Application Of Magnetic Field Research Articles

Inception of positive wire-cylinder corona discharges in air in crossed electric and magnetic fields

A computational study of the inception of positive wire-cylinder corona discharges in low-pressure air in crossed electric and magnetic fields is performed. The inception voltages are calculated for a wide range of gas densities, wire radii, and applied magnetic fields. Conditions are considered when the reduced electric fields at wire electrodes reach extremely high values of about 10 kTd. An expression applicable at such strong fields for the ionization coefficient, which is a key parameter of the corona inception model, is presented against the values of electric and magnetic fields. Calculated inception voltages agree with a large quantity of available experimental data on low-pressure positive corona discharges, obtained both with and without the application of magnetic fields. The calculation results describe specific details of the non-monotonous dependence of the inception voltages on the magnetic field values, similar to those obtained in experiments.

Beyond the Passive Diffusion: Core@Satellite Magneto‐Plasmonic Particles for Rapid and Sensitive Colorimetric Immunosensor Response

AbstractMagneto‐plasmonic particles, comprising gold and iron oxide, exhibit substantial potential for biosensing applications due to their distinct properties. Gold nanoparticles (AuNPs) provide plasmonic features, while iron oxide composites, responsive to an external magnetic field, significantly reduce detection time compared to passive diffusion. This study explores core@satellite magneto‐plasmonic particles (CSMPs), featuring magnetic nanoparticle clusters and numerous satellite‐like AuNPs, to amplify the optical response on a nanostructured gold surface. Using a sandwich scheme, target analytes are detected as hybrid nanoparticles bind to the pre‐immobilized target on the AuNPs surface, inducing changes in the immunosensor's extinction spectrum. Application of an external magnetic field notably enhances biosensor response and sensitivity, reducing assay time from hours to minutes. Leveraging the properties of CSMPs, the immunosensor detects specific immune protein at low concentrations within minutes. CSMPs hold considerable promise for precise and sensitive analyte detection, offering potential applications in rapid testing and mass screening.

Interplay between the reversibility of the inverse magnetocaloric effect and kinetic arrest in Ni-Co-Mn-Sn Heusler alloys

The nature of martensitic phase transitions and its modification as a function of composition and application of magnetic field have been studied in detail for Ni40Co10Mn40Sn10-xGax (x=0, 0.3, 0.4 and 0.5). The phase transition temperature (TM) increases with increasing x. The kinetic arrest (KA) of the austenitic phase has been observed for x=0 and 0.3, which disappeared for x>0.3. The KA results in a decrease in the change of magnetization (ΔM) across TM. However, the isothermal entropy change ΔS varies almost linearly with [dTM/d(μ0H)]−1 (field-induced shift in TM) irrespective of the composition variation and thermal cycling. This behavior indicates that the variation of dTM/d(μ0H) is the dominant factor determining the magnitude of the ΔS rather than ΔM. Consequently, the effect of KA on ∆M has a negligible influence on ΔS in the studied Heusler alloys. The reduced field-sensitivity in TM associated with the temperature-induced decrease of magnetization in the ferromagnetic austenitic phase leads to a decrease of the thermal hysteresis and an increase of ΔS. As a result, a large reversible (|ΔSrev|=21 J/kg K for Δμ0H=5 T) has been observed for x=0.5, which exceeds previously reported values for Sn-based Heusler alloys.

Modelling the mechanics of 32 T REBCO superconductor magnet using numerical simulation

