Applications In Information Processing Research Articles

Synchronous micromechanically resonant programmable photonic circuits

Programmable photonic integrated circuits (PICs) are emerging as powerful tools for control of light, with applications in quantum information processing, optical range finding, and artificial intelligence. Low-power implementations of these PICs involve micromechanical structures driven capacitively or piezoelectrically but are often limited in modulation bandwidth by mechanical resonances and high operating voltages. Here we introduce a synchronous, micromechanically resonant design architecture for programmable PICs and a proof-of-principle 1×8 photonic switch using piezoelectric optical phase shifters. Our design purposefully exploits high-frequency mechanical resonances and optically broadband components for larger modulation responses on the order of the mechanical quality factor Qm while maintaining fast switching speeds. We experimentally show switching cycles of all 8 channels spaced by approximately 11 ns and operating at 4.6 dB average modulation enhancement. Future advances in micromechanical devices with high Qm, which can exceed 10000, should enable an improved series of low-voltage and high-speed programmable PICs.

Enhancement of microwave fields in pulse EPR of quantum paraelectrics

The pulse electron paramagnetic resonance (EPR) is widely used in different branches of material and life sciences, including promising applications in quantum information processing and quantum sensing. Here, we study the effect of the high polarizability of KTaO3 and SrTiO3 quantum paraelectrics on local electric and magnetic field components of microwaves (MW) at Fe3+ and Mn2+ paramagnetic ions. The measurements are performed with a commercial EPR spectrometer using dielectric and split-ring resonators. It is found that the power of MW pulses used in coherent spin manipulation at nanoseconds timescale decreases to milliwatts as compared to the tens–hundreds of watts usually used for spins in conventional materials. The amplification of MW fields is related to the very high dielectric permittivity (up to 25 000 in SrTiO3) of quantum paraelectrics at GHz frequencies and temperatures below 20 K. This creates the large induced polarization and, thus, huge displacement current and in turn the secondary MW magnetic field. Numerical simulations support the observation of the enhanced magnetic MW field in the high-permittivity sample. The low MW power for excitation of spin transitions in quantum paraelectrics eliminates the requirement of expensive high-power MW equipment. This approach also allows to globally control spin qubits in tandem with integrated devices based on conventional semiconductor MW circuits working at mW powers. It is suggested that quantum paraelectrics can also be used as substrates for deposition of nanoparticles or films of other materials, which would be manipulated by the low-power MW pulses.

Polarization-Sensitive Detector Based on MoTe2/WTe2 Heterojunction for Broadband Optoelectronic Imaging.

Polarization-sensitive detectors have significant applications in modern communication and information processing. In this study. We present a polarization-sensitive detector based on a MoTe2/WTe2 heterojunction, where WTe2 forms a favorable bandgap structure with MoTe2 after forming the heterojunction. This enhances the carrier separation efficiency and photoelectric response. We successfully achieved wide spectral detection ranging from visible to near-infrared light. Specifically, under zero bias, our photodetector exhibits a responsivity (R) of 0.6 A/W and a detectivity (D*) of 3.6 × 1013 Jones for 635 nm laser illumination. Moreover, the photoswitching ratio can approach approximately 6.3 × 105. Importantly, the polarization sensitivity can reach 3.5 (5.2) at 635 (1310) nm polarized light at zero bias. This study both unveils potential for utilizing MoTe2/WTe2 heterojunctions as polarization-sensitive detectors and provides novel insights for developing high-performance optoelectronic devices.

Nonequilibrium dynamics of the Jaynes-Cummings dimer.

We investigate the nonequilibrium dynamics of a Josephson-coupled Jaynes-Cummings dimer in the presence of Kerr nonlinearity, which can be realized in the cavity and circuit quantum electrodynamics systems. The semiclassical dynamics is analyzed systematically to chart out a variety of photonic Josephson oscillations and their regime of stability. Different types of transitions between the dynamical states lead to the self-trapping phenomenon, which results in photon population imbalance between the two cavities. We also study the dynamics quantum mechanically to identify characteristic features of different steady states and to explore fascinating quantum effects, such as spin dephasing, phase fluctuation, and revival phenomena of the photon field, as well as the entanglement of spin qubits. For a particular "self-trapped" state, the mutual information between the atomic qubits exhibits a direct correlation with the photon population imbalance, which is promising for generating photon mediated entanglement between two non interacting qubits in a controlled manner. Under a sudden quench from stable to unstable regime, the photon distribution exhibits phase space mixing with a rapid loss of coherence, resembling a thermal state. Finally, we discuss the relevance of the new results in experiments, which can have applications in quantum information processing and quantum technologies.

