Effects Of Aerosols Research Articles

Understanding the response of tropical overturning circulations to greenhouse gas and aerosol forcing

Abstract While observational records provide evidence for strengthening of the Pacific Walker circulation and the boreal winter Hadley cell (HC) over the last few decades, the underlying causes are not well understood. This study investigates the radiative effects of CO2 and anthropogenic aerosols on regional variations in the intensity of tropical meridional (Hadley-like) and zonal (Walker-like) overturning circulations, based on a suite of experiments using the IITM Earth System Model (IITM-ESM) along with supplementary analysis of observed and reanalysis datasets. Two key findings emerge from our study (i) strengthening of the Pacific Walker circulation with enhanced zonal sea surface temperature (SST) gradients and precipitation increase over the tropical Indo-Pacific, in response to global warming via ocean-atmosphere coupled feedbacks (ii) aerosol-induced intensification of regional meridional overturning circulation over the (0 − 120◦E) longitudinal domain resulting from inter hemispheric energy imbalance and southward shift of the southern hemispheric (SH) rainfall belt extending eastward from Africa across the Indian Ocean. Our results suggest that the combined radiative influence of increased CO2 and northern hemispheric (NH) anthropogenic aerosols reinforces the regional meridional overturning circulation, by enhancing convection over the SH and promoting widespread descent over the NH subtropics and mid-latitudes covering northern Africa, Mediterranean, parts of middle-East, West and South Asia. The present findings have important implications for the regional water resources, agriculture and environment.

Distinct structure, radiative effects, and precipitation characteristics of deep convection systems in the Tibetan Plateau compared to the tropical Indian Ocean

Abstract. Using spaceborne lidar and radar observations, this study identifies deep convection systems (DCSs), including deep convection cores (DCCs) and anvils, over the Tibetan Plateau (TP) and tropical Indian Ocean (TO) and finds that DCSs over the TP are less frequent, exhibiting narrower and thinner DCCs and anvils compared to those over the TO. The thinner DCCs over the TP exert weaker radiative cooling effects at the top of atmosphere (TOA) compared to the TO. But, the shortwave TOA cloud radiative effect (CRE) of TP anvils is stronger than that of the TO possibly due to more densely packed cloud tops over the TP. It results in a stronger TOA CRE of DCSs over the TP than that of TO. In particular, the longwave CRE of DCSs over the TP is notably greater at surface and low-level atmosphere due to the distinct lower temperature and less water vapour. The width of DCSs shows a positive correlation with wind shear and atmospheric instability, and the underlying mechanisms are discussed. We also find that the impact of aerosols on cloud top heights and precipitation displays significant discrepancies between the two regions. It is because that the aerosol invigoration effect is less efficient on the TP DCSs, mainly attributed to the significantly colder cloud base. Due to competition between invigoration and direct/semi-direct radiative effects of aerosols, the correlation between precipitation and aerosols over the TP is not obvious. However, precipitation in the TO experiences invigoration followed by suppression with increasing aerosols, due to the dominance of aerosol radiative effects and enhancement entrainment under polluted conditions.

Large effects of fine and coarse aerosols on tropical deep convective systems throughout their lifecycle

Previous studies have shown that aerosols invigorate deep convective systems (DCS). However, the magnitude or even the existence of aerosol invigoration of DCS remains controversial. Here, we aimed to observationally quantify the full aerosol effects on DCS by tracking their entire lifecycle and spatial extent in tropical regions. We found that fine aerosols (FA) can invigorate DCS, making them taller and longer lived, and resulting in up to ×5 increase in total area and rainfall amount. In contrast, added coarse sea salt aerosols (CSA) over the ocean can inhibit the vertical development of DCS through enhancing warm rain formation, yet resulting in longer lived and extensive DCSs. Notably, combining FA and CSA generates the strongest aerosol invigoration effect at the concentrations of ~5 and ~80 μg/m³, leading up to ×10 increase in rainfall amount. Our results indicate that aerosols significantly redistribute convective precipitation and climate effects, greatly underestimated in previous studies.