High-temperature REBCO superconducting tapes are very promising for high-field magnets. With high magnetic field applications there are high electromechanical forces, and thus a concern for mechanical damage. Due to the presence of large screening currents and the composite structure of the tape, the mechanical design of these magnets is not straightforward. In addition, many contemporary designs use insulated winding. In this work, we develop a novel two-dimensional axi-symmetric finite element tool programmed in MATLAB that assumes the displacement field to be within a linear elastic range. The stack of pancakes and the large number of REBCO tape turns are approximated as an anisotropic bulk hollow cylinder. Our results agree with uni-axial stress experiments in the literature, validating the bulk approximation. Here, we study the following configuration. The current is first ramped up to below the critical current and we calculate the screening currents and the forces that they cause using the minimum electromagnetic entropy production method (MEMEP) model. This electromagnetic model can now take insulated magnets into account. As a case study, a 32 T REBCO superconductor magnet is simulated numerically. We perform a complete mechanical analysis of the magnet by including the axial and shear mechanical quantities for each pancake, unlike in previous work where only radial and circumferential quantities were focused on. The effect on mechanical quantities without the screening current is also calculated and compared. It is shown that including the screening current-induced field strongly affects the mechanical quantities, especially the shear stress. The latter may be a critical quantity for certain magnet configurations. Additionally, in order to overcome high stresses, a stiff overbanding of different materials is considered and numerically modelled, which significantly reduces the mechanical stresses. The finite element-based model developed is efficient in calculating the mechanical behaviour of any general superconductor magnet and its devices.

Contactless magnetically responsive injectable hydrogel for aligned tissue regeneration

Cellular alignment plays a pivotal role in several human tissues, including skeletal muscle, spinal cord and tendon. Various techniques have been developed to control cellular alignment using 3D biomaterials. However, the majority of 3D-aligned scaffolds require invasive surgery for implantation. In contrast, injectable hydrogels provide a non-invasive delivery method, gaining considerable attention for the treatment of diverse conditions, including osteochondral lesions, volumetric muscle loss, and traumatic brain injury.We engineered a biomimetic hydrogel with magnetic responsiveness by combining gellan gum, hyaluronic acid, collagen, and magnetic nanoparticles (MNPs). Collagen type I was paired with MNPs to form magnetic collagen bundles (MCollB), allowing the orientation control of these bundles within the hydrogel matrix through the application of a remote low-intensity magnetic field. This resulted in the creation of an anisotropic architecture. The hydrogel mechanical properties were comparable to those of human soft tissues, such as skeletal muscle, and proof of the aligned hydrogel concept was demonstrated.In vitro findings confirmed the absence of toxicity and pro-inflammatory effects. Notably, an increased fibroblast cell proliferation and pro-regenerative activation of macrophages were observed. The in-vivo study further validated the hydrogel biocompatibility and demonstrated the feasibility of injection with rapid in situ gelation. Consequently, this magnetically controlled injectable hydrogel exhibits significant promise as a minimally invasive, rapid gelling and effective treatment for regenerating various aligned human tissues.

Development of high superconductor fraction (Ba, K)Fe2As2 wires with improved uniformity by two-axial rolling

Iron-based superconductors are regarded as prospective candidates for high magnetic field applications since they have very high upper critical field and low anisotropy. For practical applications, it is important to develop superconducting wires with strong current carrying capability. In this work, Cu/Ag composite sheathed (Ba, K)Fe2As2 (Ba-122) iron-based superconducting wires were fabricated by a two-axial rolling deformation process and a subsequent hot isostatic pressing (HIP) heat treatment. Compared with the previously reported Cu/Ag/Ba-122 wires prepared by groove rolling, the two-axial rolling allowed to use much thinner Cu/Ag composite sheath for wire fabrication, thus greatly increasing the filling factor of superconducting materials by about 5 times to 24 %, and lowering the volume fraction of silver down to 16 % in wires. By a comparative study on the microstructure and superconducting properties between the wires made by two-axial rolling and groove rolling processes, it is found that besides the significantly increased engineering critical current density, the former also exhibits improved homogeneity of mass distribution and uniformity of Ba-122/Ag interfaces, resulting in significantly enhanced n-values over 40 in magnetic fields up to 14 T. Our work suggests that two-axial rolling, combined with HIP processes, presents a promising approach to prepare iron-based superconducting wires with high filling factor, high uniformity and low cost for practical applications.