Research Progress on the Application of Topological Phase Transition Materials in the Field of Memristor and Neuromorphic Computing.

Topological phase transition materials have strong coupling between their charge, spin orbitals, and lattice structure, which makes them have good electrical and magnetic properties, leading to promising applications in the fields of memristive devices. The smaller Gibbs free energy difference between the topological phases, the stable oxygen vacancy ordered structure, and the reversible topological phase transition promote the memristive effect, which is more conducive to its application in information storage, information processing, information calculation, and other related fields. In particular, extracting the current resistance or conductance of the two-terminal memristor to convert to the weight of the synapse in the neural network can simulate the behavior of biological synapses in their structure and function. In addition, in order to improve the performance of memristors and better apply them to neuromorphic computing, methods such as ion doping, electrode selection, interface modulation, and preparation process control have been demonstrated in memristors based on topological phase transition materials. At present, it is considered an effective method to obtain a unique resistive switching behavior by improving the process of preparing functional layers, regulating the crystal phase of topological phase transition materials, and constructing interface barrier-dependent devices. In this review, we systematically expound the resistance switching mechanism, resistance switching performance regulation, and neuromorphic computing of topological phase transition memristors, and provide some suggestions for the challenges faced by the development of the next generation of non-volatile memory and brain-like neuromorphic devices based on topological phase transition materials.

Microwave‐Optics Entanglement Via Cavity Optomagnomechanics

AbstractMicrowave‐optics entanglement is a vital component for building hybrid quantum networks. Here, a new mechanism for preparing stationary entanglement between microwave and optical cavity fields in a cavity optomagnomechanical system is proposed. It consists of a magnon mode in a ferrimagnetic crystal that couples directly to a microwave cavity mode via the magnetic dipole interaction and indirectly to an optical cavity through the deformation displacement of the crystal. The mechanical displacement is induced by the magnetostrictive force and coupled to the optical cavity via radiation pressure. Both the opto‐ and magnomechanical couplings are dispersive. Magnon–phonon entanglement is created via magnomechanical parametric down‐conversion, which is further distributed to optical and microwave photons via simultaneous optomechanical beamsplitter interaction and electromagnonic state‐swap interaction, yielding stationary microwave‐optics entanglement. The microwave‐optics entanglement is robust against thermal noise, which will find broad potential applications in quantum networks and quantum information processing with hybrid quantum systems.

Adapted poling to break the nonlinear efficiency limit in nanophotonic lithium niobate waveguides.

Nonlinear frequency mixing is a method to extend the wavelength range of optical sources with applications in quantum information and photonic signal processing. Lithium niobate with periodic poling is the most widely used material for frequency mixing due to its strong second-order nonlinear coefficient. The recent development using nanophotonic lithium niobate waveguides promises to improve nonlinear efficiencies by orders of magnitude thanks to subwavelength optical confinement. However, the intrinsic nanoscale inhomogeneity of nanophotonic lithium niobate waveguides limits the coherent interaction length, leading to low nonlinear efficiencies. Here we show improved second-order nonlinear efficiency in nanophotonic lithium niobate waveguides that breaks the limit imposed by nanoscale inhomogeneity. This is realized by developing the adapted poling approach to eliminate the impact of nanoscale inhomogeneity. We realize an overall second-harmonic efficiency of 104% W-1 (without cavity enhancement), approaching the theoretical performance for nanophotonic lithium niobate waveguides. The ideal square dependence of the nonlinear efficiency on the waveguide length is recovered. Phase-matching bandwidths and temperature tuneability are improved through dispersion engineering. We finally demonstrate a conversion ratio from pump to second-harmonic power greater than 80% in a single-pass configuration with pump power as low as 20 mW. Our work therefore breaks the trade-off between the conversion ratio and pump power, offering a potential solution for highly efficient and scalable nonlinear-optical sources, amplifiers and converters.

Edge-Confined Excitons in Monolayer Black Phosphorus.