Aerosol effects during heat waves in summer 2022 and responses to emission change over China

This study explores aerosol direct, indirect, and feedback effects on meteorology and fine particulate matter during heat waves of August 2022 over eastern China by using an online coupled regional climate–chemistry–aerosol model. In this period, aerosols exerted mean direct (DRE) and indirect (IRE) radiative effects of −3.9 Wm−2 and −2.4 Wm−2 at TOA, which totally caused a decrease in average surface air temperature by 0.3 °C over east China, accompanied by decreases in PBLH (planetary boundary layer height) and precipitation and an increase in PM2.5 concentration. With the anthropogenic emission reduction from 2013 to 2022, DRE apparently decreased while IRE changed little, leading to a decrease in total aerosol radiative effect (TRE) by 27% at TOA. The weakened TRE resulted in increases in surface air temperature and precipitation by 0.14 °C and 2.7 mm, respectively, on average over east China, with the maximum warming exceeding 0.5 °C in BTH (Beijing–Tianjin–Hebei province). This study highlights a warming trend due to weakened TRE, which may exacerbate heat wave, and an increasing importance of aerosol IRE relative to DRE due to weak sensitivity of cloud properties to aerosol change during the emission reduction.

Effects of mixed aerosol on the path loss of NLOS UV communication system

Effects of mixed aerosol on the path loss of NLOS UV communication system

The atmospheric effect of aerosols on future tropical cyclone frequency and precipitation in the Energy Exascale Earth System Model

This study uses experiments from the Energy Exascale Earth System Model (E3SM) to compare the influence on tropical cyclone (TC) activity of: (i) the atmospheric effect of aerosols under specified sea-surface temperatures (SSTs); and (ii) the net effect of greenhouse gases (GhGs) (including changes in SSTs). The experiments were performed using the CMIP6 Shared Socioeconomic Pathway SSP5-8.5 emissions scenario with GhG-induced SST warming specified and atmospheric aerosol effects simulated but without explicit ocean coupling. Insignificant changes in global TC frequency are found in response to the atmospheric effect of future aerosols and GhGs, as significant regional responses in TC frequency counteract each other. Future GhGs contribute to more frequent TCs in the North Atlantic, and reductions over the Northwestern Pacific and Southern Indian Ocean. The atmospheric effect of future aerosols drives more frequent TCs over the Northwestern Pacific and reductions over the Northeast Pacific and North Atlantic. Along with increases in TC intensity, global TC precipitation (TCP) is projected to increase by 52.8% (14.1%/K) due to the combined effect of future aerosols and GhGs. Although both forcings contribute to TCP increases (14.7–19.3% from reduced aerosols alone and 28.1–33.3% from increased GhGs alone), they lead to different responses in the spatial structure of TCP. TCP increases preferentially in the inner-core due to increased GhGs, whereas TCP decreases in the inner-core and increases in the outer-bands in response to the atmospheric effects of decreased aerosols. These changes are distinct from those caused by aerosol-induced SST changes, which have been considered in other studies.

Residential Wood Burning and Vehicle Emissions as Major Sources of Environmentally Persistent Free Radicals in Fairbanks, Alaska.

Environmentally persistent free radicals (EPFRs) play an important role in aerosol effects on air quality and public health, but their atmospheric abundance and sources are poorly understood. We measured EPFRs contained in PM2.5 collected in Fairbanks, Alaska, in winter 2022. We find that EPFR concentrations were enhanced during surface-based inversion and correlate strongly with incomplete combustion markers, including carbon monoxide and elemental carbon (R2 > 0.75). EPFRs exhibit moderately good correlations with PAHs, biomass burning organic aerosols, and potassium (R2 > 0.4). We also observe strong correlations of EPFRs with hydrocarbon-like organic aerosols, Fe and Ti (R2 > 0.6), and single-particle mass spectrometry measurements reveal internal mixing of PAHs, with potassium and iron. These results suggest that residential wood burning and vehicle tailpipes are major sources of EPFRs and nontailpipe emissions, such as brake wear and road dust, may contribute to the stabilization of EPFRs. Exposure to the observed EPFR concentrations (18 ± 12 pmol m-3) would be equivalent to smoking ∼0.4-1 cigarette daily. Very strong correlations (R2 > 0.8) of EPFR with hydroxyl radical formation in surrogate lung fluid indicate that exposure to EPFRs may induce oxidative stress in the human respiratory tract.

