the application of SRM algorithm in the field of aerosol three-dimensional reconstruction. The average aerosol matching rate for this channel combination can reach 90.57%, 81.64%, 78.6%, 74.12%, and 65.96% at extended distances of 5, 20, 30, 50, and 100 km, respectively. In addition, the combination of the average correct match rate and the reconstructed aerosol structure revealed that the most suitable extension distance is up to 100 km. Then, for the reconstruction profile validation, lidar sites under four weather conditions (clean sky, aerosol loading, thin clouds, and thick clouds) were selected for validation. The comparison results reveal that the average relative errors are about 30%, 60%, 30%–60%, and 70% for these four conditions, respectively. Overall, the average relative error of the reconstructed profiles within 100 km of the orbital track of CALIPSO (except under thick cloud conditions) is less than 60%, which is within a reasonable error envelop. There are also some limitations that can be improved later by adding more constraints: 1) it is difficult to reconstruct some short-time, small-scale aerosol or cloud features; 2) it is difficult to reconstruct some hierarchical structures under thick clouds due to signal attenuation caused by thick clouds; 3) there is an underestimation of the attenuated backscatter coefficient under clouds. Finally, for aerosol optical depth (AOD), the SRM algorithm largely underestimates AOD. The reconstructed AOD is in good agreement with aerosol robotic network (AERONET), with R2=0.8231 after removal of outliers.

Validation of initial observation from the first spaceborne high-spectral-resolution lidar with a ground-based lidar network

Abstract. On 16 April 2022, China successfully launched the world's first spaceborne high-spectral-resolution lidar (HSRL), which is called the Aerosol and Carbon Detection Lidar (ACDL), on board the Atmospheric Environment Monitoring Satellite known as Daqi-1 (DQ-1). The ACDL is expected to precisely detect the three-dimensional distribution of aerosol and cloud globally with high spatial–temporal resolutions. To assess the performance of the newly launched satellite lidar, the ACDL-retrieved observations were compared with ground-based lidar measurements of atmospheric aerosol and cloud over northwest China from May to July 2022 using the Belt and Road lidar network (BR-lidarnet) initiated by Lanzhou University in China and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) lidar observations. A total of six cases in the daytime and nighttime, including clear days, dust events, and cloudy conditions, were selected for further analysis. Moreover, profiles of the total attenuated backscatter coefficient (TABC) and the volume depolarization ratio (VDR) at 532 nm measured by the ACDL, the CALIPSO lidar, and ground-based lidar are compared in detail. Comparison is made between the 532 nm extinction coefficient and lidar ratio obtained from ACDL HSRL retrieval and the Raman retrieval results obtained from BR-lidarnet. The achieved results revealed that the ACDL observations were in good agreement with the ground-based lidar measurements during dust events with a relative deviation of about −10.5 ± 25.4 % for the TABC and −6.0 ± 38.5 % for the VDR. Additionally, the heights of the cloud top and bottom from these two measurements were well matched and comparable. Compared with the observation of CALIPSO, the ACDL also shows high consistency. This study proves that the ACDL provides reliable observations of aerosol and cloud in the presence of various climatic conditions, which helps to further evaluate the impacts of aerosol on climate and the environment, as well as on the ecosystem in the future.

Challenges in Detecting Clouds in Polar Regions Using a Drone with Onboard Low-Cost Particle Counter

It is expected that uncrewed aerial vehicles (UAVs) will be used increasingly for operational atmospheric soundings to cover a broader area of the lower troposphere, including that in the polar regions and over the oceans. During the Japanese Antarctic Research Expedition of 2022/2023, 172 vertical profiles up to a maximum height of 1000 m a.s.l. were conducted from mid-December 2022 to mid-March 2023 using a commercially available inexpensive drone launched from the icebreaker RV Shirase. Over a quarter of the flights encountered clouds and snow, of which half produced icing on the body and blades of the drone. The onboard aerosol counter detected an increase in the particle number concentration in the cloud layers, which was synchronized with an increase in the attenuated backscatter coefficient of a shipboard lidar ceilometer. In the presence of icing, the concentration of particles >1.0μm exceeded 5000 particles L−1 as a median value, while the concentration was <1000 particles L−1 for cases without icing. Using an onboard aerosol counter and/or land-based ceilometer would be useful for detecting the icing environments.