Quantum confinement of two-dimensional excitons in van der Waals materials via electrostatic trapping, lithographic patterning, Moiré potentials, and chemical implantation has enabled significant advances in tailoring light emission from nanostructures. While such approaches rely on complex preparation of materials, natural edges are a ubiquitous feature in layered materials and provide a different approach for investigating quantum-confined excitons. Here, we observe that certain edge sites of monolayer black phosphorus (BP) strongly localize the intrinsic quasi-one-dimensional excitons, yielding sharp spectral lines in photoluminescence, with nearly an order of magnitude line width reduction. Through structural characterization of BP edges using transmission electron microscopy and first-principles GW plus Bethe-Salpeter equation (GW-BSE) calculations of exemplary BP nanoribbons, we find that certain atomic reconstructions can strongly quantum-confine excitons resulting in distinct emission features, mediated by local strain and screening. We observe linearly polarized luminescence emission from edge reconstructions that preserve the mirror symmetry of the parent BP lattice, in agreement with calculations. Furthermore, we demonstrate efficient electrical switching of localized edge excitonic luminescence, whose sites act as excitonic transistors for emission. Localized emission from BP edges motivates exploration of nanoribbons and quantum dots as hosts for tunable narrowband light generation, with future potential to create atomic-like structures for quantum information processing applications as well as exploration of exotic phases that may reside in atomic edge structures.

Quantum Combinational Logics and their Realizations with Circuits

AbstractClassical combinational logic circuits (CCLCs) are widely used in various fields. Corresponding to the CCLCs, here schemes are given for some quantum combinational logic circuits (QCLCs) based on the quantum NAND tree. Three typical circuits, adder, comparator, and seven‐segment display decoder, are discussed in detail as examples. All the designs of the schemes are based on the quantum random walk theory. Furthermore, these QCLCs are mapped onto the classical circuit networks and design new types of CCLCs, and take advantage of the fact that there is a good correspondence between the voltage in the circuit satisfying Kirchhoff's law and the system wave function satisfying the Schrodinger equation. These CCLCs that are designed have exponential speedup functions compared with conventional ones, which have been demonstrated experimentally. Because classical circuit networks possess good scalability and stability, the realization of QCLCs on classical circuits is expected to have potential applications for information processing in the era of big data.

Bragg grating based entangled biphoton dispersion management

In the realm of quantum information processing and precision measurements, a range of non-classical effects based on entangled photon pairs are employed. Non-local dispersion cancellation is one of these properties, in which the second photon (idler) can be manipulated to cancel the effects of dispersion on the first photon (signal). In the present study, a thorough investigation is conducted into non-local dispersion cancellation by using excitation modes within a Bragg grating slab waveguide. We present a complete theoretical analysis of non-local dispersion cancellation for frequency-limited entangled photon pairs. For the analysis of the effect of dispersion cancellation, we use a spontaneous parametric down-conversion (SPDC) photon pair source with frequency correlation and anti-correlation as the entangled source. To evaluate the dispersion cancellation effect for information processing applications, the second correlation function is used and calculated as a practical and tangible metric. Considering different cases for Bragg Grating waveguide the results on both photons are extracted and discussed. Moreover, we will show that the physical parameters of the waveguide that the second photon is propagated inside will be effective in minimizing the width of the temporal correlation function. Hence, this study underscores the feasibility of achieving non-local dispersion cancellation through strategic optimization of optical and geometric parameters in the Bragg Grating waveguide, with potential implications for quantum information processing and high-resolution sensing endeavors.

Integrated programmable controlled phase gate design for quantum information processing

An integrated programmable controlled-phase (CPHASE) gate has been proposed for quantum information processing applications. This gate can introduce arbitrary phase difference to the target qubit in the case of the control qubit being in the state of |1〉. As the desired phase difference can be utilized after fabrication, unlike the conventional controlled-phase gates that provide hard-coded phase shift, such an integrated gate is expected to pave the way for more versatile operations of current integrated optical circuits as well as possible new applications.

Giant nonlocal Kerr nonlinearity and polaritonic solitons in a Rydberg-dressed Bose-Einstein condensate.