A review of vortex pinning in REBa2Cu3O7‐x coated conductors

AbstractREBa2Cu3O7‐x (REBCO) exhibits outstanding qualities such as a high irreversible field (7 T) and strong current‐carrying capacity (77 K, 106 A cm−2), making it ideal for high magnetic field applications such as fusion, accelerators, and nuclear magnetic resonance. However, the degradation of in‐field critical current density (Jc) due to vortex motion is a significant hurdle. Research indicates that improving vortex pinning can notably enhance Jc in REBCO, showing promise for its future high‐field applications. This review explores vortex pinning mechanisms, artificial pinning centers (APCs), and how environmental conditions affect pinning characteristics, highlighting advancements in vortex pinning for REBCO in magnetic fields. Different methods for introducing APCs are discussed and compared for evaluating their efficacy in achieving optimal nanoparticle distributions and consequent superconducting performance improvements, underscoring the importance of nano‐defect features (type, size, and distribution) in optimizing the superconducting properties of the REBCO. Additionally, the review tackles current challenges, shares recent research breakthroughs, and outlines future research directions for designing pinning landscapes to further improve REBCO performance.

Electronic structure and room temperature colossal magnetodielectric effect in La0.4Dy0.1Ca0.5MnO3 manganite

Present communication reports the possible origin of the colossal magnetodielectric (MD) effect observed at room temperature in La0.4Re0.1Ca0.5MnO3 (with Re = Eu, Gd, and Dy) polycrystalline manganites. This study reveals that all the samples are half–doped (% Mn3+ = % Mn4+ = 50 %) and room temperature X-ray absorption measurement at Mn L-edges confirms the presence of both Mn3+ and Mn4+ ions in these oxides. All these specimens are paramagnetic at room temperature with the presence of metastable charge–ordered domains. The application of a low constant magnetic field of 0.6 T and 1.2 T collapses some of the charge-ordered domains that lead to the charge delocalization and colossal values of the MD effect. The Dy–based sample exhibits the strongest charge ordering state, ascribed to the important cationic mismatch effect.

Boosting the Efficiency of Photoactive Rod-Shaped Nanomotors via Magnetic Field-Induced Charge Separation.

Photocatalytic nanomotors have attracted a lot of attention because of their unique capacity to simultaneously convert light and chemical energy into mechanical motion with a fast photoresponse. Recent discoveries demonstrate that the integration of optical and magnetic components within a single nanomotor platform offers novel advantages for precise motion control and enhanced photocatalytic performance. Despite these advancements, the impact of magnetic fields on energy transfer dynamics in photocatalytic nanomotors remains unexplored. Here, we introduce dual-responsive rod-like nanomotors, made of a TiO2/NiFe heterojunction, able to (i) self-propel upon irradiation, (ii) align with the direction of an external magnetic field, and (iii) exhibit enhanced photocatalytic performance. Consequently, when combining light irradiation with a homogeneous magnetic field, these nanomotors exhibit increased velocities attributed to their improved photoactivity. As a proof-of-concept, we investigated the ability of these nanomotors to generate phenol, a valuable chemical feedstock, from benzene under combined optical and magnetic fields. Remarkably, the application of an external magnetic field led to a 100% increase in the photocatalytic phenol generation in comparison with light activation alone. By using various state-of-the-art techniques such as photoelectrochemistry, electrochemical impedance spectroscopy, photoluminescence, and electron paramagnetic resonance, we characterized the charge transfer between the semiconductor and the alloy component, revealing that the magnetic field significantly improved charge pair separation and enhanced hydroxyl radical generation. Consequently, our work provides valuable insights into the role of magnetic fields in the mechanisms of light-driven photocatalytic nanomotors for designing more effective light-driven nanodevices for selective oxidations.

Impact of constant magnetic field on enhancing the microalgal biomass and biomolecules accumulations and life cycle assessment of the approach

Three freshwater microalgal species such as Chlorella protothecoides, Micractinium sp. and Scenedesmus obliquus were cultured under static magnetic field (SMF) and its influence on the accumulation of biomolecules (lipids, proteins, carbohydrates) and biomass production have been evaluated. This study involved the cultivation of the three microalgal species under the electromagnetic intensity of 80mT which was achieved using ferrite magnets. The SMF treatment showed a significant enhancement in biomass productivity of S. obliquus (0.098 g L−1 d−1) and C. protothecoides (0.114 g L−1 d−1). On compared to SMF untreated culture, Micractinium sp. resulted in a considerable reduction in biomass productivity by 10.9 % was observed. The constant SMF treatment for the total cultivation period (17 days) has significantly promoted the biomolecules accumulation (9 % lipids, 39 % protein, 16 % carbohydrates) and biomass (55 %) productivity of S. obliquus. The results suggested that SMF treatment exhibited a species-specific response in biomass productivity and biomolecules accumulation. Finally, to assess the feasibility of this strategy, economic feasibility and LCA simulation for SMF treated microalgal biomass and biomolecules production have been evaluated. LCA revealed that the magnetic field application for microalgal cultivation processes showed diversified impacts on environment as few indicators (Abiotic depletion, Acidification and Global warming) were better under magnetic application as compared to non-magnetic cultivation process.