Laser light propagation in a turbid medium: solution including multiple scattering effects

We have shown that solutions to the radiative transfer equation for a homogeneous slab yield a zenith radiance reflectance that for collimated beam incidence in the nadir direction can be expressed in terms of the lidar ratio, defined as the extinction coefficient divided by the 180^circ backscattering coefficient. The recently developed QlblC method, which allows one to quantify layer-by-layer contributions to radiances emerging from a slab illuminated with a collimated beam of radiation, was used to show explicitly that in the single-scattering approximation the attenuated backscatter coefficient estimated by the new QlblC method gives the same result as the lidar equation. Originally developed for the continuous wave (CW) lidar problem, we have extended the new QlblC method to apply to the pulsed lidar problem. A specific example is provided to illustrate the challenge encountered for ocean property retrievals from space observations due to the fact that a very significant fraction of the signal is due to aerosol scattering/absorption; typically only about 10% (or less) comes from the ocean.Graphical abstract

Computation of the Attenuated Backscattering Coefficient by the Backscattering Lidar Signal Simulator (BLISS) in the Framework of the CALIOP/CALIPSO Observations

This paper presents the Backscattering Lidar Signal Simulator (BLISS), an end-to-end lidar simulator developed by the Centre National d’Etudes Spatiales (CNES). We computed the constant multiple-scattering (MS) coefficient of BLISS with a Monte Carlo (MC) code in the framework of CALIOP/CALIPSO observations for different homogeneous and plane-parallel stratocumulus and cirrus cloud geophysical scenes. The MS coefficient varies from 0.46 to 0.63. Then we evaluated the Level 1 products of BLISS. Above and in-cloud relative difference between the attenuated backscattering coefficient vertical profile simulated by BLISS and by the MC code is smaller than 0.5% under single-scattering regime and smaller than 10% (30% if optical depth of cirrus is large) under multiple-scattering regime, thus confirming the robustness of BLISS.

Nearshore bathymetry and seafloor property studies from Space lidars: CALIPSO and ICESat-2.

In shallow nearshore waters, seafloor heights and properties can be accurately measured by the current generation of space-based elastic backscatter lidars: CALIOP, flying aboard the CALIPSO satellite and ATLAS aboard ICESat-2. CALIOP's 532 nm volume depolarization ratios, together with the ratios of the attenuated backscatter coefficients measured at 532 nm and 1064 nm, can efficiently distinguish optically shallow waters from nearby land surfaces and deep oceans. ATLAS's high vertical resolution photon measurements can accurately determine seafloor depths in shallow water bodies, characterize seafloor reflectance, and provide assessments of ocean biomass concentrations in the intervening water column. By adding bathymetry, seafloor optical properties (e.g., reflectance, depolarization ratio and attenuated backscatter), and nighttime observations, space lidar measurements obtained in nearshore waters can provide a wealth of unique information to complement existing satellite-based ocean color remote sensing capabilities. The results reported here demonstrate the feasibility of using satellite lidars for nearshore seafloor ecosystem analyses, which in turn provide critical insights for studies of coastal navigation and seabed topography changes due to disasters, as well as the temporal and spatial morphological evolution of coastal systems.

Spatio-Temporal Evolution of a Typical Sandstorm Event in an Arid Area of Northwest China in April 2018 Based on Remote Sensing Data