We present a scheme to generate nonlocal optical Kerr nonlinearity and polaritonic solitons via matter-wave superradiance in a Rydberg-dressed Bose-Einstein condensate (BEC). We show that the polariton spectrum of the scattered field generated by the superradiance is changed significantly due to the existence of the long-range Rydberg-Rydberg interaction between atoms, i.e. it has a roton-maxon form; moreover, the BEC structure factor displays a strong dependence on the Rydberg-dressing, which can be tuned in a controllable way. We also show that such a Rydberg-dressed BEC system can support a giant nonlocal optical Kerr nonlinearity, and hence allow the formation and stable propagation of polaritonic solitons, which have ultraslow propagation velocity and ultralow generation power. The results reported here are useful to understand the unique properties of Rydberg-dressing in BECs and have potential applications in optical information processing and transmission.

High-frame-rate reconfigurable diffractive neural network based on superpixels.

The existing implementations of reconfigurable diffractive neural networks rely on both a liquid-crystal spatial light modulator and a digital micromirror device, which results in complexity in the alignment of the optical system and a constrained computational speed. Here, we propose a superpixel diffractive neural network that leverages solely a digital micromirror device to control the neuron bias and connection. This approach considerably simplifies the optical system and achieves a computational speed of 326 Hz per neural layer. We validate our method through experiments in digit classification, achieving an accuracy of 82.6%, and action recognition, attaining a perfect accuracy of 100%. Our findings demonstrate the effectiveness of the superpixel diffractive neural network in simplifying the optical system and enhancing computational speed, opening up new possibilities for real-time optical information processing applications.

Gain-loss-induced non-Abelian Bloch braids

Onsite gain-loss-induced topological braiding principle of non-Hermitian energy bands is theoretically formulated in multiband lattice models with Hermitian hopping amplitudes. Braid phase transition occurs when the gain-loss parameter is tuned across exceptional point degeneracy. Laboratory realizable effective-Hamiltonians are proposed to realize braid groups B2 and B3 of two and three bands, respectively. While B2 is trivially Abelian, the group B3 features non-Abelian braiding and energy permutation originating from the collective behavior of multiple exceptional points. Phase diagrams with respect to lattice parameters to realize braid group generators and their non-commutativity are shown. The proposed theory is conducive to synthesizing exceptional materials for applications in topological computation and information processing.

On-Surface Synthesis of Graphene Nanoribbons with Atomically Precise Structural Heterogeneities and On-Site Characterizations.

Graphene nanoribbons (GNRs) are strips of graphene, with widths of a few nanometers, that are promising candidates for future applications in nanodevices and quantum information processing due to their highly tunable structure-dependent electronic, spintronic, topological, and optical properties. Implantation of periodic structural heterogeneities, such as heteroatoms, nanopores, and non-hexagonal rings, has become a powerful manner for tailoring the designer properties of GNRs. The bottom-up synthesis approach, by combining on-surface chemical reactions based on rationally designed molecular precursors and in situ tip-based microscopic and spectroscopic techniques, promotes the construction of atomically precise GNRs with periodic structural modulations. However, there are still obstacles and challenges lying on the way toward the understanding of the intrinsic structure-property relations, such as the strong screening and Fermi level pinning effect of the normally used transition metal substrates and the lack of collective tip-based techniques that can cover multi-internal degrees of freedom of the GNRs. In this Perspective, we briefly review the recent progress in the on-surface synthesis of GNRs with diverse structural heterogeneities and highlight the structure-property relations as characterized by the noncontact atomic force microscopy and scanning tunneling microscopy/spectroscopy. We furthermore motivate to deliver the need for developing strategies to achieve quasi-freestanding GNRs and for exploiting multifunctional tip-based techniques to collectively probe the intrinsic properties.

Dephasing-assisted preparation of asymmetric steering in coupled quantum wells.

It is shown that the dephasing rates are usually harmful for quantum correlations in various systems. Nevertheless, we explore that the dephasing rates in the coupled quantum wells (QWs), as a major contribution of the decay processes, can assist to generate one-way Einstein-Podolsky-Rosen (EPR) steering. By applying two strong fields to drive two dipole-allowed transitions while the other transitions are coupled with two quantized modes, the asymmetric EPR steering is possible to obtain at steady state through a single-pathway dissipation in the three-well system. According to dressed-state and Bogoliubov mode transformation, we find that the dephasing rates play a role in modifying the dressed-state populations and the dissipation rate through multiple quantum interference mechanisms. The positive effect of the dephasing rates from a nanostructure on quantum correlation is expected to find potential applications in quantum information processing.