Aerosol-Induced Changes in Atmospheric and Oceanic Heat Transports in the CESM2 Large Ensemble

Abstract The total poleward energy transport (PET) is set by the top of atmosphere radiation flux, and is therefore sensitive to any process which can alter those fluxes, particularly in the shortwave. One example is the direct and indirect effects of anthropogenic aerosols, which increase the local reflection of solar radiation back to space. The historic emission of sulphur dioxide, which peaked in the northern midlatitudes during the 1980s, has been proposed as a primary contributor to historic anomalies in cross-equatorial energy transport, as well as related processes such as a shift in the tropical rainband. In this study, we analyze simulations from the CESM2 large ensemble and single-forcing projects to better understand the forced response of PET to historical forcings. First, analysis of the single-forcing project reveals that the position of the ITCZ responds in a non-linear manner to greenhouse gas forcing in CESM2. This type of non-linearity has been found previously in the context of the aerosol-only simulations in the CESM2 single-forcing project, but may be the first identification of a similar effect in the greenhouse gas-only simulations. Second, through analysis of the full CESM2 large ensemble simulations, we find that anomalous heat transport occurred in both the atmosphere (through the mean meridional circulation and atmospheric eddies) and in the oceans (through the Atlantic and Indo-Pacific sectors) due to a variety of related processes including the Hadley cells, the midlatitude storm tracks, the Atlantic Meridional Overturning Circulation (AMOC), and the Pacific wind-driven subtropical gyre.

Tiny rain makers: How aerosols shape extreme rainfall simulation accuracy

Given the rapid spatiotemporal variability of aerosols and their complex impacts on the Earth system, investigating the role of aerosols in modelling extreme weather events, particularly various extreme rainfalls, remains limited. This study explored extreme rainfall simulation sensitivity to aerosol properties, transport and seasonality over the UK and Ireland during four seasons in 2020 by the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) model. Two sets of high-resolution simulations, one including aerosol direct and indirect effects and the other one without any aerosol effects, were conducted to investigate the improvements due to aerosol inputs. Meteorological results were verified using ground and satellite observations to examine the reliability of simulations. The 12 extreme rainfall events during the study months were classified by their backward trajectories from the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model, and their simulation accuracies were quantified through six spatiotemporal metrics and one overall score. By comprehensive analyses of the simulation performances under different conditions, it is found that the model performs better in simulating rainfall events driven by sea salt aerosols (SSA) compared to those promoted by anthropogenic aerosols. Air masses transported from the Arctic and North Atlantic Ocean also help achieve higher rainfall simulation accuracy than European air masses. Rainfall simulations for winter and autumn events outperform those for spring and summer events. When considering aerosol effects in simulations, almost half of the events showed improved performance, while an equal number experienced a decrease and a small proportion remained unchanged. The most remarkable improvements are observed in rainfall simulations with higher concentrations of SSA and the participation of anthropogenic aerosols, while simulations promoted only by anthropogenic aerosols all experience performance reductions. The aerosol effects also led to significant increases in monthly rainfalls, accompanied by great reductions of Cl in larger particle size aerosols and NO3 in smaller particle size aerosols.

Combined effects of fine and coarse marine aerosol on vertical raindrop size distribution

Climate models commonly overestimate warm rain frequency and underestimate its intensity over the ocean, primarily due to insufficient representation of the aerosol effects. This pertains to both fine aerosols (FA) and coarse sea spray aerosols (CSA), where the latter is mostly absent in the models. Here, our observations show that adding CSA enhances vertical warm rain structure, in contrast to the effect of FA. The magnitude of the effect of CSA is larger than the opposite effect of the FA. For rain with top heights of 2–3 km, the raindrop size, concentration, and rain rate can be increased by factors of 1.03, 1.47, and 1.60, respectively. These CSA-induced changes are larger for thicker clouds, reaching a maximum by factors of 1.12, 1.85, and 2.21, respectively. Therefore, the combined FA and CSA effects should be incorporated into climate models for accurately simulated precipitation microphysical processes.