Magnetically Induced Near-Infrared Circularly Polarized Electroluminescence from an Achiral Perovskite Light-Emitting Diode

Circularly polarized electroluminescent devices are conventionally fabricated by incorporating an optically active chiral luminophore into their emission layer. Herein, we developed a circularly polarized perovskite light-emitting diode (PeLED) system with an optically inactive perovskite luminophore that can emit near-infrared circularly polarized electroluminescence (CPEL) upon application of an external magnetic field. The magnitude of the magnetic CPEL (gMCPEL) was in the order of 10−3 in the near-infrared wavelength range of 771–773 nm. Although the Pb perovskite quantum dots were achiral, the rotation direction of the CPEL of the magnetic circularly polarized PeLED system was successfully reversed by switching the Faraday geometry of the applied magnetic field. The use of achiral luminophores exhibiting magnetic-field-induced CPEL represents a new approach for the development of circularly polarized electroluminescent devices.

Cu(II)-Ln(III) (Ln = Gd, Tb and Dy) complexes of an unsymmetrical N2O3 donor ligand: field induced SMM behaviour of Cu(II)-Tb(III) complexes.

Three new hetero-metallic CuII-LnIII complexes [(CuL)Gd(NO3)3(CH3OH)]n (1), [(CuL)Tb(NO3)3(H2O)]·[CuL] (2) and [(CuL)Dy(NO3)3(H2O)]·[CuL] (3) have been synthesized using a mono-nuclear Cu(II) complex, [CuL], of an unsymmetrically di-condensed N2O3 donor Schiff base ligand, N-(3-methoxysalicylidene)-N-(salicylidene)-1,2-ethylenediamine (H2L). Single crystal X-ray crystallography revealed that complex 1 is a nitrate bridged 1D chain of dinuclear Cu(II)-Gd(III) units whereas in 2 and 3, the dinuclear Cu(II)-Ln(III) units are co-crystallized with a [CuL] unit. The Ln(III) centers are nine coordinated with the geometry of a spherical capped square antiprism for Gd and spherical tricapped trigonal prism for Tb and Dy. The geometry of the Cu(II) center is distorted octahedral for complex 1 and distorted square planar for complexes 2 and 3. Temperature-dependent molar magnetic susceptibility measurements in 1-3 revealed the presence of overall ferromagnetic coupling between the Cu(II) and Ln(III) centers. Notably, field induced single-molecule magnet behavior was witnessed in the Tb(III) derivative (2). The ab initio calculations indicated that upon application of an external magnetic field, the tunneling in the ground state of complex 2 gets reduced and thereby field-induced SMM behaviour is observed. Besides, in the case of complex 1, BS-DFT calculations were carried out to gain further insights into the magnetic exchange coupling interactions between the Cu(II) and Gd(III) centers.

IKVAV functionalized oriented PCL/Fe3O4 scaffolds for magnetically modulating DRG growth behavior

The re-bridging of the deficient nerve is the main problem to be solved after the functional impairment of the peripheral nerve. In this study, a directionally aligned polycaprolactone/triiron tetraoxide (PCL/Fe3O4) fiber scaffolds were firstly prepared by electrospinning technique, and further then grafted with IKVAV peptide for regulating DRG growth and axon extension in peripheral nerve regeneration. The results showed that oriented aligned magnetic PCL/Fe3O4 composite scaffolds were successfully prepared by electrospinning technique and possessed good mechanical properties and magnetic responsiveness. The PCL/Fe3O4 scaffolds containing different Fe3O4 concentrations were free of cytotoxicity, indicating the good biocompatibility and low cytotoxicity of the scaffolds. The IKVAV-functionalized PCL/Fe3O4 scaffolds were able to guide and promote the directional extension of axons, the application of external magnetic field and the grafting of IKVAV peptides significantly further promoted the growth of DRGs and axons. The ELISA test results showed that the AP-10 F group scaffolds promoted the secretion of nerve growth factor (NGF) from DRG under a static magnetic field (SMF), thus promoting the growth and extension of axons. Importantly, the IKVAV-functionalized PCL/Fe3O4 scaffolds could significantly up-regulate the expression of Cntn2, PCNA, Sox10 and Isca1 genes related to adhesion, proliferation and magnetic receptor function under the stimulation of SMF. Therefore, IKVAV-functionalized PCL/Fe3O4 composite oriented scaffolds have potential applications in neural tissue engineering.

