All-optical Magnetization Switching Research Articles

Engineering Single-Shot All-Optical Switching of Ferromagnetic Materials.

Since it was recently demonstrated in a spin-valve structure, magnetization reversal of a ferromagnetic layer using a single ultrashort optical pulse has attracted attention for future ultrafast and energy-efficient magnetic storage or memory devices. However, the mechanism and the role of the magnetic properties of the ferromagnet as well as the time scale of the magnetization switching are not understood. Here, we investigate single-shot all-optical magnetization switching in a GdFeCo/Cu/[CoxNi1-x/Pt] spin-valve structure. We demonstrate that the threshold fluence for switching both the GdFeCo and the ferromagnetic layer depends on the laser pulse duration and the thickness and the Curie temperature of the ferromagnetic layer. We are able to explain most of the experimental results using a phenomenological model. This work provides a way to engineer ferromagnetic materials for energy efficient single-shot all-optical magnetization switching.

Magnetic and all-optical switching properties of amorphousTbxCo100−xalloys

Amorphous Tb$_{x}$Co$_{100-x}$ magnetic alloys exhibit a list of intriguing properties, such as perpendicular magnetic anisotropy, high magneto-optical activity and magnetization switching using ultrashort optical pulses. Varying the Tb:Co ratio in these alloys allows for tuning properties such as the saturation magnetic moment, coercive field and the performance of the light-induced magnetization switching. In this work, we investigate the magnetic, optical and magneto-optical properties of various Tb$_{x}$Co$_{100-x}$ thin film alloy compositions. We report on the effect the choice of different seeding layers has on the structural and magnetic properties of Tb$_{x}$Co$_{100-x}$ layers. We also demonstrate that for a range of alloys, deposited on fused silica substrates, with Tb content of 24-30 at.$\%$, helicity dependent all-optical switching of magnetization can be achieved, albeit in a multi-shot framework. We explain this property to arise from the helicity-dependent laser induced magnetization on the Co sublattice due to the inverse Faraday effect. Our study provides an insight into material aspects for future potential hybrid magneto-plasmonic TbCo-based architectures.

Element-Specific Magnetization Dynamics of Complex Magnetic Systems Probed by Ultrafast Magneto-Optical Spectroscopy

The vision to manipulate and control magnetism with light is driven on the one hand by fundamental questions of direct and indirect photon-spin interactions, and on the other hand by the necessity to cope with ever growing data volumes, requiring radically new approaches on how to write, read and process information. Here, we present two complementary experimental geometries to access the element-specific magnetization dynamics of complex magnetic systems via ultrafast magneto-optical spectroscopy in the extreme ultraviolet spectral range. First, we employ linearly polarized radiation of a free electron laser facility to demonstrate decoupled dynamics of the two sublattices of an FeGd alloy, a prerequisite for all-optical magnetization switching. Second, we use circularly polarized radiation generated in a laboratory-based high harmonic generation setup to show optical inter-site spin transfer in a CoPt alloy, a mechanism which only very recently has been predicted to mediate ultrafast metamagnetic phase transitions.

Dynamics of all-optically switched magnetic domains in Co/Gd heterostructures with Dzyaloshinskii-Moriya interaction

Given the development of hybrid spintronic-photonic devices and chiral magnetic structures, a combined interest in all-optical switching (AOS) of magnetization and current-induced domain wall motion in synthetic ferrimagnetic structures with strong Dzyaloshinskii-Moriya Interaction (DMI) is emerging. In this study, we report a study on single-pulse all-optical toggle switching and asymmetric bubble expansion in specially engineered Co/Gd-based multilayer structures. In the absence of any external magnetic fields, we look into the AOS properties and the potential role of the DMI on the AOS process as well as the stability of optically written micro-magnetic domains. Particularly, interesting dynamics are observed in moon-shaped structures written by two successive laser pulses. The stability of domains resulting from an interplay of the dipolar interaction and domain-wall energy are compared to simple analytical models and micromagnetic simulations.

Interlayer exchange coupling modulated all-optical magnetic switching in synthetic ferrimagnetic heterostructures

All-optical magnetic switching in ferromagnetic thin films reveals an unprecedented route to manipulate magnetic configurations for future ultrafast and energy-efficient magnetic storage. In this study, the relationship between the all-optical magnetic switching and interlayer exchange coupling was investigated in a [Co/Pt]n/Ru/GdFeCo synthetic ferrimagnetic heterostructure. While a thermal demagnetization is dominant in a single GdFeCo alloy film after laser sweep, the magneto-optical interaction transits to a clear all-optical magnetic switching after GdFeCo film being exchange coupled with a [Co/Pt]n multilayer. Meanwhile, the established interlayer exchange coupling can also significantly increase the optical-induced magnetization switching ratio in [Co/Pt]n multilayer after single-pulse laser illumination. A threshold interlayer exchange coupling strength of ∼0.31 erg cm−2 was confirmed for achieving a deterministic (∼90%) optical-induced magnetization switching ratio after multi-pulse laser illumination. This study demonstrates a clear correlation between interlayer exchange coupling and all-optical magnetic switching, offering a promising engineering pathway for high density all-optical magnetic recording.