Northwest China is significantly affected by sandstorm disasters. To mitigate the negative impacts of sandstorm events, it is critical to understand the spatio-temporal variations in typical sand and dust storms and their influencing factors. In this work, using ground-based measurements of particulate matter and remote sensing data such as MODIS, OMI, and CALIPSO data, the sources of aerosol pollution and aerosol optical properties of a typical sandstorm event that occurred in Northwest China in 2018 was studied. In addition, the HYSPLIT model was used to explore the air mass trajectories in order to analyze the sand and dust migration process during the sandstorm event. Furthermore, the wind erosion sensitivity of Northwest China was analyzed via single factor analysis and multi-factor superposition of wind field intensity, soil drought index, vegetation coverage, and relief amplitude. Finally, the region of the study area having a high comprehensive wind erosion sensitivity was identified. The results showed that the PM10 concentrations exceeded 400 µg/m3 and the PM2.5/PM10 ratio did not exceeded 0.6 during the sandstorm event, indicating that natural particulate matter was dominant in the ambient air. At the epicenter of pollution, the aerosol optical depth (AOD) at 550 nm was 0.75–1. By combining AOD data with wind speed and direction data from field observation stations, it was found that the sandstorm event in 2018 mainly occurred between 1 April and 3 April, and affected all of Northwest China on 2 April and 3 April. The absorbed aerosol index (AAI) ranged between 2.5 and 4, indicating that the Taklimakan Desert was the main source of sandstorm events in Northwest China. The CALIPSO total attenuated backscatter coefficient at 532 nm indicated that the main component of tropospheric aerosol in this region was distributed in the range of 0–12.5 km. The simulated airflow track showed that it had the same dust source regions as AAI index studies. Moreover, investigation of wind erosion sensitivity in the study areas indicated that the Taklimakan Desert and other desert regions were the main ecologically sensitive areas. These conclusions can provide references and suggestions for the mitigation of damage caused by sandstorm events, in addition to the enhancement of ecological governance.

Wildfire Smoke Observations in the Western United States from the Airborne Wyoming Cloud Lidar during the BB-FLUX Project. Part I: Data Description and Methodology

Abstract During the summer of 2018, the upward-pointing Wyoming Cloud Lidar (WCL) was deployed on board the University of Wyoming King Air (UWKA) research aircraft for the Biomass Burning Flux Measurements of Trace Gases and Aerosols (BB-FLUX) field campaign. This paper describes the generation of calibrated attenuated backscatter coefficients and aerosol extinction coefficients from the WCL measurements. The retrieved aerosol extinction coefficients at the flight level strongly correlate (correlation coefficient, rr &gt; 0.8) with in situ aerosol concentration and carbon monoxide (CO) concentration, providing a first-order estimate for converting WCL extinction coefficients into vertically resolved CO and aerosol concentration within wildfire smoke plumes. The integrated CO column concentrations from the WCL data in nonextinguished profiles also correlate (rr = 0.7) with column measurements by the University of Colorado Airborne Solar Occultation Flux instrument, indicating the validity of WCL-derived extinction coefficients. During BB-FLUX, the UWKA sampled smoke plumes from more than 20 wildfires during 35 flights over the western United States. Seventy percent of flight time was spent below 3 km above ground level (AGL) altitude, although the UWKA ascended up to 6 km AGL to sample the top of some deep smoke plumes. The upward-pointing WCL observed a nearly equal amount of thin and dense smoke below 2 km and above 5 km due to the flight purpose of targeted fresh fire smoke. Between 2 and 5 km, where most of the wildfire smoke resided, the WCL observed slightly more thin smoke than dense smoke due to smoke spreading. Extinction coefficients in dense smoke were 2–10 times stronger, and dense smoke tended to have larger depolarization ratio, associated with irregular aerosol particles.

Spatial variability of forward modelled attenuated backscatter in clear-sky conditions over a megacity: Implications for observation network design.

Sensors that measure the attenuated backscatter coefficient (e.g., automatic lidars and ceilometers [ALCs]) provide information on aerosols that can impact urban climate and human health. To design an observational network of ALC sensors for supporting data assimilation and to improve prediction of urban weather and air quality, a methodology is needed. In this study, spatio‐temporal patterns of aerosol‐attenuated backscatter coefficient are modelled using Met Office numerical weather prediction (NWP) models at two resolutions, 1.5 km (UKV) and 300 m (London Model [LM]), for 28 clear‐sky days and nights. Initially, attenuated backscatter coefficient data are analysed using S‐mode principal component analysis (PCA) with varimax rotation. Four to seven empirical orthogonal functions (EOFs) are produced for each model level, with common EOFs found across different heights (day and night) for both NWP models. EOFs relate strongly to orography, wind, and emissions source location, highlighting these as critical controls of attenuated backscatter coefficient spatial variability across the megacity. Urban–rural differences are largest when wind speeds are low and vertical boundary‐layer dynamics can more effectively distribute near‐surface aerosol emissions vertically. In several night‐time EOFs, gravity‐wave features are found for both NWP models. Increasing the horizontal resolution of native ancillaries (model input parameters) and improving the urban surface scheme in the LM may enhance the urban signal in the EOFs. PCA output, with agglomerative Ward cluster analysis (CA), minimises intra‐group variance. The UKV and LM CA shape and size results are similar and strongly related to orography. PCA‐CA is a simple, but adaptable methodology, allowing close alignment with observation network design goals. Here, CA is used with wind roses to suggest the optimised ALC deployment is one in the city to observe the urban plume and others surrounding the city, with priority given to cluster size and frequency of upwind advection.