An Investigation on Causes of the Detected Surface Solar Radiation Brightening in Europe Using Satellite Data

AbstractSurface solar radiation is fundamental for terrestrial life. It provides warmth to make our planet habitable, drives atmospheric circulation, the hydrological cycle and photosynthesis. Europe has experienced an increase in surface solar radiation, termed “brightening,” since the 1980s. This study investigates the causative factors behind this brightening. A novel algorithm from the EUMETSAT satellite application facility on climate monitoring (CM SAF) provides the unique opportunity to simulate surface solar radiation under various atmospheric conditions for clouds (clear‐sky or all‐sky), aerosol optical depth (time‐varying or climatological averages) and water vapor content (with or without its direct influence on surface solar radiation). Through a multiple linear regression approach, the study attributes brightening trends to changes in these atmospheric parameters. Analyzing 61 locations distributed across Europe from 1983 to 2020, aerosols emerge as key driver during 1983–2002, with Southern Europe and high elevations showing subdued effects (0%/decade–1%/decade) versus more pronounced impacts in Northern and Eastern Europe (2%/decade–6%/decade). Cloud effects exhibit spatial variability, inducing a negative effect on surface solar radiation (−3%/decade–−2%/decade) at most investigated locations in the same period. In the period 2001–2020, aerosol effects are much smaller, while cloud effects dominate the observed brightening (2%/decade–5%/decade). This study therefore finds a substantial decrease in the cloud radiative effect over Europe in the first two decades of the 21st century. Water vapor exerts negligible influence in both sub‐periods.

Interdecadal variations of aerosol and its composition over the Fenwei Plain based on multi-source observations

Understanding the variations and potential source of air pollution is essential for implementing targeted mitigation actions. However, the distribution and long-term trends of Aerosol Optical Depth (AOD) and its components over the Fenwei Plain (FWP) have not been thoroughly investigated. Furthermore, the potential source contribution of AOD loading is still unclear. Thus, maximum synthesis and Mann-Kendall trend (MK) test with Sen's Slope methods are employed to reveal the spatiotemporal variation characteristics of AOD over the FWP. The Potential Source Contribution Function (PSCF) model was applied to analyze the potential source contribution of AOD over the FWP. Results demonstrated that the AOD in spatial pattern exhibited consistency with the topography. AOD over the FWP fluctuated annually from 2000 to 2020, with an increase in the previous decade followed by a gradual decline after 2011. There was a significant monthly variation in AOD with higher values in August (0.47±0.21) and lower in November (0.29±0.12). A positive AOD trend was confirmed from 2000 to 2010 yet a negative trend is identified from 2011 to 2020. The sulfate aerosol (AODSU) exhibited an increasing trend over an extended period. Clear-sky radiation shows a negative trend at the surface and the top of the atmosphere (TOA) from 2000 to 2010, which is consistent with the trend in AOD. The AOD in FWP was primarily influenced by local emissions, with contributions from northern and northwestern sources. This research offers an enhanced overarching comprehension of the distribution and regional climate effects of aerosols over the FWP.

Changes in the Direct Climate Effect of Black Carbon Aerosols in East Asia Under the “Dual Carbon” Goal of China