Exchange-driven all-optical magnetic switching in compensated 3d ferrimagnets

The authors experimentally resolve the pulse- and temperature-dependent limits of single-shot alloptical magnetic switching in the compensated three dimensional ferrimagnet, revealing that the process is driven by exchange relaxation.

Deterministic all-optical magnetization writing facilitated by non-local transfer of spin angular momentum

Ever since its discovery around a decade ago, all-optical magnetization switching (AOS) using femtosecond laser pulses has shown potential for future data storage and logic devices. In particular, single pulse helicity independent AOS in certain ferrimagnetic alloys and multilayers is highly efficient and ultrafast. However, in most cases it is a toggle mechanism, which is not desirable for applications. Here we experimentally demonstrate conversion from toggle switching to a deterministic mechanism by biasing AOS in a Co/Gd bilayer with a spin polarized current which is optically generated in an adjacent ferromagnetic reference layer. We show deterministic writing of an ‘up’ and ‘down’ state using a sequence of one or two pulses, respectively, and demonstrate the non-local origin by varying the magnitude of the generated spin current. Our demonstration of deterministic magnetization writing could provide an essential step towards the implementation of future optically addressable spintronic memory devices.

Enhanced ultrafast optomagnetic effects in room-temperature ferromagnetic Pt nanoclusters embedded in silica by ion implantation

Ferromagnetic-like behavior at room temperature (300 K) was observed in Pt particles embedded in ion-implanted silica matrices. Results in samples integrated by ultra-small photoluminescent Pt clusters (<2 nm) were compared with samples containing exclusively larger plasmonic Pt nanoparticles (>3 nm). The ferromagnetic behavior coexists simultaneously with a diamagnetic response. Enhanced diamagnetic response of one order of magnitude was observed compared to typical diamagnetism in pure silica, and it is increased with the mean diameter of the Pt particles. Besides, a larger sensitivity to an external field was observed in the ferromagnetic response of the nanostructures with a characteristic saturation at 20 kOe. This ferromagnetic behavior was only observed in the samples with nucleated Pt particles. The magnitude of the saturation magnetization shows up to a fivefold increase in the samples with smaller particle size and larger particle density. Saturation magnetization was observed between 3–15 × 10−4 emu g−1, with remanent magnetization of 0.2–0.6 × 10−4emu g−1, measured at 300 K. Coercitive fields also decrease in samples with smaller size and particles density, with values of 114 and 300 Oe. At lower temperatures (5 K) the saturation magnetization increases, as it would be expected from a ferromagnetic state. Optomagnetic response was studied by inverse Faraday effects and induced photomagnetization with circular polarized picosecond pulsed light at 1064 nm wavelength. Results showed that samples with a stronger ferromagnetic response exhibit larger Faraday rotation up to 5.3 × 103deg cm−1 by light excitations with irradiances between 50 and 180 GW cm−2. These findings have immediate applications in multifunctional solid-state magneto-optical devices such as optical isolators, high-data storage devices and ultrafast all-optical switching of magnetization.

Single-shot all-optical switching of magnetization in Tb/Co multilayer-based electrodes

Ever since the first observation of all-optical switching of magnetization in the ferrimagnetic alloy GdFeCo using femtosecond laser pulses, there has been significant interest in exploiting this process for data-recording applications. In particular, the ultrafast speed of the magnetic reversal can enable the writing speeds associated with magnetic memory devices to be potentially pushed towards THz frequencies. This work reports the development of perpendicular magnetic tunnel junctions incorporating a stack of Tb/Co nanolayers whose magnetization can be all-optically controlled via helicity-independent single-shot switching. Toggling of the magnetization of the Tb/Co electrode was achieved using either 60 femtosecond-long or 5 picosecond-long laser pulses, with incident fluences down to 3.5 mJ/cm2, for Co-rich compositions of the stack either in isolation or coupled to a CoFeB-electrode/MgO-barrier tunnel-junction stack. Successful switching of the CoFeB-[Tb/Co] electrodes was obtained even after annealing at 250 °C. After integration of the [Tb/Co]-based electrodes within perpendicular magnetic tunnel junctions yielded a maximum tunneling magnetoresistance signal of 41% and RxA value of 150 Ωμm2 with current-in-plane measurements and ratios between 28% and 38% in nanopatterned pillars. These results represent a breakthrough for the development of perpendicular magnetic tunnel junctions controllable using single laser pulses, and offer a technologically-viable path towards the realization of hybrid spintronic-photonic systems featuring THz switching speeds.

