Abstract
Preparation of radical cation salts based on 1,3-dithiane derivatives (1,2 and 5–8) was investigated. Although attempts to prepare stable radical cation salts derived from 1 and 2 were unsuccessful, various radical cation salts composed of TTF (tetrathiafulvalene) derivatives fused with a 2-(1,3-dithiol-2-ylidene)-1,3-dithiane (DTDT) unit (5–8) were formed with ease by electrochemical oxidation. Several radical cation salts of 6–8 exhibited metallic conducting behaviors on a single crystal or compressed pellets.
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