The analysis of pre-monsoon dust storm over Delhi using ground-based observations

Three major sequential widespread dust events were experienced in the northern parts of India in May 2018. A significant impact of these pre-monsoon dust storms on the aerosol characteristics over the Indian National capital region (NCR) has been studied using remotely sensed ceilometer and ground-based measurements at Indira Gandhi International airport, New Delhi, India. The results show that after each dust activity, the significant inclusion of dust aerosols loaded in the free troposphere. Consequently, the direct impact on the lower atmospheric parameters like increase in daily average temperature (by 4–5 K), stepped up (stepped down) diurnal cycles of longwave fluxes (shortwave fluxes), has been recorded within 15 days of dust span. Mainly, the adverse meteorological and radiation features noticed before the first dust storm (DS1), which pinpoints the sudden dust intrusion over NCR, Delhi. However, this dust storm has extensively impacted on the atmospheric vertical dust loading, surface boundary layer mechanisms, and socioeconomic way. Therefore, the detailed analysis of vertical dust distribution and its interaction with mid-tropospheric processes has been carried by using the vertical normalized attenuated backscatter coefficients accompanying the radiosonde observation. The aloft floating dust layer up to 3–4 km has been noticed even after shallow rainfall and persisted at almost the same height for the next 34 h due to low-level clouds. Meanwhile, the sub-dust layer below 1 km is formed due to local activity, which also sustains for a long time.

Mass concentration estimates of long-range-transported Canadian biomass burning aerosols from a multi-wavelength Raman polarization lidar and a ceilometer in Finland

Abstract. A quantitative comparison study for Raman lidar and ceilometer observations, and for model simulations of mass concentration estimates of smoke particles is presented. Layers of biomass burning aerosol particles were observed in the lower troposphere, at 2 to 5 km height on 4 to 6 June 2019, over Kuopio, Finland. These long-range-transported smoke particles originated from a Canadian wildfire event. The most pronounced smoke plume detected on 5 June was intensively investigated. Optical properties were retrieved from the multi-wavelength Raman polarization lidar PollyXT. Particle linear depolarization ratios (PDRs) of this plume were measured to be 0.08±0.02 at 355 nm and 0.05±0.01 at 532 nm, suggesting the presence of partly coated soot particles or particles that have mixed with a small amount of dust or other non-spherical aerosol type. The layer-mean PDR at 355 nm (532 nm) decreased during the day from ∼0.11 (0.06) in the morning to ∼0.05 (0.04) in the evening; this decrease with time could be linked to the particle aging and related changes in the smoke particle shape properties. Lidar ratios were derived as 47±5 sr at 355 nm and 71±5 sr at 532 nm. A complete ceilometer data processing for a Vaisala CL51 ceilometer is presented from a sensor-provided attenuated backscatter coefficient to particle mass concentration (including the water vapor correction for high latitude for the first time). Aerosol backscatter coefficients (BSCs) were measured at four wavelengths (355, 532, 1064 nm from PollyXT and 910 nm from CL51). Two methods, based on a combined lidar and sun-photometer approach, are applied for mass concentration estimations from both PollyXT and the ceilometer CL51 observations. In the first method, no. 1, we used converted BSCs at 532 nm (from measured BSCs) by corresponding measured backscatter-related Ångström exponents, whereas in the second method, no. 2, we used measured BSCs at each wavelength independently. A difference of ∼12 % or ∼36 % was found between PollyXT and CL51 estimated mass concentrations using method no. 1 or no. 2, showing the potential of mass concentration estimates from a ceilometer. Ceilometer estimations have an uncertainty of ∼50 % in the mass retrieval, but the potential of the data lies in the great spatial coverage of these instruments. The mass retrievals were compared with the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) meteorological and aerosol reanalysis. The inclusion of dust (as indicated by MERRA-2 data) in the retrieved mass concentration is negligible considering the uncertainties, which also shows that ceilometer observations for mass retrievals can be used even without exact knowledge of the composition of the smoke-dominated aerosol plume in the troposphere.