AbstractIn the context of China's “dual carbon” goal, emissions of air pollutants are expected to significantly decrease in the future. Thus, the direct climate effects of black carbon (BC) aerosols in East Asia are investigated under this goal using an updated regional climate and chemistry model. The simulated annual average BC concentration over East Asia is approximately 1.29 μg/m3 in the last decade. Compared to those in 2010–2020, both the BC column burden and instantaneous direct radiative forcing in East Asia decrease by more than 55% and 80%, respectively, in the carbon peak year (2030s) and the carbon neutrality year (2060s). Conversely, the BC effective radiative forcing (ERF) and regional climate responses to BC exhibit substantial nonlinearity to emission reduction, possibly resulting from different adjustments of thermal‐dynamic fields and clouds from BC‐radiation interactions. The regional mean BC ERF at the tropopause over East Asia is approximately +1.11 W/m2 in 2010–2020 while negative in the 2060s. BC‐radiation interactions in the present‐day impose a significant annual mean cooling of −0.2 to −0.5 K in central China but warming +0.3 K in the Tibetan Plateau. As China's BC emissions decline, surface temperature responses show a mixed picture compared to 2010–2020, with more cooling in eastern China and Tibet of −0.2 to −0.3 K in the 2030s, but more warming in central China of approximately +0.3 K by the 2060s. The Indian BC might play a more important role in East Asian climate with reduction of BC emissions in China.

First atmospheric aerosol-monitoring results from the Geostationary Environment Monitoring Spectrometer (GEMS) over Asia

Abstract. Aerosol optical properties have been provided by the Geostationary Environment Monitoring Spectrometer (GEMS), the world's first geostationary-Earth-orbit (GEO) satellite instrument designed for air quality monitoring. This study describes improvements made to the GEMS aerosol retrieval (AERAOD) algorithm, including spectral binning, surface reflectance estimation, cloud masking, and post-processing, along with validation results. These enhancements aim to provide more accurate and reliable aerosol-monitoring results for Asia. The adoption of spectral binning in the lookup table (LUT) approach reduces random errors and enhances the stability of satellite measurements. In addition, we introduced a new high-resolution database for surface reflectance estimation based on the minimum-reflectance method, which was adapted to the GEMS pixel resolution. Monthly background aerosol optical depth (BAOD) values were used to estimate hourly GEMS surface reflectance consistently. Advanced cloud-removal techniques have been implemented to significantly improve the effectiveness of cloud detection and enhance aerosol retrieval quality. An innovative post-processing correction method based on machine learning has been introduced to address artificial diurnal biases in aerosol optical depth (AOD) observations. In this study, we investigated selected aerosol events, highlighting the capability of GEMS in monitoring and providing insights into hourly aerosol optical properties during various atmospheric events. The performance of the GEMS AERAOD products was validated against the Aerosol Robotic Network (AERONET) and Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data for the period from November 2021 to October 2022. GEMS AOD at 443 nm demonstrated a strong correlation with AERONET AOD at 443 nm (R = 0.792). However, it exhibited biased patterns, including the underestimation of high AOD values and overestimation of low-AOD conditions. Different aerosol types (highly absorbing fine aerosols, dust aerosols, and non-absorbing aerosols) exhibited distinct validation results. The retrievals of GEMS single-scattering albedo (SSA) at 443 nm agreed well with the AERONET SSA at 440 nm within reasonable error ranges, with variations observed among aerosol types. For GEMS AOD at 443 nm exceeding 0.4 (1.0), 42.76 % (56.61 %) and 67.25 % (85.70 %) of GEMS SSA data points fell within the ±0.03 and ±0.05 error bounds, respectively. Model-enforced post-processing correction improved GEMS AOD and SSA performance, thereby reducing the diurnal variation in the biases. The validation of the retrievals of GEMS aerosol layer height (ALH) against the CALIOP data demonstrates good agreement, with a mean bias of −0.225 km and 55.29 % (71.70 %) of data points falling within ±1 km (1.5 km).

Anthropogenic effects on tropical cyclones near Western Europe

There is less consensus on whether human activities have significantly altered tropical cyclone (TC) statistics, given the relatively short duration of reliable observed records. Understanding and projecting TC frequency change is more challenging in certain coastal regions with lower TC activity yet high exposure, such as Western Europe. Here, we show, with large-ensemble simulations, that the observed increase in TC frequency near Western Europe from 1966 to 2020 is likely linked to the anthropogenic aerosol effect. Under a future scenario featuring regionally controlled aerosol emissions and substantially increased greenhouse gas concentrations (Shared Socioeconomic Pathway 5-85), our simulations show a potential decrease in TC frequency near Western Europe by the end of the 21st century. These contrasting trends in historical and future TC frequencies are primarily due to the rise for 1966–2020 and potentially subsequent fall for 2030–2100 in TC genesis frequency in the North Atlantic. The response of large-scale environmental conditions to anthropogenic forcing is found to be crucial in explaining the historical and future changes in TC frequency near Western Europe.

