Abstract

The nuclear and electronic magnetic dipole moments of 21Fr and the nuclear ground-state spin of 207Fr have been measured directly by on-line atomic-beam magnetic resonance techniques at the ISOLDE facility at CERN. The following results have been obtained: μI(211Fr) = 4.00(8) nm, gJ(Fr, 7s 2S1/2) = 2.00497(9) and I(207Fr) = 9/2. A large deviation of the electronic magnetic moment from the free electron value was found. Using the measured nuclear magnetic moment μI(211Fr), a comparison is made between different theoretical calculations of the magnetic dipole hyperfine constants and with the available experimental data in 211Fr. An analysis of the electric quadrupole interaction is also given. Nuclear magnetic dipole and electric quadrupole moments are deduced for the sequences 207-213Fr and 220-228Fr, using the data on 211Fr as reference values. The nuclear quantities are discussed within the framework of the shell model and the core-quasiparticle model, giving information on the nuclear single-particle structure and on the variation in deformation along the sequences of francium isotopes.

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