Abstract

Abstract. Methane is the second most important greenhouse gas in terms of anthropogenic radiative forcing. Since pre-industrial times, the globally averaged dry mole fraction of methane in the atmosphere has increased considerably. Emissions from coal mining are one of the primary anthropogenic methane sources. However, our knowledge about different sources and sinks of methane is still subject to great uncertainties. Comprehensive measurement campaigns and reliable chemistry–climate models, are required to fully understand the global methane budget and to further develop future climate mitigation strategies. The CoMet 1.0 campaign (May to June 2018) combined airborne in situ, as well as passive and active remote sensing measurements to quantify the emissions from coal mining in the Upper Silesian Coal Basin (USCB, Poland). Roughly 502 kt of methane is emitted from the ventilation shafts per year. In order to help with the flight planning during the campaigns, we performed 6 d forecasts using the online coupled, three-time nested global and regional chemistry–climate model MECO(n). We applied three-nested COSMO/MESSy instances going down to a spatial resolution of 2.8 km over the USCB. The nested global–regional model system allows for the separation of local emission contributions from fluctuations in the background methane. Here, we introduce the forecast set-up and assess the impact of the model's spatial resolution on the simulation of methane plumes from the ventilation shafts. Uncertainties in simulated methane mixing ratios are estimated by comparing different airborne measurements to the simulations. Results show that MECO(3) is able to simulate the observed methane plumes and the large-scale patterns (including vertically integrated values) reasonably well. Furthermore, we obtain reasonable forecast results up to forecast day four.

Highlights

  • In terms of radiative forcing methane is the second most important anthropogenically altered greenhouse gas (Myhre et al, 2013)

  • The instrument is an integrated-path differential absorption (IPDA) lidar called CHARM-F (Amediek et al, 2017), which was installed on board the German Research Aircraft High Altitude and Long Range Research Aircraft (HALO) (High Altitude and LOng Range)

  • Modelling the smaller-scale features observed by P is, challenging, which is reflected in the Overall, the comparison of the analysis simulation with airborne-derived measurements shows that MECO(n) is able to simulate the observed methane plumes reasonably well

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Summary

Introduction

In terms of radiative forcing methane is the second most important anthropogenically altered greenhouse gas (Myhre et al, 2013). The reason for the rapid methane growth in the atmosphere is currently under debate and discussed in several studies (Schaefer et al, 2016; Nisbet et al, 2016, 2019; Saunois et al, 2017; Thompson et al, 2018). A depletion in global δ13C indicates a shift from fossil fuel emissions towards more microbial sources (Schaefer et al, 2016; Nisbet et al, 2016, 2019). Increasing fossil fuel emissions could explain the rise in atmospheric methane (Thompson et al, 2018). A reduction of anthropogenic emissions is attractive and inexpensive, and due to its relatively short lifetime (∼ 9 years), it could rapidly cause a change in the global methane budget (Dlugokencky et al, 2011). Comprehensive measurements and the use of chemistry–climate models can help to improve further climate change projections and to develop potential climate change mitigation strategies

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