Abstract

This research focused on enhancement of mechanical properties in carbon fiber (CF)-filler-reinforced linear low-density polyethylene (PE) matrix composites. A hand layup method using an oven was used as the fabrication method. Improvement in adhesion was achieved by oxygen plasma treatment to the PE matrix. CF and PE were initially mixed by normal stirring, ultrasonication and mechanical stirring before being filtered and dried for fabrication. Better tensile results were observed with a plasma-treated polyethylene (PEP)/10 wt.% CF combination, with a maximum tensile strength of 21.5 MPa and improvement in the properties of up to 12.57% compared to non-plasma PE with the same CF addition. The addition of carbon fibers at 13 and 15 wt.% resulted in a reduction in the tensile strength properties to 18.2 MPa and 17.7 MPa, respectively. This reduction in tensile strength was due to agglomeration of CF with plasma- and non-plasma-treated PE. The fabrication condition of 180 °C temperature for 20 min showed better tensile properties than other conditions. The SEM results following tensile testing revealed enhanced CF filler adherence with plasma PE results, as well as fewer surface deformations. A higher flexural strength of 25.87 MPa was observed for the plasma treated PE/7 wt.% CF combination.

Highlights

  • Polyethylene is one of the most effective polymers used in various fields for thin films, adhesives, medical implants, electronics, battery and orthopedic applications [1,2].It is usually fabricated using rotomolding for industrial applications

  • Radiofrequency plasma treatment, using air, argon and a combination of air and argon, for both PEEK and carbon fibers, increased surface roughness and provided good mechanical interlocking with CF and PEEK

  • There was good interfacial adhesion with the PE matrix and 5% CF filler resulting in good properties (Figure 3c)

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Summary

Introduction

Polyethylene is one of the most effective polymers used in various fields for thin films, adhesives, medical implants, electronics, battery and orthopedic applications [1,2]. Fiber and matrix adhesion are vital factors in determining the mechanical properties of the composites These can be improved by plasma treatment of polyethylene matrices, which significantly enhances compatibility between fibers and matrices [2–4]. The shape memory of polymers of an epoxy-based matrix resulted in improved mechanical properties with incorporation of continuous and short carbon fibers into the combination [20] Carbon reinforced materials, such as carbon fibers, single and multi-wall carbon nanotubes and carbon black (CB), have been used for electrical conductivity applications with various thermo- and thermo-setting plastics. Radiofrequency plasma treatment, using air, argon and a combination of air and argon, for both PEEK and carbon fibers, increased surface roughness and provided good mechanical interlocking with CF and PEEK This enhanced the interfacial strength of the PEEK composites [25]. Carbon fibers were treated with plasma in the final stage for confirmation

Materials
Fabrication
Methods
Tensile Testing
Tensile
Flexural
13. Normal
15. Surface
Conclusions
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