Abstract
We generalize the multimode Brownian oscillator model for a two-level system to optical four wave mixing spectroscopy of a multilevel system, based on the recent work of Sung and Silbey [J. Chem. Phys. 115, 9266 (2001)]. For the Ohmic limit where the phenomenological Langevin equation becomes correct, we present exact expressions for energy-gap correlation functions in the strong damping case as well as in the weak damping case.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.