Capabilities of an Automatic Lidar Ceilometer to Retrieve Aerosol Characteristics within the Planetary Boundary Layer

Continuous observation and quantitative retrieval of aerosol backscatter coefficients are important in the study of air quality and climate in metropolitan areas such as New York City. Ceilometers are ideal for this application, but aerosol backscatter coefficient retrievals from ceilometers are challenging and require proper calibration. In this study, we calibrate the ceilometer (Lufft CHM15k, 1064 nm) system constant with the molecular backscatter coefficient and evaluate the calibrated profiles with other independent methods, including the water-phase cloud method and comparison with the NASA Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) attenuated backscatter coefficient profile. Multiple-day calibration results show a stable system constant with a relative uncertainty of about 7%. We also evaluate the overlap correction for the CHM15k ceilometer (provided by Lufft) with a Vaisala CL-31 ceilometer, and the results show good consistency between two ceilometers’ range-corrected signal (RCS) profiles above 200 m. Next, we implement a forward iterative method to retrieve aerosol backscatter coefficients from continuous ceilometer measurements. In the retrieval, the lidar ratio is constrained by the co-located NASA AERONET radiometer aerosol optical depth (AOD) retrieval and agrees with the AERONET lidar-ratio products, derived from aerosol microphysical parameters. The aerosol backscatter coefficient retrievals are validated with co-located elastic-Raman lidar retrievals and indicate a good correlation (R2≥0.95) in the planetary boundary layer (PBL). Furthermore, a case study shows that the ceilometer retrieved aerosol extinction coefficient profiles can be used to estimate the AOD of the PBL and the aloft plumes. Finally, simulations of the uncertainty of aerosol backscatter coefficient retrieval show that a calibration error of 10% results in 10–20% of relative error in the aerosol backscatter coefficient retrievals, while relative error caused by a lidar-ratio error of 10% is less than 4% in the PBL.

Global Ocean Studies from CALIOP/CALIPSO by Removing Polarization Crosstalk Effects

Recent studies indicate that the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) aboard the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite provides valuable information about ocean phytoplankton distributions. CALIOP’s attenuated backscatter coefficients, measured at 532 nm in receiver channels oriented parallel and perpendicular to the laser’s linear polarization plane, are significantly improved in the Version 4 data product. However, due to non-ideal instrument effects, a small fraction of the backscattered optical power polarized parallel to the receiver polarization reference plane is misdirected into the perpendicular channel, and vice versa. This effect, known as polarization crosstalk, typically causes the measured perpendicular signal to be higher than its true value and the measured parallel signal to be lower than its true value. Therefore, the ocean optical properties derived directly from CALIOP’s measured signals will be biased if the polarization crosstalk effect is not taken into account. This paper presents methods that can be used to estimate the CALIOP crosstalk effects from on-orbit measurements. The global ocean depolarization ratios calculated both before and after removing the crosstalk effects are compared. Using CALIOP crosstalk-corrected signals is highly recommended for all ocean subsurface studies.

Classification of atmospheric aerosols and clouds by use of dual-polarization lidar measurements.

Accurate identification of aerosols and cloud from remote sensing observations is of importance for quantitatively evaluating their radiative forcing and related impacts. Even though polarization lidar has exhibited a unique advantage of classifying atmospheric aerosols and clouds over the past several decades, polarization measurements are often achieved at one wavelength (UV or VIS) using laser remote sensing. To better identify the types of aerosols and clouds, we developed a ground-based dual-polarization lidar system that can simultaneously detect polarization measurements at wavelengths of 355 nm and 532 nm. Our results show that the volume depolarization ratios (VDRs) at 355 nm and 532 nm markedly differ for typical types of aerosols and clouds in the atmosphere. For non-spherical particles, the ratio of VDRs at 532 nm and 355 nm are 2.87 ± 1.35 for ice cloud and 1.51 ± 0.29 for dust-dominated aerosols, respectively. However, for spherical particles, the ratios are 0.43 ± 0.26 for water cloud and 0.56 ± 0.05 for air pollutants. Consequently, we proposed a simple reliable method for classifying atmospheric aerosols and clouds from polarization measurements observed by the developed lidar system. The proposed method first distinguishes clouds from aerosols using a combination of the color ratio (CR, 532 nm/355 nm) and attenuated backscattering coefficients (ABC) at 532 nm. Then, subtypes of clouds and aerosols are identified based on the ratio of VDRs at 532 nm and 355 nm. The results showed that dual-polarization lidar measurements can remarkably improve the classification of atmospheric aerosols and clouds, compared with results using a traditional method. This study illustrates that more information on atmospheric aerosols and clouds can be obtained from polarization measurements at multiple wavelengths by active remote sensing.