Magnetization reversal more rapidly by using an ultrashort square-wave laser

With the feature of low-power and ultrashort time magnetization manipulation, all optical magnetic switching (AOMS) has been propelled to the forefront in investigations. To further speed up the magnetization reversal, in this paper, based on the combination of heating and Inverse Faraday Effect (IFE), an ultrashort square-wave laser (USWL) pulse is explored to excite the reversal of magnetization in a Co/Pt system, and all the parameters necessary for our simulation are well within the current theoretical estimates. Simulation results show that the switching time of magnetization is 3 times faster than the using of a traditional ultrashort Gaussian wave laser (UGWL) under the same laser fluence F = 4 mJ/cm2 and pulse duration t0 = 35 fs, and the threshold of AOMS for the ferromagnet is 0.67 mJ/cm2. We furthermore demonstrate that the heat accumulating effect of a laser-pulse is an important factor that influences the switching time, and a USWL has a larger effect of heat accumulating than a UGWL. At present, the debate on the origin of helicity dependent AOMS is still going on, and the model we propose provide a guideline for achieving helicity dependent AOMS more rapidly. We believe that the results could potentially be used to the field of storage technology especially for the using of AOMS.

Application of Layered Structure for Efficient Light Absorption and Ultra-thin Film Formation in Material that Induces All-Optical Magnetization Switching

Application of Layered Structure for Efficient Light Absorption and Ultra-thin Film Formation in Material that Induces All-Optical Magnetization Switching

Pathways for Single-Shot All-Optical Switching of Magnetization in Ferrimagnets

We resolve a significant controversy about how to understand and engineer single-shot all-optical switching of magnetization in ferrimagnets using femto- or picosecond-long heat pulses. By realistically modelling a generic ferrimagnet as two coupled macrospins, we comprehensively show that the net magnetization can be reversed via different pathways, using a heat pulse with duration spanning all relevant timescales within the non-adiabatic limit. This conceptual understanding is fully validated by experiments studying the material and optical limits at which the switching process in GdFeCo alloys loses its reliability. Our interpretation and results constitute a blueprint for understanding how deterministic all-optical switching can be achieved in alternative ferrimagnets using short thermal pulses.

Hysteretic optomagnetic bistability based on the plasmon-induced inverse Faraday effect in magnetoplasmonic disk resonators

We investigate the inverse Faraday effect (IFE) by surface plasmon traveling modes in an ultracompact magnetoplasmonic disk resonator side-coupled to a plasmonic waveguide. The magnetic field by the IFE reacts to the traveling modes and leads to a nonlinear shift of the resonance in the disk resonator. Describing those nonlinear phenomena analytically by using the temporal coupled mode theory and the Lorentz reciprocity theorem, we propose a conception of hysteretic optomagnetic bistability that the system has two stable states of optically induced magnetic field to switch on and off, depending upon the history of the incident optical power. The numerical simulations agree well with the analytical prediction. The proposed conception may find potential applications in all-optical magnetic recording and switching with nanometer resolution.

Magneto-optical painting of heat current

Active control of heat flow is crucial for the thermal management of increasingly complex electronic and spintronic devices. In addition to conventional heat transport engineering, spin caloritronics has received extensive attention as a heat control principle owing to its high controllability and unique thermal energy conversion symmetry. Here we demonstrate that the direction of heat currents generated by spin-caloritronic phenomena can be changed simply by illuminating magnetic materials with visible light. The optical control of heat currents is realized through a combination of the spin-driven thermoelectric conversion called an anomalous Ettingshausen effect and all-optical helicity-dependent switching of magnetization. This approach enables not only pinpoint manipulation and flexible design of the heat current distribution by patterning the illuminating light but also on/off control of the resulting temperature modulation by tuning the light polarization. These versatile heat control functionalities will open up a pathway for nanoscale thermal energy engineering.

Multi-layer magnetic recording driven by a tunable laser

All-optical magnetization switching with features of low-power consumption and high writing speed is a promising road map to satisfy the demand for volume data storage. To promote denser and faster magnetic recording technologies, herein, all-optical helicity-dependent switching (AO-HDS) in multi-layer magnetic recording is proposed based on the chromatic aberration of an optical lens (Thorlabs’s N-BK7 plano-convex uncoated lens). The power of the incident beams and the thickness of the multi-layer magnetic recording film are designed carefully. Besides, the uniformity of this multi-layer magnetic recording is optimized. At last, a prototype system of information multiplexing based on this multi-layer magnetic recording technology is constructed as well. Flexible and controllable magnetization reversals in different layers are also demonstrated by tuning the wavelength and helicity of working beams. We believe that such a prototype system can pave the way for increasing the storage density in an effective and low-cost mode.

