Abstract
Data are given on the mathematical modelling of the radiation-chemical behaviour of U, Np, Pu, Am in HClO 4 and HNO 3 solutions. Based on the comparison between the calculated and experimental data the optimized reaction schemes were developed for each system; the previously unknown rate constants were found for a lot of radiation-chemical reactions; mechanisms and kinetic regularities were established in the radiolytic behaviour of individual valent forms of a given actinide in a solution under study.
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