Magnetic Field Effect on Photocatalytic Dye Degradation: A Review

AbstractIn the present day, photocatalysis has become the primary and most promising technology to generate renewable energy and degrade environmental pollutants. Remarkable efforts have been made to improve photocatalytic efficiency. Among these, introducing an external magnetic field is considered a promising strategy to boost photocatalytic performance. This review explores the dynamic realm of improving photocatalytic efficiency, with a particular emphasis on the strategic integration of external magnetic fields. Examining recent breakthroughs, we reviewed the influence of magnetic fields on diverse catalyst materials, including both magnetic and nonmagnetic variants, 2D materials, and semiconductors. Comprehensive coverage is provided on the mechanisms governing photocatalytic dye degradation, materials utilized for catalysis, and the profound impact of magnetic fields on enhancing reaction kinetics. This review also focuses on recent advances in the application and effect of magnetic fields in the magnetic and nonmagnetic catalysts towards dye degradation. This review provides a forward‐looking view, highlighting the potential of magnetic field‐enhanced photocatalysis to play a central role in sustainable energy and environmental management.

Enhancing thermal stability of optimal magnetization reversal in nanoparticles

Energy-efficient switching of nanoscale magnets requires application of a time-varying magnetic field characterized by microwave frequency. At finite temperatures, even weak thermal fluctuations induce perturbations in the magnetization that can accumulate in time, disrupt the phase locking between the magnetization and the applied field, and eventually compromise magnetization switching. It is demonstrated here that the magnetization reversal is mostly disturbed by unstable perturbations arising in a certain domain of the configuration space of a nanomagnet. The instabilities can be suppressed and the probability of magnetization switching enhanced by applying an additional stimulus such as a weak longitudinal magnetic field that ensures bounded dynamics of the perturbations. Application of the stabilizing longitudinal field to a uniaxial nanomagnet makes it possible to reach a desired probability of magnetization switching even at elevated temperatures. The principle of suppressing instabilities provides a general approach to enhancing thermal stability of magnetization dynamics. Published by the American Physical Society 2024

Barkhausen Noise as A Magnetic Nondestructive Testing Technique

Magnetic Barkhausen Noise (MBN) is a magnetic-based non-destructive electromagnetic testing method. Due to the electromagnetic working principle of MBN, it can be used for ferromagnetic materials, which consist of small magnetic fields discredited by domain walls and oriented in various directions. In an external magnetic field application, the fields turn to the magnetic direction, and the domain walls move and cause magnetic flux jumps. The jumps are named Barkhausen Noise (BN). The domain wall movements are sometimes pushed down by microstructure, composition, and defects. As the magnetic domain walls break away from the pinning sites produce MBN signal. MBN can be used for different material properties such as microstructure, composition, residual stress, and hardness. The paper's purpose is to analyze MBN as an improved NDT, clarify the relationship between material properties and MBN profile, and introduce MBN's applications and test equipment of MBN.

3D and 4D Printing of PETG-ABS-Fe3O4 Nanocomposites with Supreme Remotely Driven Magneto-Thermal Shape-Memory Performance.