Observation of clouds, aerosols, and precipitation by multiple-field-of-view multiple-scattering polarization lidar at 355 nm

We developed a multiple-field-of-view multiple-scattering polarization lidar at 355 nm (MFMSPL-355) to study the microphysics of clouds and aerosols, and understand the multiple scattering effects on space lidar measurements. The MFMSPL-355 is used to simulate and interpret multiple scattering signals by the 355 nm lidar installed on the Earth Clouds, Aerosol and Radiation Explorer satellite. This is the first multiple scattering lidar developed at 355 nm in the world. The system has five receiver modules and can observe both parallel and perpendicular attenuated backscatter coefficients for the on-beam direction and four off-beam directions with different tilting angles. Thus, the MFMSPL-355 can measure the single scattering signal and multiple scattering signal independently; accordingly, it can provide microphysical properties, such as the effective radius, of clouds and aerosols. We demonstrated that the MFMSPL-355 could observe multiple scattering signals for water clouds, ice clouds, aerosols, and drizzle. The observed features of the water clouds and drizzle were consistent with those observed by a previously developed 532-nm MFMSPL. Furthermore, we found that aerosol signals and their multiple scattering contributions were generally more pronounced at 355 nm, which is the advantage of performing measurements at 355 nm. Off-beam channels can offer a unique opportunity to study aerosol microphysics.

Atmospheric boundary layer height estimation from aerosol lidar: a new approach based on morphological image processing techniques

Abstract. The atmospheric boundary layer (ABL) represents the lowermost part of the atmosphere directly in contact with the Earth's surface. The estimation of its depth is of crucial importance in meteorology and for anthropogenic pollution studies. ABL height (ABLH) measurements are usually far from being adequate, both spatially and temporally. Thus, different remote sensing sources can be of great help in growing both the spatial and temporal ABLH measurement capabilities. To this aim, aerosol backscatter profiles are widely used as a proxy to retrieve the ABLH. Hence, the scientific community is making remarkable efforts in developing automatic ABLH retrieval algorithms applied to lidar observations. In this paper, we propose a ABLH estimation algorithm based on image processing techniques applied to the composite image of the total attenuated backscatter coefficient. A pre-processing step is applied to the composite total backscatter image based on morphological filters to properly set-up and adjust the image to detect edges. As final step, the detected edges are post-processed through both mathematical morphology and an object-based analysis. The performance of the proposed approach is assessed on real data acquired by two different lidar systems, deployed in Potenza (Italy) and Évora (Portugal), belonging to the European Aerosol Research Lidar Network (EARLINET). The proposed approach has shown higher performance than the benchmark consisting of some state-of-the-art ABLH estimation methods.

Observed and modelled cloud cover up to 6 km height at Station Nord in the high Arctic

AbstractWe present results from an analyses of cloud cover based on profiles of the attenuated backscatter coefficient from an 8‐year‐long data series (July 2011–April 2019). The observations are carried out in the high Arctic by a ceilometer with a maximum range setting of 7.7 km from the Villum Research Station at Station Nord, Greenland. Results show that the hourly cloud cover turned out to follow a U‐shaped rather than Gaussian‐like distribution. Annual and seasonal cloud cover variation is illustrated. The cloud cover is larger during the autumn and winter as compared to summer and spring. The cloud cover exhibits a substantial variation from year to year without a clear trend. The cloud cover during spring is low and decreasing between 2012 and 2017. The cloud cover during the autumn of 2016 is lowest compared to the other years. The observed cloud cover is compared to the cloud cover provided in the ERA5 reanalysis dataset. The cloud cover for low clouds and medium clouds are combined to represent a total height of 6 km. Both the observed and modelled cloud cover is larger during winter as compared to summer‐time cloud cover. The measured reduction in the cloud cover for the autumn of 2016 is present in the reanalysis data as well but the measured low cloud cover during spring is not apparent in the reanalysis data. Because the cloud cover distribution is U‐shaped rather than of a Gaussian nature, standard metrics are not applicable. We apply a generalized skill score that is developed for contingency tables or joint histograms. Three skill scores were calculated. It was found that for all three methods, skills for the predictability of the cloud cover by the ERA5 modelling is better for winter than summer and is poor during the spring.