Theoretical Investigation of All Optical Switching by Intersystem Crossing

The dynamics of spin flips induced by the femtosecond laser are theoretically investigated in this article. The spin flips in this scenario are attributed to the intersystem crossing (ISC) described within the frame of the Rabi model. This new explanation is a step attempting to explain the mechanism of the all-optical magnetic orientation switching in the perspective of the conservation of the angular momentum and breaks of the selection rule, which is ignored in the Raman scattering related explanations. The final spin states discussed herein are closely related to the intensity of the incident laser and the ISC decay rate. The quantitative analysis of the relation between decay rate, temperature and the intensity of the laser is discussed.

Role of compensation points in all-optical magnetization switching

We study theoretically the role of compensation points in all-optical magnetization switching (AOS) in rare-earth transition-metal ferrimagnets. We use the s-d model in which localized spins are coupled with spins of itinerant electrons via the s-d exchange interaction. The main advantage of the model is that it considers the dynamics of both localized and itinerant spin population. We show that the compensation temperature, which is relevant to AOS, is determined by the net spin polarization, i.e., by the sum of the spin polarizations of localized and itinerant spins. This temperature does not coincide exactly with either the magnetization compensation temperature or the angular momentum compensation temperature.

Plasmonic layer-selective all-optical switching of magnetization with nanometer resolution

All-optical magnetization reversal with femtosecond laser pulses facilitates the fastest and least dissipative magnetic recording, but writing magnetic bits with spatial resolution better than the wavelength of light has so far been seen as a major challenge. Here, we demonstrate that a single femtosecond laser pulse of wavelength 800 nm can be used to toggle the magnetization exclusively within one of two 10-nm thick magnetic nanolayers, separated by just 80 nm, without affecting the other one. The choice of the addressed layer is enabled by the excitation of a plasmon-polariton at a targeted interface of the nanostructure, and realized merely by rotating the polarization-axis of the linearly-polarized ultrashort optical pulse by 90°. Our results unveil a robust tool that can be deployed to reliably switch magnetization in targeted nanolayers of heterostructures, and paves the way to increasing the storage density of opto-magnetic recording by a factor of at least 2.

Writing magnetic memory with ultrashort light pulses

Laser pulses are the shortest stimulus known to control the magnetization of materials and to switch magnetic devices on the picosecond to femtosecond timescales. Femtosecond laser pulses have been able to trigger the fastest changes in the magnetic state of matter, and thus these pulses may lead to technologies with increased speed and energy efficiency of magnetic data storage and memory. In the past decade, materials enabling optical control of magnetism and concepts of devices employing such opto-magnetic phenomena have been shown. In this Review, we explore ultrafast all-optical switching (AOS) of magnetization as the least-dissipative and fastest method for magnetic writing. We outline the physical processes responsible for mechanisms of AOS, define the materials suitable for optical control of magnetism and test these mechanisms and materials against three important criteria of recording: speed, accompanying dissipations and scalability. In particular, we emphasize that switching magnetization with the help of light outperforms other methods in terms of the speed of the write–read magnetic recording event (less than 20 ps) and the unprecedentedly low heat load (<6 J cm−3). Finally, we outline the integration of AOS in spintronic devices and the perspective of large-scale integration towards magnetic random access memory and other memory applications with low-energy dissipations. Laser pulses can trigger fast changes in magnetic state, facilitating new magnetic data storage and memory devices. This Review outlines the mechanisms of all-optical switching and the materials suitable for the optical control of magnetism and tests these mechanisms and materials in terms of speed, accompanying dissipations and scalability. Finally, the large-scale integration of devices in memory applications with low-energy dissipations is discussed.

All-optical magnetization switching by counterpropagataion or two-frequency pulses using the plasmon-induced inverse Faraday effect in magnetoplasmonic structures

In this Letter we study the generation of quasi-static magnetic fields by the plasmon-induced inverse Faraday effect and propose a magneto-optical waveguide structure for achieving magnetization switching at sub-ps time in a nano-confined magneto-optical structure. In particular we show that the direction of the generated quasi-static field in a magneto-optical dielectric cavity side-coupled to a metal-insulator-metal (MIM) waveguide depends sensitively on the wavelength of the surface plasmon polaritions (SPP). This phenomenon could open up a new energy-efficient ultrafast method for nano-confined all-optical magnetization switching by two-frequency pulses.