Abstract

The treatment of large-scale air pollution models is not only important for modern society, but also an extremely difficult task. Five important physical and chemical processes: (1) horizontal advection, (2) horizontal diffusion, (3) vertical exchange, (4) emission of different pollutants and (5) dry and wet deposition have to be united and handled together. This leads to huge computational problems which have to be treated on modern high-speed parallel architectures by using advanced numerical methods. The computational difficulties are vastly increased when such models are used in the investigation of the impact of climatic changes on high pollution levels that are often exceeding certain critical concentrations and, therefore, are becoming harmful for plants, animals and human beings. There are two major reasons for the great increase in computational difficulties: (a) it is necessary to run the discretized data on fine spatial grid models over very long time-periods consisting of many consecutive years and (b) different scenarios are to be used in order to investigate the sensitivity of the pollution levels to systematic variations of several carefully selected key parameters. How the major difficulties can be resolved is explained here. Furthermore, many results are presented in order to demonstrate the ability of the model to handle successfully the huge computational tasks by using fine space and time discretization and by applying a chemical scheme with many chemical species participating in several hundred chemical reactions. Our results indicate that the climatic changes will often lead to some increases in the pollution levels.

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