Cloud Susceptibility to Aerosols: Comparing Cloud‐Appearance Versus Cloud‐Controlling Factors Regimes

AbstractClouds can be classified into regimes based on their appearance or meteorological controlling factors. The cloud appearance regimes inherently include adjustments to aerosol effects, such as transitions between closed and open cells. Therefore, calculating cloud susceptibilities to aerosols for each cloud‐appearance regime individually and then aggregating them excludes much of the cloud adjustment component of the susceptibilities. In contrast, aggregating susceptibilities over regimes defined by cloud‐controlling factors includes the full effects of cloud adjustments. Here we compared the susceptibilities of the two kinds of cloud regimes and demonstrated this effect. Overall, increasing cloud droplet number concentration (Nd) consistently correlates to weaker precipitation, higher cloud fraction (CF), and reduced liquid water path, regardless of how the regime is defined. However, their susceptibilities to Nd aggregated over cloud‐appearance regimes are significantly lower than those aggregated over cloud‐controlling factors regimes, with lower‐tropospheric stability (LTS) serving as an example to define cloud‐controlling factors regimes. This underestimation is more pronounced for CF susceptibility, where the susceptibility for cloud appearance regimes is only 1/4 of the susceptibility for cloud controlling regimes. These findings imply that relying solely on cloud‐appearance regimes may underestimate the effective radiative forcing produced by cloud adjustment (ERFaci). Nevertheless, the substantial variability in the magnitude of cloud adjustment across appearance regimes at similar LTS also suggests that a single cloud‐controlling factor is not sufficient to fully separate cloud regimes to quantify cloud adjustment. Therefore, identifying a comprehensive set of cloud‐controlling factors is essential for accurately quantifying cloud adjustments in future studies.

Revisiting Aerosol–Cloud Interactions From Weekly Cycles

AbstractWeekly cycles (WCs) in cloud properties have been reported and linked to aerosol effects. Yet the extent to which human activities contribute to their occurrence remains unclear. Here, we revisit aerosol–cloud interactions from the WCs over central Europe using long‐term satellite and reanalysis data. Significant WCs in aerosol and cloud droplet number concentration (Nd) are detected with minima/maxima on Monday/Friday, indicating a clear signal of the Twomey effect. Notably, Nd–to–aerosol sensitivity from WCs is found to decrease at larger aerosol concentrations, confirming the nonlinear behavior of the aerosol–Nd relation (in log–log space) reported previously, but from a distinct perspective. Nevertheless, no discernible WCs in liquid water path are found. The pronounced WCs in cloud cover are demonstrated to be driven by natural variability. Our results indicate that the WCs offer a useful pathway for investigating the Twomey effect, but are not as effective for detecting cloud adjustments.

Studying the Aerosol Effect on Deep Convective Clouds over the Global Oceans by Applying Machine Learning Techniques on Long-Term Satellite Observation

Long-term (1982–2019) satellite climate data records (CDRs) of aerosols and clouds, reanalysis data of meteorological fields, and machine learning techniques are used to study the aerosol effect on deep convective clouds (DCCs) over the global oceans from a climatological perspective. Our analyses are focused on three latitude belts where DCCs appear more frequently in the climatology: the northern middle latitude (NML), tropical latitude (TRL), and southern middle latitude (SML). It was found that the aerosol effect on marine DCCs may be detected only in NML from long-term averaged satellite aerosol and cloud observations. Specifically, cloud particle size is more susceptible to the aerosol effect compared to other cloud micro-physical variables (e.g., cloud optical depth). The signature of the aerosol effect on DCCs can be easily obscured by meteorological covariances for cloud macro-physical variables, such as cloud cover and cloud top temperature (CTT). From a machine learning analysis, we found that the primary aerosol effect (i.e., the aerosol effect without meteorological feedbacks and covariances) can partially explain the aerosol convective invigoration in CTT and that meteorological feedbacks and covariances need to be included to accurately capture the aerosol convective invigoration. From our singular value decomposition (SVD) analysis, we found the aerosol effects in the three leading principal components (PCs) may explain about one third of the variance of satellite-observed cloud variables and significant positive or negative trends are only observed in the lead PC1 of cloud and aerosol variables. The lead PC1 component is an effective mode for detecting the aerosol effect on DCCs. Our results are valuable for the evaluation and improvement of aerosol-cloud interactions in the long-term climate simulations of global climate models.