New attenuated backscatter profile by removing the CALIOP receiver's transient response

The photomultiplier tubes (PMTs) used to measure altitude-resolved 532 nm backscatter intensity by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) do not recover rapidly following exposure to very high light levels (e.g., from optically dense water clouds). Instead, they exhibit exponentially decaying “noise tails” that can cause substantial misestimates when determining layer base altitudes and deriving cloud extinction coefficients. Here we present a deconvolution correction algorithm to remove these noise tails in the CALIOP level 1 science data products. The corrected 532 nm attenuated backscatter profiles generated by the deconvolution algorithm are evaluated using the corresponding CALIOP observations at 1064 nm and coincident profiles measured at 532 nm by the NASA-Langley airborne high spectral resolution lidar. Results indicate that our deconvolution correction algorithm effectively removes the non-ideal PMT recovery effects on the CALIOP level 1 vertical profiles, showing excellent performance for surface and water cloud lidar returns when the attenuated backscatter coefficients are greater than 0.01 km−1 sr−1.

Dust Lidar Ratios Retrieved from the CALIOP Measurements Using the MODIS AOD as a Constraint

Lidar ratio for dust aerosols is retrieved from a synergetic use of the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) Total Attenuated Backscatter coefficients and the Moderate Resolution Imaging Spectroradiometer (MODIS) Aerosol Optical Depths (AODs) for 5 years from 2007 to 2011. MODIS AODs from the Dark Target (DT) algorithm over ocean and from the Deep Blue (DB) algorithm over land are used as a constraint for the retrieval. The dust lidar ratio is retrieved larger over land (46.6 ± 36.3 sr) than ocean (39.5 ± 16.8 sr) and shows distinct regional variation. Lidar ratio for Saharan dust (49.5 ± 36.8 sr) is larger than Arabian dust (42.5 ± 26.2 sr). Lidar ratios for dust aerosols transported to Mediterranean Sea (44.4 ± 15.9 sr), Mid Atlantic (40.3 ± 12.4 sr), and Arabian Sea (37.5 ± 12.1 sr) show lower values relative to their source regions. Retrieved dust lidar ratios for Taklamakan and Gobi Deserts region (35.0 ± 31.1 sr) and Australia (35.4 ± 34.4 sr) are slightly lower than the above-mentioned regions. AOD comparison between CALIOP and MODIS shows that the CALIOP AOD is biased low. When including clear air AOD for CALIOP, however, AODs from two sensors become more comparable.

Long-term aerosol optical hygroscopicity study at the ACTRIS SIRTA observatory: synergy between ceilometer and in situ measurements

Abstract. An experimental setup to study aerosol hygroscopicity is proposed based on the temporal evolution of attenuated backscatter coefficients from a ceilometer colocated with an instrumented tower equipped with meteorological sensors at different heights. This setup is used to analyze a 4.5-year database at the ACTRIS SIRTA observatory in Palaiseau (Paris, France, 2.208∘ E, 48.713∘ N; 160 m above sea level). A strict criterion-based procedure has been established to identify hygroscopic growth cases using ancillary information, such as online chemical composition, resulting in 8 hygroscopic growth cases from a total of 107 potential cases. For these eight cases, hygroscopic growth-related properties, such as the attenuated backscatter enhancement factor fβ (RH) and the hygroscopic growth coefficient γ, are evaluated. This study shows that the hygroscopicity parameter γ is negatively correlated with the aerosol organic mass fraction but shows a positive correlation with the aerosol inorganic mass fraction. Among inorganic species, nitrate exhibited the highest correlation. This is the first time that hygroscopic enhancement factors are directly retrieved under ambient aerosols using remote-sensing techniques, which are combined with online chemical composition in situ measurements to evaluate the role of the different aerosol species in aerosol hygroscopicity.