Semi-empirical Haken–Strobl model for molecular spin qubits

Understanding the physical processes that determine the relaxation T 1 and dephasing T 2 times of molecular spin qubits is critical for envisioned applications in quantum metrology and information processing. Recent spin-echo measurements of solid-state molecular spin qubits have stimulated the development of quantum mechanical models for predicting intrinsic qubit timescales using first-principles electronic structure methods. We develop an alternative semi-empirical approach to construct Redfield quantum master equations for molecular spin qubits using a stochastic Haken–Strobl theory for a central spin with fluctuating gyromagnetic tensor due to spin-lattice interaction and fluctuating local magnetic field due to interactions with lattice spins. Using two vanadium-based spin qubits as case studies, we compute qubit population and decoherence times as a function of temperature and magnetic field, using a bath spectral density parametrized with a small number of T 1 measurements. The theory quantitatively agrees with experimental data over a range of conditions beyond those used to parameterize the model, demonstrating the generalization potential of the method. The ability of the model to describe the temperature dependence of the ratio is discussed and possible applications for designing novel molecule-based quantum magnetometers are suggested.

Hilbert Space in Isotopologue Dy(III) SMM Dimers: Dipole Interaction Limit in [163/164Dy2(tmhd)6(tape)]0 Complexes.

Single-molecule magnets are molecular complexes proposed to be useful for information storage and quantum information processing applications. In the quest for multilevel systems that can act as Qudits, two dysprosium-based isotopologues were synthesized and characterized. The isotopologues are [164Dy2(tmhd)6(tape)] (1(I=0)) and [163Dy2(tmhd)6(tape)] (2(I=5/2)), where tmhd = 2,2,6,6-tetramethylheptandionate and tape = 1,6,7,12-tetraazaperylene. Both complexes showed slow relaxation at a zero applied magnetic field with dominant Orbach and Raman relaxation mechanisms. μSQUID studies at milli-Kelvin temperatures reveal quasi-single ion loops, in contrast with the expected S-shape (near zero field) butterfly loops, characteristic of antiferromagnetically coupled dimeric complexes. Through analysis of the low-temperature data, we find that the interaction operating between Dy(III) is small, leading to a small exchange biasing from the zero-field transition. The resulting indirectly coupled nuclear states are degenerate or possess a small energy difference between them. We, therefore, conclude that for the creation of Qudits with enlarged Hilbert spaces, shorter Dy(III)···Dy(III) distances are deemed essential.

Selective and Scalable Control of Spin Quantum Memories in a Photonic Circuit.

A central goal in many quantum information processing applications is a network of quantum memories that can be entangled with each other while being individually controlled and measured with high fidelity. This goal has motivated the development of programmable photonic integrated circuits (PICs) with integrated spin quantum memories using diamond color center spin-photon interfaces. However, this approach introduces a challenge into the microwave control of individual spins within closely packed registers. Here, we present a quantum memory-integrated photonics platform capable of (i) the integration of multiple diamond color center spins into a cryogenically compatible, high-speed programmable PIC platform, (ii) selective manipulation of individual spin qubits addressed via tunable magnetic field gradients, and (iii) simultaneous control of qubits using numerically optimized microwave pulse shaping. The combination of localized optical control, enabled by the PIC platform, together with selective spin manipulation opens the path to scalable quantum networks on intrachip and interchip platforms.

Polarization dependent light propagation in textrm{WTe}_2 multilayer structure

textrm{WTe}_2 is one of the exciting and outstanding semimetallic members of TMDCs, which has attracted immense attention for manipulating light propagation due to its inherent optical anisotropy and hyperbolic characteristic in the infrared frequency range. We investigate the dependence of the reflectance and transmittance of structures with a single and double textrm{WTe}_2 thin film in terms of frequency and polarization angle of the incident wave. We find rich behaviors in the optical response of these structures due to their anisotropic permittivity tensors. Furthermore, we analyze the polarization state of transmitted and reflected waves through these structures. We demonstrate that these structures provide the ability to achieve desired polarization rotation for outgoing waves by tuning the frequency and polarization angle of the incident wave with respect to the principal axes of textrm{WTe}_2 thin film. In particular, we elucidate the essential relevance of the optical response and polarization rotation of the double thin film structure to the in-plain twist angle of textrm{WTe}_2 thin films. We explain that this structure permits comprehensive control of the polarization rotation of the outgoing waves by adjusting the twist angle of thin films. The proposed structure can be employed as an efficient light manipulator with the aim of application in communication, imaging, and information processing.