Aerosol impacts on summer precipitation forecast over the North China Plain by using Thompson aerosol aware scheme in WRF: Process analysis and response sensitivity to aerosol concentrations during a Heavy Rainfall Event in Beijing

Aerosol-Cloud-Interactions (ACIs) are possibly important factors affecting precipitation while are usually not considered in numerical weather prediction systems (NWP) due to the complexities and uncertainties involved by considering aerosol information. This research focused on the use of the Thompson aerosol-aware scheme in WRF (Weather Research and Forecasting model). This paper summarized the process analysis and response sensitivity to aerosol concentrations during a heavy rainfall event in Beijing. The July 16, 2018 rainfall event -a typical precipitation case involving both warm and cold-phase clouds was thoroughly analyzed, including cloud fraction, downward shortwave radiation, water vapor consumption, cloud microphysical processes, net latent heat etc., which verified that the aerosol-cloud interaction paths were accurately and adequately considered in Thompson aerosol-ware scheme. By tracking key parameter changes, it is confirmed that the CCN/IN activation and relative roles in changing precipitation at different stages are reasonable in Thompson aerosol-aerosol scheme. According to the rainfall characteristics, the precipitation was divided into two phases. And the difference in the aerosol effect on precipitation in the two precipitation phases is mainly due to the complexity of cold rain process and hypothesis. Sensitivity simulations also revealed that the current concentrations of background aerosol in Beijing are actually high enough and further ten-times of aerosol concentration increase didn't bring significant additional precipitation response.

Effects of Combustible Cigarettes and Heated Tobacco Products on Systemic Inflammatory Response in Patients with Chronic Inflammatory Diseases.

Smoke derived from combustible cigarettes (CCs) contains numerous harmful chemicals that can impair the viability, proliferation, and activation of immune cells, affecting the progression of chronic inflammatory diseases. In order to avoid the detrimental effects of cigarette smoking, many CC users have replaced CCs with heated tobacco products (HTPs). Due to different methods of tobacco processing, CC-sourced smoke and HTP-derived aerosols contain different chemical constituents. With the exception of nicotine, HTP-sourced aerosols contain significantly lower amounts of harmful constituents than CC-derived smoke. Since HTP-dependent effects on immune-cell-driven inflammation are still unknown, herein we used flow cytometry analysis, intracellular staining, and an enzyme-linked immunosorbent assay to determine the impact of CCs and HTPs on systemic inflammatory response in patients suffering from ulcerative colitis (UC), diabetes mellitus (DM), and chronic obstructive pulmonary disease (COPD). Both CCs and HTPs significantly modulated cytokine production in circulating immune cells, affecting the systemic inflammatory response in COPD, DM, and UC patients. Compared to CCs, HTPs had weaker capacity to induce the synthesis of inflammatory cytokines (IFN-γ, IL-1β, IL-5, IL-6, IL-12, IL-23, IL-17, TNF-α), but more efficiently induced the production of immunosuppressive IL-10 and IL-35. Additionally, HTPs significantly enhanced the synthesis of pro-fibrotic TGF-β. The continuous use of CCs and HTPs aggravated immune-cell-driven systemic inflammation in COPD and DM patients, but not in UC patients, suggesting that the immunomodulatory effects of CC-derived smoke and HTP-sourced aerosols are disease-specific, and need to be determined for specific immune-cell-driven inflammatory diseases.