Abstract

Fission products deposited in the coolant circuit outside of the active core play a dominant role in source term estimations for advanced small pebble bed HTRs, particularly in design basis accidents (DBA). The deposited fission products may be released in depressurization accidents because present pebble bed HTR concepts abstain from a gas tight containment. Contamination of the circuit also hinders maintenance work. Experiments, performed from 1972 to 88 on the AVR, an experimental pebble bed HTR, allow for a deeper insight into fission product transport behavior. The activity deposition per coolant pass was lower than expected and was influenced by fission product chemistry and by presence of carbonaceous dust. The latter lead also to inconsistencies between Cs plate out experiments in laboratory and in AVR. The deposition behavior of Ag was in line with present models. Dust as activity carrier is of safety relevance because of its mobility and of its sorption capability for fission products. All metal surfaces in pebble bed reactors were covered by a carbonaceous dust layer. Dust in AVR was produced by abrasion in amounts of about 5 kg/y. Additional dust sources in AVR were ours oil ingress and peeling of fuel element surfaces due to an air ingress. Dust has a size of about 1 m, consists mainly of graphite, is partly remobilized by flow perturbations, and deposits with time constants of 1 to 2 hours. In future reactors, an efficient filtering via a gas tight containment is required because accidents with fast depressurizations induce dust mobilization. Enhanced core temperatures in normal operation as in AVR and broken fuel pebbles have to be considered, as inflammable dust concentrations in the gas phase.

Highlights

  • Fission product transport during HTR normal operation plays a major role in safety examinations for normal operation and for accidents as in maintenance and in dismantling

  • The fission products released during reactor normal operation and accumulated within the coolant circuit are most relevant contributions to the source terms of design basis accidents (DBAs) for advanced small HTRs

  • These activities are released into the coolant circuit during long-term normal operation at high temperatures from intact- and defect coated fuel particles and from uranium contamination in the graphite by diffusion through kernel, coating layers, and graphite as well as by diffusion out of the kernels of defective coated fuel particles without further retention

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Summary

Introduction

Fission product transport during HTR normal operation plays a major role in safety examinations for normal operation and for accidents as in maintenance and in dismantling. The intact coated particle is a very efficient barrier for nonmetals, but low melting metallic fission products diffuse through intact coatings, at temperatures >1000◦C. Condensable fission products are mainly deposited in the coolant circuit: plate out on metals competes with sorption on graphitic dust. Except for noble gases, the gas-borne activities are low in steady-state operation due to this deposition

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