This study introduces novel PETG-ABS-Fe3O4 nanocomposites that offer impressive 3D- and 4D-printing capabilities. These nanocomposites can be remotely stimulated through the application of a temperature-induced magnetic field. A direct granule-based FDM printer equipped with a pneumatic system to control the output melt flow is utilized to print the composites. This addresses challenges associated with using a high weight percentage of nanoparticles and the lack of control over geometry when producing precise and continuous filaments. SEM results showed that the interface of the matrix was smooth and uniform, and the increase in nanoparticles weakened the interface of the printed layers. The ultimate tensile strength (UTS) increased from 25.98 MPa for the pure PETG-ABS sample to 26.3 MPa and 27.05 MPa for the 10% and 15% Fe3O4 nanocomposites, respectively. This increase in tensile strength was accompanied by a decrease in elongation from 15.15% to 13.94% and 12.78%. The results of the shape-memory performance reveal that adding iron oxide not only enables indirect and remote recovery but also improves the shape-memory effect. Improving heat transfer and strengthening the elastic component can increase the rate and amount of shape recovery. Nanocomposites containing 20% iron oxide demonstrate superior shape-memory performance when subjected to direct heat stimulation and a magnetic field, despite exhibiting low print quality and poor tensile strength. Smart nanocomposites with magnetic remote-control capabilities provide opportunities for 4D printing in diverse industries, particularly in medicine, where rapid speed and remote control are essential for minimally invasive procedures.

Magnetically Controlled Strategies for Enhanced Tissue Vascularization

AbstractTissue vascularization plays a critical role in the regeneration and repair of damaged tissues. However, in certain instances of tissue injury, the pace and effectiveness of vascularization can be limited. Innovative strategies leveraging magnetic fields and magnetic nanoparticles (MNPs) are devised to enhance the efficacy of tissue vascularization. This review explores the potential of magnetic field‐assisted strategies in augmenting tissue vascularization and repair. Direct application of static or dynamic magnetic fields, alone or in combination with MNPs, offers a means to modulate cellular behaviors and gene expression, thereby promoting angiogenesis and tissue regeneration. Techniques such as cell labeling, gene delivery using MNPs, and magnetic targeting have shown promise in efficiently repairing various ischemic tissue injuries by enhancing tissue vascularization. These strategies have broad applications in bone and skin tissue regeneration, limb ischemia treatment, myocardial injury treatment, and diabetic wound therapy. By summarizing recent advancements in magnetically controlled strategies, this review aims to shed light on their future prospects in tissue regeneration and clinical treatment.

Dichotomous dynamics of magnetic monopole fluids

A recent advance in the study of emergent magnetic monopoles was the discovery that monopole motion is restricted to dynamical fractal trajectories [J. N. Hallén et al., Science 378, 1218 (2022)], thus explaining the characteristics of magnetic monopole noise spectra [R. Dusad et al., Nature 571, 234 (2019); A. M. Samarakoon et al., Proc. Natl. Acad. Sci. U.S.A. 119, e2117453119 (2022)]. Here, we apply this novel theory to explore the dynamics of field-driven monopole currents, finding them composed of two quite distinct transport processes: initially swift fractal rearrangements of local monopole configurations followed by conventional monopole diffusion. This theory also predicts a characteristic frequency dependence of the dissipative loss angle for AC field-driven currents. To explore these novel perspectives on monopole transport, we introduce simultaneous monopole current control and measurement techniques using SQUID-based monopole current sensors. For the canonical material Dy2Ti2O7, we measure [Formula: see text], the time dependence of magnetic flux threading the sample when a net monopole current [Formula: see text] is generated by applying an external magnetic field [Formula: see text] These experiments find a sharp dichotomy of monopole currents, separated by their distinct relaxation time constants before and after t ~[Formula: see text] from monopole current initiation. Application of sinusoidal magnetic fields [Formula: see text] generates oscillating monopole currents whose loss angle [Formula: see text] exhibits a characteristic transition at frequency [Formula: see text] over the same temperature range. Finally, the magnetic noise power is also dichotomic, diminishing sharply after t ~[Formula: see text]. This complex phenomenology represents an unprecedented form of dynamical heterogeneity generated by the interplay of fractionalization and local spin configurational symmetry.

Застосування індукційного топлення та постійного магнетного поля для впливу на перерозподіл компонентів з різними магнетними властивостями в зернах стопу на ос-нові Al–Cu–РЗМ

Застосування індукційного топлення та постійного магнетного поля для впливу на перерозподіл компонентів з різними магнетними властивостями в зернах стопу на ос-нові Al–Cu–РЗМ